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Adrian Bachtold

Publications and source records attributed to Adrian Bachtold.

At least 19 recordsLinked to original sources

Current-based RF charge sensing in a carbon nanotube

Ultra-sensitive charge detection is a widely used tool for quantum electronics with applications in quantum information processing and in probing the physics of condensed matter systems. Existing approaches require either an impedance-matched resonant circuit, or millimeter-scale proximity between amplifier and sample, both adding complexity and constraining device design. In this work, we introduce a current-mode charge sensor in a suspended carbon nanotube, operating at the $1.25$ MHz resonance of an RLC tank circuit and achieving a charge sensitivity of $0.15~μe/\sqrt{\mathrm{Hz}}$. We utilize it to measure a double quantum dot (DQD) electrostatically defined in the same nanotube, revealing a highly regular charge stability diagram. We perform single-shot readout of the DQD charge state at an integration time of $3.56~μ\mathrm{s}$, without any false assignments over $10^{7}$ measurements and a signal-to-noise ratio of 17 exceeding the state of the art.

cond-mat.mes-hall

Tunable nonlinear electromechanics at the zero-point motion scale

Nonlinearity at the scale of zero-point motion opens new possibilities for the control and readout of nanomechanical systems, but achieving this remains a formidable challenge. Here we demonstrate that ultrastrong coupling (USC) between a nanotube mechanical oscillator and a double-quantum-dot electronic two-level system enables a mechanical Kerr (Duffing) nonlinearity at the zero-point motion scale. In the dispersive regime, this large coupling yields a mechanical anharmonicity of $α= 1.4\%$ - three orders of magnitude larger than in previous work - while preserving the predominantly mechanical nature of the lowest energy states. We further demonstrate a purely quadratic cavity-based continuous readout of the mechanical motion. This continuous nonlinear optomechanical readout is enforced by a double-quantum dot symmetry, which can be broken by gate tuning to introduce a large linear transduction. These results establish a tunable USC platform that enables strong mechanical anharmonicity and nonlinear continuous readout at the zero-point motion scale.

quant-ph

Imaging superconducting weak spots through vortex-assisted THz near-field photovoltage

Nanoscale inhomogeneities are a defining feature of many superconducting materials, yet their local electromagnetic response has remained difficult to access experimentally. This is because their relevant energy scale lies in the terahertz range, where wavelengths -- on the order of hundreds of microns -- are too large to spatially resolve nanoscopic variations. Here, we demonstrate the first application of THz near-field photovoltage nanoscopy in a superconductor, achieving 300 nm spatial resolution at 2.52 THz. Scanning a current-biased NbN strip, we reveal photovoltage peaks within the bulk associated with nanoscopic defects of reduced superfluid density. The observed photovoltage follows the evolution of the vortex-dissipative state and is attributed to enhanced vortex-antivortex pair nucleation at defect sites. Together, these results open a direct route to probing how material inhomogeneities influence light-matter interactions in superconductors, with implications for superconducting devices and strongly inhomogeneous systems such as high-Tc and moiré materials.

cond-mat.supr-con

Emergent Bell Phase in an Electro-Nanomechanical Quantum Simulator

Suspended carbon nanotubes hosting electrostatically defined quantum dots allow for exceptionally strong and tunable electromechanical coupling as well as mechanical modes that can reach the quantum ground state of motion simply by cryogenic cooling. This makes them a unique platform for quantum simulation of electron-phonon coupling. Here, we propose an experimentally realisable setup with two such carbon nanotubes in parallel, each hosting four quantum dots. Our system not only exhibits phonon-mediated electron-electron attraction, but also supports a robust, maximally entangled Bell phase at mesoscopic scales shared across the subsystems. These features highlight its potential as a simulator of strongly correlated quantum systems.

quant-ph

Coherent Thermal Emission from Large-Scale Suspended Nanomechanical Membranes

Thermal radiation is an abundant form of incoherent light. Generating coherent infrared light through incandescence promises a cheap alternative to the costly and epitaxially complex quantum cascade laser, however it remains a fundamental challenge. Previous approaches leveraged the spatial coherence of polaritonic excitations that occur in the thermal near-field, by diffracting them into the far-field zone via patterned micro- or nano-scatterers. This approach requires high-resolution lithography, is difficult to scale-up, and yields limited outcoupled radiation due to the intrinsically polarized nature of polaritons. We overcome these limitations and report coherent thermal emission through simple wave interference. We show that unpatterned, millimeter-scale, suspended nanomechanical membranes of SiC operate for both linear polarizations and exhibit antenna-like directionality without relying on the excitation of near-field polaritons. The ability to generate polarization-insensitive, narrowband and spatially coherent incandescent light without lithography at large scales paves the way towards democratizing thermal infrared technologies.

