arXiv subjects

Ali A. Husain

Publications and source records attributed to Ali A. Husain.

15 recordsLinked to original sources

arXiv2026

Computing with many encoded logical qubits beyond break-even

High-rate quantum error correcting (QEC) codes encode many logical qubits in a given number of physical qubits, making them promising candidates for quantum computation. Implementing high-rate codes at a scale that both frustrates classical computing and improves performance by encoding requires both high fidelity gates and long-range qubit connectivity -- both of which are offered by trapped-ion quantum computers. Here, we demonstrate computations that outperform their unencoded counterparts in the high-rate $[[ k+2,\, k,\, 2 ]]$ iceberg quantum error detecting (QED) and $[[ (k_2 + 2)(k_1 + 2),\, k_2k_1,\, 4 ]]$ two-level concatenated iceberg QEC codes, using the 98-qubit Quantinuum Helios trapped-ion quantum processor. Utilizing new gadgets for encoded operations, we realize this "beyond break-even" performance with reasonable postselection rates across a range of fault-tolerant (FT) and partially-fault-tolerant (pFT) component and application benchmarks with between $48$ and $94$ logical qubits. These benchmarks include FT state preparation and measurement, QEC cycle benchmarking, logical gate benchmarking, GHZ state preparation, and a pFT quantum simulation of the three-dimensional $XY$ model of quantum magnetism. Additionally, we illustrate that postselection rates can be suppressed by increasing the code distance via concatenation. Our results represent state-of-the-art logical component and state fidelities and provide evidence that high-rate QED/QEC codes are viable on contemporary quantum computers for near-term beyond-classical-scale computation.

quant-ph↗

arXiv2025

Helios: A 98-qubit trapped-ion quantum computer

We report on Quantinuum Helios, a 98-qubit trapped-ion quantum processor based on the quantum charge-coupled device (QCCD) architecture. Helios features $^{137}$Ba$^{+}$ hyperfine qubits, all-to-all connectivity enabled by a rotatable ion storage ring connecting two quantum operation regions by a junction, speed improvements from parallelized operations, and a new software stack with real-time compilation of dynamic programs. Averaged over all operational zones in the system, we achieve average infidelities of $2.5(1)\times10^{-5}$ for single-qubit gates, $7.9(2)\times10^{-4}$ for two-qubit gates, and $4.8(6)\times10^{-4}$ for state preparation and measurement, none of which are fundamentally limited and likely able to be improved. These component infidelities are predictive of system-level performance in both random Clifford circuits and random circuit sampling, the latter demonstrating that Helios operates well beyond the reach of classical simulation and establishes a new frontier of fidelity and complexity for quantum computers.

quant-ph↗

arXiv2025

Certified randomness amplification by dynamically probing remote random quantum states

Cryptography depends on truly unpredictable numbers, but physical sources emit biased or correlated bits. Quantum mechanics enables the amplification of imperfect randomness into nearly perfect randomness, but prior demonstrations have required physically co-located, loophole-free Bell tests, constraining the feasibility of remote operation. Here we realize certified randomness amplification across a network by dynamically probing large, entangled quantum states on Quantinuum's 98-qubit Helios trapped-ion quantum processor. Our protocol is secure even if the remote device acts maliciously or is compromised by an intercepting adversary, provided the samples are generated quickly enough to preclude classical simulation of the quantum circuits. We stream quantum gates in real time to the quantum processor, maintain quantum state coherence for $\approx 0.9$ seconds, and then reveal the measurement bases to the quantum processor only milliseconds before measurement. This limits the time for classical spoofing to 30 ms and constrains the location of hypothetical adversaries to a $4{,}500$ km radius. We achieve a fidelity of 0.586 on random circuits with 64 qubits and 276 two-qubit gates, enabling the amplification of realistic imperfect randomness with a low entropy rate into nearly perfect randomness.

quant-ph↗

arXiv2025

Realization of a Quantum Streaming Algorithm on Long-lived Trapped-ion Qubits

Large classical datasets are often processed in the streaming model, with data arriving one item at a time. In this model, quantum algorithms have been shown to offer an unconditional exponential advantage in space. However, experimentally implementing such streaming algorithms requires qubits that remain coherent while interacting with an external data stream. In this work, we realize such a data-streaming model using Quantinuum Helios trapped-ion quantum computer with long-lived qubits that communicate with an external server. We implement a quantum pair sketch, which is the primitive underlying many quantum streaming algorithms, and use it to solve Hidden Matching, a problem known to exhibit a theoretical exponential quantum advantage in space. Furthermore, we compile the quantum streaming algorithm to fault-tolerant quantum architectures based on surface and bivariate bicycle codes and show that the quantum space advantage persists even with the overheads of fault-tolerance.

