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Abhijit Biswas

Publications and source records attributed to Abhijit Biswas.

At least 19 recordsLinked to original sources

Adaptive Diagonally Implicit Runge-Kutta Methods Devoid of Order Reduction for Semilinear ODEs

Diagonally implicit Runge-Kutta (DIRK) methods are a prominent class of numerical methods for solving stiff systems of ordinary differential equations (ODEs). Stiffness does not only impose stability challenges on Runge-Kutta methods; it can also degrade the order of convergence. This so-called order reduction phenomenon occurs when assumptions used for classical convergence analysis, e.g., an asymptotically small step size, fail to hold. In a prior paper by the authors, sharp order conditions and global error bounds for Runge-Kutta methods were developed, which hold uniformly with respect to stiffness when applied to a wide class of semilinear ODEs. In this work, those conditions are leveraged to construct the first DIRK methods of order four and five which satisfy these conditions and thus do not exhibit order reduction. Numerical results demonstrate that for a broad class of relevant nonlinear test problems, these new methods successfully mitigate order reduction, accurately estimate local error via an embedding for adaptive step size control, and can outperform classical DIRK methods.

math.NA

Diamond-to-graphite transformation under hypersonic impact

Diamond to graphite transformation is a complex kinetically driven process which has been studied under various conditions for its fundamental importance. We report the transformation of diamond embedded ceramic matrix composites during hypersonic impact. Diamond particles embedded in cubic boron nitride matrix provide a superhard composite that was subjected to high impact collisions of metal projectiles travelling at speeds reaching Mach 8.45. Our observations suggest that the energy absorption and fracture of the composite is primarily enabled via the phase change of diamond into graphite. Characterization of the impact-fractured composite shows transformed diamond particles and provides details of the shock-induced phase transformation and the nature of diamond-graphite interfaces formed during rapid phase change. The study provides new understanding of phase transformation of diamond under extreme conditions.

cond-mat.mtrl-sci

A Stiff Order Condition Theory for Runge-Kutta Methods Applied to Semilinear ODEs

Classical convergence theory of Runge-Kutta methods assumes that the time step is small relative to the Lipschitz constant of the ordinary differential equation (ODE). For stiff problems, that assumption is often violated, and a problematic degradation in accuracy, known as order reduction, can arise. Methods with high stage order, e.g., Gauss-Legendre and Radau, are known to avoid order reduction, but they must be fully implicit. For the broad class of semilinear ODEs, which consist of a stiff linear term and non-stiff nonlinear term, we show that weaker conditions suffice. Our new semilinear order conditions are formulated in terms of orthogonality relations and can be enumerated by rooted trees. Finally, we prove global error bounds that hold uniformly with respect to stiffness of the linear term.

math.NA

Optical spin defect pairs in cubic boron nitride

Room-temperature optically active solid-state spin defects are widely known to be useful in quantum sensing applications, however, only a select range of materials have been found to host such systems. Recent measurements in the van der Waals material hexagonal boron nitride (hBN) have shown optically detected magnetic resonance (ODMR) with spin-1/2-like signatures can be explained by a charge transfer mechanism where charges move between adjacent defects forming weakly coupled spin pairs. Interestingly, these ODMR signatures have been reported in a variety of materials aside from hBN, suggesting the spin pair model provides a potentially material agnostic approach for enabling ODMR. Here, we test whether the charge transfer mechanism is supported in a different crystal phase, and report on ODMR signatures in cubic boron nitride (cBN), showing all the characteristic properties identified in hBN are preserved. We consider a selection of different cBN samples of varying size and observe ODMR from a single sub-micron cBN particle, paving the way towards sensing applications. This work further expands understanding of the ubiquity of optical spin defect pairs, and establishes the potential for exploring quantum technologies with a wider range of materials.

cond-mat.mes-hall

Exploring the Anomalous Nernst Effect in SrRuO$_3$

We investigate the anomalous Nernst effect in epitaxial SrRuO$_3$ thin films grown on c-cut Al$_2$O$_3$ substrates, and in a polycrystalline SrRuO$_3$ slab. Through comprehensive measurements of the transverse thermoelectric response as a function of temperature and magnetic field, we observe a pronounced Nernst signal near $T_c$ in the (111) oriented SrRuO$_3$ thin films. The strong temperature and nontrivial field dependence underscore the pivotal role of the magnetic anisotropy in tuning the Berry curvature and, consequently, the anomalous Nernst effect in SrRuO$_3$.