physics.optics

Giant ultra-broadband photoconductivity in twisted graphene heterostructures

The requirements for broadband photodetection are becoming exceedingly demanding in hyperspectral imaging. Whilst intrinsic photoconductor arrays based on mercury cadmium telluride represent the most sensitive and suitable technology, their optical spectrum imposes a narrow spectral range with a sharp absorption edge that cuts their operation to < 25 um. Here, we demonstrate a giant ultra-broadband photoconductivity in twisted double bilayer graphene heterostructures spanning a spectral range of 2 - 100 um with internal quantum efficiencies ~ 40 % at speeds of 100 kHz. The giant response originates from unique properties of twist-decoupled heterostructures including pristine, crystal field induced terahertz band gaps, parallel photoactive channels, and strong photoconductivity enhancements caused by interlayer screening of electronic interactions by respective layers acting as sub-atomic spaced proximity screening gates. Our work demonstrates a rare instance of an intrinsic infrared-terahertz photoconductor that is complementary metal-oxide-semiconductor compatible and array integratable, and introduces twist-decoupled graphene heterostructures as a viable route for engineering gapped graphene photodetectors with 3D scalability.

cond-mat.mes-hall

Steady-state Peierls transition in nanotube quantum simulator

Quantum dots placed along a vibrating nanotube provide a quantum simulation platform that can directly address the electron-phonon interaction. This offers promising prospects for the search of new quantum materials and the study of strong correlation effects. As this platform is naturally operated by coupling the dots to an electronic reservoir, state preparation is straightforwardly achieved by driving into the steady state. Here we show that for intermediate electron-phonon coupling strength, the system with spin-polarized quantum dots undergoes a Peierls transition into an insulating regime which exhibits charge-density wave order in the steady state as a consequence of the competition between electronic Coulomb repulsive interactions and phonon-induced attractive interactions. The transport phenomena can be directly observed as fingerprints of electronic correlations. We also present powerful methods to numerically capture the physics of such an open electron-phonon system at large numbers of phonons. Our work paves the way to study and detect correlated electron-phonon physics in the nanotube quantum simulator with current experimentally accessible techniques.

cond-mat.str-el

Engineering high quality graphene superlattices via ion milled ultra-thin etching masks

Nanofabrication research pursues the miniaturization of patterned feature size. In the current state of the art, micron scale areas can be patterned with features down to ~ 30 nm pitch using electron beam lithography. Our work demonstrates a new nanofabrication technique which allows patterning periodic structures with a pitch down to 16 nm. It is based on focused ion beam milling of suspended membranes, with minimal proximity effects typical to electron beam lithography. The membranes are then transferred and used as hard etching masks. We benchmark our technique by engineering a superlattice potential in single layer graphene using a thin graphite patterned gate electrode. Our electronic transport characterization shows high quality superlattice properties and a rich Hofstadter butterfly spectrum. Our technique opens the path towards the realization of very short period superlattices in 2D materials, comparable to those in natural moire systems, but with the ability to control lattice symmetries and strength. This can pave the way for a versatile solid-state quantum simulator platform and the study of correlated electron phases.

cond-mat.mes-hall

Nanomechanical Resonators: Toward Atomic Scale

The quest for realizing and manipulating ever smaller man-made movable structures and dynamical machines has spurred tremendous endeavors, led to important discoveries, and inspired researchers to venture to new grounds. Scientific feats and technological milestones of miniaturization of mechanical structures have been widely accomplished by advances in machining and sculpturing ever shrinking features out of bulk materials such as silicon. With the flourishing multidisciplinary field of low-dimensional nanomaterials, including one-dimensional (1D) nanowires/nanotubes, and two-dimensional (2D) atomic layers such as graphene/phosphorene, growing interests and sustained efforts have been devoted to creating mechanical devices toward the ultimate limit of miniaturization--genuinely down to the molecular or even atomic scale. These ultrasmall movable structures, particularly nanomechanical resonators that exploit the vibratory motion in these 1D and 2D nano-to-atomic-scale structures, offer exceptional device-level attributes, such as ultralow mass, ultrawide frequency tuning range, broad dynamic range, and ultralow power consumption, thus holding strong promises for both fundamental studies and engineering applications. In this Review, we offer a comprehensive overview and summary of this vibrant field, present the state-of-the-art devices and evaluate their specifications and performance, outline important achievements, and postulate future directions for studying these miniscule yet intriguing molecular-scale machines.

