arXiv subjects

Alexander Mook

Publications and source records attributed to Alexander Mook.

At least 37 records · Page 2Linked to original sources

arXiv2025

Spontaneous magnon decays from nonrelativistic time-reversal symmetry breaking in altermagnets

Quasiparticles are central to condensed matter physics, but their stability can be undermined by quantum many-body interactions. Magnons, quasiparticles in quantum magnets, are particularly intriguing because their properties are governed by both real and spin space. While crystal symmetries may be low, spin interactions often remain approximately isotropic, limiting spontaneous magnon decay. Textbook wisdom holds that collinear Heisenberg magnets follow a dichotomy: ferromagnets host stable magnons, while antiferromagnetic magnons may decay depending on dispersion curvature. Up to now, relativistic spin-orbit coupling and noncollinear order that connect spin space to real space, were shown to introduce more complex magnon instability mechanisms. Here, we show that even in nonrelativistic isotropic collinear systems, this conventional dichotomy is disrupted in altermagnets. Altermagnets, a newly identified class of collinear magnets, exhibit compensated spin order with nonrelativistic time-reversal symmetry breaking and even-parity band splitting. Using kinematic analysis, nonlinear spin-wave theory, and quantum simulations, we reveal that even weak band splitting opens a decay phase space, driving quasiparticle breakdown. Additionally, d-wave altermagnets form a rare ``island of stability'' at the Brillouin zone center. Our findings establish a quasiparticle stability trichotomy in collinear Heisenberg magnets and position altermagnets as a promising platform for unconventional spin dynamics.

cond-mat.str-el↗

arXiv2025

Large Thermal Hall Effect in MnPS$_3$

Recent studies have demonstrated that the thermal Hall effect can originate from magnons (magnon Hall effect), phonons (phonon Hall effect), or their combination (magnon-polaron Hall effect). The magnon-polaron Hall effect, first observed in Fe2Mo3O8, is particularly intriguing as its thermal Hall signal can be remarkably large. In this study, we explore the thermal Hall effect in MnPS3, an insulating antiferromagnetic material exhibiting a spin-flop transition and significant magnetoelastic coupling, making it a strong candidate for studying the thermal Hall effect originating from spin-lattice coupling. We report an exceptionally large thermal Hall angle down to 4 K and show that it cannot be accounted for by standard calculations based on the intrinsic magnon-polaron Berry curvature. Our findings provide an in-depth analysis of the role of the spin-flop transition in the thermal properties of MnPS3 and call for further theory development on magnon-phonon coupling and scattering to reveal their influence on transverse heat transport.

cond-mat.mtrl-sci↗

arXiv2025

Spin demons in d-wave altermagnets

Demons are a type of plasmons, which consist of out-of-phase oscillations of electrons in different bands. Here, we show that $d$-wave altermagnets, a recently discovered class of collinear magnetism, naturally realize a spin demon, which consists of out-of-phase movement of the two spin species. The spin demon lives outside of the particle-hole continuum of one of the spin species, and is therefore significantly underdamped, reaching quality factors of $>10$. We show that the spin demon carries a magnetic moment, which inherits the $d$-wave symmetry. Finally, we consider both three and two dimensional $d$-wave altermagnets, and show that spin demons exists in both.

cond-mat.str-el↗

arXiv2025

Altermagnetic splitting of magnons in hematite ($α$-Fe$_2$O$_3$)

We develop a four-sublattice spin-wave theory for the $g$-wave altermagnet candidate hematite ($α$-Fe$_2$O$_3$), considering both its easy-axis phase below and its weak ferromagnetic phase above the Morin temperature. A key question is whether the defining altermagnetic feature - magnon spin splitting (also called chirality or polarization splitting) due to nonrelativistic time-reversal symmetry breaking - remains intact when relativistic corrections, which contribute to hematite's magnetic order, are included. Using a detailed symmetry analysis supported by density functional theory, we show that capturing the magnon splitting within a Heisenberg model requires exchange interactions extending at least to the 13th neighbor. We find an altermagnetic band splitting of approximately 2 meV, which contrasts with the total band width of about 100 meV. To evaluate the experimental observability of this splitting, we analyze relativistic corrections to the magnon spectrum in both magnetic phases. We show that spin-orbit coupling - manifesting as magnetocrystalline anisotropies and the Dzyaloshinskii-Moriya interaction (DMI) - does not obscure the key altermagnetic features. These findings indicate that inelastic neutron scattering can directly probe altermagnetic magnon splitting in hematite. We also discuss implications for magnon transport, particularly magnonic contributions to the thermal Hall effect (which requires spin-orbit coupling) and to spin splitter effects (which do not). Notably, we predict a third-order nonlinear magnon spin splitter effect. This result suggests that the $g$-wave magnon spin splitting in hematite enables transverse heat-to-spin conversion without requiring an external magnetic field.

