arXiv subjects

A. V. Malyshev

Publications and source records attributed to A. V. Malyshev.

At least 37 records · Page 2Linked to original sources

arXiv2021

Relativistic calculations of the chemical properties of the superheavy element with $Z=119$ and its homologues

Relativistic calculations of the electronic structure of the superheavy element of the eighth period $-$ eka-francium ($Z=119$) and its homologues, which form the group of alkali metals, are performed in the framework of the configuration-interaction method and many-body perturbation theory using the basis of the Dirac-Fock-Sturm orbitals (DFS). The obtained values of the ionization potentials, electron affinities, and root-mean-square radii are compared with the corresponding values calculated within the non-relativistic approximation. A comparison with the available experimental data and the results of previous theoretical calculations is given as well. The analysis of the obtained results indicates a significant influence of the relativistic effects for the francium and eka-francium atoms, which leads to a violation of the monotonic behaviour of the listed above chemical properties as a function of the alkaline-element atomic number. In addition, the quantum electrodynamics corrections to the ionization potentials are evaluated by employing the model Lamb-shift operator (QEDMOD).

physics.atom-ph↗

arXiv2021

Ab initio calculations of energy levels in Be-like xenon: strong interference between electron-correlation and QED effects

The strong mixing of close levels with two valence electrons in Be-like xenon greatly complicates ab initio QED calculations beyond the first-order approximation. Due to a strong interplay between the electron-electron correlation and QED effects, the standard single-level perturbative QED approach may fail, even if it takes into account the second-order screened QED diagrams. In the present Letter, the corresponding obstacles are overcome by working out the QED perturbation theory for quasidegenerate states. The contributions of all the Feynman diagrams up to the second order are taken into account. The many-electron QED effects are rigorously evaluated in the framework of the extended Furry picture to all orders in the nuclear-strength parameter $αZ$. The higher-order electron-correlation effects are considered within the Breit approximation. The nuclear recoil effect is accounted for as well. The developed approach is applied to high-precision QED calculations of the ground and singly excited energy levels in Be-like xenon. The most accurate theoretical predictions for the binding and excitation energies are obtained. These results deviate from the most precise experimental value by $3σ$ but perfectly agree with a more recent measurement.

physics.atom-ph↗

arXiv2020

QED theory of the normal mass shift in few-electron atoms

The electron-electron interaction correction of first order in $1/Z$ to the one-electron part of the nuclear recoil effect on binding energies in atoms and ions is considered within the framework of the rigorous QED approach. The calculations to all orders in $αZ$ are performed for the $1s^2$ state in heliumlike ions and the $1s^2 2s$ and $1s^2 2p_{1/2}$ states in lithiumlike ions in the range $Z=5$--$100$. The results obtained are compared with the Breit-approximation values. The performed calculations complete a systematic treatment of the QED nuclear recoil effect up to the first order in $1/Z$. The correction obtained is combined with the previously studied two-electron part as well as the higher-order electron-correlation corrections evaluated within the Breit approximation to get the total theoretical predictions for the mass shifts.

physics.atom-ph↗

arXiv2020

QED corrections to the $^2P_{1/2}-{}^2P_{3/2}$ fine structure in fluorinelike ions: model Lamb shift operator approach

In [Li ${\it et \, al.}$, Phys. Rev. A ${\bf 98}$, 020502(R) (2018)] it was claimed that the model-potential computations of the Lamb shift on the $^2P_{1/2}-{}^2P_{3/2}$ fine structure in fluorinelike uranium lead to a discrepancy between theory and experiment. Later, it was reported by [Volotka ${\it et \, al.}$, Phys. Rev. A ${\bf 100}$, 010502(R) (2019)] that {\it ab initio} QED calculation, including the first-order one-electron QED contributions and the related effects of two-electron screening, yields the result which restores the agreement between theory and experiment and strongly disagrees with the model-potential Lamb shift values. In the present paper, the model Lamb shift operator [Shabaev ${\it et \, al.}$, Phys. Rev. A ${\bf 88}$, 012513 (2013)] is used to evaluate the QED effects on the $^2P_{1/2}-{}^2P_{3/2}$ fine structure in F-like ions. The calculations are performed by incorporating this operator into the Dirac-Coulomb-Breit equation employing different methods. It is demonstrated that the methods, based on including the Lamb shift operator either into the Dirac-Fock equations or into the calculations by perturbation theory, lead to the theoretical results which are in good agreement with each other and with experiment. The restriction of these results to the first order in the QED effects leads to a value which agrees with the aforementioned ${\it ab\, initio}$ QED result.