cond-mat.mes-hall

Mesoscopic physics of nanomechanical systems

Nanomechanics has brought mesoscopic physics into the world of vibrations. Because nanomechanical systems are small, fluctuations are significant, the vibrations become nonlinear already for comparatively small amplitudes, and new mechanisms of dissipation come into play. At the same time, the exquisite control of these systems makes them a platform for studying many problems of classical and quantum physics far from thermal equilibrium in a well-characterized setting. This review describes, at a conceptual level, basic theoretical ideas and explicative experiments pertaining to mesoscopic physics of nanomechanical systems. Major applications of nanomechanics in science and technology are also outlined. A broad range of phenomena related to the conservative as well as dissipative nonlinearity and fluctuations are discussed within a unifying framework. They include the linear response of single and coupled vibrational modes as well as nonlinear effects of periodic driving. Such driving breaks the continuous time-translation symmetry and the detailed balance, with conspicuous consequences for fluctuations, particularly in the presence of the driving-induced bi- and multistability. Mathematical techniques are described in the appendices to streamline the reading, but also to provide an introduction to the theory. The goal of the review is to show the richness of the physics at work. The continuous experimental and theoretical advances make nanomechanical systems a vibrant area of research, with many new phenomena to discover.

cond-mat.mes-hall

Phonon-induced pairing in quantum dot quantum simulator

Quantum simulations can provide new insights into the physics of strongly correlated electronic systems. A well studied system, but still open in many regards, is the Hubbard-Holstein Hamiltonian, where electronic repulsion is in competition with attraction generated by the electron-phonon coupling. In this context we study the phase diagram of four quantum dots in a suspended carbon nanotube and coupled to its flexural degrees of freedom. The system is described by a Hamiltonian of the Hubbard-Holstein class, where electrons on different sites interact with the same phonon. We find that the system presents a transition from the Mott insulating state to a polaronic state, with the appearance of pairing correlations and the breaking of the translational symmetry. Our study shows that this system thus constitutes a relevant example of a correlated system that could be studied by experimental realization.

cond-mat.str-el

Optomechanical measurement of thermal transport in two-dimensional MoSe2 lattices

Nanomechanical resonators have emerged as sensors with exceptional sensitivities. These sensing capabilities open new possibilities in the studies of the thermodynamic properties in condensed matter. Here, we use mechanical sensing as a novel approach to measure the thermal properties of low-dimensional materials. We measure the temperature dependence of both the thermal conductivity and the specific heat capacity of a transition metal dichalcogenide (TMD) monolayer down to cryogenic temperature, something that has not been achieved thus far with a single nanoscale object. These measurements show how heat is transported by phonons in two-dimensional systems. Both the thermal conductivity and the specific heat capacity measurements are consistent with predictions based on first-principles.

cond-mat.mes-hall

Layering transitions in superfluid helium adsorbed on a carbon nanotube mechanical resonator

Helium is recognized as a model system for the study of phase transitions. Of particular interest is the superfluid phase in two dimensions. We report measurements on superfluid helium films adsorbed on the surface of a suspended carbon nanotube. We measure the mechanical vibrations of the nanotube to probe the adsorbed helium film. We demonstrate the formation of helium layers up to five atoms thickness. Upon increasing the vapour pressure, we observe layer-by-layer growth with discontinuities in both the number of adsorbed atoms and the speed of sound in the adsorbed film. These hitherto unobserved discontinuities point to a series of first-order layering transitions. Our results show that helium multilayers adsorbed on a nanotube are of unprecedented quality compared to previous works. They pave the way to new studies of quantized superfluid vortex dynamics on cylindrical surfaces, of the Berezinskii-Kosterlitz-Thouless phase transition in this new geometry, perhaps also to supersolidity in crystalline single layers as predicted in quantum Monte Carlo calculations.

cond-mat.mes-hall

Superconductors, Orbital Magnets, and Correlated States in Magic Angle Bilayer Graphene