quant-ph↗

arXiv2023

Orbital-selective time-domain signature of nematicity dynamics in the charge-density-wave phase of La$_{1.65}$Eu$_{0.2}$Sr$_{0.15}$CuO$_4$

Understanding the interplay between charge, nematic, and structural ordering tendencies in cuprate superconductors is critical to unraveling their complex phase diagram. Using pump-probe time-resolved resonant x-ray scattering on the (0 0 1) Bragg peak at the Cu $L_3$ and O $K$ resonances, we investigate non-equilibrium dynamics of $Q_a = Q_b = 0$ nematic order and its association with both charge density wave (CDW) order and lattice dynamics in La$_{1.65}$Eu$_{0.2}$Sr$_{0.15}$CuO$_4$. The orbital selectivity of the resonant x-ray scattering cross-section allows nematicity dynamics associated with the planar O 2$p$ and Cu 3$d$ states to be distinguished from the response of anisotropic lattice distortions. A direct time-domain comparison of CDW translational-symmetry breaking and nematic rotational-symmetry breaking reveals that these broken symmetries remain closely linked in the photoexcited state, consistent with the stability of CDW topological defects in the investigated pump fluence regime.

cond-mat.str-el↗

arXiv2022

Incommensurate magnetic orders and topological Hall effect in the square-net centrosymmetric EuGa$_2$Al$_2$ system

Neutron diffraction on the centrosymmetric square-net magnet EuGa$_2$Al$_2$ reveals multiple incommensurate magnetic states (AFM1,2,3) in zero field. In applied field, a new magnetic phase (A) is identified from magnetization and transport measurements, bounded by two of the $μ_0H$~=~0 incommensurate magnetic phases (AFM1,helical and AFM3, cycloidal) with different moment orientations. Moreover, magneto-transport measurements indicate the presence of a topological Hall effect, with maximum values centered in the A phase. Together, these results render EuGa$_2$Al$_2$ a material with non-coplanar or topological spin texture in applied field. X-ray diffraction reveals an out-of-plane (OOP) charge density wave (CDW) below $T_{CDW} \sim$ 50 K while the magnetic propagation vector lies in plane below $T_N$ = 19.5 K. Together these data point to a new route to realizing in-plane non-collinear spin textures through an OOP CDW. In turn, these non-collinear spin textures may be unstable against the formation of topological spin textures in an applied field.

cond-mat.str-el↗

arXiv2021

Generic character of charge and spin density waves in superconducting cuprates

Understanding the nature of charge density waves (CDW) in cuprate superconductors has been complicated by material specific differences. A striking example is the opposite doping dependence of the CDW ordering wavevector in La-based and Y-based compounds, the two families where charge ordering is strongest and best characterized. Here we report a combined resonant soft X-ray scattering (RSXS) and neutron scattering study of charge and spin density waves in isotopically enriched La$_{1.8-x}$ Eu$_{0.2}$ Sr$_{x}$ CuO$_{4}$ over a range of doping $0.07 \leq x \leq 0.20$. For all dopings studied by RSXS, we find that the CDW amplitude is approximately temperature-independent and develops well above experimentally accessible temperatures. Surprisingly, the CDW ordering wavevector shows a non-monotonic temperature dependence, with a sudden change occurring at temperatures near the SDW onset temperature. We describe this behavior with a Landau-Ginzburg theory for an incommensurate CDW in a metallic system with a finite charge compressibility and CDW-SDW coupling. Our Landau-Ginzburg analysis suggests that the ordering wavevector at high temperatures decreases with increased doping. This behavior is opposite to the trend at low temperatures and highly reminiscent of the doping dependence seen in YBa$_2$ Cu$_3$ O$_{6+δ}$ , suggesting a common origin of the CDW in hole-doped cuprate superconductors.

cond-mat.supr-con↗

arXiv2021

Ultrafast renormalization of the onsite Coulomb repulsion in a cuprate superconductor

