arXiv subjects

Alexander Marsteller

Publications and source records attributed to Alexander Marsteller.

9 recordsLinked to original sources

arXiv2026

Gaseous Tritium Activity Monitoring with Scintillators (GaTAMoS)

We present a novel device for the inline activity monitoring of gaseous tritium, named Gaseous Tritium Activity Monitoring with Scintillators (GaTAMOS). Unlike established methods that often rely on liquid scintillation or plastic scintillators with limited chemical resistance, this system utilises a chemically inert, inorganic Terbium-activated Gadolinium Oxysulfide (Gd2O2S:Tb) ceramic. A specialised soldering technique was developed to join the ceramic scintillator to a stainless-steel flange, achieving a vacuum-tight seal fully compatible with high-purity tritium applications. The device was characterised using pure tritium gas, demonstrating a linear response and high sensitivity across a dynamic range from < 1 kBq to >10 GBq. A key advantage of the ceramic material over organic alternatives is its high tolerance to aggressive cleaning agents. We demonstrate that the inevitable tritium memory effect can be significantly mitigated by flushing the cell with ethanol, removing >95% of residual contamination within minutes. The proposed system offers a compact, robust, and cost-effective alternative to ionisation chambers or BIXS systems for process monitoring in tritium handling facilities.

physics.ins-det↗

arXiv2026

A precision 32 keV angular-selective photoelectron source for calibration measurements at the KATRIN experiment

The Karlsruhe Tritium Neutrino (KATRIN) experiment measures the neutrino mass from a precise measurement of the endpoint region of the kinematic tritium beta-decay spectrum by using a spectrometer combining magnetic adiabatic collimation and electrostatic filtering (MAC-E filter). For calibration purposes, KATRIN uses a monoenergetic angular-selective photoelectron source. We present an upgrade of this source, which was installed in the KATRIN beamline in February 2022. The source allows for a wide range of accessible electron energies up to 32 keV and a variation of the angle with regard to the magnetic field. These features are used for precise measurements of electron scattering effects off tritium molecules in KATRIN's gaseous tritium source, for investigations of angular-dependent backscattering for example at KATRIN's focal-plane detector, and for studies on adiabatic transport in the main spectrometer.

physics.ins-det↗

arXiv2025

First results of the Tritium Absorption InfraRed Spectroscopy (T2ApIR) experiment

The literature on experimentally verified material properties of tritium is sparse but information about this is crucial in fusion for pellet production (Magnetic Confined Fusion), target fueling (Inertial Confined Fusion), cryogenic distillation, as well as in astroparticle physics for neutrino experiments, and search for rare physics. To improve on this, the T$_2$ApIR experiment has been designed and built at the Tritium Laboratory Karlsruhe (TLK), and is in its scientific commissioning phase. The main focus of this experiment is to enable the investigation of the properties of all six hydrogen isotopologues and their mixtures in the gaseous, liquid, and solid phase, as well as the dynamics of their phase changes. In addition, mixtures with noble gases such as xenon and neon can be investigated. This is achieved using a cryogenic setup capable of reaching less than 10 in a measurement cell that allows optical access for infrared absorption spectroscopy, Raman spectroscopy and a polariscope setup, as well as temperature and pressure measurement.

physics.ins-det↗

arXiv2025

Commissioning of an experiment for thermodynamic and spectroscopic studies of hydrogen isotopologues at cryogenic conditions

To study thermodynamic properties and dynamic phase space behavior of hydrogen isotopologues (Q$_2$) at cryogenic temperatures and at high density, the Tritium Absorption InfraRed Spectroscopy 2 (T$_2$ApIR) experiment has been set up and commissioned at Tritium Laboratory Karlsruhe (TLK). In the frame of the experiment, Q$_2$ behavior in different phases, ortho/para states, temperatures (10 K - 300 K) and pressures (up to 2.5 bar a) will be investigated with optical methods, infrared and Raman spectroscopy. The facility consists of a fully tritium compatible cryostat, which includes an optical cell, ortho/para converter and windows for optical and spectroscopic studies. The cryostat can be cooled below the H$_2$ triple point by a two-stage cryocooler and contains openings in the cryogenic shielding for the optical access. The challenge of combining these scientific requirements in a design with high amounts of tritium (14 g), in a limited space, all while maintaining the TLK safety philosophy was solved by the presented design. The experiment is ready to be fully integrated into the TLK closed loop tritium infrastructure. This contribution reports a comprehensive overview of the commissioning phase of the experimental facility and the results of the first commissioning experiments, including cryogenic performance tests, commissioning experiments with non-radioactive gases, and tests of the analytical instruments.

