arXiv subjects

Alejandro V. Silhanek

Publications and source records attributed to Alejandro V. Silhanek.

At least 19 recordsLinked to original sources

arXiv2026

Cryogenic Voltage Control of Magnetism in Silicon-Integrated \newline SrTiO$_3$/Fe Heterostructures

Cryogenic electronics forms a rapidly emerging research domain for high-performance and power-efficient computing applications. Incorporating nanomagnetic components in cryogenic circuitry adds highly valuable functionality, facilitating downscaling, reducing energy consumption and introducing time-reversal symmetry breaking. Furthermore, low-temperature environments enhance magnetic stability and switching efficiency at nanoscale dimensions, reinforcing the potential of cryogenic nanomagnets. To fully leverage these opportunities, magnetic control schemes require alternative options to current-based writing, which is the main bottleneck regarding power consumption and downscaling. In this regard, voltage-based gating of the magnetic state could drastically enhance operational efficiency and integration density. In this work, we investigate cryogenic Voltage Control of Magnetism (VCM) in epitaxial SrTiO$_3$/Fe thin film heterostructures on a CMOS compatible Si substrate. We demonstrate and quantify voltage-controlled modifications of the magnetic domain structure, consistent with electric field-controlled magnetic anisotropy at the Fe/SrTiO$_3$ interface. These findings provide a viable material system for the development of next-generation magnetic domain-based devices for classical and quantum computing.

cond-mat.mes-hall↗

arXiv2026

Electrical manipulation of oxygen stoichiometry in multiterminal YBa$_2$Cu$_3$O$_{7-δ}$ junctions

Local manipulation of oxygen stoichiometry offers a route to control the electronic properties of complex oxides, yet the selective modification of individual current-carrying branches through oxygen redistribution remains unexplored in multiterminal high-temperature superconducting junctions. In a YBa$_2$Cu$_3$O$_{7-δ}$ Y-shaped three-terminal device, we demonstrate the possibility to electrically control oxygen vacancy migration on a hand-picked terminal while largely preserving the other two. Oxygen-depleted propagating fronts are directly visualized by the resulting change in optical reflectivity and they are linked to the evolution of the electrical response. The process is highly directional and determined by the polarity of the applied current, allowing for the creation of either a converging or a diverging propagating front from the central node of the Y-shaped device. The associated changes in resistance exhibit relaxation on a timescale of minutes, driven by the vacancy concentration gradient. Effects of oxygen migration are also mapped by Kelvin Probe Force Microscopy and Scanning Laser Microscopy, which probe work-function changes and spatially resolved variations in the superconducting transition, respectively. Notably, the Tc contrast revealed by the latter provides a quantitative handle on the underlying oxygen content, enabling direct visualization of oxygen redistribution. Finite-element modeling and nanoprobe X-ray diffraction qualitatively reproduce the observed vacancy redistribution. These results establish a post-fabrication route to locally tune properties of superconducting multiterminal devices such as nanocryotrons, yTron, and tunable weak links.

cond-mat.supr-con↗

arXiv2026

Time-Resolved Thermal Susceptibility Mapping via Low-Temperature Scanning Laser Microscopy

We present a multiharmonic lock-in detection approach that utilizes the inverse Fast Fourier Transform to reconstruct the time evolution of thermal susceptibility with high spatial resolution. The method is implemented on a custom-built, modular scanning laser microscope designed for operation in low working-distance optical cryostats and thoroughly calibrated for spatial accuracy. A demonstrative case study using a superconducting resonator highlights the capability of this technique to generate thermal images on time scales significantly shorter than the intrinsic scanning speed, thus enabling dynamic thermal characterization with high spatial fidelity. The proposed technique of low-temperature time-resolved scanning laser microscopy offers unique opportunities to explore superconducting devices, 2D materials, hybrid planar structures, and other low-dimensional systems.

cond-mat.supr-con↗

arXiv2026

Nanoscale Spatial Tuning of Superconductivity in Cuprate Thin Films via Direct Laser Writing

