arXiv subjects

Alex S. Clark

Publications and source records attributed to Alex S. Clark.

At least 19 recordsLinked to original sources

arXiv2026

Generation and detection of squeezed light on a single silicon photonic chip

The ability to generate and detect quantum states of light on a single integrated photonic device is essential to scale quantum photonics into useful quantum technologies. Integrating the required capabilities into complementary-metal-oxide-semiconductor compatible monolithic chips can reduce cost and unlock new functionality through miniaturisation. In this work we demonstrate a single silicon-on-insulator photonic integrated circuit for the monolithic generation and detection of quantum light on a commercially available platform that operates entirely at room temperature. Specifically, we leverage spontaneous four-wave mixing in silicon waveguides to produce squeezed light which is subsequently detected by photodiodes operating in a pulsed homodyne detector configuration on the same chip as the source. We directly measure $0.25(1)$ dB of squeezing, including contributions from waveguide propagation loss and detection inefficiency, and include a detailed analysis of the impact of nonlinear loss on the squeezing levels achievable using this platform.

quant-ph↗

arXiv2026

Indistinguishablity from dephased emitters using combined plasmonic-dielectric cavities

The concept of cavity funneling has emerged recently as a promising route towards creating indistinguishable photons from highly dephased emitters. So far, all suggested solutions are solely based on dielectric cavities that require extremely high quality factors that are difficult to reach at visible wavelengths. Here we suggest a hybrid funneling architecture where a dephased emitter is coupled to a plasmonic nanoresonator that is enclosed by an outer dielectric cavity. The estimated lower limit of the outer cavity quality factor is found to be $\sim2$ orders of magnitude lower compared to a cascaded cavity system. Furthermore, the surrounding topology of our approach allows for a partial direct coupling between the emitter and the outer cavity which in turn can increase the overall system extraction efficiency $\left(\beta\right)$ by a factor of 12, boosting the probability of photon collection.

quant-ph↗

arXiv2026

Heralding efficiency and brightness optimization of a micro-ring resonator via tunable coupling

Efficient and bright single photon sources on photonic chips are key to scaling quantum technologies. Spontaneous four wave mixing in micro-ring resonators creates excellent narrowband and tunable photon sources. We experimentally demonstrate the optimization of heralding efficiency and brightness by tuning the coupling of the pump, signal and idler modes into the resonator whilst operating in a pulsed pump regime. We observe a maximum detected pair rate of over 93,000~coincidences per second in a moderately over-coupled regime, alongside a high intrinsic idler heralding efficiency of 97.87$\pm$8.97\% when operating close to maximal over-coupling. The measured dependence on coupling strength is in strong agreement with theoretical predictions, experimentally validating the predicted trade-off between brightness and heralding efficiency.

quant-ph↗

arXiv2025

Open-Path Methane Sensing via Backscattered Light in a Nonlinear Interferometer

Nonlinear interferometry has widespread applications in sensing, spectroscopy, and imaging. However, most implementations require highly reflective mirrors and precise optical alignment, drastically reducing their versatility and usability in outdoor applications. This work is based on stimulated parametric down conversion (ST-PDC), demonstrating methane absorption spectroscopy in the mid-infrared (MIR) region by detecting near-infrared (NIR) photons using a silicon-based CMOS camera. The MIR light, used to probe methane, is diffusely backscattered from a Lambertian surface, experiencing significant transmission loss. We implement a single-mode confocal illumination and collection scheme, using a two-lens system to mode-match the interfering beams to achieve background methane detection at a distance of 4.6 meters under a 60 dB loss. Our method is also extended to real-world surfaces, such as glass, brushed metal, and a leaf, showing robust background methane sensing with various target materials.