cond-mat.str-el↗

arXiv2025

Thermal Hall Effect of Magnons from Many-Body Skew Scattering

We present a theory of magnonic thermal Hall transport driven by many-body skew scattering. In field-polarized chiral magnets, the Dzyaloshinskii-Moriya interaction induces three-magnon interactions that violate time-reversal symmetry and interfere with the four-magnon scattering, thereby breaking microscopic detailed balance and causing thermal Hall currents. This mechanism operates without disorder or Berry curvature and is intrinsic to interacting spin systems. We argue that it can be as significant as the band-geometric anomalous velocity, highlighting the importance of magnon interactions in thermal Hall physics.

cond-mat.str-el↗

arXiv2024

Tunable band topology and optical conductivity in altermagnets

We study two-dimensional $d$-wave altermagnetic metals taking into account the presence of substrate-induced Rashba spin-orbit coupling. We consider the altermagnet bandstructure using a 2D band Hamiltonian near the $Γ$ point under external magnetic field. It is shown that time-reversal-symmetry breaking due to altermagnetism, together with Rashba coupling and external magnetic field, can result in non-trivial band topology. The topological phases can be tuned by magnetic field strength and directions, and are classified by their Chern numbers. Furthermore, we investigate the charge response by computing the full optical conductivity tensor with and without magnetic field. In particular, we focus on magneto-optical responses, which are the finite-frequency analog of the Berry curvature-induced anomalous Hall conductivity. Finally, using experimentally realistic parameters for RuO$_2$, we estimate the Faraday angle in the absence of magnetic fields.

cond-mat.str-el↗

arXiv2024

Electrical Non-Hermitian Control of Topological Magnon Spin Transport

Magnonic topological phases realize chiral edge spin waves that are protected against backscattering, potentially enabling highly efficient spin transport. Here we show that the spin transport through these magnonic chiral edge states can be electrically manipulated by non-Hermitian control. We consider the paradigmatic magnon Haldane model and show that it is transformed into an effective non-Hermitian magnon Chern insulator by including a sublattice-dependent spin-orbit torque. In linear spin-wave theory, this electrically induced torque reduces the damping of the chiral edge magnons along certain edge directions, leading to an enhancement of the spin-wave amplitude. This prediction is confirmed by numerical simulations based on the Landau-Lifshitz-Gilbert equation. For a spin-wave transport setup, in which magnons are excited by a microwave field and detected with a normal metal conductor, we find that the magnon amplification is remarkably robust against disorder, establishing non-Hermitian control as a promising avenue for topological magnonics.

cond-mat.mes-hall↗

arXiv2024

Spontaneous Crystal Thermal Hall Effect in Insulating Altermagnets

We show that magnetic insulators with a collinear and compensated order can exhibit a thermal Hall effect even at zero magnetic field if they have altermagnetic symmetries. We predict a finite thermal Hall conductivity vector $\boldsymbolκ_\text{H}$ for a rutile-inspired effective spin model with Dzyaloshinskii-Moriya interaction. Within the linear spin-wave theory, we identify two magnon branches that carry identical Berry curvature and give rise to a finite $\boldsymbolκ_\text{H}$, which can be controlled by the Néel vector orientation and by strain. The thermal Hall response is further complemented with a spin Nernst response to contrast spin and heat transport in altermagnetic insulators with those in ferromagnets and antiferromagnets. Our results establish the crystal thermal Hall effect of magnons and we discuss material candidates for experimental realization, such as MnF$_2$, CoF$_2$, and NiF$_2$.

cond-mat.mes-hall↗

arXiv2023

Electrical Activity of Topological Chiral Edge Magnons

Topological magnon insulators support chiral edge excitations, whose lack of electric charge makes them notoriously difficult to detect experimentally. We show that relativistic magnetoelectric coupling universally renders chiral edge magnons electrically active, thereby facilitating electrical probes of magnon topology. Considering a two-dimensional out-of-plane magnetized topological magnon insulator, we predict a fluctuation-activated electric polarization perpendicular to the sample edges. Furthermore, the chiral topological electromagnons give rise to a unique in-gap signal in electrical absorption experiments. These results suggest THz spectroscopy as a promising probe for topological magnons.

cond-mat.mes-hall↗

arXiv2023

Spontaneous Formation of Altermagnetism from Orbital Ordering

Altermagnetism has emerged as a third type of collinear magnetism. In contrast to standard ferromagnets and antiferromagnets, altermagnets exhibit extra even-parity wave spin order parameters resulting in a spin-splitting of electronic bands in momentum space. In real space, sublattices of opposite spin polarization are anisotropic and related by rotational symmetry. In the hitherto identified altermagnetic candidate materials the anisotropies arise from the local crystallographic symmetry. Here, we show that altermagnetism can also form as an interaction-induced electronic instability in a lattice without the crystallographic sublattice anisotropy. We provide a microscopic example of a two-orbital model showing that the coexistence of staggered antiferromagnetic and orbital order can realize robust altermagnetism. We quantify the spin-splitter conductivity as a key experimental observable and discuss material candidates for the interaction-induced realization of altermagnetism.

