arXiv subjects

Alexander Melville

Publications and source records attributed to Alexander Melville.

At least 19 recordsLinked to original sources

arXiv2025

Machine Learning Enables Optimization of Diamond for Quantum Applications

Spins in solid-state materials, molecules, and other chemical systems have the potential to impact the fields of quantum sensing, communication, simulation, and computing. In particular, color centers in diamond, such as negatively charged nitrogen vacancy (NV$^-$) and silicon vacancy centers (SiV$^-$), are emerging as quantum platforms poised for transition to commercial devices. A key enabler stems from the semiconductor-like platform that can be tailored at the time of growth. The large growth parameter space makes it challenging to use intuition to optimize growth conditions for quantum performance. In this paper, we use supervised machine learning to train regression models using different synthesis parameters in over 100 quantum diamond samples. We train models to optimize NV$^-$ defects in diamond for high sensitivity magnetometry. Importantly, we utilize a magnetic-field sensitivity figure of merit (FOM) for NV magnetometry and use Bayesian optimization to identify critical growth parameters that lead to a 300% improvement over an average sample and a 55% improvement over the previous champion sample. Furthermore, using Shapley importance rankings, we gain new physical insights into the most impactful growth and post-processing parameters, namely electron irradiation dose, diamond seed depth relative to the plasma, seed miscut angle, and reactor nitrogen concentration. As various quantum devices can have significantly different material requirements, advanced growth techniques such as plasma-enhanced chemical vapor deposition (PE-CVD) can provide the ability to tailor material development specifically for quantum applications.

cond-mat.mtrl-sci↗

arXiv2024

An integrated photonic engine for programmable atomic control

Solutions for scalable, high-performance optical control are important for the development of scaled atom-based quantum technologies. Modulation of many individual optical beams is central to the application of arbitrary gate and control sequences on arrays of atoms or atom-like systems. At telecom wavelengths, miniaturization of optical components via photonic integration has pushed the scale and performance of classical and quantum optics far beyond the limitations of bulk devices. However, these material platforms for high-speed telecom integrated photonics are not transparent at the short wavelengths required by leading atomic systems. Here, we propose and implement a scalable and reconfigurable photonic architecture for multi-channel quantum control using integrated, visible-light modulators based on thin-film lithium niobate. Our approach combines techniques in free-space optics, holography, and control theory together with a sixteen-channel integrated photonic device to stabilize temporal and cross-channel power deviations and enable precise and uniform control. Applying this device to a homogeneous constellation of silicon-vacancy artificial atoms in diamond, we present techniques to spatially and spectrally address a dynamically-selectable set of these stochastically-positioned point emitters. We anticipate that this scalable and reconfigurable optical architecture will lead to systems that could enable parallel individual programmability of large many-body atomic systems, which is a critical step towards universal quantum computation on such hardware.

quant-ph↗

arXiv2023

Characterization of superconducting through-silicon vias as capacitive elements in quantum circuits

The large physical size of superconducting qubits and their associated on-chip control structures presents a practical challenge towards building a large-scale quantum computer. In particular, transmons require a high-quality-factor shunting capacitance that is typically achieved by using a large coplanar capacitor. Other components, such as superconducting microwave resonators used for qubit state readout, are typically constructed from coplanar waveguides which are millimeters in length. Here we use compact superconducting through-silicon vias to realize lumped element capacitors in both qubits and readout resonators to significantly reduce the on-chip footprint of both of these circuit elements. We measure two types of devices to show that TSVs are of sufficient quality to be used as capacitive circuit elements and provide a significant reductions in size over existing approaches.

quant-ph↗

arXiv2023

High-Fidelity, Frequency-Flexible Two-Qubit Fluxonium Gates with a Transmon Coupler