cond-mat.stat-mech↗

arXiv2025

Sterile-neutrino search based on 259 days of KATRIN data

Neutrinos are the most abundant fundamental matter particles in the Universe and play a crucial role in particle physics and cosmology. Neutrino oscillation, discovered about 25 years ago, reveals that the three known species mix with each other. Anomalous results from reactor and radioactive-source experiments suggest a possible fourth neutrino state, the sterile neutrino, which does not interact via the weak force. The KATRIN experiment, primarily designed to measure the neutrino mass via tritium $β$-decay, also searches for sterile neutrinos suggested by these anomalies. A sterile-neutrino signal would appear as a distortion in the $β$-decay energy spectrum, characterized by a discontinuity in curvature (kink) related to the sterile-neutrino mass. This signature, which depends only on the shape of the spectrum rather than its absolute normalization, offers a robust, complementary approach to reactor experiments. KATRIN examined the energy spectrum of 36 million tritium $β$-decay electrons recorded in 259 measurement days within the last 40 electronvolt below the endpoint. The results exclude a substantial part of the parameter space suggested by the gallium anomaly and challenge the Neutrino-4 claim. Together with other neutrino-disappearance experiments, KATRIN probes sterile-to-active mass splittings from a fraction of an electron-volt squared to several hundred electron-volts squared, excluding light sterile neutrinos with mixing angles above a few percent.

hep-ex↗

arXiv2022

ViMA -- the spinning rotor gauge to measure the viscosity of tritium between 77 and 300 K

Experimental values for the viscosity of the radioactive hydrogen isotope tritium (T$_2$) are currently unavailable in literature. The value of this material property over a wide temperature range is of interest for applications in the field of fusion, neutrino physics, as well as to test ab initio calculations. As a radioactive gas, tritium requires careful experiment design to ensure safe and environmental contamination free measurements. In this contribution, we present a spinning rotor gauge based, tritium compatible design of a gas viscosity measurement apparatus (ViMA) capable of covering the temperature range from 80 K to 300 K.

physics.ins-det↗

arXiv2022

Operation Modes of the KATRIN Experiment Tritium Loop System using $^{83\mathrm{m}}$Kr

The KArlsruhe TRItium Neutrino (KATRIN) experiment aims to search for the effective electron antineutrino mass with a sensitivity of 0.2 eV (90 % C.L.). In order to achieve this goal, KATRIN measurement phases focusing on the neutrino mass search are alternated with phases of investigations of systematic effects. During these phases, metastable $^{83\mathrm{m}}$Kr is used as a calibration source. The monoenergetic conversion electrons emitted accompanying the decay of $^{83\mathrm{m}}$Kr allow a direct access to the starting conditions of $β$-electrons produced inside the windowless gaseous tritium source (WGTS) of KATRIN. To make use of $^{83\mathrm{m}}$Kr in the WGTS, the Tritium Loop System, which provides a stable flow of tritium to the WGTS, needs to be operated in special modes. This paper focuses on the technical implementation of these modes and their performance with regard to the achievable $^{83\mathrm{m}}$Kr-rates, gas densities, and gas compositions inside the WGTS.

physics.ins-det↗

arXiv2022

Viscosity measurements of gaseous H2 between 200 K to 300 K with a spinning rotor gauge

Experimental values for the viscosity of the radioactive hydrogen isotopologue tritium are still unknown in literature. Existing values from ab initio calculations disregard quantum mechanic effects and are therefore only good approximations for room temperature and above. To fill in these missing experimental values, a measurement setup has been designed, to measure the viscosity of gaseous hydrogen and its isotopologues (H$_2$, HD, HT, D$_2$, DT, T$_2$) at cryogenic temperatures. In this paper, the first results with this Cryogenic Viscosity Measurement Apparatus (Cryo-ViMA) of the viscosity of gaseous hydrogen between 200 K to 300 K are presented.

physics.ins-det↗

arXiv2020

Neutral tritium gas reduction in the KATRIN differential pumping sections

The KArlsruhe TRItium Neutrino experiment (KATRIN) aims to measure the effective electron anti-neutrino mass with an unprecedented sensitivity of $0.2\,\mathrm{eV}/\mathrm{c}^2$, using $β$-electrons from tritium decay. The electrons are guided magnetically by a system of superconducting magnets through a vacuum beamline from the windowless gaseous tritium source through differential and cryogenic pumping sections to a high resolution spectrometer and a segmented silicon pin detector. At the same time tritium gas has to be prevented from entering the spectrometer. Therefore, the pumping sections have to reduce the tritium flow by more than 14 orders of magnitude. This paper describes the measurement of the reduction factor of the differential pumping section performed with high purity tritium gas during the first measurement campaigns of the KATRIN experiment. The reduction factor results are compared with previously performed simulations, as well as the stringent requirements of the KATRIN experiment.

physics.ins-det↗