Cuprate high-temperature superconductors, such as Yttrium Barium Copper Oxide (YBCO), are extremely promising for emerging technologies such as low-power computing, data storage, quantum sensors and superconducting electronics. However, the realization of high-performance functional nanostructures presents formidable challenges due to the difficulty of applying conventional nanofabrication methods to such sensitive materials, making the search for alternative methods a key enabling factor. Since YBCO's superconducting and normal-state properties are highly dependent on oxygen stoichiometry, precise nanoscale control of the oxygen content represents a highly appealing approach for creating advanced nanoengineered devices. In this work, we demonstrate the precise fabrication of sub-micrometer, grayscale patterns over large areas in epitaxial YBCO thin films, achieving finely tuned optical and superconducting transport properties by locally controlling the stoichiometry through maskless direct laser writing under ambient conditions. Cryogenic magneto-optical imaging and transport measurements in irradiated devices directly demonstrate the spatial tuning of the critical temperature and carrier density with the patterning conditions. Correlated Raman microscopy and reflectometry indicate a laser-power dependent oxygen depletion in the irradiated regions. The proposed laser-controlled stoichiometry approach provides a direct and scalable method to navigate the phase diagram of high-TC superconducting oxides, offering new possibilities for integrating functional nanostructures into superconducting devices.

cond-mat.supr-con↗

arXiv2026

Probing Electromigration of Oxygen Vacancies in YBa$_2$Cu$_3$O$_{7-δ}$ Devices by Multimodal X-ray Techniques

Control of oxygen vacancies by electrical currents in complex oxides such as YBa$_2$Cu$_3$O$_{7-δ}$ (YBCO) has attracted considerable interest due to the relative simplicity of its implementation and its potential for both fundamental studies and the tuning of superconducting device properties. However, the structural evolution and depth-dependent effects associated with current-based techniques remain largely unexplored, particularly with respect to the connection between optical signatures and the spatial distribution of oxygen vacancies. Here, we combine nanoprobe X-ray Diffraction (NanoXRD), Cu K-edge X-ray Absorption Near-Edge Structure (XANES), X-ray Photoelectron Spectroscopy (XPS), electrical transport, and optical measurements to reveal modifications induced in YBCO microbridges by pulsed electromigration. We observe a c-axis expansion correlated with spectroscopic features of oxygen depletion in the Cu-O chains, and we confirm that oxygen redistribution, crystallographic changes, and copper coordination evolve consistently across techniques. Notably, the spatial profile of unit-cell expansion closely follows the optical contrast observed after electromigration, demonstrating that the different signatures capture the same underlying oxygen reordering. We further show that optical microscopy cannot reliably capture bipolar electromigration involving strong resistance modifications, as surface deoxygenation appears largely irreversible. Taken together, our findings provide a significant step toward a microscopic understanding of current-assisted oxygen migration in YBCO and establish a framework for effectively exploiting vacancy control in high-temperature superconducting devices.

cond-mat.supr-con↗

arXiv2026

Effect of pulse duration on current-induced selective oxygen migration in high-Tc superconductors

High current densities can induce the directional diffusion of atoms in metallic films. In YBa$_2$Cu$_3$O$_{7-δ}$ (YBCO), this electromigration process selectively acts on oxygen atoms lying in the Cu-O chains, permitting to vary the oxygen concentration in a targeted spot of high current density. This approach has proven successful in mapping the phase diagram of the material as a function of carrier concentration or as a way to manufacture memristive devices owing to its reversibility under small bipolar excitations. Thus far, most of the investigations have been limited to pulsed excitation with current/voltage pulses on a millisecond or longer scale, for which thermal effects undeniably influence the process. In the present work, we explore the impact of pulse length $δt$ on the onset current of electromigration, $I_{\text{EM}}$, of YBCO bridges, covering the range from 200 ns to 1 ms. As $δt$ decreases below $\sim 10~μ$s, $I_{\text{EM}}$ exhibits a rapid increase. Analytical and numerical estimates of the local temperature show that as pulses shorten, the temperature decreases, making the electromigration process more athermal. These findings are relevant for the operation of memristors and should be taken into account when describing the effects of thermomagnetic instabilities in thin films.

cond-mat.supr-con↗

arXiv2026

Engineering Magnetic Anisotropy in Permalloy Films via Atomic Force Nanolithography