Ultrafast lasers are an increasingly important tool to control and stabilize emergent phases in quantum materials. Among a variety of possible excitation protocols, a particularly intriguing route is the direct light-engineering of microscopic electronic parameters, such as the electron hopping and the local Coulomb repulsion (Hubbard $U$). In this work, we use time-resolved x-ray absorption spectroscopy to demonstrate the light-induced renormalization of the Hubbard $U$ in a cuprate superconductor, La$_{1.905}$Ba$_{0.095}$CuO$_4$. We show that intense femtosecond laser pulses induce a substantial redshift of the upper Hubbard band, while leaving the Zhang-Rice singlet energy unaffected. By comparing the experimental data to time-dependent spectra of single- and three-band Hubbard models, we assign this effect to a $\sim140$ meV reduction of the onsite Coulomb repulsion on the copper sites. Our demonstration of a dynamical Hubbard $U$ renormalization in a copper oxide paves the way to a novel strategy for the manipulation of superconductivity, magnetism, as well as to the realization of other long-range-ordered phases in light-driven quantum materials.

cond-mat.str-el↗

arXiv2021

Search for $Q \sim 0$ order near a forbidden Bragg position in Bi$_{2.1}$Sr$_{1.9}$CaCu$_2$O$_{8+x}$ with resonant soft x-ray scattering

Identifying what broken symmetries are present in the cuprates has become a major area of research. Many authors have reported evidence for so-called "$Q \sim 0$" order that involves broken inversion, mirror, chiral, or time-reversal symmetry that is uniform in space. Not all these observations are well understood and new experimental probes are needed. Here we use resonant soft x-ray scattering (RSXS) to search for $Q \sim 0$ order in Bi$_{2.1}$Sr$_{1.9}$CaCu$_2$O$_{8+x}$ (Bi-2212) by measuring the region of a forbidden Bragg peak, $(0,0,3)$, which is normally extinguished by symmetry but may become allowed on resonance if valence band order is present. Using circularly polarized light, we found that this reflection becomes allowed on the Cu $L_3$ resonance for temperatures $T_c < T < T^\ast$, though remains absent in linear polarization and at other temperatures. This observation suggests the existence of spatially uniform valence band order near the pseudogap temperature. In addition, we observed periodic oscillations in the specular reflectivity from the sample surface that resemble thin film interference fringes, though no known film is present. These fringes are highly resonant, appear in all polarizations, and exhibit a period that depends on the location where the beam strikes the sample surface. We speculate that these fringes arise from interaction between some intrinsic valence band instability and extrinsic structural surface morphologies of the material. Our study supports the existence of some kind of $Q \sim 0$ broken symmetry state in Bi-2212 at intermediate temperatures, and calls for further study using a microfocused beam that could disentangle microscopic effects from macroscopic heterogeneities.

cond-mat.str-el↗

arXiv2020

Extracting correlation effects from Momentum-Resolved Electron Energy Loss Spectroscopy (M-EELS): Synergistic origin of the dispersion kink in Bi$_{2.1}$Sr$_{1.9}$CaCu$_2$O$_{8+x}$

We employ Momentum-Resolved Electron Energy Loss Spectroscopy (M-EELS) on Bi2.1Sr1.9CaCu2O8+x to resolve the issue of the kink feature in the electron dispersion widely observed in the cuprates. To this end, we utilize the GW approximation to relate the density response function measured in in M-EELS to the self-energy, isolating contributions from phonons, electrons, and the momentum dependence of the effective interaction to the decay rates. The phononic contributions, present in the M-EELS spectra due to electron-phonon coupling, lead to kink features in the corresponding single-particle spectra at energies between 40 meV and 80 meV, independent of the doping level. We find that a repulsive interaction constant in momentum space is able to yield the kink attributed to phonons in ARPES. Hence, our analysis of the M-EELS spectra points to local repulsive interactions as a factor that enhances the spectroscopic signatures of electron-phonon coupling in cuprates. We conclude that the strength of the kink feature in cuprates is determined by the combined action of electron-phonon coupling and electron-electron interactions.

cond-mat.supr-con↗

arXiv2019

Evidence for photoinduced sliding of the charge-order condensate in La$_{1.875}$Ba$_{0.125}$CuO$_4$

We use femtosecond resonant soft x-ray scattering to measure the ultrafast optical melting of charge-order correlations in La$_{1.875}$Ba$_{0.125}$CuO$_4$. By analyzing both the energy-resolved and energy-integrated order parameter dynamics, we find evidence of a short-lived nonequilibrium state, whose features are compatible with a sliding charge density wave coherently set in motion by the pump. This transient state exhibits shifts in both the quasielastic line energy and its wave vector, as expected from a classical Doppler effect. The wave vector change is indeed found to directly follow the pump propagation direction. These results demonstrate the existence of sliding charge order behavior in an unconventional charge density wave system and underscore the power of ultrafast optical excitation as a tool to coherently manipulate electronic condensates.

