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Alexander Mook

Publications and source records attributed to Alexander Mook.

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Chiral Hinge Magnons in Second-Order Topological Magnon Insulators

When interacting spins in condensed matter order ferromagnetically, their ground state wave function is topologically trivial. Nonetheless, in two dimensions, the ferromagnetic state can support spin excitations with nontrivial topology, an exotic state known as topological magnon insulator (TMI). Here, we theoretically unveil and numerically confirm a novel ferromagnetic state in three dimensions dubbed second-order TMI, whose hallmarks are excitations at its hinges, where facets intersect. Since ferromagnetism naturally comes with broken time-reversal symmetry, the hinge magnons are chiral, rendering backscattering impossible. Hence, they trace out a three-dimensional path about the sample unimpeded by defects and are topologically protected by the spectral gap. They are remarkably robust against disorder and simultaneously highly tunable by atomic-level engineering of the sample termination. Our findings empower magnonics with the tools of higher-order topology, a promising route to combine low-energy information transfer free of Joule heating with three-dimensional vertical integration.

cond-mat.mes-hall↗

Orbital Magnetic Moment of Magnons

In experiments and applications usually the spin magnetic moment of magnons is considered. In this Paper we identify an additional degree of freedom of magnons: an \emph{orbital} magnetic moment brought about by spin-orbit coupling.Our microscopic theory uncovers that spin magnetization $\vec{M}^\mathrm{S}$ and orbital magnetization $\vec{M}^\mathrm{O}$ are independent quantities. They are not necessarily collinear; thus, even when the total spin moment is compensated due to antiferromagnetism ($\vec{M}^\mathrm{S} = \vec{0}$), $\vec{M}^\mathrm{O}$ may be nonzero. This scenario of orbital weak ferromagnetism is realized in paradigmatic kagome antiferromagnets with Dzyaloshinskii-Moriya interaction. We demonstrate that magnets exhibiting a magnonic orbital moment are omnipresent and propose transport experiments for probing it.

cond-mat.str-el↗

Compensated Quantum and Topological Hall Effects of Electrons in Polyatomic Stripe Lattices

The quantum Hall effect is generally understood for free electron gases, in which topologically protected edge states between Landau levels (LLs) form conducting channels at the edge of the sample. In periodic crystals, the LLs are imprinted with lattice properties; plateaus in the transverse Hall conductivity are not equidistant in energy anymore. Herein, crystals with a polyatomic basis are considered. For a stripe arrangement of different atoms, the band structure resorts nontrivially and exhibits strong oscillations that form a salient pattern with very small bandgaps. The Hall conductivity strongly decreases for energies within these bands, and only sharp peaks remain for energies in the gap. These effects are traced back to open orbits in the initial band structure; the corresponding LLs are formed from states with positive and negative effective mass. The partial cancellation of transverse charge conductivity also holds for different polyatomic stripe lattices and even when the magnetic field is replaced by a topologically nontrivial spin texture. The topological Hall effect is suppressed in the presence of magnetic skyrmions. The discussion is complemented by calculations of Hofstadter butterflies and orbital magnetization.

cond-mat.str-el↗

Quantum Damping of Skyrmion Crystal Eigenmodes due to Spontaneous Quasiparticle Decay

The elementary excitations of skyrmion crystals experience both emergent magnetic fields and anharmonic interactions brought about by the topologically nontrivial noncollinear texture. The resulting flat bands cause strong spontaneous quasiparticle decay, dressing the eigenmodes of skyrmion crystals with a finite zero-temperature quantum lifetime. Sweeping the flat bands through the spectrum by changing the magnetic field leads to an externally controllable energy-selective magnon breakdown. In particular, we uncover that the three fundamental modes, i.e., the anticlockwise, breathing, and clockwise mode, exhibit distinct decay behavior, with the clockwise (anticlockwise) mode being the least (most) stable mode out of the three.

