arXiv subjects

A. W. Rushforth

Publications and source records attributed to A. W. Rushforth.

At least 19 recordsLinked to original sources

arXiv2025

Unconventional relativistic spin polarization of electronic bands in an altermagnet

Altermagnetism is a recently identified phase with a d, g or i-wave spin symmetry of magnetic ordering. Its discovery opens new research fronts at intersections of magnetism and spintronics with fields ranging from superconductivity to topological and relativistic quantum physics. Here we demonstrate an unconventional relativistic spin polarization in an altermagnet by spin and angle resolved photoemission spectroscopy of electronic bands in single-domain MnTe. The relativistic spin-orbit coupling origin is revealed by observing that the alternating momentum-dependent spin polarization is orthogonal to the magnetic-ordering vector. The collinearity, even-parity and time-reversal-odd nature of the demonstrated relativistic spin polarization in the altermagnet is unparalleled in conventional forms of the relativistic spin polarization. Our experimental results and methodology are supported by non-relativistic spin-symmetry and relativistic magnetic-symmetry analyses, and microscopic ab initio ground-state and photoemission theory.

cond-mat.mes-hall↗

arXiv2024

Altermagnetism imaged and controlled down to the nanoscale

Nanoscale detection and control of the magnetic order underpins a broad spectrum of fundamental research and practical device applications. The key principle involved is the breaking of time-reversal ($\cal{T}$) symmetry, which in ferromagnets is generated by an internal magnetization. However, the presence of a net-magnetization also imposes severe limitations on compatibility with other prominent phases ranging from superconductors to topological insulators, as well as on spintronic device scalability. Recently, altermagnetism has been proposed as a solution to this restriction, since it shares the enabling $\cal{T}$-symmetry breaking characteristic of ferromagnetism, combined with the antiferromagnetic-like vanishing net-magnetization. To date, altermagnetic ordering has been inferred from spatially averaged probes. Here, we demonstrate nanoscale imaging and control of altermagnetic ordering ranging from nanoscale vortices to domain walls to microscale single-domain states in MnTe. We combine the $\cal{T}$-symmetry breaking sensitivity of X-ray magnetic circular dichroism with magnetic linear dichroism and photoemission electron microscopy, to achieve detailed imaging of the local altermagnetic ordering vector. A rich variety of spin configurations can be imposed using microstructure patterning or thermal cycling in magnetic fields. The demonstrated detection and control of altermagnetism paves the way for future research ranging from ultra-scalable digital and neuromorphic spintronic devices, to the interplay of altermagnetism with non-dissipative superconducting or topological phases.

cond-mat.mtrl-sci↗

arXiv2022

Transition magnon modes in thin ferromagnetic nanogratings

This work presents micromagnetic simulations in ferromagnetic nanogratings for the full range of directions of an applied in-plane external magnetic field. We focus on the modification of the magnon mode characteristics when the magnetic field orientation is gradually changed between the classical Damon-Eshbach (DE) and backward-volume (BV) geometries. We found that in a specific range of field directions, the magnon mode parameters differ significantly from the parameters in the classical cases, namely, the modes are characterized by complex spatial distributions and have low group velocities. The center of this range corresponds to the direction of the external magnetic field, which gives the maximal nonuniform distribution of the static magnetization in the nanogratings.

cond-mat.mes-hall↗

arXiv2022

Antiferromagnetic half-skyrmions electrically generated and controlled at room temperature

Topologically protected magnetic textures, such as skyrmions, half-skyrmions (merons) and their antiparticles, constitute tiny whirls in the magnetic order. They are promising candidates for information carriers in next-generation memory devices, as they can be efficiently propelled at very high velocities using current-induced spin torques. Antiferromagnets have been shown to host versions of these textures, which have gained significant attention because of their potential for terahertz dynamics, deflection free motion, and improved size scaling due to the absence of stray field. Here we show that topological spin textures, merons and antimerons, can be generated at room temperature and reversibly moved using electrical pulses in thin film CuMnAs, a semimetallic antiferromagnet that is a testbed system for spintronic applications. The electrical generation and manipulation of antiferromagnetic merons is a crucial step towards realizing the full potential of antiferromagnetic thin films as active components in high density, high speed magnetic memory devices.

