arXiv subjects

Akimasa Sakuma

Publications and source records attributed to Akimasa Sakuma.

At least 19 recordsLinked to original sources

arXiv2025

Light-induced torque in ferromagnetic metals via orbital angular momentum generated by photon-helicity

We investigated photon-helicity-induced magnetization precession in Co$_{1-x}$Pt$_{x}$ alloy thin films. In addition to field-like torque, attributable to magnetic field generation owing to {\it the inverse Faraday effect}, we observed non-trivial and large damping-like torque which has never been discussed for single ferromagnetic layer. The composition dependence of those two torques is effectively elucidated by a model that considers mutual coupling via spin-orbit interaction between magnetization and the electronic orbital angular momentum generated by photon-helicity. This work significantly enhances our understanding of the physics relevant to the interplay of photon-helicity and magnetization in magnetic metals.

cond-mat.mtrl-sci↗

arXiv2024

First-principles study of exchange stiffness constant of half-metallic Heusler alloys Co2MnZ (Z= Si, Al) at finite temperatures: Spin fluctuation-induced effective half metallicity

We performed first-principles calculations at finite temperatures to investigate the temperature dependence of the magnetic properties, such as exchange stiffness constants and Curie temperatures, of Co2MnZ (Z= Si, Al) assuming L21 and B2 structures. In L21 structures, we confirmed a relatively high Curie temperature for Co2MnAl, compatible with that of Co2MnSi; however, its exchange stiffness constant and single site magnetic excitation energy at zero temperature are much smaller than those of Co2MnSi. This might indicate that the Curie temperature of itinerant magnets cannot be determined by the exchange interaction at zero temperature. We also investigated the temperature dependence of the exchange stiffness constants of both alloys, and we found robustness in the temperature dependence of the exchange stiffness constant for Co2MnAl, assuming an L21 structure. This might lead to a high Curie temperature, contrary to the small exchange stiffness constant. Finally, we examined the temperature dependence of the electronic structure to investigate the origin of the behavior of the exchange stiffness constant at finite temperatures. We confirmed that the spin polarization at chemical potential effectively increases with an increasing temperature due to the altered electronic structure induced by the spin disorder. This might contribute to the robustness of the exchange stiffness constant at finite temperatures. Our results might indicate that renomarization of the electronic structure due to spin disorder at finite temperature influences the exchange interactions of Co2MnAl.

cond-mat.mtrl-sci↗

arXiv2024

Magnetization and exchange-stiffness constants of Fe-Al-Si alloys at finite-temperatures: A first-principles study

We investigated the magnetic properties of Sendust (Fe-Al-Si) alloys not only at 0 K but also at finite-temperatures by means of the first-principles calculations assuming A2, B2, and DO3 structures. We confirmed that the itinerant characteristics of 3d electrons of Fe are not negligible for A2 and B2 structures and a significantly small exchange stiffness constant exists at zero-temperature in a B2 structure. However, the calculated Curie temperatures are in the same order for all structures; this indicates that the Curie temperature cannot be determined only by the exchange interactions at zero-temperature in itinerant electron systems. Temperature dependence of the exchange interaction, namely spin configuration dependence, also might be important for determining it. In addition, this property might also be related to the unique behavior of the temperature dependence of the exchange stiffness constant for the B2 structure, which does not decrease monotonically as temperatures increase, contrary to the behavior expected from the Heisenberg model. In addition, we investigated composition dependence on the exchange stiffness constant at zero-temperature and confirmed that the substitution of Si with Al could improve the amplitude of the exchange stiffness constant at zero-temperature for all structures.

cond-mat.mtrl-sci↗

arXiv2023

Finite-temperature second-order perturbation analysis of magnetocrystalline anisotropy energy of L10-type ordered alloys

We present a novel finite-temperature second-order perturbation method incorporating spin-orbit coupling to investigate the temperature-dependent site-resolved contributions to the magnetocrystalline anisotropy energy (MAE), specifically K1(T), in FePt, MnAl, and FeNi alloys. Our developed method successfully reproduces the results obtained using the force theorem from our previous work. By employing this method, we identify the key sites responsible for the distinctive behaviors of MAE in these alloys, shedding light on the inadequacy of the spin model in capturing the temperature dependence of MAE in itinerant magnets. Moreover, we explore the lattice expansion effect on the temperature dependence of on-site contributions to K1(T) in FeNi. Our results not only provide insights into the limitations of the spin model in explaining the temperature dependence of MAE in itinerant ferromagnets but also highlight the need for further investigations. These findings contribute to a deeper understanding of the complex nature of MAE in itinerant magnetic systems.

