arXiv subjects

Alexander A. Govyadinov

Publications and source records attributed to Alexander A. Govyadinov.

9 recordsLinked to original sources

arXiv2026

Quantum cascade laser roadmap

Quantum cascade lasers (QCLs) are unipolar semiconductor lasers first demonstrated in 1994. Since then, they have played a central role in advancing mid-infrared and terahertz photonics, becoming among the most reliable light sources in these regions of the electromagnetic spectrum. Their importance is further reinforced by their ability to generate self-starting optical frequency combs, whose investigation is motivated both by fundamental physics and by a wide range of applications, including molecular spectroscopy and free-space optical communications. This Roadmap provides a unified overview of current advances and emerging directions in QCL research. The chapters are organized into three main sections: device design and technology; frequency combs and pulse formation; and applications of QCLs. Each chapter reviews the relevant background, summarizes the current state of the art, and identifies key challenges and future directions within its specific research area.

physics.optics↗

arXiv2021

Understanding the image contrast of material boundaries in IR nanoscopy reaching 5 nm spatial resolution

Scattering-type scanning near-field optical microscopy (s-SNOM) allows for nanoscale resolved Infrared (IR) and Terahertz (THz) imaging, and thus has manifold applications ranging from materials to biosciences. However, a quantitatively accurate understanding of image contrast formation at materials boundaries, and thus spatial resolution is a surprisingly unexplored terrain. Here we introduce the write/read head of a commercial hard disk drive (HDD) as a most suitable test sample for fundamental studies, given its well20 defined sharp material boundaries perpendicular to its ultra-smooth surface. We obtainunprecedented and unexpected insights into the s-SNOM image formation process, free of topography-induced artifacts that often mask and artificially modify the pure near-field optical contrast. Across metal-dielectric boundaries, we observe non-point-symmetric line profiles for both IR and THz illumination, which are fully corroborated by numericalsimulations. We explain our findings by a sample-dependent confinement and screening of the near fields at the tip apex, which will be of crucial importance for an accurate understanding and proper interpretation of high-resolution s-SNOM images of nanocomposite materials. We also demonstrate that with ultra-sharp tungsten tips the apparent width (and thus resolution) of sharp material boundaries can be reduced to about 5 nm.

physics.optics↗

arXiv2016

Probing low-energy hyperbolic polaritons in van der Waals crystals with an electron microscope

Van der Waals (vdW) materials exhibit intriguing structural, electronic and photonic properties. Electron Energy Loss Spectroscopy (EELS) within Scanning Transmission Electron Microscope (STEM) allows for nanoscale mapping of such properties. However, typical STEM-EELS detection is limited to energy losses in the eV range, which are too large for probing important low-energy excitation such as phonons or mid-IR plasmons. Here we adapt a conventional STEM-EELS system to probe energy loss down to 100 meV, and apply it to map phononic states in h-BN, a representative van der Waals (vdW) material. The h-BN EELS spectra, surprisingly, depend on the h-BN thickness and the distance of the electron beam to h-BN flake edges. To explain this observation, we developed a classical response theory describing the interaction of fast electrons with (anisotropic) slabs of vdW materials. Theoretical and numerical calculations perfectly match the experimental h-BN spectra, and reveal that the electron loss is dominated by the excitation of hyperbolic phonon polaritons, and not of bulk phonons as often reported. Thus, STEM-EELS offers the possibility to probe low-energy polaritons in vdW materials, with our theory being of fundamental importance for interpreting future experiments.

cond-mat.mes-hall↗

arXiv2011

Theoretical and numerical investigation of the size-dependent optical effects in metal nanoparticles

We further develop the theory of quantum finite-size effects in metallic nanoparticles, which was originally formulated by Hache, Ricard and Flytzanis [J. Opt. Soc. Am. B 3, 1647 (1986)] and (in a somewhat corrected form) by Rautian [Sov. Phys. JETP 85, 451 (1997)]. These references consider a metal nanoparticle as a degenerate Fermi gas of conduction electrons in an infinitely-high spherical potential well. This model (referred to as the HRFR model below) yields mathematical expressions for the linear and the third-order nonlinear polarizabilities of a nanoparticle in terms of infinite nested series. These series have not been evaluated numerically so far and, in the case of nonlinear polarizability, they can not be evaluated with the use of conventional computers due to the high computational complexity involved. Rautian has derived a set of remarkable analytical approximations to the series but direct numerical verification of Rautian's approximate formulas remained a formidable challenge. In this work, we derive an expression for the third-order nonlinear polarizability, which is exact within the HRFR model but amenable to numerical implementation. We then evaluate the expressions obtained by us numerically for both linear and nonlinear polarizabilities. We investigate the limits of applicability of Rautian's approximations and find that they are surprizingly accurate in a wide range of physical parameters. We also discuss the limits of small frequencies (comparable or below the Drude relaxation constant) and of large particle sizes (the bulk limit) and show that these limits are problematic for the HRFR model, irrespectively of any additional approximations used. Finally, we compare the HRFR model to the purely classical theory of nonlinear polarization of metal nanoparticles developed by us earlier [Phys. Rev. Lett. 100, 47402 (2008)].