cond-mat.other↗

arXiv2021

Spectrum evolution and chirping of laser-induced spin wave packets in thin iron films

We present the experimental study of ultrafast optical excitation of magnetostatic surface spin wave (MSSW) packets and their spectral properties in thin films of pure iron. As the packets leave the excitation area and propagate in space, their spectra evolve non-trivially. Particularly, low or high frequency components are suppressed at the border of the excitation area depending on the orientation of the external magnetic field with respect to the magnetocrystolline anisotropy axes of the film. The effect is ascribed to the ultrafast local heating of the film. Further, the time resolution of the implemented all-optical technique allows us to extract the chirp of the MSSW packet in the time domain via wavelet analysis. The chirp is a result of the group velocity dispersion of the MSSW and, thus, is controlled by the film magnetic parameters, magnetization and anisotropy, and external field orientation. The demonstrated tunable modulation of MSSW wave packets with femtosecond laser pulses may find application in future magnonic-photonic hybrid devices for wave-based data processing.

cond-mat.str-el↗

arXiv2021

Effect of magnetic anisotropy relaxation on laser-induced magnetization precession in thin galfenol films

The rate and pathways of relaxation of a magnetic medium to its equilibrium following excitation with intense and short laser pulses are the key ingredients of ultrafast optical control of spins. Here we study experimentally the evolution of the magnetization and magnetic anisotropy of thin films of a ferromagnetic metal galfenol (Fe$_{0.81}$Ga$_{0.19}$) resulting from excitation with a femtosecond laser pulse. From the temporal evolution of the hysteresis loops we deduce that the magnetization $M_S$ and magnetic anisotropy parameters $K$ recover within a nanosecond, and the ratio between $K$ and $M_S$ satisfies the thermal equilibrium's power law in the whole time range spanning from a few picoseconds to 3 nanoseconds. We further use the experimentally obtained relaxation times of $M_S$ and $K$ to analyze the laser-induced precession and demonstrate how they contribute to its frequency evolution at the nanosecond timescale.

cond-mat.mtrl-sci↗

arXiv2021

Spin flop and crystalline anisotropic magnetoresistance in CuMnAs

Recent research works have shown that the magnetic order in some antiferromagnetic materials can be manipulated and detected electrically, due to two physical mechanisms: Neel-order spin-orbit torques and anisotropic magnetoresistance. While these observations open up opportunities to use antiferromagnets for magnetic memory devices, different physical characterization methods are required for a better understanding of those mechanisms. Here we report a magnetic field induced rotation of the antiferromagnetic Neel vector in epitaxial tetragonal CuMnAs thin films. Using soft x-ray magnetic linear dichroism spectroscopy, x-ray photoemission electron microscopy, integral magnetometry and magneto-transport methods, we demonstrate spin-flop switching and continuous spin reorientation in antiferromagnetic films with uniaxial and biaxial magnetic anisotropies, respectively. From field-dependent measurements of the magnetization and magnetoresistance, we obtain key material parameters including the anisotropic magnetoresistance coefficients, magnetocrystalline anisotropy, spin-flop and exchange fields.

cond-mat.mtrl-sci↗

arXiv2021

Low-Energy Switching of Antiferromagnetic CuMnAs/ GaP Using sub-10 Nanosecond Current Pulses

The recently discovered electrical-induced switching of antiferromagnetic (AF) materials that have spatial inversion asymmetry has enriched the field of spintronics immensely and opened the door for the concept of antiferromagnetic MRAM. CuMnAs is one promising AF material that exhibits such electrical switching ability, and has been studied to switch using electrical pulses of length millisecond down to picosecond, but with little focus on nanosecond regime. We demonstrate here switching of CuMnAs/GaP using nanosecond pulses. Our results showed that in the nanosecond regime low-energy switching, high readout signal with highly reproducible behaviour down to a single pulse can be achieved. Moreover, a comparison of the two switching methods of orthogonal switching and polarity switching was done on same device showing two different behaviours that can be exploited selectively for different future memory/processing applications.

cond-mat.mtrl-sci↗

arXiv2018

Optical excitation of single- and multi-mode magnetization precession in Galfenol nanolayers