Atomic force nanolithography provides a precise method for sculpting magnetic thin films, enabling controlled engineering of magnetic anisotropy in soft ferromagnets at the microscale. We demonstrate that nanoscale groove arrays patterned into permalloy (Ni80Fe20) films induce a robust in-plane uniaxial anisotropy, with the easy axis aligned along the groove direction. The anisotropy field is shown to increase with decreasing groove period and increasing engraving depth, offering continuous tunability of magnetic hardness within a single fabrication step. Artificially engraved microstructures further allow domain configurations and domain-wall trajectories to be directed along predefined pathways, exemplified by the creation of a chessboard-like magnetic landscape. Owing to its adaptability to diverse ferromagnetic materials and arbitrary corrugation geometries, this approach provides a versatile platform for tailoring in-plane magnetic anisotropy. Concrete applications are demonstrated in the design of magnonic elements and anisotropic magnetoresistance sensors.

cond-mat.mtrl-sci↗

arXiv2025

Impact of border defects on the magnetic flux penetration in superconducting films

Defects in superconducting systems are ubiquitous and nearly unavoidable. They can vary in nature, geometry, and size, ranging from microscopic-size defects such as dislocations, grain boundaries, twin planes, and oxygen vacancies, to macroscopic-size defects such as segregations, indentations, contamination, cracks, or voids. Irrespective of their type, defects perturb the otherwise laminar flow of electric current, forcing it to deviate from its path. In the best-case scenario, the associated perturbation can be damped within a distance of the order of the size of the defect if the rigidity of the superconducting state, characterized by the creep exponent $n$, is low. In most cases, however, this perturbation spans macroscopic distances covering the entire superconducting sample and thus dramatically influences the response of the system. In this work, we review the current state of theoretical understanding and experimental evidence on the modification of magnetic flux patterns in superconductors by border defects, including the influence of their geometry, temperature, and applied magnetic field. We scrutinize and contrast the picture emerging from a continuous media standpoint, i.e. ignoring the granularity imposed by the vortex quantization, with that provided by a phenomenological approach dictated by the vortex dynamics. In addition, we discuss the influence of border indentations on the nucleation of thermomagnetic instabilities. Assessing the impact of surface and border defects is of utmost importance for all superconducting technologies, including superconducting resonators, superconducting single-photon detectors, superconducting radio-frequency cavities and accelerators, superconducting cables, superconducting metamaterials, superconducting diodes, and many others.

cond-mat.supr-con↗

arXiv2024

DC-operated Josephson junction arrays as a cryogenic on-chip microwave measurement platform

Providing radio frequency (RF) signals to circuits working in cryogenic conditions requires bulky and expensive transmission cabling interfacing specialized RF electronics anchored at room temperature. Superconducting Josephson junction arrays (JJAs) can change this paradigm by placing the RF source and detector inside the chip. In this work, we demonstrate that DC-biased JJAs can emit signals in the C-band frequency spectrum and beyond. We fabricate reproducible JJAs comprised of amorphous MoGe or NbTiN superconducting islands and metallic Au weak links. Temperature, magnetic fields, applied currents, and device design are explored to control the operation of the RF sources, while we also identify important features that affect the ideal source behavior. Combined with the proven ability of these JJAs to detect microwave radiation, these sources allow us to propose a fully DC-operated cryogenic on-chip measurement platform that is a viable alternative to the high-frequency circuitry currently required for several quantum applications.

cond-mat.supr-con↗

arXiv2024

Non-Invasive Readout of the Kinetic Inductance of Superconducting Nanostructures

The energy landscape of multiply connected superconducting structures is ruled by fluxoid quantization due to the implied single-valuedness of the complex wave function. The transitions and interaction between these energy states, each defined by a specific phase winding number, are governed by classical and/or quantum phase slips. Understanding these events requires the ability to probe, non-invasively, the state of the ring. Here, we employ a niobium resonator to examine the superconducting properties of an aluminum loop. By applying a magnetic field, adjusting temperature, and altering the loop's dimensions via focused ion beam milling, we correlate resonance frequency shifts with changes in the loop's kinetic inductance. This parameter is a unique indicator of the superconducting condensate's state, facilitating the detection of phase slips in nanodevices and providing insights into their dynamics. Our method presents a proof-of-principle spectroscopic technique with promising potential for investigating the Cooper pair density in inductively coupled superconducting nanostructures.