cond-mat.str-el

Asymptotic-preserving and energy-conserving methods for a hyperbolic approximation of the BBM equation

We study the hyperbolic approximation of the Benjamin-Bona-Mahony (BBM) equation proposed recently by Gavrilyuk and Shyue (2022). We develop asymptotic-preserving numerical methods using implicit-explicit (additive) Runge-Kutta methods that are implicit in the stiff linear part. The new discretization of the hyperbolization conserves important invariants converging to invariants of the BBM equation. We use the entropy relaxation approach to make the fully discrete schemes energy-preserving. Numerical experiments demonstrate the effectiveness of these discretizations.

math.NA

Cavity Enhanced Emission from Telecom Rare-Earth System in Colloidal Host

Erbium incorporated in a ceria (CeO2) host offers strong potential as a spin qubit platform, providing a pathway toward telecom-compatible quantum memory. But erbium is a dim emitter due to its long excited state lifetime. Methods to enhance its emission rate and efficiency through nanophotonic cavity integration are therefore essential. In this work, we demonstrate cavity-enhanced emission from erbium doped CeO2. We couple colloidally synthesized erbium doped CeO2 nanocrystals to a silicon nanobeam cavity and show a 30-fold improvement in emitter brightness combined with a 2-fold lifetime enhancement. We estimate a lower bound of 12 for the Purcell factor of cavity-coupled emitters after accounting for non-radiative decay. These results pave the way towards utilizing colloidally synthesized optically addressable spin qubits emitting at telecom wavelength for quantum networking and distributed quantum computing.

physics.optics

Traveling-wave solutions and structure-preserving numerical methods for a hyperbolic approximation of the Korteweg-de Vries equation

We study the recently-proposed hyperbolic approximation of the Korteweg-de Vries equation (KdV). We show that this approximation, which we call KdVH, possesses a rich variety of solutions, including solitary wave solutions that approximate KdV solitons, as well as other solitary and periodic solutions that are related to higher-order water wave models, and may include singularities. We analyze a class of implicit-explicit Runge-Kutta time discretizations for KdVH that are asymptotic preserving, energy conserving, and can be applied to other hyperbolized systems. We also develop structure-preserving spatial discretizations based on summation-by-parts operators in space including finite difference, discontinuous Galerkin, and Fourier methods. We use the entropy relaxation approach to make the fully discrete schemes energy-preserving. Numerical experiments demonstrate the effectiveness of these discretizations.

math.NA

A Hyperbolic Approximation of the Nonlinear Schrödinger Equation

We study a first-order hyperbolic approximation of the nonlinear Schrödinger (NLS) equation. We show that the system is strictly hyperbolic and possesses a modified Hamiltonian structure, along with at least three conserved quantities that approximate those of NLS. We provide families of explicit standing-wave solutions to the hyperbolic system, which are shown to converge uniformly to ground-state solutions of NLS in the relaxation limit. The system is formally equivalent to NLS in the relaxation limit, and we develop asymptotic preserving discretizations that tend to a consistent discretization of NLS in that limit, while also conserving mass. Examples for both the focusing and defocusing regimes demonstrate that the numerical discretization provides an accurate approximation of the NLS solution.

math.AP

Anomalous properties of spark plasma sintered boron nitride solids

Hexagonal boron nitride (h-BN) is a brittle ceramic with a layered structure, however, recent experiments have suggested that inter-layer structural engineering could be key to new structural and functional properties. Here we report the scalable bulk synthesis of high-density crystalline h-BN solids, by using high-temperature spark plasma sintering (SPS) of h-BN powders, which show high values of mechanical strength, ductility, dielectric constant, thermal conductivity, and exceptional neutron radiation shielding capability. Through exhaustive characterizations we reveal that SPS induces non-basal plane crystallinity, twisting of layers, and facilitates inter-grain fusion with a high degree of in-plane alignment across macroscale dimensions, resulting in near-theoretical density and improved properties. Our findings highlight the importance of material design, via new approaches such as layer twisting and interlayer interconnections, to create novel ceramics with properties that could go beyond their intrinsic limits.