physics.optics↗

arXiv2025

Entanglement-inspired frequency-agile rangefinding

Entanglement, a key feature of quantum mechanics, is recognized for its non-classical correlations which have been shown to provide significant noise resistance in single-photon rangefinding and communications. Drawing inspiration from the advantage given by energy-time entanglement, we developed an energy-time correlated source based on a classical laser that preserves the substantial noise reduction typical of quantum illumination while surpassing the quantum brightness limitation by over six orders of magnitude, making it highly suitable for practical remote sensing applications. A frequency-agile pseudo-random source is realized through fibre chromatic dispersion and pulse carving using an electro-optic intensity modulator. Operating at a faint transmission power of 48 {\mu}W, the distance between two buildings 154.8182 m apart can be measured with a precision better than 0.1 mm, under varying solar background levels and weather conditions with an integration time of only 100 ms. These trials verified the predicted noise reduction of this system, demonstrating advantages over quantum illumination-based rangefinding and highlighting its potential for practical remote sensing applications.

physics.optics↗

arXiv2025

Phase-Matching-Free Sensing with Undetected Light Using a Nonlinear Thin-Film Metasurface

In this article, we report classical sensing with undetected light at a wavelength of 1500 nm, detected on a silicon camera at 580 nm, using four-wave mixing from a plasmonic metasurface. The bidirectional nonlinear scattering due to inherent reflections from such thin nonlinear materials modifies their operation within a nonlinear interferometer. The theoretical model for visibility accounting for such bidirectionality as well as pulsed illumination accurately predicts visibility in the system as a function of transmission in the near-infrared seed (idler) arm. Spectrally resolving the visible signal emission evaluates the total dispersion within the interferometer, highlighting the prospect of ultrafast sensing with undetected photons.

physics.optics↗

arXiv2025

Quantum undetected optical projection tomography

Quantum imaging with undetected photons (QIUP) is an emerging technique that decouples the processes of illuminating an object and projecting its image. The properties of the illuminating and detected light can thus be simultaneously optimised for both contrast on a sample and sensitivity on a camera. Here, we combine QIUP with computed tomography to enable three-dimensional (3D) infrared imaging. The image data is registered with a standard silicon camera at a wavelength of 810 nm, but the extracted 3D images map the sample's absorption at a wavelength of 1550 nm, well beyond the camera's sensitivity. Quantum Undetected Optical Projection Tomography (QUOPT) enables label-free volumetric sensing at difficult to detect wavelengths, such as those that allow molecular imaging contrast, or those within the infrared biological transmission windows.

quant-ph↗

arXiv2024

Methane Sensing via Unbalanced Nonlinear Interferometry using a CMOS Camera

Here we present a high-sensitivity, rapid, and low-cost method for methane sensing based on a nonlinear interferometer. This method utilizes signal photons generated by stimulated parametric down-conversion (ST-PDC), enabling the use of a silicon detector to capture high-precision methane absorption spectra in the mid-infrared region. By controlling the system loss, we achieve more significant changes in visibility, thereby increasing sensitivity. The methane concentration within a gas cell is determined accurately. In addition, ST-PDC enables long-distance sensing and the capability to measure low ambient methane concentrations in the real world. A low-cost CMOS camera is employed to capture spatial interference fringes, ensuring fast and efficient detection.

physics.optics↗

arXiv2024

Single-frame transmission and phase imaging using off-axis holography with undetected photons

Imaging with undetected photons relies upon nonlinear interferometry to extract the spatial image from an infrared probe beam and reveal it in the interference pattern of an easier-to-detect visible beam. Typically, the transmission and phase images are extracted using phase-shifting techniques and combining interferograms from multiple frames. Here we show that off-axis digital holography enables reconstruction of both transmission and phase images at the infrared wavelength from a single interferogram, and hence a single frame, recorded in the visible. This eliminates the need for phase stepping and multiple acquisitions, thereby greatly reducing total measurement time for imaging with long acquisition times at low flux or enabling video-rate imaging at higher flux. With this single-frame acquisition technique, we are able to reconstruct transmission images of an object in the infrared beam with a signal-to-noise ratio of $1.78\,\pm\,0.06$ at 10 frames per second, and record a dynamic scene in the infrared beam at 33 frames per second.