We demonstrate a variety of precessional responses of the magnetization to ultrafast optical excitation in nanolayers of Galfenol (Fe,Ga), which is a ferromagnetic material with large saturation magnetization and enhanced magnetostriction. The particular properties of Galfenol, including cubic magnetic anisotropy and weak damping, allow us to detect up to 6 magnon modes in a 120-nm layer, and a single mode with effective damping $α_{eff}$ = 0.005 and frequency up to 100 GHz in a 4-nm layer. This is the highest frequency observed to date in time-resolved experiments with metallic ferromagnets. We predict that detection of magnetization precession approaching THz frequencies should be possible with Galfenol nanolayers.

cond-mat.mes-hall↗

arXiv2018

Optically driven spin pumping mediating collective magnetization dynamics in a spin valve structure

We demonstrate spin pumping, i.e. the generation of a pure spin current by precessing magnetization, without application of microwave radiation commonly used in spin pumping experiments. We use femtosecond laser pulses to simultaneously launch the magnetization precession in each of two ferromagnetic layers of a Galfenol-based spin valve and monitor the temporal evolution of the magnetizations. The spin currents generated by the precession cause a dynamic coupling of the two layers. This coupling has dissipative character and is especially efficient when the precession frequencies in the two layers are in resonance, where coupled modes with strongly different decay rates are formed.

cond-mat.mes-hall↗

arXiv2018

Negative spin-Hall angle and anisotropic spin-orbit torques in epitaxial IrMn

A spin-torque ferromagnetic resonance study is performed in epitaxial $\mathrm{Fe / Ir_{15}Mn_{85}}$ bilayers with different Fe thicknesses. We measure a negative spin-Hall angle of a few percent in the antiferromagnetic IrMn in contrast to previously reported positive values. A large spin-orbit field with Rashba symmetry opposing the Oersted field is also present. Magnitudes of measured spin-orbit torques depend on the crystallographic direction of current and are correlated with the exchange bias direction set during growth. We suggest that the uncompensated moments at the Fe / IrMn interface are responsible for the observed anisotropy. Our findings highlight the importance of crystalline and magnetic structures for the spin-Hall effect in antiferromagnets.

cond-mat.mes-hall↗

arXiv2017

Generation of a localized microwave magnetic field by coherent phonons in a ferromagnetic nanograting

A high-amplitude microwave magnetic field localized at the nanoscale is a desirable tool for various applications within the rapidly developing field of nanomagnetism. Here, we drive magnetization precession by coherent phonons in a metal ferromagnetic nanograting and generate ac-magnetic induction with extremely high amplitude (up to $10$ mT) and nanometer scale localization in the grating grooves. We trigger the magnetization by a laser pulse which excites localized surface acoustic waves. The developed technique has prospective uses in several areas of research and technology, including spatially resolved access to spin states for quantum technologies.

cond-mat.mes-hall↗

arXiv2017

The effect of dynamical compressive and shear strain on magnetic anisotropy in low symmetry ferromagnetic film

Dynamical strain generated upon excitation of a metallic film by a femtosecond laser pulse may become a versatile tool enabling control of magnetic state of thin films and nanostructures via inverse magnetostriction on a picosecond time scale. Here we explore two alternative approaches to manipulate magnetocrystalline anisotropy and excite magnetization precession in a low-symmetry film of a magnetic metallic alloy galfenol (Fe,Ga) either by injecting picosecond strain pulse into it from a substrate or by generating dynamical strain of complex temporal profile in the film directly. In the former case we realize ultrafast excitation of magnetization dynamics solely by strain pulses. In the latter case optically-generated strain emerged abruptly in the film modifies its magnetocrystalline anisotropy, competing with heat-induced change of anisotropy parameters. We demonstrate that the optically-generated strain remains efficient for launching magnetization precession, when the heat-induced changes of anisotropy parameters do not trigger the precession anymore. We emphasize that in both approaches the ultrafast change of magnetic anisotropy mediating the precession excitation relies on mixed, compressive and shear, character of the dynamical strain, which emerges due to low-symmetry of the metallic film under study.

cond-mat.mes-hall↗

arXiv2017

Effect of lithographically-induced strain relaxation on the magnetic domain configuration in microfabricated epitaxially grown Fe81Ga19

