SearcharxivSearch

arXiv · 2606.16616

Gaseous Tritium Activity Monitoring with Scintillators (GaTAMoS)

Abstract

We present a novel device for the inline activity monitoring of gaseous tritium, named Gaseous Tritium Activity Monitoring with Scintillators (GaTAMOS). Unlike established methods that often rely on liquid scintillation or plastic scintillators with limited chemical resistance, this system utilises a chemically inert, inorganic Terbium-activated Gadolinium Oxysulfide (Gd2O2S:Tb) ceramic. A specialised soldering technique was developed to join the ceramic scintillator to a stainless-steel flange, achieving a vacuum-tight seal fully compatible with high-purity tritium applications. The device was characterised using pure tritium gas, demonstrating a linear response and high sensitivity across a dynamic range from < 1 kBq to >10 GBq. A key advantage of the ceramic material over organic alternatives is its high tolerance to aggressive cleaning agents. We demonstrate that the inevitable tritium memory effect can be significantly mitigated by flushing the cell with ethanol, removing >95% of residual contamination within minutes. The proposed system offers a compact, robust, and cost-effective alternative to ionisation chambers or BIXS systems for process monitoring in tritium handling facilities.

Explore related subjects

Keep this discovery

BibTeXRIS

Florian Priester, Alexander Marsteller, Johanna Wydra, Robin Größle. 2026-06-15. Gaseous Tritium Activity Monitoring with Scintillators (GaTAMoS). https://arxiv.org/abs/2606.16616

Cite the original work for its findings. Save a collection to share your selection of sources.

KEEP EXPLORING

Related papers

High-Speed Semi-FE Readout Module for ATLAS MDT at HL-LHC: Design and Production-Level Characterization

The High-Luminosity upgrade of the Large Hadron Collider (HL-LHC) introduces increased demands on the ATLAS Muon Spectrometer, particularly in terms of data throughput, timing distribution and system reliability. The Phase-II Chamber Service Module (CSM) is a key component of the upgraded Monitored Drift Tube (MDT) trigger and readout system, providing a high-speed interface between the front-end electronics and the backend systems. This paper describes the design and implementation of the Phase-II CSM, together with its validation. The results show that the CSM supports two independent optical uplinks, each operating at a line rate of 10.24 Gbps, together with clock distribution and slow control in the expected operating environment. Integration with small-diameter MDT (sMDT) chambers and tests with the prototype L0MDT trigger system are also presented. The CSM boards are now in production and will be used for installation and integration during the upcoming LHC Long Shutdown.

physics.ins-det

Spectral Discrimination of Deposited Gamma-Ray Energies in a Simulated CeBr$_3$ Scintillator

We show that wavelength measurements of individual detected optical photons may provide additional information about gamma-ray energy deposited in a CeBr$_3$ crystal when the detected-photon-count distributions overlap for nearby gamma-ray energies. Monoenergetic 662 and 629 keV gammas are used in a Geant4 simulation of a $25\times25\times20~\mathrm{mm^3}$ CeBr$_3$ crystal. Assuming a light yield of $6.0\times10^4$ photons/MeV, a wavelength-independent photon-detection efficiency of 30%, and a wavelength resolution of $\sigma_{\lambda}=40$ nm, we find that the fraction of photons reconstructed above 385 nm gives an event-level separation of $\sim$ 2 standard deviations between the 662 and 629 keV event populations selected within the same $\sim$ 1%-wide detected-photon-count interval. No timing or reconstructed interaction-position information is used. The result demonstrates, within the present simulation model, that event-dependent optical spectra can retain energy information beyond an undifferentiated photon count.

physics.ins-det

Operation of a negative ion gas time projection chamber without electronegative fill gases

The high fidelity reconstruction of particle tracks in micropatterned gaseous time projection chambers renders this technology ideal for future rare-event searches, including direction-sensitive dark matter experiments. Large drift distances are typically required for such experiments, so that the overall spatial resolution is limited by diffusion. Negative ion drift exhibits lower diffusion than electron drift and is thus an attractive option for realising a large-scale detector. The use of electronegative gases to create negative ions introduces technical challenges, most notably a reduction in gain when compared to conventional gas mixtures. In this study, we demonstrate a new method for negative ion generation via dissociative electron attachment using the conventional molecular fill gas CF$_4$. Our optical measurements of negative ion drift indicate electron attachment lengths of $<$1 mm and comparable gain to electron avalanches. The individual negative ion avalanches were also time-resolved, allowing the number of ions reaching the readout to be counted. We measure an improved energy resolution by single ion counting, relative to an integrated electron avalanche signal measured under identical gain conditions.

physics.ins-det