cond-mat.str-el↗

arXiv2023

Zero-frequency chiral magnonic edge states protected by non-equilibrium topology

Topological bosonic excitations must, in contrast to their fermionic counterparts, appear at finite energies. This is a key challenge for magnons, as it prevents straightforward excitation and detection of topologically-protected magnonic edge states and their use in magnonic devices. In this work, we show that in a non-equilibrium state, in which the magnetization is pointing against the external magnetic field, the topologically-protected chiral edge states in a magnon Chern insulator can be lowered to zero frequency, making them directly accessible by existing experimental techniques. We discuss the spin-orbit torque required to stabilize this non-equilibrium state, and show explicitly using numerical Landau-Lifshitz-Gilbert simulations that the edge states can be excited with a microwave field. Finally, we consider a propagating spin wave spectroscopy experiment, and demonstrate that the edge states can be directly detected.

cond-mat.mes-hall↗

arXiv2023

Breakdown of Chiral Edge Modes in Topological Magnon Insulators

Topological magnon insulators (TMI) are ordered magnets supporting chiral edge magnon excitations. These edge states are envisioned to serve as topologically protected information channels in low-loss magnonic devices. The standard description of TMI is based on linear spin-wave theory (LSWT), which approximates magnons as free non-interacting particles. However, magnon excitations of TMI are genuinely interacting even at zero temperature, calling into question descriptions based on LSWT alone. Here we perform a detailed non-linear spin-wave analysis to investigate the stability of chiral edge magnons. We identify three general breakdown mechanisms: (1) The edge magnon couples to itself, generating a finite lifetime that can be large enough to lead to a spectral annihilation of the chiral state; (2) The edge magnon hybridizes with the extended bulk magnons and, as a consequence, delocalizes away from the edge; (3) Due to a bulk-magnon mediated edge-to-edge coupling, the chiral magnons at opposite edges hybridize. We argue that, in general, these breakdown mechanisms may invalidate predictions based on LSWT and violate the notion of topological protection. We discuss strategies how the breakdown of chiral edge magnons can be avoided, e.g. via the application of large magnetic fields. Our results highlight a challenge for the realization of chiral edge states in TMI and in other bosonic topological systems without particle number conservation.

cond-mat.str-el↗

arXiv2022

Spurious Symmetry Enhancement and Interaction-Induced Topology in Magnons

Linear spin wave theory (LSWT) is the standard technique to compute the spectra of magnetic excitations in quantum materials. In this paper, we show that LSWT, even under ordinary circumstances, may fail to implement the symmetries of the underlying ordered magnetic Hamiltonian leading to spurious degeneracies. In common with pseudo-Goldstone modes in cases of quantum order-by-disorder these degeneracies tend to be lifted by magnon-magnon interactions. We show how, instead, the correct symmetries may be restored at the level of LSWT. In the process we give examples, supported by nonperturbative matrix product based time evolution calculations, where symmetries dictate that there should be a topological magnon gap but where LSWT fails to open up this gap. We also comment on possible spin split magnons in MnF$_2$ and similar rutiles by analogy to recently proposed altermagnets.

cond-mat.other↗

arXiv2022

Magnetoelectric Cavity Magnonics in Skyrmion Crystals

We present a theory of magnetoelectric magnon-photon coupling in cavities hosting noncentrosymmetric magnets. Analogously to nonreciprocal phenomena in multiferroics, the magnetoelectric coupling is time-reversal and inversion asymmetric. This asymmetry establishes a means for exceptional tunability of magnon-photon coupling, which can be switched on and off by reversing the magnetization direction. Taking the multiferroic skyrmion-host Cu$_2$OSeO$_3$ with ultralow magnetic damping as an example, we reveal the electrical activity of skyrmion eigenmodes and propose it for magnon-photon splitting of ``magnetically dark'' elliptic modes. Furthermore, we predict a cavity-induced magnon-magnon coupling between magnetoelectrically active skyrmion excitations. We discuss applications in quantum information processing by proposing protocols for all-electrical magnon-mediated photon quantum gates, and a photon-mediated SPLIT operation of magnons. Our study highlights magnetoelectric cavity magnonics as a novel platform for realizing quantum-hybrid systems and the coherent transduction between photons and magnons in topological magnetic textures.

