arXiv subjects

A. Vishwanath

Publications and source records attributed to A. Vishwanath.

At least 19 recordsLinked to original sources

arXiv2021

Magnetic crystalline-symmetry-protected axion electrodynamics and field-tunable unpinned Dirac cones in EuIn2As2

Knowledge of magnetic symmetry is vital for exploiting nontrivial surface states of magnetic topological materials. EuIn$_{2}$As$_{2}$ is an excellent example, as it is predicted to have collinear antiferromagnetic order where the magnetic moment direction determines either a topological-crystalline-insulator phase supporting axion electrodynamics or a higher-order-topological-insulator phase with chiral hinge states. Here, we use neutron diffraction, symmetry analysis, and density functional theory results to demonstrate that EuIn$_{2}$As$_{2}$ actually exhibits low-symmetry helical antiferromagnetic order which makes it a stoichiometric magnetic topological-crystalline axion insulator protected by the combination of a 180$^{\circ}$ rotation and time-reversal symmetries: $C_{2}\times\mathcal{T}=2^{\prime}$. Surfaces protected by $2^{\prime}$ are expected to have an exotic gapless Dirac cone which is unpinned to specific crystal momenta. All other surfaces have gapped Dirac cones and exhibit half-integer quantum anomalous Hall conductivity. We predict that the direction of a modest applied magnetic field of $H\approx1$ to $2$ T can tune between gapless and gapped surface states.

cond-mat.str-el↗

arXiv2016

Observation of a Discrete Time Crystal

Spontaneous symmetry breaking is a fundamental concept in many areas of physics, ranging from cosmology and particle physics to condensed matter. A prime example is the breaking of spatial translation symmetry, which underlies the formation of crystals and the phase transition from liquid to solid. Analogous to crystals in space, the breaking of translation symmetry in time and the emergence of a "time crystal" was recently proposed, but later shown to be forbidden in thermal equilibrium. However, non-equilibrium Floquet systems subject to a periodic drive can exhibit persistent time-correlations at an emergent sub-harmonic frequency. This new phase of matter has been dubbed a "discrete time crystal" (DTC). Here, we present the first experimental observation of a discrete time crystal, in an interacting spin chain of trapped atomic ions. We apply a periodic Hamiltonian to the system under many-body localization (MBL) conditions, and observe a sub-harmonic temporal response that is robust to external perturbations. Such a time crystal opens the door for studying systems with long-range spatial-temporal correlations and novel phases of matter that emerge under intrinsically non-equilibrium conditions.

quant-ph↗

arXiv2016

Strain-induced nonsymmorphic symmetry breaking and removal of Dirac semimetallic nodal line in an orthoperovskite iridate

By using a combination of heteroepitaxial growth, structure refinement based on synchrotron x-ray diffraction and first-principles calculations, we show that the symmetry-protected Dirac line nodes in the topological semimetallic perovskite SrIrO3 can be lifted simply by applying epitaxial constraints. In particular, the Dirac gap opens without breaking the Pbnm mirror symmetry. In virtue of a symmetry-breaking analysis, we demonstrate that the original symmetry protection is related to the n-glide operation, which can be selectively broken by different heteroepitaxial structures. This symmetry protection renders the nodal line a nonsymmorphic Dirac semimetallic state. The results highlight the vital role of crystal symmetry in spin-orbit-coupled correlated oxides and provide a foundation for experimental realization of topological insulators in iridate-based heterostructures.

cond-mat.str-el↗

arXiv2015

Photoexcited states of the harmonic honeycomb iridate γ-Li$_2$IrO$_3$

We report equilibrium and nonequilibrium optical measurements on the recently synthesized "harmonic" honeycomb iridate γ-Li$_2$IrO$_3$ (LIO), as well as the layered honeycomb iridate Na$_2$IrO$_3$ (NIO). Using Fourier transform infrared microscopy we performed reflectance measurements on LIO, from which we obtained the optical conductivity below 2 eV. In addition we measured the photoinduced changed in reflectance, ΔR, as a function of time, t, temperature, T, and probe field polarization in both LIO and NIO. In LIO, ΔR(t,T) is anisotropic and comprised of three T dependent components. Two of these components are related to the onset of magnetic order and the third is related to a photoinduced population of metastable electronic excited states. In NIO, ΔR(t,T) has a single T dependent component that is strikingly similar to the electronic excitation component of ΔR in LIO. Through analysis and comparison of ΔR(t,T) for two compounds, we extract information on the onset of magnetic correlations at and above the transition temperature in LIO, the bare spin-flip scattering rate in equilibrium, the lifetime of low-lying quasiparticle excitations, and the polarization dependence of optical transitions that are sensitive to magnetic order.