physics.atom-ph↗

arXiv2020

Manipulating photonic signals by a multipurpose quantum junction

We show that photon wave packets can be manipulated and reshaped in various ways by a quantum junction comprising a set of three-level atoms coupling two waveguides. We consider atomic nodes with the $Λ$-scheme of allowed optical transitions, one of which is driven by an external classical control field. Addressing the dynamics of wave packets in such a system, we demonstrate that a photon pulse can be either stored partially in the junction, delayed by a controlled time, split into several parts, or routed into one of the selected output channels. We argue, therefore, that our proposed design is a promising prototype of a multipurpose quantum junction.

quant-ph↗

arXiv2019

Relativistic calculation of the nuclear recoil effect on the $g$ factor of the $^2P_{3/2}$ state in highly charged B-like ions

The nuclear recoil effect on the $^2 P_{3/2}$-state $g$ factor of B-like ions is calculated to first order in the electron-to-nucleus mass ratio $m/M$ in the range $Z=18$--$92$. The calculations are performed by means of the $1/Z$ perturbation theory. Within the independent-electron approximation, the one- and two-electron recoil contributions are evaluated to all orders in the parameter $αZ$ by employing a fully relativistic approach. The interelectronic-interaction correction of first order in $1/Z$ is treated within the Breit approximation. Higher orders in $1/Z$ are partially taken into account by incorporating the screening potential into the zeroth-order Hamiltonian. The most accurate to date theoretical predictions for the nuclear recoil contribution to the bound-electron $g$ factor are obtained.

physics.atom-ph↗

arXiv2019

Interelectronic-interaction contribution to the nuclear recoil effect on the $g$ factor of boronlike ions

The nuclear recoil effect on the ground-state $g$ factor of highly charged boronlike ions is considered within the relativistic framework. The interelectronic-interaction contribution is evaluated within the Breit approximation employing two independent approaches: the second-order perturbation theory and the configuration-interaction Dirac-Fock-Sturm method. The uncertainty of the nuclear recoil $g$-factor contributions is significantly reduced, especially for low- and middle-$Z$ ions.

physics.atom-ph↗

arXiv2019

QED calculations of the nuclear recoil effect on the bound-electron $g$ factor

Fully relativistic approach is applied to evaluation of the nuclear recoil effect on the bound-electron $g$ factor in hydrogenlike ions to first order in the electron-to-nucleus mass ratio $m/M$ and to all orders in $αZ$. The calculations are performed in the range $1 \leqslant Z \leqslant 20$ for the $g$ factors of $1s$, $2s$, $2p_{1/2}$, and $2p_{3/2}$ states. The $αZ$-dependence of the nontrivial QED recoil contribution as a function of $Z$ is studied.

physics.atom-ph↗

arXiv2019

QED with heavy ions: on the way from strong to supercritical fields

The current status of tests of quantum electrodynamics with heavy ions is reviewed. The theoretical predictions for the Lamb shift and the hyperfine splitting in heavy ions are compared with available experimental data. Recent achievements and future prospects in studies of the $g$ factor with highly charged ions are also reported. These studies can provide precise determination of the fundamental constants and tests of QED within and beyond the Furry picture at the strong-coupling regime. Theoretical calculations of the electron-positron pair creation probabilities in low-energy heavy-ion collisions are also considered. Special attention is paid to tests of QED in supercritical-field regime, which can be accessed in slow collisions of two bare nuclei with the total charge number larger than the critical value, $Z_{\rm crit} \approx 173$. In the supercritical field, the initially neutral vacuum can spontaneously decay into the charged vacuum and two positrons. It is demonstrated that this fundamental phenomenon can be observed via impact-sensitive measurements of the pair-production probabilities.

physics.atom-ph↗

arXiv2019

QED calculation of electron-electron correlation effects in heliumlike ions

Fully relativistic approach to evaluate the correlation effects in highly charged ions is presented. The interelectronic-interaction contributions of first and second orders in $1/Z$ are treated rigorously within the framework of bound-state quantum electrodynamics, whereas the calculations of the third- and higher-order contributions are based on the Dirac-Coulomb-Breit Hamiltonian. The developed approach allows one to deal with single as well as degenerate or quasi-degenerate states. We apply this approach to the calculations of the correlation contributions to the $n=1$ and $n=2$ energy levels in heliumlike ions. The obtained contributions are combined with the one-electron and screened QED corrections, nuclear recoil and nuclear polarization corrections to get the total theoretical predictions for the ionization and transition energies in high-$Z$ heliumlike ions.

physics.atom-ph↗

arXiv2019

QED theory of the specific mass shift in atoms

The quantum electrodynamics formalism to treat the interelectronic-interaction correction of first order in $1/Z$ to the two-electron part of the nuclear recoil effect on binding energies in atoms and ions is developed. The nonperturbative in $αZ$ calculations of the corresponding contribution to the energies of the $1s^2$ state in He-like and the $1s^2 2s$ and $1s^2 2p_{1/2}$ states in Li-like ions are performed in the range $Z=5-100$. The behavior of the two-electron part of the nuclear recoil effect beyond the lowest-order relativistic approximation as $Z$ grows is studied.