cond-mat.mtrl-sci

Approximation of arbitrarily high-order PDEs by first-order hyperbolic relaxation

We present a framework for constructing a first-order hyperbolic system whose solution approximates that of a desired higher-order evolution equation. Constructions of this kind have received increasing interest in recent years, and are potentially useful as either analytical or computational tools for understanding the corresponding higher-order equation. We perform a systematic analysis of a family of linear model equations and show that for each member of this family there is a stable hyperbolic approximation whose solution converges to that of the model equation in a certain limit. We then show through several examples that this approach can be applied successfully to a very wide range of nonlinear PDEs of practical interest.

math.AP

Room-Temperature High-Purity Single Photon Emission from Carbon-Doped Boron Nitride Thin Films

Hexagonal boron nitride (hBN) has emerged as an excellent host material for generating room temperature single photons exhibiting high brightness and spin-photon entanglement. However, challenges in improving purity, stability, and scalability limit its use in quantum technologies. Here, we demonstrate highly pure and stable single photon emitters (SPEs) in hBN by directly growing carbon-doped, centimeter-scale hBN thin films using the pulsed laser deposition (PLD) method. These SPEs exhibit room temperature operation with polarized emission, achieving a g(2)(0) value of 0.015, which is among the lowest reported for room temperature SPEs and the lowest achieved for hBN SPEs. It also exhibits high brightness ( around 0.5 million counts per second), remarkable stability during continuous operation (> 15 minutes), and a Debye-Waller factor of 45%. First-principles calculations reveal unique carbon defects responsible for these properties, enabled by PLD's low-temperature synthesis and in-situ doping. Our results demonstrate an effective method for large-scale production of high-purity, stable SPEs in hBN, enabling robust quantum optical sources for various applications.

physics.app-ph

Dynamically Encircled Higher-order Exceptional Points in an Optical Fiber

The unique properties of exceptional point (EP) singularities, arising from non-Hermitian physics, have unlocked new possibilities for manipulating light-matter interactions. A tailored gain-loss variation, while encircling higher-order EPs dynamically, can significantly enhance the control of the topological flow of light in multi-level photonic systems. In particular, the integration of dynamically encircled higher-order EPs within fiber geometries holds remarkable promise for advancing specialty optical fiber applications, though a research gap remains in exploring and realizing such configurations. Here, we report a triple-core specialty optical fiber engineered with customized loss and gain to explore the topological characteristics of a third-order exceptional point (EP3), formed by two interconnected second-order exceptional points (EP2s). We elucidate chiral and nonchiral light transmission through the fiber, grounded in second- and third-order branch point behaviors and associated adiabatic and nonadiabatic modal characteristics, while considering various dynamical parametric loops to encircle the embedded EPs. We investigate the persistence of EP-induced light dynamics specifically in the parametric regions immediately adjacent to, though not encircling, the embedded EPs, potentially leading to improved device performance. Our findings offer significant implications for the design and implementation of novel light management technologies in all-fiber photonics and communications.

physics.optics

Algebraic Structure of the Weak Stage Order Conditions for Runge-Kutta Methods

Runge-Kutta (RK) methods may exhibit order reduction when applied to stiff problems. For linear problems with time-independent operators, order reduction can be avoided if the method satisfies certain weak stage order (WSO) conditions, which are less restrictive than traditional stage order conditions. This paper outlines the first algebraic theory of WSO, and establishes general order barriers that relate the WSO of a RK scheme to its order and number of stages for both fully-implicit and DIRK schemes. It is shown in several scenarios that the constructed bounds are sharp. The theory characterizes WSO in terms of orthogonal invariant subspaces and associated minimal polynomials. The resulting necessary conditions on the structure of RK methods with WSO are then shown to be of practical use for the construction of such schemes.