Superconductivity often occurs close to broken-symmetry parent states and is especially common in doped magnetic insulators. When twisted close to a magic relative orientation angle near 1 degree, bilayer graphene has flat moire superlattice minibands that have emerged as a rich and highly tunable source of strong correlation physics, notably the appearance of superconductivity close to interaction-induced insulating states. Here we report on the fabrication of bilayer graphene devices with exceptionally uniform twist angles. We show that the reduction in twist angle disorder reveals insulating states at all integer occupancies of the four-fold spin/valley degenerate flat conduction and valence bands, i.e. at moire band filling factors nu = 0, +(-) 1, +(-) 2, +(-) 3, and superconductivity below critical temperatures as high as 3 K close to - 2 filling. We also observe three new superconducting domes at much lower temperatures close to the nu = 0 and nu = +(-) 1 insulating states. Interestingly, at nu = +(-) 1 we find states with non-zero Chern numbers. For nu = - 1 the insulating state exhibits a sharp hysteretic resistance enhancement when a perpendicular magnetic field above 3.6 tesla is applied, consistent with a field driven phase transition. Our study shows that symmetry-broken states, interaction driven insulators, and superconducting domes are common across the entire moire flat bands, including near charge neutrality.

cond-mat.str-el

Improving the read-out of the resonance frequency of nanotube mechanical resonators

We report on an electrical detection method of ultrasensitive carbon nanotube mechanical resonators. The noise floor of the detection method is reduced using a RLC resonator and an amplifier based on a high electron mobility transistor cooled at 4.2 K. This allows us to resolve the resonance frequency of nanotube resonators with an unprecedented quality. We show that the noise of the resonance frequency measured at 4.2 K is limited by the resonator itself, and not by the imprecision of the measurement. The Allan deviation reaches ~10^-5 at 125 ms integration time. When comparing the integration time dependence of the Allan deviation to a power law, the exponent approaches ~1/4. The Allan deviation might be limited by the diffusion of particles over the surface of the nanotube. Our work holds promise for mass spectrometry and surface science experiments based on mechanical nano-resonators.

cond-mat.mes-hall

Electrostatically induced phononic crystal

The possibility of realizing an electrostatically induced phononic crystal is investigated numerically in an acoustic waveguide based on a graphene sheet that is suspended over periodically arrayed electrodes. The application of dc voltage to these electrodes exerts electrostatic force on the graphene and this results in the periodic formation of stress in the waveguide structure in a non-invasive way, unlike the cases with mass loading and air holes. This non-invasive scheme enables a bandgap, namely a phononic crystal, to be created in the waveguide that can be used to dynamically tune the acoustic transparency in the medium. Our approach will allow the dispersion relation to be locally modified, thus modulating the temporal response of traveling acoustic phonon waves. This novel phonon architecture is promising in terms of realizing the advanced control of phonon dynamics such as waveform and dissipation engineering in the device.

cond-mat.mes-hall

Force sensitivity of multilayer graphene optomechanical devices

Mechanical resonators based on low-dimensional materials are promising for force and mass sensing experiments. The force sensitivity in these ultra-light resonators is often limited by the imprecision in the measurement of the vibrations, the fluctuations of the mechanical resonant frequency, and the heating induced by the measurement. Here, we strongly couple multilayer graphene resonators to superconducting cavities in order to achieve a displacement sensitivity of $1.3$ fm Hz$^{-1/2}$. This coupling also allows us to damp the resonator to an average phonon occupation of $7.2$. Our best force sensitivity, $390$ zN Hz$^{-1/2}$ with a bandwidth of $200$ Hz, is achieved by balancing measurement imprecision, optomechanical damping, and heating. Our results hold promise for studying the quantum capacitance of graphene, its magnetization, and the electron and nuclear spins of molecules adsorbed on its surface.

cond-mat.mes-hall

High quality-factor mechanical resonators based on WSe2 monolayers

Suspended monolayer transition metal-dichalcogenides (TMD) are membranes that combine ultra-low mass and exceptional optical properties, making them intriguing materials for opto-mechanical applications. However, the low measured quality factor of TMD resonators has been a roadblock so far. Here, we report an ultrasensitive optical readout of monolayer TMD resonators that allows us to reveal their mechanical properties at cryogenic temperatures. We find that the quality factor of monolayer WSe2 resonators greatly increases below room temperature, reaching values as high as 1.6E^4 at liquid nitrogen temperature and 4.7E^4 at liquid helium temperature. This surpasses the quality factor of monolayer graphene resonators with similar surface areas. Upon cooling the resonator, the resonant frequency increases significantly due to the thermal contraction of the WSe2 lattice. These measurements allow us to experimentally study the thermal expansion coefficient of WSe2 monolayers for the first time. High Q-factors are also found in resonators based on MoS2 and MoSe2 monolayers. The high quality-factor found in this work opens new possibilities for coupling mechanical vibrational states to two-dimensional excitons, valley pseudospins, and single quantum emitters, and for quantum opto-mechanical experiments based on the Casimir interaction.

cond-mat.mes-hall