cond-mat.str-el↗

arXiv2014

Probing the chiral anomaly with nonlocal transport in three dimensional topological semimetals

Weyl semimetals are three-dimensional crystalline systems where pairs of bands touch at points in momentum space, termed Weyl nodes, that are characterized by a definite topological charge: the chirality. Consequently, they exhibit the Adler-Bell-Jackiw anomaly, which in this condensed matter realization implies that application of parallel electric ($\mathbf{E}$) and magnetic ($\mathbf{B}$) fields pumps electrons between nodes of opposite chirality at a rate proportional to $\mathbf{E}\cdot\mathbf{B}$. We argue that this pumping is measurable via nonlocal transport experiments, in the limit of weak internode scattering. Specifically, we show that as a consequence of the anomaly, applying a local magnetic field parallel to an injected current induces a valley imbalance that diffuses over long distances. A probe magnetic field can then convert this imbalance into a measurable voltage drop far from source and drain. Such nonlocal transport vanishes when the injected current and magnetic field are orthogonal, and therefore serves as a test of the chiral anomaly. We further demonstrate that a similar effect should also characterize Dirac semimetals --- recently reported to have been observed in experiments --- where a pair of Weyl nodes coexisting at a single point in the Brillouin zone are protected by a crystal symmetry. Since the nodes are analogous to valley degrees of freedom in semiconductors, this suggests that valley currents in three dimensional topological semimetals can be controlled using electric fields, which has potential practical `valleytronic' applications.

cond-mat.str-el↗

arXiv2014

Non-coplanar and counter-rotating incommensurate magnetic order stabilized by Kitaev interactions in $γ$-Li2IrO3

Materials that realize Kitaev spin models with bond-dependent anisotropic interactions have long been searched for, as the resulting frustration effects are predicted to stabilize novel forms of magnetic order or quantum spin liquids. Here we explore the magnetism of $γ$-Li$_2$IrO$_3$, which has the topology of a 3D Kitaev lattice of inter-connected Ir honeycombs. Using resonant magnetic x-ray diffraction we find a complex, yet highly-symmetric incommensurate magnetic structure with non-coplanar and counter-rotating Ir moments. We propose a minimal Kitaev-Heisenberg Hamiltonian that naturally accounts for all key features of the observed magnetic structure. Our results provide strong evidence that $γ$-Li$_2$IrO$_3$ realizes a spin Hamiltonian with dominant Kitaev interactions.

cond-mat.str-el↗

arXiv2013

Tuning the electronic properties of J_eff=1/2 correlated semimetal in epitaxial perovskite SrIrO3

We investigated the electronic properties of epitaxially stabilized perovskite SrIrO3 and demonstrated the effective strain-control on its electronic structure. Comprehensive transport measurements showed that the strong spin-orbit coupling renders a novel semimetallic phase for the J_eff=1/2 electrons rather than an ordinary correlated metal, elucidating the nontrivial mechanism underlying the dimensionality-controlled metal-insulator transition in iridates. The electron-hole symmetry of this correlated semimetal was found to exhibit drastic variation when subject to bi-axial strain. Under compressive strain, substantial electron-hole asymmetry is observed in contrast to the tensile side, where the electron and hole effective masses are comparable, illustrating the susceptivity of the J_eff=1/2 to structural distortion. Tensile strain also shrinks the Fermi surface, indicative of an increasing degree of correlation which is consistent with optical measurements. These results pave a pathway to investigate and manipulate the electronic states in spin-orbit-coupled correlated oxides, and lay the foundation for constructing 5d transition metal heterostructures.