physics.atom-ph↗

arXiv2019

Ground-State Energy of Uranium Diatomic Quasimolecules with One and Two Electrons

Ground-state energies of the one- and two-electron uranium dimers are calculated for internuclear distances in the range D=40--1000 fm and compared with the previous calculations. The generalization of the dual-kinetic-balance approach for axially symmetric systems is employed to solve the two-center Dirac equation without the partial-wave expansion for the potential of two nuclei. The one-electron one-loop QED contributions (self-energy and vacuum polarization) to the ground-state energy are evaluated using the monopole approximation for the two-center potential. Interelectronic interaction of the first and second order is taken into account for the two-electron quasimolecule. Within the QED approach one-photon-exchange contribution is calculated in the two-center potential, while the two-photon-exchange contribution is treated in the monopole approximation.

physics.atom-ph↗

arXiv2019

Relativistic calculations of the ground and inner-L-shell excited energy levels of berylliumlike ions

Large-scale relativistic configuration-interaction method combined with many-body perturbation theory is consistently applied to calculations of the energy levels of the ground and inner-L-shell excited states of berylliumlike ions in the range $10 \leq Z \leq 92$. The quantum electrodynamics, nuclear recoil, and frequency-dependent Breit corrections are taken into account. The obtained results are supplemented with the systematical estimation of the uncertainties.

physics.atom-ph↗

arXiv2019

Isotope shifts of the $1s^22s2p(J)$ -$1s^22s^2$ transition energies in Be-like thorium and uranium

Precise calculations of the isotope shifts in berylliumlike thorium and uranium ions are presented. The main contributions to the field and mass shifts are calculated within the framework of the Dirac-Coulomb-Breit Hamiltonian employing the configuration-interaction Dirac-Fock-Sturm method. These calculations include the relativistic, electron-electron correlation, and Breit-interaction effects. The QED, nuclear deformation, and nuclear polarization corrections are also evaluated.

physics.atom-ph↗

arXiv2019

A tunable single photon quantum router

We propose an efficient single-photon router comprising two resonator waveguide channels coupled by several sequential cavities with embedded three-level atoms. We show that the system can operate as a perfect four-way single-photon switch. We also demonstrate that an incident single-photon propagating in one of the waveguides can be routed into one or the other output channels; such routing can be controlled by the external classical electromagnetic field driving the atoms. We argue that, under appropriate conditions, the efficiency of such routing can be close to 100\% within a broad operational bandwidth, suggesting various applications in photonics.

quant-ph↗

arXiv2018

QED calculations of the $n=2$ to $n=1$ x-ray transition energies in middle-$Z$ heliumlike ions

Ab initio QED calculations of the four x-ray transitions from the $L$ to $K$ shell in heliumlike argon, titanium, iron, copper, and krypton are performed. The binding energies for all the $n=1$ and $n=2$ states are evaluated as well. The calculation approach combines the rigorous QED treatment in the first two orders of the perturbation theory constructed within the extended Furry picture with the third- and higher-order correlation effects evaluated in the Breit approximation. The obtained results are compared with the previous evaluations and available experimental data.

physics.atom-ph↗

arXiv2018

Stringent tests of QED using highly charged ions

The present status of tests of QED with highly charged ions is reviewed. The theoretical predictions for the Lamb shift and the transition energies are compared with available experimental data. Recent achievements in studies of the hyperfine splitting and the $g$-factor isotope shift with highly charged ions are reported. Special attention is paid to tests of QED within and beyond the Furry picture at strong-coupling regime. Prospects for tests of QED at supercritical fields that can be created in low-energy heavy-ion collisions are discussed as well.

physics.atom-ph↗

arXiv2018

Relativistic nuclear recoil effect on the $g$ factor of highly charged boronlike ions

The nuclear recoil effect on the $g$ factor of the ground state of highly charged B-like ions is studied to first order in the electron-to-nucleus mass ratio $m/M$. The leading one-electron and two-electron recoil contributions are calculated nonperturbatively in the parameter $αZ$ within the rigorous QED formalism. The interelectronic-interaction correction to the nuclear recoil effect is evaluated in the Breit approximation by means of perturbation theory to the first order in $1/Z$. The higher-order interelectronic-interaction corrections are taken into account partially by performing the calculations with the effective screening potential. The results obtained represent the most accurate up-to-date treatment of the nuclear recoil effect on the $g$ factor of highly charged B-like ions in the range $Z = 20$--$92$.

physics.atom-ph↗