arXiv subjects

Andrew K. Mitchell

Publications and source records attributed to Andrew K. Mitchell.

At least 37 records · Page 2Linked to original sources

arXiv2022

Automatic Differentiable Numerical Renormalization Group

Machine learning techniques have recently gained prominence in physics, yielding a host of new results and insights. One key concept is that of backpropagation, which computes the exact gradient of any output of a program with respect to any input. This is achieved efficiently within the differentiable programming paradigm, which utilizes automatic differentiation (AD) of each step of a computer program and the chain rule. A classic application is in training neural networks. Here, we apply this methodology instead to the numerical renormalization group (NRG), a powerful technique in computational quantum many-body physics. We demonstrate how derivatives of NRG outputs with respect to Hamiltonian parameters can be accurately and efficiently obtained. Physical properties can be calculated using this differentiable NRG scheme--for example, thermodynamic observables from derivatives of the free energy. Susceptibilities can be computed by adding source terms to the Hamiltonian, but still evaluated with AD at precisely zero field. As an outlook, we briefly discuss the derivatives of dynamical quantities and a possible route to the vertex.

cond-mat.str-el↗

arXiv2022

Quantum simulation of an exotic quantum critical point in a two-site charge Kondo circuit

Tuning a material to the cusp between two distinct ground states can produce exotic physical properties, unlike those in either of the neighboring phases. The prospect of designing a model experimental system to capture such behavior is tantalizing. An array of tunnel-coupled quantum dots, each hosting a local spin, should have an appropriately complex phase diagram, but scaling up from individual dots to uniform clusters or lattices has proven difficult: though each site can be tuned to the same occupancy, each has a different set of localized wavefunctions whose couplings to neighboring sites cannot be made fully uniform. An array of metal nanostructures has complementary strengths and weaknesses: simple electrostatic tuning can make each element behave essentially identically, but intersite coupling is not tunable. In this work, we study a tunable nanoelectronic circuit comprising two coupled hybrid metallic-semiconductor islands, combining the strengths of the two types of materials, and demonstrating the potential for scalability. With two charge states of an island acting as an effective spin-1/2, the new architecture also offers a rich range of coupling interactions, and we exploit this to demonstrate a novel quantum critical point. Experimental results in the vicinity of the critical point match striking theoretical predictions.

cond-mat.mes-hall↗

arXiv2022

Monolithic Integration of Quantum Resonant Tunneling Gate on a 22nm FD-SOI CMOS Process

The proliferation of quantum computing technologies has fueled the race to build a practical quantum computer. The spectrum of the innovation is wide and encompasses many aspects of this technology, such as the qubit, control and detection mechanism, cryogenic electronics, and system integration. A few of those emerging technologies are poised for successful monolithic integration of cryogenic electronics with the quantum structure where the qubits reside. In this work, we present a fully integrated Quantum Processor Unit in which the quantum core is co-located with control and detection circuits on the same die in a commercial 22-nm FD-SOI process from GlobalFoundries. The system described in this work comprises a two dimensional (2D) 240 qubits array integrated with 8 detectors and 32 injectors operating at 3K and inside a two-stage Gifford-McMahon cryo-cooler. The power consumption of each detector and injector is 1mW and 0.27mW, respectively. The control sequence is programmed into an on-chip pattern generator that acts as a command and control block for all hardware in the Quantum Processor Unit. Using the aforementioned apparatus, we performed a quantum resonant tunneling experiment on two qubits inside the 2D qubit array. With supporting lab measurements, we demonstrate the feasibility of the proposed architecture in scaling-up the existing quantum core to thousands of qubits.

quant-ph↗

arXiv2021

SO(5) non-Fermi liquid in a Coulomb box device

Non-Fermi liquid (NFL) physics can be realized in quantum dot devices where competing interactions frustrate the exact screening of dot spin or charge degrees of freedom. We show that a standard nanodevice architecture, involving a dot coupled to both a quantum box and metallic leads, can host an exotic SO(5) symmetry Kondo effect, with entangled dot and box charge and spin. This NFL state is surprisingly robust to breaking channel and spin symmetry, but destabilized by particle-hole asymmetry. By tuning gate voltages, the SO(5) state evolves continuously to a spin and then "flavor" two-channel Kondo state. The expected experimental conductance signatures are highlighted.

cond-mat.str-el↗

arXiv2021

SO(5) critical point in a spin-flavor Kondo device -- Bosonization and refermionization solution