We propose and demonstrate an architecture for fluxonium-fluxonium two-qubit gates mediated by transmon couplers (FTF, for fluxonium-transmon-fluxonium). Relative to architectures that exclusively rely on a direct coupling between fluxonium qubits, FTF enables stronger couplings for gates using non-computational states while simultaneously suppressing the static controlled-phase entangling rate ($ZZ$) down to kHz levels, all without requiring strict parameter matching. Here we implement FTF with a flux-tunable transmon coupler and demonstrate a microwave-activated controlled-Z (CZ) gate whose operation frequency can be tuned over a 2 GHz range, adding frequency allocation freedom for FTF's in larger systems. Across this range, state-of-the-art CZ gate fidelities were observed over many bias points and reproduced across the two devices characterized in this work. After optimizing both the operation frequency and the gate duration, we achieved peak CZ fidelities in the 99.85-99.9\% range. Finally, we implemented model-free reinforcement learning of the pulse parameters to boost the mean gate fidelity up to $99.922\pm0.009\%$, averaged over roughly an hour between scheduled training runs. Beyond the microwave-activated CZ gate we present here, FTF can be applied to a variety of other fluxonium gate schemes to improve gate fidelities and passively reduce unwanted $ZZ$ interactions.

quant-ph↗

arXiv2023

Evolution of $1/f$ Flux Noise in Superconducting Qubits with Weak Magnetic Fields

The microscopic origin of $1/f$ magnetic flux noise in superconducting circuits has remained an open question for several decades despite extensive experimental and theoretical investigation. Recent progress in superconducting devices for quantum information has highlighted the need to mitigate sources of qubit decoherence, driving a renewed interest in understanding the underlying noise mechanism(s). Though a consensus has emerged attributing flux noise to surface spins, their identity and interaction mechanisms remain unclear, prompting further study. Here we apply weak in-plane magnetic fields to a capacitively-shunted flux qubit (where the Zeeman splitting of surface spins lies below the device temperature) and study the flux-noise-limited qubit dephasing, revealing previously unexplored trends that may shed light on the dynamics behind the emergent $1/f$ noise. Notably, we observe an enhancement (suppression) of the spin-echo (Ramsey) pure dephasing time in fields up to $B=100~\text{G}$. With direct noise spectroscopy, we further observe a transition from a $1/f$ to approximately Lorentzian frequency dependence below 10 Hz and a reduction of the noise above 1 MHz with increasing magnetic field. We suggest that these trends are qualitatively consistent with an increase of spin cluster sizes with magnetic field. These results should help to inform a complete microscopic theory of $1/f$ flux noise in superconducting circuits.

cond-mat.mes-hall↗

arXiv2022

Lindblad Tomography of a Superconducting Quantum Processor

As progress is made towards the first generation of error-corrected quantum computers, robust characterization and validation protocols are required to assess the noise environments of physical quantum processors. While standard coherence metrics and characterization protocols such as T1 and T2, process tomography, and randomized benchmarking are now ubiquitous, these techniques provide only partial information about the dynamic multi-qubit loss channels responsible for processor errors, which can be described more fully by a Lindblad operator in the master equation formalism. Here, we introduce and experimentally demonstrate Lindblad tomography, a hardware-agnostic characterization protocol for tomographically reconstructing the Hamiltonian and Lindblad operators of a quantum noise environment from an ensemble of time-domain measurements. Performing Lindblad tomography on a small superconducting quantum processor, we show that this technique characterizes and accounts for state-preparation and measurement (SPAM) errors and allows one to place bounds on the fit to a Markovian model. Comparing the results of single- and two-qubit measurements on a superconducting quantum processor, we demonstrate that Lindblad tomography can also be used to identify and quantify sources of crosstalk on quantum processors, such as the presence of always-on qubit-qubit interactions.