cond-mat.mtrl-sci↗

arXiv2022

Perpendicularly Polarized Spin Hall Effects Induced by Spin-Dependent Scattering in Ferromagnetic Metals

Spin currents in ferromagnets afford diverse functionalities. We evaluate the extrinsic spin Hall effects of magnetic impurity scattering in ferromagnetic metals. We show that spin-dependent scattering can provide a high spin current polarized perpendicularly to the magnetization direction and is a dominant mechanism in the moderate-conductivity regime. We find that the superposition of the spin-conserve and spin-flip channels causes the spin currents. These findings suggest that optimizing alloy composition is an effective strategy to control the spin Hall effect.

cond-mat.mtrl-sci↗

arXiv2022

Temperature Dependence of Magnetocrystalline Anisotropy in Itinerant Ferromagnets

We theoretically investigated magnetocrystalline anisotropy (MA) at a finite temperature $T$ in ferromagnetic metals. Assuming a Rashba-type ferromagnet with uniaxial MA, we defined the MA constants $K_\mathrm{u}(T)$ derived from several different concepts. Our purpose was to examine the equality between them and to confirm a power law between $K_\mathrm{u}(T)$ and magnetization $M(T)$ in the form of $K_\mathrm{u}(T)/K_\mathrm{u}(0)=[M(T)/M(0)]^α$. We demonstrate that $α$ equals 2 in the itinerant-electron limit and increases with the localized feature of electrons passing through $α=3$, predicted for the single-ion MA in spin models.

cond-mat.str-el↗

arXiv2021

Theoretical Study of Temperature Dependence of Spin Susceptibility in Anisotropic Itinerant Ferromagnets

We developed a framework for directly calculating the spin susceptibility of anisotropic itinerant ferromagnets in the full temperature range within the coherent potential approximation in the disordered local moment picture. As a test of our formulation, we demonstrate the computation for the temperature ($T$) dependence of the spin susceptibility for Rashba-type ferromagnets with the Curie temperature $T_\mathrm{C}$. In a certain parameter, we found that the inverse transverse susceptibility $1/χ_\perp\simeq\mathrm{const.}$ for $T T_\mathrm{C}$, which reflects characteristics of itinerant ferromagnets including a spin-orbit interaction.

cond-mat.str-el↗

arXiv2021

Theoretical Study of Extrinsic Spin-current Generation in Ferromagnets Induced by Anisotropic Spin-flip Scattering

The spin Hall effect (SHE) and the magnetic spin Hall effect (MSHE) are responsible for electrical spin current generation, which is a key concept of modern spintronics. We theoretically investigated the spin conductivity induced by spin-dependent s-d scattering in a ferromagnetic 3d alloy model by employing microscopic transport theory based on the Kubo formula. We derived a novel extrinsic mechanism that contributes to both the SHE and MSHE. This mechanism can be understood as the contribution from anisotropic (spatial-dependent) spin-flip scattering due to the combination of the orbital-dependent anisotropic shape of s-d hybridization and spin flipping, with the orbital shift caused by spin-orbit interaction with the d-orbitals. We also show that this mechanism is valid under crystal-field splitting among the d-orbitals in either the cubic or tetragonal symmetry.

cond-mat.mtrl-sci↗

arXiv2020

Detecting quadrupole: a hidden source of magnetic anisotropy for Manganese alloys

Mn-based alloys exhibit unique properties in the spintronics materials possessing perpendicular magnetic anisotropy (PMA) beyond the Fe and Co-based alloys. It is desired to figure out the quantum physics of PMA inherent to Mn-based alloys, which have never been reported. Here, the origin of PMA in ferrimagnetic Mn$_{3-δ}$Ga ordered alloys is investigated to resolve antiparallel-coupled Mn sites using x-ray magnetic circular and linear dichroism (XMCD/XMLD) and a first-principles calculation. We found that the contribution of orbital magnetic moments in PMA is small from XMCD and that the finite quadrupole-like orbital distortion through spin-flipped electron hopping is dominant from XMLD and theoretical calculations. These findings suggest that the spin-flipped orbital quadrupole formations originate from the PMA in Mn$_{3-δ}$Ga and bring the paradigm shift in the researches of PMA materials using x-ray magnetic spectroscopies.