physics.app-ph↗

arXiv2023

Catastrophic magnetic flux avalanches in NbTiN superconducting resonators

Macroscopic superconducting components are an important building block of various quantum circuits. Since several of the envisioned applications require exposure to magnetic fields, it is of utmost importance to explore the impact of magnetic fields on their performance. Here we explore the complex pattern of magnetic field penetration and identify its impact on the resonance frequency of NbTiN superconducting resonators by combining magneto-optical imaging and high-frequency measurements. At temperatures below approximately half of the superconducting critical temperature, the development of magnetic flux avalanches manifests itself as a noisy response in the field-dependent resonance frequency. Magneto-optical imaging reveals different regimes and distinguishes the impact of avalanches in the ground plane and resonator. Our findings demonstrate that superconducting resonators represent a valuable tool to investigate magnetic flux dynamics. Moreover, the current blooming of niobium-based superconducting radio-frequency devices makes this report timely by unveiling the severe implications of magnetic flux dynamics.

cond-mat.supr-con↗

arXiv2020

A roadmap for the design of four-terminal spin valves and the extraction of spin diffusion length

Graphene is a promising substrate for future spintronics devices owing to its remarkable electronic mobility and low spin-orbit coupling. Hanle precession in spin valve devices is commonly used to evaluate the spin diffusion and spin lifetime properties. In this work, we demonstrate that this method is no longer accurate when the distance between inner and outer electrodes is smaller than six times the spin diffusion length, leading to errors as large as 50% for the calculations of the spin figures of merit of graphene. We suggest simple but efficient approaches to circumvent this limitation by addressing a revised version of the Hanle fit function. Complementarily, we provide clear guidelines for the design of four-terminal spin valves able to yield flawless estimations of the spin lifetime and the spin diffusion coefficient.

cond-mat.mes-hall↗

arXiv2020

On the origin of the giant spin detection efficiency in tunnel barrier based electrical spin detector

Efficient conversion of a spin signal into an electric voltage in mainstream semiconductors is one of the grand challenges of spintronics. This process is commonly achieved via a ferromagnetic tunnel barrier where non-linear electric transport occurs. In this work, we demonstrate that non-linearity may lead to a spin-to-charge conversion efficiency larger than 10 times the spin polarization of the tunnel barrier when the latter is under bias of a few mV. We identify the underlying mechanisms responsible for this remarkably efficient spin detection as the tunnel barrier deformation and the conduction band shift resulting from a change of applied voltage. In addition, we derive an approximate analytical expression for the detector spin sensitivity $P_{\textrm{det}}(V)$. Calculations performed for different barrier shapes show that this enhancement is present in oxide barriers as well as in Schottky tunnel barriers even if the dominant mechanisms differs with the barrier type. Moreover, although the spin signal is reduced at high temperatures, it remains superior to the value predicted by the linear model. Our findings shed light into the interpretation and understanding of electrical spin detection experiments and open new paths to optimize the performance of spin transport devices.

physics.app-ph↗

arXiv2019

Non-Volatile Superconductivity in an Insulating Copper Oxide Induced via Ionic Liquid Gating

Manipulating the superconducting states of high-T_c cuprate superconductors in an efficient and reliable way is of great importance for their applications in next-generation electronics. Traditional methods are mostly based on a trial-and-error method that is difficult to implement and time consuming. Here, employing ionic liquid gating, a selective control of volatile and non-volatile superconductivity is achieved in pristine insulating Pr_2CuO_{4\pmδ} film, based on two distinct mechanisms: 1) with positive electric fields, the film can be reversibly switched between non-superconducting and superconducting states, attributed to the carrier doping effect. 2) The film becomes more resistive by applying negative bias voltage up to -4 V, but strikingly, a non-volatile superconductivity is achieved once the gate voltage is removed. Such a persistent superconducting state represents a novel phenomenon in copper oxides, resulting from the doping healing of oxygen vacancies in copper-oxygen planes as unraveled by high-resolution scanning transmission electron microscope and in-situ x-ray diffraction experiments. The effective manipulation and mastering of volatile/non-volatile superconductivity in the same parent cuprate opens the door to more functionalities for superconducting electronics, as well as supplies flexible samples for investigating the nature of quantum phase transitions in high-T_c superconductors.