cond-mat.str-el↗

arXiv2018

Ultrafast time-resolved x-ray scattering reveals diffusive charge order dynamics in La$_{2-x}$Ba$_x$CuO$_4$

Charge order is universal among high-T$_c$ cuprates but its relevance to superconductivity is not established. It is widely believed that, while static order competes with superconductivity, dynamic order may be favorable and even contribute to Cooper pairing. We use time-resolved resonant soft x-ray scattering to study the collective dynamics of the charge order in the prototypical cuprate, La$_{2-x}$Ba$_x$CuO$_4$. We find that, at energy scales $0.4$ meV $ \lesssim ω\lesssim 2$ meV, the excitations are overdamped and propagate via Brownian-like diffusion. At energy scales below 0.4 meV the charge order exhibits dynamic critical scaling, displaying universal behavior arising from propagation of topological defects. Our study implies that charge order is dynamic, so may participate tangibly in superconductivity.

cond-mat.str-el↗

arXiv2018

Inequivalence of the zero-momentum Limits of Transverse and Longitudinal Dielectric Response in the Cuprates

We address the question of the mismatch between the zero momentum limits of the transverse and longitudinal dielectric functions for a fixed direction of the driving field observed in the cuprates. This question translates to whether or not the order in which the longitudinal and transverse momentum transfers are taken to zero commute. While the two limits commute for both isotropic and anisotropic Drude metals, we argue that a scaleless vertex interaction that depends solely on the angle between scattered electron momenta is sufficient to achieve non-commutativity of the two limits even for a system that is inherently isotropic. We demonstrate this claim for a simple case of the Drude conductivity modified by electron-boson interactions through appropriate vertex corrections, and outline possible consequences of our result to optical and electron energy loss spectroscopy (EELS) measurements close to zero momentum transfer

cond-mat.str-el↗

arXiv2018

Signatures of exciton condensation in a transition metal dichalcogenide

Bose condensation has shaped our understanding of macroscopic quantum phenomena, having been realized in superconductors, atomic gases, and liquid helium. Excitons are bosons that have been predicted to condense into either a superfluid or an insulating electronic crystal. Using the recently developed momentum-resolved electron energy-loss spectroscopy (M-EELS), we study electronic collective modes in the transition metal dichalcogenide semimetal, 1T-TiSe$_2$. Near the phase transition temperature, T$_c$ = 190 K, the energy of the electronic mode falls to zero at nonzero momentum, indicating dynamical slowing down of plasma fluctuations and crystallization of the valence electrons into an exciton condensate. Our study provides compelling evidence for exciton condensation in a three-dimensional solid and establishes M-EELS as a versatile technique sensitive to valence band excitations in quantum materials.

cond-mat.str-el↗

arXiv2017

Measurement of the dynamic charge response of materials using low-energy, momentum-resolved electron energy-loss spectroscopy (M-EELS)

One of the most fundamental properties of an interacting electron system is its frequency- and wave-vector-dependent density response function, $χ({\bf q},ω)$. The imaginary part, $χ''({\bf q},ω)$, defines the fundamental bosonic charge excitations of the system, exhibiting peaks wherever collective modes are present. $χ$ quantifies the electronic compressibility of a material, its response to external fields, its ability to screen charge, and its tendency to form charge density waves. Unfortunately, there has never been a fully momentum-resolved means to measure $χ({\bf q},ω)$ at the meV energy scale relevant to modern elecronic materials. Here, we demonstrate a way to measure $χ$ with quantitative momentum resolution by applying alignment techniques from x-ray and neutron scattering to surface high-resolution electron energy-loss spectroscopy (HR-EELS). This approach, which we refer to here as "M-EELS," allows direct measurement of $χ''({\bf q},ω)$ with meV resolution while controlling the momentum with an accuracy better than a percent of a typical Brillouin zone. We apply this technique to finite-q excitations in the optimally-doped high temperature superconductor, Bi$_2$Sr$_2$CaCu$_2$O$_{8+x}$ (Bi2212), which exhibits several phonons potentially relevant to dispersion anomalies observed in ARPES and STM experiments. Our study defines a path to studying the long-sought collective charge modes in quantum materials at the meV scale and with full momentum control.

cond-mat.supr-con↗