cond-mat.mtrl-sci↗

arXiv2019

Voltage-Controlled Magnonic Spin Tunneling Junction

We theoretically investigate the effective exchange interaction, $J_\mathrm{eff}$, mediated by conductive electrons within a nonmagnetic metal spacer, in the presence of a bias voltage, sandwiched by two ferromagnetic insulators. On the basis of the tight-binding model, we show the voltage and spacer thickness dependences of $J_\mathrm{eff}$, and its contorollability is demonstrated. We also propose a new magnonic device with the functions of both field effect transistor and non-volatile memory.

cond-mat.mes-hall↗

arXiv2019

Theoretical Study on Four-fold Symmetric Anisotropic Magnetoresistance Effect in Cubic Single-crystal Ferromagnetic Model

In this study, we present a theoretical interpretation of the experimental results that the anisotropic magnetoresistance (AMR) effect has a four-fold symmetric component, $c_4$, in cubic ferromagnetic metals. The theoretical model that we employ is based on the Anderson impurity model that includes a four-fold symmetric crystalline electric field, and we assume that the impurities have 3d electron orbitals and spin--orbit interaction (SOI). We describe the DC conductivity on the basis of the Kubo formula, and we investigate $c_4$ by analyzing the magnetization direction dependence of the resultant AMR ratio. Analytical and numerical calculations are performed; the analytical calculation reveals that $c_4$ arises from the fourth-order contribution of the SOI, and the numerical calculation provides the parameter dependencies of $c_{4}$ in our model. From the calculation results, we observe that the splitting of impurity 3d levels due to SOI is responsible for the existence of $c_{4}$ in cubic ferromagnetic metals.

physics.app-ph↗

arXiv2019

Analytic Expression for Magnetic Activation Energy

We theoretically investigate the magnetic activation energy of permanent magnets. Practically, it is widely used in a phenomenological form as $\mathcal{F}_\mathrm{B}(H_\mathrm{ext})=\mathcal{F}_\mathrm{B}^0\left(1-H_\mathrm{ext}/H_0\right)^n,$ where $\mathcal{F}_\mathrm{B}^0$ is the activation energy in the absence of an external magnetic field $H_\mathrm{ext}$, $n$ is a real parameter, and $H_0$ is defined by the equation $\mathcal{F}_\mathrm{B}(H_0)=0$. We derive the general and direct expressions for these phenomenological parameters under the restriction of uniform rotation of magnetization and on the basis of the perturbative theory with respect to $H_\mathrm{ext}$. Further,we apply our results to Nd$_2$Fe$_{14}$B magnets and confirm the validity of the proposed method by comparing with the Monte Carlo calculations.

cond-mat.mtrl-sci↗

arXiv2019

Noncollinearity effects on magnetocrystalline anisotropy for $R_2$Fe$_{14}$B magnets

We present a theoretical investigation of the magnetocrystalline anisotropy (MA) in $R_2$Fe$_{14}$B ($R$ is a rare-earth element) magnets in consideration of the non-collinearity effect (NCE) between the $R$ and Fe magnetization directions. In particular, the temperature dependence of the MA of Dy$_2$Fe$_{14}$B magnets is detailed in terms of the $n$th-order MA constant (MAC) $K_n(T)$ at a temperature $T$. The features of this constant are as follows: $K_1(T)$ has a broad plateau in the low-temperature range and $K_2(T)$ persistently survives in the high-temperature range. The present theory explains these features in terms of the NCE on the MA by using numerical calculations for the entire temperature range, and further, by using a high-temperature expansion. The high-temperature expansion for $K_n(T)$ is expressed in the form of $K_n(T)=κ_1(T)\left[1+δ(T)\right][-δ(T)]^{n-1}$, where $κ_1(T)$ is the part without the NCE and $δ(T)$ is a correction factor for the NCE introduced in this study. We also provide a convenient expression to evaluate $K_n(T)$, which can be determined only by a second-order crystalline electric field coefficient and an effective exchange field.

cond-mat.mtrl-sci↗

arXiv2018

Tunable Spin Seebeck Diode with Magnonic Spin Tunneling Junction

We theoretically investigate the spin--wave spin current induced by the spin Seebeck effect in magnonic spin tunneling junctions (MSTJs) for arbitrary magnetization directions. We show that the MSTJ functions as a \textit{tunable} spin Seebeck diode in which the tunneling spin current can be turned on and off with high efficiency by controlling the magnetization direction.