cond-mat.str-el↗

arXiv2022

Long-distance coupling of spin qubits via topological magnons

We consider two distant spin qubits in quantum dots, both coupled to a two-dimensional topological ferromagnet hosting chiral magnon edge states at the boundary. The chiral magnon is used to mediate entanglement between the spin qubits, realizing a fundamental building block of scalable quantum computing architectures: a long-distance two-qubit gate. Previous proposals for long-distance coupling with magnons involved off-resonant coupling, where the detuning of the spin-qubit frequency from the magnonic band edge provides protection against spontaneous relaxation. The topological magnon mode, on the other hand, lies in-between two magnonic bands far away from any bulk magnon resonances, facilitating strong and highly tuneable coupling between the two spin qubits. Even though the coupling between the qubit and the chiral magnon is resonant for a wide range of qubit splittings, we find that the magnon-induced qubit relaxation is vastly suppressed if the coupling between the qubit and the ferromagnet is antiferromagnetic. A fast and high-fidelity long-distance coupling protocol is presented capable of achieving spin-qubit entanglement over micrometer distances with $1\,$MHz gate speed and up to $99.9\%$ fidelities. The resulting spin-qubit entanglement may be used as a probe for the long-sought detection of topological edge magnons.

cond-mat.mes-hall↗

arXiv2022

Topological Hybrids of Magnons and Magnon Bound Pairs

We consider quantum condensed matter systems without particle-number conservation. Since the particle number is not a good quantum number, states belonging to different particle-number sectors can hybridize, which causes topological anticrossings in the spectrum. The resulting spectral gaps support chiral edge excitations whose wavefunction is a superposition of states in the two hybridized sectors. This situation is realized in fully saturated spin-anisotropic quantum magnets without spin conservation, in which single magnons hybridize with magnon bound pairs, i.e., two-magnon bound states. The resulting chiral edge excitations are exotic composites that carry mixed spin-multipolar character, inheriting spin-dipolar and spin-quadrupolar character from their single-particleness and two-particleness, respectively. In contrast to established topological magnons, the topological effects discussed here are of genuine quantum mechanical origin and vanish in the classical limit. We discuss implications for both intrinsic anomalous Hall-type transport and beyond-spintronics computation paradigms. We conclude that fully polarized quantum magnets are a promising platform for topology caused by hybridizations between particle-number sectors, complementing the field of ultracold atoms working with a conserved number of particles.

cond-mat.mes-hall↗

arXiv2021

Thermal Hall effect of magnons in collinear antiferromagnetic insulators: signatures of magnetic and topological phase transitions

We demonstrate theoretically that the thermal Hall effect of magnons in collinear antiferromagnetic insulators is an indicator of magnetic and topological phase transitions in the magnon spectrum. The transversal heat current of magnons caused by a thermal gradient is calculated for an antiferromagnet on a honeycomb lattice. An applied magnetic field drives the system from the antiferromagnetic phase via a spin-flop phase into the field-polarized phase. Besides these magnetic phase transitions we find topological phase transitions within the spin-flop phase. Both types of transitions manifest themselves in prominent and distinguishing features in the thermal conductivities; depending on the temperature, the conductivity changes by several orders of magnitude, providing a tool to discern experimentally the two types of phase transitions. We include numerical results for the van der Waals magnet MnPS$_3$.

cond-mat.str-el↗

arXiv2020

Interaction-stabilized topological magnon insulator in ferromagnets

Condensed matter systems admit topological collective excitations above a trivial ground state, an example being Chern insulators formed by Dirac bosons with a gap at finite energies. However, in contrast to electrons, there is no particle-number conservation law for collective excitations. This gives rise to particle number-nonconserving many-body interactions whose influence on single-particle topology is an open issue of fundamental interest in the field of topological quantum materials. Taking magnons in ferromagnets as an example, we uncover topological magnon insulators that are stabilized by interactions through opening Chern-insulating gaps in the magnon spectrum. This can be traced back to the fact that the particle-number nonconserving interactions break the effective time-reversal symmetry of the harmonic theory. Hence, magnon-magnon interactions are a source of topology that can introduce chiral edge states, whose chirality depends on the magnetization direction. Importantly, interactions do not necessarily cause detrimental damping but can give rise to topological magnons with exceptionally long lifetimes. We identify two mechanisms of interaction-induced topological phase transitions---one driven by an external field, the other by temperature---and show that they cause unconventional sign reversals of transverse transport signals, in particular of the thermal Hall conductivity. We identify candidate materials where this many-body mechanism is expected to occur, such as the metal-organic kagome-lattice magnet Cu(1,3-benzenedicarboxylate), the van der Waals honeycomb-lattice magnet CrI$_3$, and the multiferroic kamiokite (Fe$_2$Mo$_3$O$_8$). Our results demonstrate that interactions can play an important role in generating nontrivial topology.

cond-mat.str-el↗