cond-mat.supr-con↗

arXiv2019

Calculation of currents around a triangular indentation by the hodograph method

Border indentations in non-linear conductors, such as superconducting thin films in the creep regime, alter the distribution of currents and magnetic fields near and far from the indentation. One of such disturbances are the discontinuity lines, or \textit{d}-lines, a parabolic-like line originating from the indentation where the current density direction changes abruptly. Hodograph series results are obtained for the currents around a triangular indentation and its corresponding $d$-lines in a conducting stripe of finite width and in an infinite half plane, considering two cases: uniform creep exponent and mixed infinite and ohmic exponents. The mixed creep exponent case presents currents distributions resembling the purely ohmic case, with significant current disturbances only near the indentation. For uniform creep exponent, results similar to a planar indentation are obtained, with far ranged currents features and parabolic-like $d$-lines with shapes depending on the creep exponent. In particular, the same $d$-line asymptotic behaviour is obtained for the triangle indentation as that of the planar defect in the critical state, a result obtained here just on continuity considerations of the hodograph expansions. This equivalence is due to identical contributions to the Fourier series of the current stream-function in the hodograph space, obtained from an images method expansion.

cond-mat.supr-con↗

arXiv2017

Imaging of super-fast dynamics and flow instabilities of superconducting vortices

Quantized magnetic vortices driven by electric current determine key electromagnetic properties of superconductors. While the dynamic behavior of slow vortices has been thoroughly investigated, the physics of ultrafast vortices under strong currents remains largely unexplored. Here we use a nanoscale scanning superconducting quantum interference device to image vortices penetrating into a superconducting Pb film at rates of tens of GHz and moving with velocities up to tens of km/s, which are not only much larger than the speed of sound but also exceed the pair-breaking speed limit of superconducting condensate. These experiments reveal formation of mesoscopic vortex channels which undergo cascades of bifurcations as the current and magnetic field increase. Our numerical simulations predict metamorphosis of fast Abrikosov vortices into mixed Abrikosov-Josephson vortices at even higher velocities. This work offers an insight into the fundamental physics of dynamic vortex states of superconductors at high current densities, crucial for many applications.

cond-mat.supr-con↗

arXiv2015

Microwave-stimulated superconductivity due to presence of vortices

The response of superconducting devices to electromagnetic radiation is a core concept implemented in diverse applications, ranging from the currently used voltage standard to single photon detectors in astronomy. Suprisingly, a sufficiently high power subgap radiation may stimulate superconductivity itself. The possibility of stimulating type II superconductors, in which the radiation may interact also with vortex cores, remains however unclear. Here we report on superconductivity enhanced by GHz radiation in type II superconducting Pb films in the presence of vortices. The stimulation effect is more clearly observed in the upper critical field and less pronounced in the critical temperature. The magnetic field dependence of the vortex related microwave losses in a film with periodic pinning reveals a reduced dissipation of mobile vortices in the stimulated regime due to a reduction of the core size. Results of numerical simulations support the validy of this conclusion. Our findings may have intriguing connections with holographic superconductors in which the possibility of stimulation is under current debate.

cond-mat.supr-con↗

arXiv2014

Near-field aperture-probe as a magnetic dipole source and optical magnetic field detector

Scanning near-field field optical microscopy (SNOM) is a technique, which allows sub-wavelength optical imaging of photonic structures. While the electric field components of light can be routinely obtained, imaging of the magnetic components has only recently become of interest. This is so due to the development of artificial materials, which enhance and exploit the typically weak magnetic light-matter interactions to offer extraordinary optical properties. Consequently, both sources and detectors of the magnetic field of light are now required. In this paper, assisted by finite-difference time-domain simulations, we suggest that the circular aperture at the apex of a metal coated hollow-pyramid SNOM probe can be approximated by a lateral magnetic dipole source. This validates its use as a detector for the lateral magnetic near-field, as illustrated here for a plasmonic nanobar sample. Verification for a dielectric sample is currently in progress. We experimentally demonstrate the equivalence of the reciprocal configurations when the probe is used as a source (illumination mode) and as a detector (collection mode). The simplification of the probe to a simple magnetic dipole facilitates the simulations and the understanding of the near-field images.

physics.optics↗