quant-ph↗

arXiv2022

Large-scale optical characterization of solid-state quantum emitters

Solid-state quantum emitters have emerged as a leading quantum memory for quantum networking applications. However, standard optical characterization techniques are neither efficient nor repeatable at scale. In this work, we introduce and demonstrate spectroscopic techniques that enable large-scale, automated characterization of color centers. We first demonstrate the ability to track color centers by registering them to a fabricated machine-readable global coordinate system, enabling systematic comparison of the same color center sites over many experiments. We then implement resonant photoluminescence excitation in a widefield cryogenic microscope to parallelize resonant spectroscopy, achieving two orders of magnitude speed-up over confocal microscopy. Finally, we demonstrate automated chip-scale characterization of color centers and devices at room temperature, imaging thousands of microscope fields of view. These tools will enable accelerated identification of useful quantum emitters at chip-scale, enabling advances in scaling up color center platforms for quantum information applications, materials science, and device design and characterization.

quant-ph↗

arXiv2022

On-Demand Directional Microwave Photon Emission Using Waveguide Quantum Electrodynamics

Routing quantum information between non-local computational nodes is a foundation for extensible networks of quantum processors. Quantum information transfer between arbitrary nodes is generally mediated either by photons that propagate between them, or by resonantly coupling nearby nodes. The utility is determined by the type of emitter, propagation channel, and receiver. Conventional approaches involving propagating microwave photons have limited fidelity due to photon loss and are often unidirectional, whereas architectures that use direct resonant coupling are bidirectional in principle, but can generally accommodate only a few local nodes. Here we demonstrate high-fidelity, on-demand, directional, microwave photon emission. We do this using an artificial molecule comprising two superconducting qubits strongly coupled to a bidirectional waveguide, effectively creating a chiral microwave waveguide. Quantum interference between the photon emission pathways from the molecule generates single photons that selectively propagate in a chosen direction. This circuit will also be capable of photon absorption, making it suitable for building interconnects within extensible quantum networks.

quant-ph↗

arXiv2022

Demonstration of tunable three-body interactions between superconducting qubits

Nonpairwise multi-qubit interactions present a useful resource for quantum information processors. Their implementation would facilitate more efficient quantum simulations of molecules and combinatorial optimization problems, and they could simplify error suppression and error correction schemes. Here we present a superconducting circuit architecture in which a coupling module mediates 2-local and 3-local interactions between three flux qubits by design. The system Hamiltonian is estimated via multi-qubit pulse sequences that implement Ramsey-type interferometry between all neighboring excitation manifolds in the system. The 3-local interaction is coherently tunable over several MHz via the coupler flux biases and can be turned off, which is important for applications in quantum annealing, analog quantum simulation, and gate-model quantum computation.

quant-ph↗

arXiv2021

Quantum transport and localization in 1d and 2d tight-binding lattices

Particle transport and localization phenomena in condensed-matter systems can be modeled using a tight-binding lattice Hamiltonian. The ideal experimental emulation of such a model utilizes simultaneous, high-fidelity control and readout of each lattice site in a highly coherent quantum system. Here, we experimentally study quantum transport in one-dimensional and two-dimensional tight-binding lattices, emulated by a fully controllable $3 \times 3$ array of superconducting qubits. We probe the propagation of entanglement throughout the lattice and extract the degree of localization in the Anderson and Wannier-Stark regimes in the presence of site-tunable disorder strengths and gradients. Our results are in quantitative agreement with numerical simulations and match theoretical predictions based on the tight-binding model. The demonstrated level of experimental control and accuracy in extracting the system observables of interest will enable the exploration of larger, interacting lattices where numerical simulations become intractable.

quant-ph↗

arXiv2021

Deep Neural Network Discrimination of Multiplexed Superconducting Qubit States

Demonstrating a quantum computational advantage will require high-fidelity control and readout of multi-qubit systems. As system size increases, multiplexed qubit readout becomes a practical necessity to limit the growth of resource overhead. Many contemporary qubit-state discriminators presume single-qubit operating conditions or require considerable computational effort, limiting their potential extensibility. Here, we present multi-qubit readout using neural networks as state discriminators. We compare our approach to contemporary methods employed on a quantum device with five superconducting qubits and frequency-multiplexed readout. We find that fully-connected feedforward neural networks increase the qubit-state-assignment fidelity for our system. Relative to contemporary discriminators, the assignment error rate is reduced by up to 25% due to the compensation of system-dependent nonidealities such as readout crosstalk which is reduced by up to one order of magnitude. Our work demonstrates a potentially extensible building block for high-fidelity readout relevant to both near-term devices and future fault-tolerant systems.