cond-mat.str-el↗

Origin of the Magnetic Spin Hall Effect: Spin Current Vorticity in the Fermi Sea

The interplay of spin-orbit coupling (SOC) and magnetism gives rise to a plethora of charge-to-spin conversion phenomena that harbor great potential for spintronics applications. In addition to the spin Hall effect, magnets may exhibit a magnetic spin Hall effect (MSHE), as was recently discovered [Kimata \textit{et al.}, Nature \textbf{565}, 627-630 (2019)]. To date, the MSHE is still awaiting its intuitive explanation. Here we relate the MSHE to the vorticity of spin currents in the Fermi sea, which explains pictorially the origin of the MSHE. For all magnetic Laue groups that allow for nonzero spin current vorticities the related tensor elements of the MSH conductivity are given. Minimal requirements for the occurrence of a MSHE are compatibility with either a magnetization or a magnetic toroidal quadrupole. This finding implies in particular that the MSHE is expected in all ferromagnets with sufficiently large SOC. To substantiate our symmetry analysis, we present various models, in particular a two-dimensional magnetized Rashba electron gas, that corroborate an interpretation by means of spin current vortices. Considering thermally induced spin transport and the magnetic spin Nernst effect in magnetic insulators, which are brought about by magnons, our findings for electron transport can be carried over to the realm of spincaloritronics, heat-to-spin conversion, and energy harvesting.

cond-mat.mes-hall↗

Magnonic Analogue of Edelstein Effect in Antiferromagnetic Insulators

We investigate the nonequilibrium spin polarization due to a temperature gradient in antiferromagnetic insulators, which is the magnonic analogue of the inverse spin-galvanic effect of electrons. We derive a linear response theory of a temperature-gradient-induced spin polarization for collinear and noncollinear antiferromagnets, which comprises both extrinsic and intrinsic contributions. We apply our theory to several noncentrosymmetric antiferromagnetic insulators, i.e., to a one-dimensional antiferromagnetic spin chain, a single layer of kagome noncollinear antiferromagnet, e.g., $\text{KFe}_3(\text{OH})_6(\text{SO}_4)_2$, and a noncollinear breathing pyrochlore antiferromagnet, e.g., LiGaCr$_4$O$_8$. The shapes of our numerically evaluated response tensors agree with those implied by the magnetic symmetry. Assuming a realistic temperature gradient of $10 \text{K}/\text{mm}$, we find two-dimensional spin densities of up to $\sim 10^6\hbar/\text{cm}^2$ and three-dimensional bulk spin densities of up to $\sim 10^{14}\hbar/\text{cm}^3$, encouraging an experimental detection.

cond-mat.mes-hall↗

Spin Seebeck and Spin Nernst Effects of Magnons in Noncollinear Antiferromagnetic Insulators

Our joint theoretical and computer experimental study of heat-to-spin conversion reveals that noncollinear antiferromagnetic insulators are promising materials for generating magnon spin currents upon application of a temperature gradient: they exhibit spin Seebeck and spin Nernst effects. Using Kubo theory and spin dynamics simulations, we explicitly evaluate these effects in a single kagome sheet of potassium iron jarosite, KFe$_3$(OH)$_6$(SO$_4$)$_2$, and predict a spin Seebeck conversion factor of $0.2 μ\mathrm{V}/\mathrm{K}$ at a temperature of $20 \mathrm{K}$.

cond-mat.mes-hall↗

Magnetic bimerons as skyrmion analogues in in-plane magnets

A magnetic bimeron is a pair of two merons and can be understood as the in-plane magnetized version of a skyrmion. Here we theoretically predict the existence of single magnetic bimerons as well as bimeron crystals, and compare the emergent electrodynamics of bimerons with their skyrmion analogues. We show that bimeron crystals can be stabilized in frustrated magnets and analyze what crystal structure can stabilize bimerons or bimeron crystals via the Dzyaloshinskii-Moriya interaction. We point out that bimeron crystals, in contrast to skyrmion crystals, allow for the detection of a pure topological Hall effect. By means of micromagnetic simulations, we show that bimerons can be used as bits of information in in-plane magnetized racetrack devices, where they allow for current-driven motion for torque orientations that leave skyrmions in out-of-plane magnets stationary.