cond-mat.str-el↗

arXiv2013

A new collective mode in YBCO observed by time-domain reflectometry

We report the observation of coherent oscillations associated with charge density wave (CDW) order in the underdoped cuprate superconductor YBa2Cu3O6+x by time-resolved optical reflectivity. Oscillations with frequency 1.87 THz onset at approximately 105 K and 130 K for dopings of x = 0.67 (ortho-VIII) and x = 0.75 (ortho-III), respectively. Upon cooling below the superconducting critical temperature (T_c), the oscillation amplitude is enhanced, the phase shifts by π, and the frequency softens by δν/ ν~7%. A bi-quadratically coupled Landau-Ginzburg model qualitatively describes this behavior as arising from competition between superconducting and CDW orders.

cond-mat.supr-con↗

arXiv2013

Epitaxy-distorted spin-orbit Mott insulator in Sr2IrO4 thin films

High quality epitaxial thin films of Jeff=1/2 Mott insulator Sr2IrO4 with increasing in-plane tensile strain have been grown on top of SrTiO3(001) substrates. Increasing the in-plane tensile strain up to ~0.3% was observed to drop the c/a tetragonality by 1.2 %. X-ray absorption spectroscopy detected a strong reduction of the linear dichroism upon increasing in-plane tensile strain towards a reduced anisotropy in the local electronic structure. While the most relaxed thin film shows a consistent dependence with previously reported single crystal bulk measurements, electrical transport reveals a charge gap reduction from 200 meV down to 50 meV for the thinnest and most epitaxy-distorted film. We argue that the reduced tetragonality plays a major role in the change of the electronic structure, which is reflected in the change of the transport properties. Our work opens the possibility for exploiting epitaxial strain as a tool for both structural and functional manipulation of spin-orbit Mott systems.

cond-mat.mtrl-sci↗

arXiv2012

Observation of Coherent Helimagnons and Gilbert damping in an Itinerant Magnet

We study the magnetic excitations of itinerant helimagnets by applying time-resolved optical spectroscopy to Fe0.8Co0.2Si. Optically excited oscillations of the magnetization in the helical state are found to disperse to lower frequency as the applied magnetic field is increased; the fingerprint of collective modes unique to helimagnets, known as helimagnons. The use of time-resolved spectroscopy allows us to address the fundamental magnetic relaxation processes by directly measuring the Gilbert damping, revealing the versatility of spin dynamics in chiral magnets. (*These authors contributed equally to this work)

cond-mat.str-el↗

arXiv2012

Dynamical Interplay between Coexisting Orders in the Electron-Doped Cuprate Superconductor Nd_{2-x}Ce_xCuO_4

We use coherent pump-probe spectroscopy to measure the photoinduced reflectivity \DeltaR, and complex dielectric function, δ\in, of the electron-doped cuprate superconductor Nd_{2-x}Ce_xCuO_{4+δ} at a value of x near optimal doping, as a function of time, temperature, and laser fluence. We observe the onset of a negative \DeltaR at T=85 K, above the superconducting transition temperature, T_c, of 23 K, that exhibits a form of scaling consistent with critical fluctuations in the time domain. A positive ΔR onsets at T_c that we associate with superconducting order. We find that the two signals are strongly coupled below T_c, in a manner that suggests a repulsive interaction between superconductivity and antiferromagnetic correlations.

cond-mat.supr-con↗

arXiv2012

Fractional topological phases and broken time reversal symmetry in strained graphene

We show that strained or deformed honeycomb lattices are promising platforms to realize fractional topological quantum states in the absence of any magnetic field. The strained induced pseudo magnetic fields are oppositely oriented in the two valleys [1-3] and can be as large as 60-300 Tesla as reported in recent experiments [4,5]. For strained graphene at neutrality, a spin or a valley polarized state is predicted depending on the value of the onsite Coulomb interaction. At fractional filling, the unscreened Coulomb interaction leads to a valley polarized Fractional Quantum Hall liquid which spontaneously breaks time reversal symmetry. Motivated by artificial graphene systems [5-8], we consider tuning the short range part of interactions, and demonstrate that exotic valley symmetric states, including a valley Fractional Topological Insulator and a spin triplet superconductor, can be stabilized by such interaction engineering.