quant-ph↗

arXiv2021

Realization of high-fidelity CZ and ZZ-free iSWAP gates with a tunable coupler

High-fidelity two-qubit gates at scale are a key requirement to realize the full promise of quantum computation and simulation. The advent and use of coupler elements to tunably control two-qubit interactions has improved operational fidelity in many-qubit systems by reducing parasitic coupling and frequency crowding issues. Nonetheless, two-qubit gate errors still limit the capability of near-term quantum applications. The reason, in part, is the existing framework for tunable couplers based on the dispersive approximation does not fully incorporate three-body multi-level dynamics, which is essential for addressing coherent leakage to the coupler and parasitic longitudinal ($ZZ$) interactions during two-qubit gates. Here, we present a systematic approach that goes beyond the dispersive approximation to exploit the engineered level structure of the coupler and optimize its control. Using this approach, we experimentally demonstrate CZ and $ZZ$-free iSWAP gates with two-qubit interaction fidelities of $99.76 \pm 0.07$% and $99.87 \pm 0.23$%, respectively, which are close to their $T_1$ limits.

quant-ph↗

arXiv2021

Probing quantum information propagation with out-of-time-ordered correlators

Interacting many-body quantum systems show a rich array of physical phenomena and dynamical properties, but are notoriously difficult to study: they are challenging analytically and exponentially difficult to simulate on classical computers. Small-scale quantum information processors hold the promise to efficiently emulate these systems, but characterizing their dynamics is experimentally challenging, requiring probes beyond simple correlation functions and multi-body tomographic methods. Here, we demonstrate the measurement of out-of-time-ordered correlators (OTOCs), one of the most effective tools for studying quantum system evolution and processes like quantum thermalization. We implement a 3x3 two-dimensional hard-core Bose-Hubbard lattice with a superconducting circuit, study its time-reversibility by performing a Loschmidt echo, and measure OTOCs that enable us to observe the propagation of quantum information. A central requirement for our experiments is the ability to coherently reverse time evolution, which we achieve with a digital-analog simulation scheme. In the presence of frequency disorder, we observe that localization can partially be overcome with more particles present, a possible signature of many-body localization in two dimensions.

quant-ph↗

arXiv2020

Programming a quantum computer with quantum instructions

The equivalence between the instructions used to define programs and the input data on which the instructions operate is a basic principle of classical computer architectures and programming. Replacing classical data with quantum states enables fundamentally new computational capabilities with scaling advantages for many applications, and numerous models have been proposed for realizing quantum computation. However, within each of these models, the quantum data are transformed by a set of gates that are compiled using solely classical information. Conventional quantum computing models thus break the instruction-data symmetry: classical instructions and quantum data are not directly interchangeable. In this work, we use a density matrix exponentiation protocol to execute quantum instructions on quantum data. In this approach, a fixed sequence of classically-defined gates performs an operation that uniquely depends on an auxiliary quantum instruction state. Our demonstration relies on a 99.7% fidelity controlled-phase gate implemented using two tunable superconducting transmon qubits, which enables an algorithmic fidelity surpassing 90% at circuit depths exceeding 70. The utilization of quantum instructions obviates the need for costly tomographic state reconstruction and recompilation, thereby enabling exponential speedup for a broad range of algorithms, including quantum principal component analysis, the measurement of entanglement spectra, and universal quantum emulation.