cond-mat.mes-hall↗

arXiv2018

Anisotropy of exchange stiffness based on atomic-scale magnetic properties in rare-earth permanent magnet Nd$_2$Fe$_{14}$B

We examine the anisotropic properties of the exchange stiffness constant, $\mathcal{A}$, for rare-earth permanent magnet, Nd$_2$Fe$_{14}$B, by connecting analyses with two different scales of length, i.e., Monte Carlo (MC) method with an atomistic spin model and Landau-Lifshitz-Gilbert (LLG) equation with a continuous magnetic model. The atomistic MC simulations are performed on the spin model of Nd$_2$Fe$_{14}$B constructed from ab-initio calculations, and the LLG micromagnetics simulations are performed with the parameters obtained by the MC simulations. We clarify that the amplitude and the thermal property of $\mathcal{A}$ depend on the orientation in the crystal, which are attributed to the layered structure of Nd atoms and weak exchange couplings between Nd and Fe atoms. We also confirm that the anisotropy of $\mathcal{A}$ significantly affects the threshold field for the magnetization reversal (coercivity) given by the depinning process.

cond-mat.mtrl-sci↗

arXiv2018

Power law analysis for temperature dependence of magnetocrystalline anisotropy constants of Nd$_2$Fe$_{14}$B magnets

Phenomenological analysis for the temperature dependence of the magnetocrystalline anisotropy (MA) in rare earth magnets is presented. We define phenomenological power laws applicable to compound magnets using the Zener theory, apply these laws to the magnetocrystalline anisotropy constants (MACs) of Nd$_2$Fe$_{14}$B magnets. The results indicate that the MACs obey the power law well, and a general understanding for the temperature-dependent MA in rare earth magnets is obtained through the analysis. Furthermore, to examine the validity of the power law, we discuss the temperature dependence of the MACs in Dy$_2$Fe$_{14}$B and Y$_2$Fe$_{14}$B magnets as examples wherein it is difficult to interpret the MA using the power law.

cond-mat.mtrl-sci↗

arXiv2017

First-principles study on the magnetic properties of ordered Nd$_{6}$(Fe,Ga)$_{14}$ alloys

We studied the stable magnetic structure of ordered Nd$_{6}$Fe$_{14-x}$Ga$_x$ ($x = 0, 1)$ alloys, which appears in the grain-boundary (GB) phase of Nd-Fe-B permanent magnets, using first-principles techniques. Slight Ga doping ($x = 1$) was shown to contribute to the stabilization of an anti-ferromagnetic (AF) state, whereas the non-doped case ($x = 0$) was revealed to favor ferromagnetic state rather than AF state with a slight energy difference.

cond-mat.mtrl-sci↗

arXiv2017

Temperature- dependence of anomalous Hall conductivity in Rashba-type ferromagnets

The applicability and usefulness of Rashba model have been extended by recent observations in the field of spintronics, such as the spin-orbit torque at the junction interfaces between ferromagnetic (FM) metals and non-magnetic (NM) metals and the perpendicular anomalous magnetoresistance (AMR) in heterostructures such as FI/NM or FM/NI (I denotes an insulator). In particular, the observations of the perpendicular AMR effect stimulate further interest in the Rashba-type spin-orbit interaction (SOI) at interfaces. Thus, the Rashba model with exchange splitting (EXS) is considered not only to play as an effective model for the physical understanding but also to reflect actual bi-layer systems in current spintronics devices. In the present work, we have first investigated the temperature dependence of anomalous Hall conductivity (AHC) of Rashba-type ferromagnets considered effects of spin fluctuations within the disordered local moment (DLM) scheme. The most distinctive feature that we observed is that intrinsic AHC increases with increasing temperature. This can be understood from the aspect of spin chirality, which indicates that the AHC increases with decreasing EXS when the SOI is much smaller than the EXS. The extrinsic part of the Fermi surface term also increases with increasing temperature and has a large contribution, comparable to that of the intrinsic part. Although, such a behaviour has not yet been observed experimentally, we suggest that the physical picture found in this work might lurk in an anomalous Hall effects in Rashbe-type ferromagnets.

cond-mat.mtrl-sci↗