cond-mat.mes-hall↗

Magnetoelectric effect and orbital magnetization in skyrmion crystals: Detection and characterization of skyrmions

Skyrmions are small magnetic quasiparticles, which are uniquely characterized by their topological charge and their helicity. In this Rapid Communication, we show via calculations how both properties can be determined without relying on real-space imaging. The orbital magnetization and topological Hall conductivity measure the arising magnetization due to the circulation of electrons in the bulk and the occurrence of topologically protected edge channels due to the emergent field of a skyrmion crystal. Both observables quantify the topological Hall effect and distinguish skyrmions from antiskyrmions by sign. Additionally, we predict a magnetoelectric effect in skyrmion crystals, which is the generation of a magnetization (polarization) by application of an electric (magnetic) field. This effect is quantified by spin toroidization and magnetoelectric polarizability. The dependence of the transverse magnetoelectric effect on the skyrmion helicity fits that of the classical toroidal moment of the spin texture and allows to differentiate skyrmion helicities: it is largest for Bloch skyrmions and zero for Neel skyrmions. We predict distinct features of the four observables that can be used to detect and characterize skyrmions in experiments.

cond-mat.str-el↗

Overcoming the speed limit in skyrmion racetrack devices by suppressing the skyrmion Hall effect

Magnetic skyrmions are envisioned as carriers of information in racetrack storage devices. Unfavorably, the skyrmion Hall effect hinders the fast propagation of skyrmions along an applied electric current and limits the device's maximum operation speed. In this Rapid Communication, we show that the maximum skyrmion velocity increases by a factor of 10 when the skyrmion Hall effect is suppressed, since the straight-line motion of the skyrmion allows for the application of larger driving currents. We consider a ferromagnet on a heavy metal layer, which converts the applied charge current into a spin current by the spin Hall effect. The spin current drives the skyrmions in the ferromagnet via spin-orbit torque. We show by analytical considerations and simulations that the deflection angle decreases, when the spin current is polarized partially along the applied current direction and derive the condition for complete suppression of the skyrmion Hall effect.

cond-mat.str-el↗

The family of topological Hall effects for electrons in skyrmion crystals

Hall effects of electrons can be produced by an external magnetic field, spin orbit-coupling or a topologically non-trivial spin texture. The topological Hall effect (THE) - caused by the latter - is commonly observed in magnetic skyrmion crystals. Here, we show analogies of the THE to the conventional Hall effect (HE), the anomalous Hall effect (AHE), and the spin Hall effect (SHE). In the limit of strong coupling between conduction electron spins and the local magnetic texture the THE can be described by means of a fictitious, 'emergent' magnetic field. In this sense the THE can be mapped onto the HE caused by an external magnetic field. Due to complete alignment of electron spin and magnetic texture, the transverse charge conductivity is linked to a transverse spin conductivity. They are disconnected for weak coupling of electron spin and magnetic texture; the THE is then related to the AHE. The topological equivalent to the SHE can be found in antiferromagnetic skyrmion crystals. We substantiate our claims by calculations of the edge states for a finite sample. These states reveal in which situation the topological analogue to a quantized HE, quantized AHE, and quantized SHE can be found.

cond-mat.str-el↗

Signatures of lattice geometry in quantum and topological Hall effect

The topological Hall effect (THE) of electrons in skyrmion crystals is strongly related to the quantum Hall effect (QHE) on lattices. This relation suggests to revisit the QHE because its Hall conductivity can be unconventionally quantized. It exhibits a jump and changes sign abruptly if the Fermi level crosses a van Hove singularity. In this Paper, we investigate the unconventional QHE features by discussing band structures, Hall conductivities, and topological edge states for square and triangular lattices; their origin are Chern numbers of bands in the skyrmion crystal (THE) or of the corresponding Landau levels (QHE). Striking features in the energy dependence of the Hall conductivities are traced back to the band structure without magnetic field whose properties are dictated by the lattice geometry. Based on these findings, we derive an approximation that allows us to determine the energy dependence of the topological Hall conductivity on any twodimensional lattice. The validity of this approximation is proven for the honeycomb lattice. We conclude that skyrmion crystals lend themselves for experiments to validate our findings for the THE and - indirectly - the QHE.