quant-ph↗

arXiv2020

Universal non-adiabatic control of small-gap superconducting qubits

Resonant transverse driving of a two-level system as viewed in the rotating frame couples two degenerate states at the Rabi frequency, an amazing equivalence that emerges in quantum mechanics. While spectacularly successful at controlling natural and artificial quantum systems, certain limitations may arise (e.g., the achievable gate speed) due to non-idealities like the counter-rotating term. Here, we explore a complementary approach to quantum control based on non-resonant, non-adiabatic driving of a longitudinal parameter in the presence of a fixed transverse coupling. We introduce a superconducting composite qubit (CQB), formed from two capacitively coupled transmon qubits, which features a small avoided crossing -- smaller than the environmental temperature -- between two energy levels. We control this low-frequency CQB using solely baseband pulses, non-adiabatic transitions, and coherent Landau-Zener interference to achieve fast, high-fidelity, single-qubit operations with Clifford fidelities exceeding $99.7\%$. We also perform coupled qubit operations between two low-frequency CQBs. This work demonstrates that universal non-adiabatic control of low-frequency qubits is feasible using solely baseband pulses.

quant-ph↗

arXiv2020

Solid-state qubits integrated with superconducting through-silicon vias

As superconducting qubit circuits become more complex, addressing a large array of qubits becomes a challenging engineering problem. Dense arrays of qubits benefit from, and may require, access via the third dimension to alleviate interconnect crowding. Through-silicon vias (TSVs) represent a promising approach to three-dimensional (3D) integration in superconducting qubit arrays -- provided they are compact enough to support densely-packed qubit systems without compromising qubit performance or low-loss signal and control routing. In this work, we demonstrate the integration of superconducting, high-aspect ratio TSVs -- 10 $μ$m wide by 20 $μ$m long by 200 $μ$m deep -- with superconducting qubits. We utilize TSVs for baseband control and high-fidelity microwave readout of qubits using a two-chip, bump-bonded architecture. We also validate the fabrication of qubits directly upon the surface of a TSV-integrated chip. These key 3D integration milestones pave the way for the control and readout of high-density superconducting qubit arrays using superconducting TSVs.

quant-ph↗

arXiv2020

Comparison of Dielectric Loss in Titanium Nitride and Aluminum Superconducting Resonators

Lossy dielectrics are a significant source of decoherence in superconducting quantum circuits. In this report, we model and compare the dielectric loss in bulk and interfacial dielectrics in titanium nitride (TiN) and aluminum (Al) superconducting coplanar waveguide (CPW) resonators. We fabricate isotropically trenched resonators to produce a series of device geometries that accentuate a specific dielectric region's contribution to resonator quality factor. While each dielectric region contributes significantly to loss in TiN devices, the metal-air interface dominates the loss in the Al devices. Furthermore, we evaluate the quality factor of each TiN resonator geometry with and without a post-process hydrofluoric (HF) etch, and find that it reduced losses from the substrate-air interface, thereby improving the quality factor.

quant-ph↗

arXiv2020

Waveguide Quantum Electrodynamics with Giant Superconducting Artificial Atoms

Models of light-matter interactions typically invoke the dipole approximation, within which atoms are treated as point-like objects when compared to the wavelength of the electromagnetic modes that they interact with. However, when the ratio between the size of the atom and the mode wavelength is increased, the dipole approximation no longer holds and the atom is referred to as a "giant atom". Thus far, experimental studies with solid-state devices in the giant-atom regime have been limited to superconducting qubits that couple to short-wavelength surface acoustic waves, only probing the properties of the atom at a single frequency. Here we employ an alternative architecture that realizes a giant atom by coupling small atoms to a waveguide at multiple, but well separated, discrete locations. Our realization of giant atoms enables tunable atom-waveguide couplings with large on-off ratios and a coupling spectrum that can be engineered by device design. We also demonstrate decoherence-free interactions between multiple giant atoms that are mediated by the quasi-continuous spectrum of modes in the waveguide-- an effect that is not possible to achieve with small atoms. These features allow qubits in this architecture to switch between protected and emissive configurations in situ while retaining qubit-qubit interactions, opening new possibilities for high-fidelity quantum simulations and non-classical itinerant photon generation.

quant-ph↗