math.NA

Non-linear optics at twist interfaces in h-BN/SiC heterostructures

Understanding the emergent electronic structure in twisted atomically thin layers has led to the exciting field of twistronics. However, practical applications of such systems are challenging since the specific angular correlations between the layers must be precisely controlled and the layers have to be single crystalline with uniform atomic ordering. Here, we suggest an alternative, simple and scalable approach where nanocrystalline two-dimensional (2D) film on three-dimensional (3D) substrates yield twisted-interface-dependent properties. Ultrawide-bandgap hexagonal boron nitride (h-BN) thin films are directly grown on high in-plane lattice mismatched wide-bandgap silicon carbide (4H-SiC) substrates to explore the twist-dependent structure-property correlations. Concurrently, nanocrystalline h-BN thin film shows strong non-linear second-harmonic generation and ultra-low cross-plane thermal conductivity at room temperature, which are attributed to the twisted domain edges between van der Waals stacked nanocrystals with random in-plane orientations. First-principles calculations based on time-dependent density functional theory manifest strong even-order optical nonlinearity in twisted h-BN layers. Our work unveils that directly deposited 2D nanocrystalline thin film on 3D substrates could provide easily accessible twist-interfaces, therefore enabling a simple and scalable approach to utilize the 2D-twistronics integrated in 3D material devices for next-generation nanotechnology.

cond-mat.mtrl-sci

Unravelling the room temperature growth of two-dimensional h-BN nanosheets for multifunctional applications

Room temperature growth of two-dimensional van der Waals (2D-vdW) materials is indispensable for state-of-the-art nanotechnology. The low temperature growth supersedes the requirement of elevated growth temperature accompanied with high thermal budgets. Moreover, for electronic applications, low or room temperature growth reduces the possibility of intrinsic film-substrate interfacial thermal diffusion related deterioration of functional properties and consequent device performance. Here, we demonstrated the growth of ultrawide-bandgap boron nitride (BN) at room temperature by using the pulsed laser deposition (PLD) process and demonstrated various functionalities for potential applications. Comprehensive chemical, spectroscopic and microscopic characterization confirms the growth of ordered nanosheet-like hexagonal BN. Functionally, nanosheets show hydrophobicity, high lubricity (low coefficient of friction), low refractive index within the visible to near-infrared wavelength range, and room temperature single-photon quantum emission. Our work unveils an important step that brings a plethora of applications potential for room temperature grown h-BN nanosheets as it can be feasible on any given substrate, thus creating a scenario for h-BN on demand at frugal thermal budget.

physics.app-ph

Explicit Runge Kutta Methods that Alleviate Order Reduction

Explicit Runge--Kutta (RK) methods are susceptible to a reduction in the observed order of convergence when applied to initial-boundary value problem with time-dependent boundary conditions. We study conditions on explicit RK methods that guarantee high-order convergence for linear problems; we refer to these conditions as weak stage order conditions. We prove a general relationship between the method's order, weak stage order, and number of stages. We derive explicit RK methods with high weak stage order and demonstrate, through numerical tests, that they avoid the order reduction phenomenon up to any order for linear problems and up to order three for nonlinear problems.

math.NA

Structural, optical, and thermal properties of BN thin films grown on diamond via pulsed laser deposition

Heterostructures based on ultrawide-bandgap (UWBG) semiconductors (bandgap >4.0 eV), boron nitride (BN) and diamond are important for next-generation high-power electronics. However, in-situ hetero-epitaxy of BN/diamond or vice-versa remains extremely challenging, due to their non-trivial growth kinetics. Here, we have grown BN thin film on (100) single crystal diamond by pulsed laser deposition and investigated its structural and magnetic properties, optical refractive index, and thermal conductivity. Structural characterizations confirm the mixed (stable hexagonal and metastable cubic) phase growth. Film shows diamagnetic behavior at room temperature. It displays anisotropic refractive index within the visible-to-near-infrared wavelength range. The room temperature cross-plane thermal conductivity of BN is ~1.53 W/(mK), and the thermal conductance of the BN/diamond interface is ~20 MW/(m2K). Our findings are useful for various device related applications based on UWBG BN/diamond heterostructures.

physics.app-ph