physics.optics↗

arXiv2023

Coupling undetected sensing modes by quantum erasure

The effect known as ``induced coherence without induced emission'' has spawned a field dedicated to imaging with undetected photons (IUP), where photons from two distinct photon-pair sources interfere if their outputs are made indistinguishable. The indistinguishability is commonly achieved in two setups. Induced coherence IUP (IC-IUP) has only the idler photons from the first source passing through the second, whilst nonlinear interferometry (NI-IUP) has both signal and idler photons from the first source passing through the second and can be simpler to implement. In both cases, changes in the idler path between sources can be detected by measuring the interference fringes in the signal path in a way that allows image information to be moved between different wavelengths. Here we model and implement a novel setup that uses a polarization state quantum eraser approach to move continuously between IC-IUP and NI-IUP operation. We find excellent agreement between experiment and theory in the low-gain or quantum regime. The system also provides a new route for optimizing IUP interference by using controllable quantum erasure to balance the interferometer.

quant-ph↗

arXiv2023

Practical quantum imaging with undetected photons

Infrared (IR) imaging is invaluable across many scientific disciplines, from material analysis to diagnostic medicine. However, applications are often limited by detector cost, resolution and sensitivity, noise caused by the thermal IR background, and the cost, portability and tunability of infrared sources. Here, we describe a compact, portable, and low-cost system that is able to image objects at IR wavelengths without an IR source or IR detector. This imaging with undetected photons (IUP) approach uses quantum interference and correlations between entangled photon pairs to transfer image information from the IR to the visible, where it can be detected with a standard silicon camera. We also demonstrate a rapid analysis approach to acquire both phase and transmission image information. These developments provide an important step towards making IUP a commercially viable technique.

quant-ph↗

arXiv2022

Enhanced nonlinear interferometry via seeding

We analyse a nonlinear interferometer, also known as an SU(1,1) interferometer, in the presence of internal losses and inefficient detectors. To overcome these limitations, we consider the effect of seeding one of the interferometer input modes with either a number state or a coherent state. We derive analytical expressions for the interference visibility, contrast, phase sensitivity, and signal-to-noise ratio, and show a significant enhancement in all these quantities as a function of the seeding photon number. For example, we predict that, even in the presence of substantial losses and highly inefficient detectors, we can achieve the same quantum-limited phase sensitivity of an unseeded nonlinear interferometer by seeding with a few tens of photons. Furthermore, we observe no difference between a number or a coherent seeding state when the interferometer operates in the low-gain regime, which enables seeding with an attenuated laser. Our results expand the nonlinear interferometry capabilities in the field of quantum imaging, metrology, and spectroscopy under realistic experimental conditions.

quant-ph↗

arXiv2022

Loss compensated and enhanced mid-infrared interaction-free sensing with undetected photons

Sensing with undetected photons enables the measurement of absorption and phase shifts at wavelengths different from those detected. Here, we experimentally map the balance and loss parameter space in a non-degenerate nonlinear interferometer, showing the recovery of sensitivity despite internal losses at the detection wavelength. We further explore an interaction-free operation mode with a detector-to-sample incident optical power ratio of >200. This allows changes in attowatt levels of power at 3.4 $μ$m wavelength to be detected at 1550 nm, immune to the level of thermal black-body background. This reveals an ultra-sensitive infrared imaging methodology capable of probing samples effectively `in the dark'.

quant-ph↗

arXiv2022

The surprising persistence of time-dependent quantum entanglement

The mismatch between elegant theoretical models and the detailed experimental reality is particularly pronounced in quantum nonlinear interferometry (QNI). In stark contrast to theory, experiments contain pump beams that start in impure states and that are depleted, quantum noise that affects -- and drives -- any otherwise gradual build up of the signal and idler fields, and nonlinear materials that are far from ideal and have a complicated time-dependent dispersive response. Notably, we would normally expect group velocity mismatches to destroy any possibility of measurable or visible entanglement, even though it remains intact -- the mismatches change the relative timings of induced signal-idler entanglements, thus generating "which path" information. Using a "positive-P" approach ideally suited to such problems, we show how the time-domain entanglement crucial for QNI can be -- and is -- recoverable despite the obscuring effects of real-world complications.