We investigate the role of lithographically-induced strain relaxation in a micron-scaled device fabricated from epitaxial thin films of the magnetostrictive alloy Fe81Ga19. The strain relaxation due to lithographic patterning induces a magnetic anisotropy that competes with the magnetocrystalline and shape induced anisotropies to play a crucial role in stabilising a flux-closing domain pattern. We use magnetic imaging, micromagnetic calculations and linear elastic modelling to investigate a region close to the edges of an etched structure. This highly-strained edge region has a significant influence on the magnetic domain configuration due to an induced magnetic anisotropy resulting from the inverse magnetostriction effect. We investigate the competition between the strain-induced and shape-induced anisotropy energies, and the resultant stable domain configurations, as the width of the bar is reduced to the nanoscale range. Understanding this behaviour will be important when designing hybrid magneto-electric spintronic devices based on highly magnetostrictive materials.

cond-mat.mes-hall↗

arXiv2016

Precise tuning of the Curie temperature of (Ga,Mn)As-based magnetic semiconductors by hole compensation: Support for valence-band ferromagnetism

For the prototype diluted ferromagnetic semiconductor (Ga,Mn)As, there is a fundamental concern about the electronic states near the Fermi level, i.e., whether the Fermi level resides in a well-separated impurity band derived from Mn doping (impurity-band model) or in the valence band that is already merged with the Mn-derived impurity band (valence-band model). We investigate this question by carefully shifting the Fermi level by means of carrier compensation. We use helium-ion implantation, a standard industry technology, to precisely compensate the hole doping of GaAs-based diluted ferromagnetic semiconductors while keeping the Mn concentration constant. We monitor the change of Curie temperature ($T_C$) and conductivity. For a broad range of samples including (Ga,Mn)As and (Ga,Mn)(As,P) with various Mn and P concentrations, we observe a smooth decrease of $T_C$ with carrier compensation over a wide temperature range while the conduction is changed from metallic to insulating. The existence of $T_C$ below 10\,K is also confirmed in heavily compensated samples. Our experimental results are naturally explained within the valence-band picture.

cond-mat.mtrl-sci↗

arXiv2015

Resonant driving of magnetization precession in a ferromagnetic layer by coherent monochromatic phonons

We realize resonant driving of the magnetization precession by monochromatic phonons in a thin ferromagnetic layer embedded into a phononic Fabry-Perot resonator. A femtosecond laser pulse excites resonant phonon modes of the structure in the 10-40 GHz frequency range. By applying an external magnetic field, we tune the precession frequency relative to the frequency of the phonons localized in the cavity and observe the enormous increase in the amplitude of the magnetization precession when the frequencies of free magnetization precession and phonons localized in the cavity are equal.

cond-mat.mes-hall↗

arXiv2015

Modification of perpendicular magnetic anisotropy and domain wall velocity in Pt/Co/Pt by voltage-induced strain

The perpendicular magnetic anisotropy K$_e$$_f$$_f$, magnetization reversal, and field-driven domain wall velocity in the creep regime are modified in Pt/Co(0.85-1.0 nm)/Pt thin films by strain applied via piezoelectric transducers. K$_e$$_f$$_f$, measured by the extraordinary Hall effect, is reduced by 10 kJ/m$^3$ by tensile strain out-of-plane ε$_z$ = 9 x 10-4, independently of the film thickness, indicating a dominant volume contribution to the magnetostriction. The same strain reduces the coercive field by 2-4 Oe, and increases the domain wall velocity measured by wide-field Kerr microscopy by 30-100 %, with larger changes observed for thicker Co layers. We consider how strain-induced changes in the perpendicular magnetic anisotropy can modify the coercive field and domain wall velocity.

cond-mat.mes-hall↗

arXiv2014

Spin-dependent phenomena and device concepts explored in (Ga,Mn)As

Over the past two decades, the research of (Ga,Mn)As has led to a deeper understanding of relativistic spin-dependent phenomena in magnetic systems. It has also led to discoveries of new effects and demonstrations of unprecedented functionalities of experimental spintronic devices with general applicability to a wide range of materials. In this article we review the basic material properties that make (Ga,Mn)As a favorable test-bed system for spintronics research and discuss contributions of (Ga,Mn)As studies in the general context of the spin-dependent phenomena and device concepts. Special focus is on the spin-orbit coupling induced effects and the reviewed topics include the interaction of spin with electrical current, light, and heat.

cond-mat.mtrl-sci↗