cond-mat.str-el↗

Antiferromagnetic skyrmion crystals: generation, topological Hall and topological spin Hall effect

Skyrmions are topologically nontrivial, magnetic quasi-particles, that are characterized by a topological charge. A regular array of skyrmions - a skyrmion crystal (SkX) - features the topological Hall effect (THE) of electrons, that, in turn, gives rise to the Hall effect of the skyrmions themselves. It is commonly believed that antiferromagnetic skyrmion crystals (AFM-SkXs) lack both effects. In this Rapid Communication, we present a generally applicable method to create stable AFM-SkXs by growing a two sublattice SkX onto a collinear antiferromagnet. As an example we show that both types of skyrmion crystals - conventional and antiferromagnetic - exist in honeycomb lattices. While AFM-SkXs with equivalent lattice sites do not show a THE, they exhibit a topological spin Hall effect. On top of this, AFM-SkXs on inequivalent sublattices exhibit a nonzero THE, which may be utilized in spintronics devices. Our theoretical findings call for experimental realization.

cond-mat.str-el↗

Unconventional Topological Hall Effect in Skyrmion Crystals Caused by the Topology of the Lattice

The hallmark of a skyrmion crystal (SkX) is the topological Hall effect (THE). In this Article, we predict and explain an unconventional behavior of the topological Hall conductivity in SkXs. In simple terms, the spin texture of the skyrmions causes an inhomogeneous emergent magnetic field whose associated Lorentz force acts on the electrons. By making the emergent field homogeneous, the THE is mapped onto the quantum Hall effect (QHE). Consequently, each electronic band of the SkX is assigned to a Landau level. This correspondence of THE and QHE allows to explain the unconventional behavior of the THE of electrons in SkXs. For example, a skyrmion crystal on a triangular lattice exhibits a quantized topological Hall conductivity with steps of $2 \cdot e^2/h$ below and with steps of $1 \cdot e^2/h$ above the van Hove singularity. On top of this, the conductivity shows a prominent sign change at the van Hove singularity. These unconventional features are deeply connected to the topology of the structural lattice.

cond-mat.str-el↗

Magnon nodal-line semimetals and drumhead surface states in anisotropic pyrochlore ferromagnets

We introduce a new type of topological magnon matter: the magnonic pendant to electronic nodal-line semimetals. Magnon spectra of anisotropic pyrochlore ferromagnets feature twofold degeneracies of magnon bands along a closed loop in reciprocal space. These magnon nodal lines are topologically protected by the coexistence of inversion and time-reversal symmetry; they require the absence of spin-orbit interaction (no Dzyaloshinskii-Moriya interaction). We calculate the topological invariants of the nodal lines and show that details of the associated magnon drumhead surface states depend strongly on the termination of the surface. Magnon nodal-line semimetals complete the family of topological magnons in three-dimensional ferromagnetic materials.

physics.comp-ph↗

Tunable magnon Weyl points in ferromagnetic pyrochlores

The dispersion relations of magnons in ferromagnetic pyrochlores with Dzyaloshinskii-Moriya interaction is shown to possess Weyl points, i.\,e., pairs of topological nontrivial crossings of two magnon branches with opposite topological charge. As a consequence of their topological nature, their projections onto a surface are connected by magnon arcs, thereby resembling closely Fermi arcs of electronic Weyl semimetals. On top of this, the positions of the Weyl points in reciprocal space can be tuned widely by an external magnetic field: rotated within the surface plane, the Weyl points and magnon arcs are rotated as well; tilting the magnetic field out-of-plane shifts the Weyl points toward the center $\barΓ$ of the surface Brillouin zone. The theory is valid for the class of ferromagnetic pyrochlores, i.\,e., three-dimensional extensions of topological magnon insulators on kagome lattices. In this Letter, we focus on the $(111)$ surface, identify candidates of established ferromagnetic pyrochlores which apply to the considered spin model, and suggest experiments for the detection of the topological features.

physics.comp-ph↗