physics.optics↗

arXiv2009

Phaseless three-dimensional optical nano-imaging

We propose a method for optical nano-imaging in which the structure of a three-dimensional inhomogeneous medium may be recovered from far-field power measurements. Neither phase control of the illuminating field nor phase measurements of the scattered field are necessary. The method is based on the solution to the inverse scattering problem for a system consisting of a weakly-scattering dielectric sample and a strongly-scattering nano-particle tip. Numerical simulations are used to illustrate the results.

cond-mat.mes-hall↗

arXiv2008

From Slow to Superluminal Propagation: Dispersive Properties of Surface Plasmon Polaritons in Linear Chains of Metallic Nanospheroids

We consider propagation of surface plasmon polaritons (SPPs) in linear periodic chains (LPCs) of prolate and oblate metallic spheroids. We show that the SPP group velocity can be efficiently controlled by varying the aspect ratio of the spheroids. For sufficiently small aspect ratios, a gap appears in the first Brillouin zone of the chain lattice in which propagating modes do not exist. depending on the SPP polarization, the gap extends to certain intervals of the Bloch wave number q. Thus, for transverse polarization, no propagating SPPs exist with wave numbers q such that q_c^\perp < | q | < π/h, h being the chain period. For longitudinally polarized SPPs, the gap spans the interval |q|<q_c^\parallel. Here q_c^\perp and q_c^\parallel are different constants which depend on the chain parameters, spheroid aspect ratio and its orientation with respect to the chain axis. The dependence of the dispersion curves on the spheroid aspect ratio leads to a number of interesting effects. In particular, bandwidth of SPPs that can propagate in an LPC can be substantially increased by utilizing prolate or oblate spheroids. When q is close to a critical value, so that |q - q_c^\perp|<<π/h or |q - q_c^\parallel|<<π/h, the decay length of the SPPs is dramatically increased. In addition, the dispersion curves acquire a very large positive or negative slope. This can be used to achieve superluminal group velocity for realistic chain parameters. We demonstrate superluminal propagation of Gaussian wave packets in numerical simulations. Both theory and simulations are based on Maxwell equations with account of retardation and, therefore, are fully relativistic.

physics.optics↗

arXiv2007

Active metamaterials: sign of refraction index and gain-assisted dispersion management

We derive an approach to define the causal direction of the wavevector of modes in optical metamaterials, which in turn, determines signs of refractive index and impedance as a function of {\it real and imaginary} parts of dielectric permittivity and magnetic permeability. We use the developed technique to demonstrate that the interplay between resonant response of constituents of metamaterials can be used to achieve efficient dispersion management. Finally we demonstrate broadband dispersion-less index and impedance matching in active nanowire-based negative index materials. Our work opens new practical applications of negative index composites for broadband lensing, imaging, and pulse-routing.

physics.optics↗

arXiv2006

Gain-assisted slow to superluminal group velocity manipulation in nano-waveguides

We study the energy propagation in subwavelength waveguides and demonstrate that the mechanism of material gain, previously suggested for loss compensation, is also a powerful tool to manipulate dispersion and propagation characteristics of electromagnetic pulses at the nanoscale. We show theoretically that the group velocity in lossy nano-waveguides can be controlled from slow to superluminal values by the material gain and waveguide geometry and develop an analytical description of the relevant physics. We utilize the developed formalism to show that gain-assisted dispersion management can be used to control the transition between ``photonic-funnel'' and ``photonic-compressor'' regimes in tapered nano-waveguides. The phenomenon of strong modulation of group velocity in subwavelength structures can be realized in waveguides with different geometries, and is present for both volume and surface-modes.

physics.optics↗

arXiv2005

Meta-material photonic funnels for sub-diffraction light compression and propagation

We present waveguides with photonic crystal cores, supporting energy propagation in subwavelength regions with a mode structure similar to that in telecom fibers. We design meta-materials for near-, mid-, and far-IR frequencies, and demonstrate efficient energy transfer to and from regions smaller than 1/25-th of the wavelength. Both positive- and negative-refractive index light transmissions are shown. Our approach, although demonstrated here in circular waveguides for some specific frequencies, is easily scalable from optical to IR to THz frequency ranges, and can be realized in a variety of waveguide geometries. Our design may be used for ultra high-density energy focusing, nm-resolution sensing, near-field microscopy, and high-speed all-optical computing.

physics.optics↗