cond-mat.str-el↗

arXiv2008

Noise Correlations in low-dimensional systems of ultracold atoms

We derive relations between standard order parameter correlations and the noise correlations in time of flight images, which are valid for systems with long range order as well as low dimensional systems with algebraic decay of correlations. Both Bosonic and Fermionic systems are considered. For one dimensional Fermi systems we show that the noise correlations are equally sensitive to spin, charge and pairing correlations and may be used to distinguish between fluctuations in the different channels. This is in contrast to linear response experiments, such as Bragg spectroscopy, which are only sensitive to fluctuations in the particle-hole channel (spin or charge). For Bosonic systems we find a sharp peak in the noise correlation at opposite momenta that signals pairing correlations in the depletion cloud. In a condensate with true long range order, this peak is a delta function and we can use Bogoliubov theory to study its temperature dependence. Interestingly we find that it is enhanced with temperature in the low temperature limit. In one dimensional condensates with only quasi-long range (i.e. power-law) order the peak in the noise correlations also broadens to a power-law singularity.

cond-mat.other↗

arXiv2008

A vortex dynamics approach to the Nernst effect in fluctuating superconductors

We present a new method to study the Nernst effect and diamagetism of an extreme type-II superconductor dominated by phase fluctuations. We work directly with vortex variables and our method allows us to tune vortex parameters (e.g., core energy and number of vortex species). We find that diamagnetic response and transverse thermoelectric conductivity ($α_{xy}$) persist well above the Kosterlitz-Thouless transition temperature, and become more pronounced as the vortex core energy is increased. However, they \textit{weaken} as the number of internal vortex states are increased. We find that $α_{xy}$ closely tracks the magnetization $(-M/T)$ over a wide range of parameters.

cond-mat.supr-con↗

arXiv2007

Noise Correlations in one-dimensional systems of ultra-cold fermions

Time of flight images reflect the momentum distribution of the atoms in the trap, but the spatial noise in the image holds information on more subtle correlations. Using Bosonization, we study such noise correlations in generic one dimensional systems of ultra cold fermions. Specifically, we show how pairing as well as spin and charge density wave correlations may be identified and extracted from the time of flight images. These incipient orders manifest themselves as power law singularities in the noise correlations, that depend on the Luttinger parameters, which suggests a general experimental technique to obtain them.

cond-mat.str-el↗

arXiv2007

Chirality induced anomalous-Hall effect in helical spin crystals

Under pressure, the itinerant helimagnet MnSi displays unusual magnetic properties. We have previously discussed a BCC helical spin crystal as a promising starting point for describing the high pressure phenomenology. This state has topologically nontrivial configurations of the magnetization field. Here we note the consequences for magneto-transport that arise generally from such spin textures. In particular a skyrmion density induced `topological' Hall effect, with unusual field dependence, is described.

cond-mat.str-el↗

arXiv2006

Theory of helical spin crystals: phases, textures and properties

Motivated by recent experiments on the itinerant helimagnet MnSi, we study general properties of helical spin crystals - magnetic structures obtained by superposing distinct spin spirals. An effective Landau description of helical spin crystals is introduced and simple rules for stabilizing various spin crystal structures over single spirals are established. Curious properties of the magnetic structures so obtained, such as symmetry stabilized topological textures and missing Bragg reflections are pointed out. The response of helical spin crystals to crystalline anisotropy, magnetic field and non-magnetic disorder are studied, with special reference to the bcc1 spin structure, a promising starting point for discussing the 'partial order' phases seen at high pressure in MnSi. Similar approaches may be applied to other crystallization problems such as Larkin-Ovchinnikov-Fulde-Ferrel states in spin-imbalanced superconductors.

cond-mat.str-el↗

arXiv2006

Theoretical proposal predicting anomalous magnetoresistance and quadratic Hall effect in the partially ordered state of MnSi

In [B. Binz, A. Vishwanath and V. Aji, Phys. Rev. Lett. 96, 207202 (2006)], a magnetic structure that breaks time reversal symmetry in the absence of net magnetization was proposed as an explanation for the high pressure "partially ordered" state of MnSi. Here we make explicit the anomalous magneto-transport properties of such a state: a magnetoresistivity which is linear and a Hall conductance which is quadratic in the applied magnetic field. Field cooling procedures for obtaining single domain samples are discussed. The anomalous effects are elaborated in the case of three geometries chosen to produce experimentally unambiguous signals of this unusual magnetic state; e.g., it is predicted that a field in z-direction induces an anisotropy in the x-y plane. Another geometry leads to a Hall voltage parallel to the magnetic field.

cond-mat.str-el↗