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Alain Pautrat

Publications and source records attributed to Alain Pautrat.

29 records · Page 2Linked to original sources

Mapping electronic reconstruction at the metal/insulator interfaces in \ce{LaVO_3/SrVO_3} heterostructures

A \ce{(LaVO_3)_6/(SrVO_3)_3} superlattice is studied with a combination of sub-Å resolved scanning transmission electron microscopy and monochromated electron energy-loss spectroscopy. The V oxidation state is mapped with atomic spatial resolution enabling to investigate electronic reconstruction at the \ce{LaVO_3}/\ce{SrVO_3} interfaces. Surprisingly, asymmetric charge distribution is found at adjacent chemically symmetric interfaces. The local structure is proposed and simulated with double channeling calculation which agrees qualitatively with our experiment. We demonstrate that local strain asymmetry is the likely cause of the electronic asymmetry of the interfaces. The electronic reconstruction at the interfaces extends much further than the chemical composition, varying from 0.5 to 1.2 nm. This distance corresponds to the length of charge transfer previously found in the \ce{(LaVO_3)_m}/\ce{(SrVO_3)_n} metal/insulating and the \ce{(LaAlO_3)_m}/\ce{(SrTiO_3)_n} insulating/insulating interfaces.

cond-mat.mtrl-sci↗

A study of flux lines lattice order and critical current with time of flight small angle neutron scattering

Small angle neutron scattering (SANS) is an historical technique to study the flux lines lattice (FLL) in a superconductor. Structural characteristics of the FLL can be revealed, providing fundamental information for the physics of vortex lattice. However, the spatial resolution is limited and all the correlation lengths of order are difficult to extract with precision. We show here that a time of flight technique reveals the Bragg peak of the FLL, and also its translational order with a better resolution. We discuss the implication of these results for pinning mechanisms in a Niobium sample.

cond-mat.supr-con↗

Dominant role of impurity scattering over crystalline anisotropy for magnetotransport properties in the quasi-1D Hollandite Ba1.2Rh8O16

Angular magnetotransport measurements have been performed to tackle the origin of the magnetoresistance in the quasi-1D Hollandite Ba1.2Rh8O16. Three samples of different impurities amount were measured. We observe that the low temperature resistivity upturn is not due to a charge density wave transition, and a dominant role of impurities scattering for low temperature transport properties is instead demonstrated. The components of magnetoresistance were separated by using the Kohler plot and the angular dependency of the resistance under magnetic field. It shows the major contribution of an isotropic, likely spin driven, negative magnetoresistance. Galvanomagnetic characteristics are then consistent with a Kondo effect and appear to be essentially 3D at low temperature.

cond-mat.mtrl-sci↗

Contrasted role of disorder for magnetic properties in an original mixed valency iron Phosphate

We have measured the magnetic properties of a mixed valency iron phosphate. It presents an original structure with crossed chains containing Fe II and orthogonal to the longest direction of the crystallites. Microstructural investigations using electron microscopy show the presence of random nano-twinning. The ac susceptibility measurements demonstrate similarities with the kinetics of a disordered magnetic, spin-glass like, state but are shown to be essentially due to this peculiar disorder. Scaling properties are characteristics of 3D second order transition implying that this disorder at a small scale does not influence significantly long range magnetic ordering. At low temperature, a decrease of the spontaneous magnetization and an irreversible metamagnetic transition is observed, and is attributed to a canting of the spins in the iron chain.

cond-mat.mtrl-sci↗

Galvanomagnetic properties and noise in a barely metallic film of V2O3

We have measured the magnetotransport properties of a strained metallic V2O3 thin film. Most of the properties are similar to V2O3 single crystals that have been submitted to a large pressure. In addition, resistance noise analysis indicates that conductivity fluctuations are freezing out at T\approx 10K. Examination of a range of measurements leads to the conclusion that spins-configuration fluctuations dominate in the low temperature regime.

cond-mat.str-el↗

Narrow-band noise due to the moving vortex lattice in superconducting niobium

We report measurements of voltage noise due to vortex motion in Niobium, a conventional low-Tc superconductor. A coherent oscillation leading to narrow band noise (NBN) is evidenced. Its characteristic frequency is a linear function of the overcritical transport current in the flux-flow regime, and hence scales as the main velocity of the vortex flow. The associated length scale is not the intervortex distance but the width of the sample, indicating temporal coherence at a large scale. NBN is also observed in the non linear part of the V(I) at the onset of depinning, in apparent disagreement with a stochastic creep motion of flux bundles. NBN exists in the peak effect region, showing that long range temporal correlations are preserved in this regime.

cond-mat.supr-con↗

Why pinning by surface irregularities can explain the peak effect in transport properties and neutron diffraction results in NbSe2 and Bi-2212 crystals?

The existence of a peak effect in transport properties (a maximum of the critical current as function of magnetic field) is a well-known but still intriguing feature of type II superconductors such as NbSe2 and Bi-2212. Using a model of pinning by surface irregularities in anisotropic superconductors, we have developed a calculation of the critical current which allows estimating quantitatively the critical current in both the high critical current phase and in the low critical current phase. The only adjustable parameter of this model is the angle of the vortices at the surface. The agreement between the measurements and the model is really very impressive. In this framework, the anomalous dynamical properties close to the peak effect is due to co-existence of two different vortex states with different critical currents. Recent neutron diffraction data in NbSe2 crystals in presence of transport current support this point of view.

cond-mat.supr-con↗

Quantitative analysis of the critical current due to vortex pinning by surface corrugation

The transport critical current of a Niobium (Nb) thick film has been measured for a large range of magnetic field. Its value and variation are quantitatively described in the framework of the pinning of vortices due to boundary conditions at the rough surface, with a contact angle well explained by the spectral analysis of the surface roughness. Increasing the surface roughness using a Focused Ion Beam results also in an increase of the superficial critical current.

cond-mat.supr-con↗

Anomaly in the dielectric response at the charge orbital ordering transition of crystalline Pr0.67Ca0.33MnO3

The complex impedance of a Pr0.67Ca0.33MnO3 crystal has been measured. The frequency dependence is studied for a wide range of temperatures (50K-403K) and is found to be characteristic of relaxation process with a single Debye time relaxation constant, which is interpreted as a dielectric constant of the material. A strong peak is observed in this dielectric constant (up to two millions) at the charge ordering transition suggesting an interpretation in terms of ordering of electric dipoles at TCO or in term of phase separation. Comparison with Pr0.63Ca0.37MnO3 - in which the phase separation is much smaller and the peak in the dielectric constant is absent - suggests an interpretation in term of phase separation between insulating and metallic states.

cond-mat.str-el↗

The vortex depinning transition in untwinned YBaCuO using complex impedance measurements

We present surface impedance measurement of the vortex linear response in a large untwinned YBCO crystal. The depinning spectra obtained over a broad frequency range (100 Hz- 30 MHz) are those of a surface pinned vortex lattice with a free flux flow resistivity (two modes response). The critical current in the "Campbell" like regime and the flux flow resistivity in the dissipative regime are extracted. Those two parameters are affected by the first order transition, showing that this transition may be related to the electronic state of vortices.

cond-mat.supr-con↗