quant-ph↗

arXiv2022

Acceleration and adiabatic expansion of multi-state fluorescence from a nanofocus

Since Purcell's seminal report 75 years ago, electromagnetic resonators have been used to control light-matter interactions to make brighter radiation sources and unleash unprecedented control over quantum states of light and matter. Indeed, optical resonators such as microcavities and plasmonic nanostructures offer excellent control but only over a limited spectral range. Strategies to tune both emission and the resonator are often required, which preclude the possibility of enhancing multiple transitions simultaneously. In this letter, we report a more than 590-fold radiative emission enhancement across the telecommunications emission band of Erbium-ions in silica using a single non-resonant plasmonic waveguide. Our plasmonic waveguide uses a novel reverse nanofocusing approach to efficiently collect emission, making these devices brighter than all non-plasmonic control samples considered. Remarkably, the high broadband Purcell factor allows us to resolve the Stark-split electric dipole transitions, which are typically only observed under cryogenic conditions. Simultaneous Purcell enhancement of multiple quantum states is of interest for photonic quantum networks as well as on-chip data communications.

physics.optics↗

arXiv2021

Photon indistinguishability measurements under pulsed and continuous excitation

The indistinguishability of successively generated photons from a single quantum emitter is most commonly measured using two-photon interference at a beam splitter. Whilst for sources excited in the pulsed regime the measured bunching of photons reflects the full wavepacket indistinguishability of the emitted photons, for continuous wave (cw) excitation the inevitable dependence on detector timing resolution and driving strength obscures the underlying photon interference process. Here we derive a method to extract the photon indistinguishability from cw measurements by considering the relevant correlation functions. The equivalence of both methods is experimentally verified through comparison of cw and pulsed excitation of an archetypal source of photons, a single molecule.

quant-ph↗

arXiv2020

Coherent characterisation of a single molecule in a photonic black box

Extinction spectroscopy is a powerful tool for demonstrating the coupling of a single quantum emitter to a photonic structure. However, it can be challenging in all but the simplest of geometries to deduce an accurate value of the coupling efficiency from the measured spectrum. Here we develop a theoretical framework to deduce the coupling efficiency from the measured transmission and reflection spectra without precise knowledge of the photonic environment. We then consider the case of a waveguide interrupted by a transverse cut in which an emitter is placed. We apply that theory to a silicon nitride waveguide interrupted by a gap filled with anthracene that is doped with dibenzoterrylene molecules. We describe the fabrication of these devices, and experimentally characterise the waveguide coupling of a single molecule in the gap.

quant-ph↗

arXiv2020

Single-photon-level sub-Doppler pump-probe spectroscopy of rubidium

We propose and demonstrate pump-probe spectroscopy of rubidium absorption which reveals the sub-Doppler hyperfine structure of the $^{5}$S$_{1/2} \leftrightarrow$ $^{5}$P$_{3/2}$ (D2) transitions. The counter propagating pump and probe lasers are independently tunable in frequency, with the probe operating at the single-photon-level. The two-dimensional spectrum measured as the laser frequencies are scanned shows fluorescence, Doppler-broadened absorption dips and sub-Doppler features. The detuning between the pump and probe lasers allows compensation of the Doppler shift for all atomic velocities in the room temperature vapor, meaning we observe sub-Doppler features for all atoms in the beam. We detail a theoretical model of the system which incorporates fluorescence, saturation effects and optical pumping and compare this with the measured spectrum, finding a mean absolute percentage error of 4.17\%. In the future this technique could assist in frequency stabilization of lasers, and the single-photon-level probe could be replaced by a single photon source.

physics.atom-ph↗