We investigate a well studied system of a quantum dot coupled to a Coulomb box and leads, realizing a spin-flavor Kondo model. It exhibits a recently discovered non-Fermi liquid (NFL) behavior with emergent SO(5) symmetry. Here, through a detailed bosonization and refermionization solution, we push forward our previous work and provide a consistent and complete description of the various exotic properties and phase diagram. A unique NFL phase emerges from the presence of an uncoupled Majorana fermion from the flavor sector, whereas FL-like susceptibilities result from the gapping out of a pair of Majroana fermions from the spin and flavor sectors. Other properties, such as a $T^{3/2}$ scaling of the conductance, stability under channel or spin symmetry breaking and a re-appearance of NFL behavior upon breaking the particle-hole symmetry, are all accounted for by a renormalization group treatment of the refermionized Majorana model.

cond-mat.str-el↗

arXiv2020

The Mott transition as a topological phase transition

We show that the Mott metal-insulator transition in the standard one-band Hubbard model can be understood as a topological phase transition. Our approach is inspired by the observation that the mid-gap pole in the self-energy of a Mott insulator resembles the zero-energy spectral pole of the localized surface state in a topological insulator. We use NRG-DMFT to solve the infinite-dimensional Hubbard model, and represent the resulting local self-energy in terms of the boundary Green's function of an auxiliary tight-binding chain without interactions. The auxiliary system is of generalized SSH model type; the Mott transition corresponds to a dissociation of domain walls.

cond-mat.str-el↗

arXiv2020

Wiedemann-Franz law in a non-Fermi liquid and Majorana central charge: Thermoelectric transport in a two-channel Kondo system

Quantum dot devices allow one to access the critical point of the two-channel Kondo model. The effective critical theory involves a free Majorana fermion quasiparticle localized on the dot. As a consequence, this critical point shows both the phenomenon of non-Fermi liquid physics and fractionalization. Although a violation of the Wiedemann-Franz law is considered a defining feature of non-Fermi liquid systems, we show by exact calculations that it holds at the critical point, providing a counterexample to this lore. Furthermore, we show that the fractionalized Majorana character of the critical point can be unambiguously detected from the heat conductivity, opening the door to a direct experimental measurement of the elusive Majorana central charge $c=\tfrac{1}{2}$.

cond-mat.str-el↗

arXiv2020

Machine learning effective models for quantum systems

The construction of good effective models is an essential part of understanding and simulating complex systems in many areas of science. It is a particular challenge for correlated many body quantum systems displaying emergent physics. We propose a machine learning approach that optimizes an effective model based on an estimation of its partition function. The success of the method is demonstrated by application to the single impurity Anderson model and double quantum dots, where non-perturbative results are obtained for the old problem of mapping to effective Kondo models. For quantum impurity parent Hamiltonians, we derive an alternative approach based on learning from observables. When mapping to minimal effective models, emergent scales may not be captured by observable learning, while partition function learning may not reproduce all observables.

cond-mat.str-el↗

arXiv2017

Kondo blockade due to quantum interference in single-molecule junctions

Molecular electronics offers unique scientific and technological possibilities, resulting from both the nanometre scale of the devices and their reproducible chemical complexity. Two fundamental yet different effects, with no classical analogue, have been demonstrated experimentally in single-molecule junctions: quantum interference due to competing electron transport pathways, and the Kondo effect due to entanglement from strong electronic interactions. Here we unify these phenomena, showing that transport through a spin-degenerate molecule can be either enhanced or blocked by Kondo correlations, depending on molecular structure, contacting geometry and applied gate voltages. An exact framework is developed, in terms of which the quantum interference properties of interacting molecular junctions can be systematically studied and understood. We prove that an exact Kondo-mediated conductance node results from destructive interference in exchange-cotunneling. Nonstandard temperature dependences and gate-tunable conductance peaks/nodes are demonstrated for prototypical molecular junctions, illustrating the intricate interplay of quantum effects beyond the single-orbital paradigm.

cond-mat.mes-hall↗

arXiv2016

Kondo impurities in the Kitaev spin liquid: Numerical renormalization group solution and gauge-flux-driven screening

Kitaev's honeycomb-lattice compass model describes a spin liquid with emergent fractionalized excitations. Here we study the physics of isolated magnetic impurities coupled to the Kitaev spin-liquid host. We reformulate this Kondo-type problem in terms of a many-state quantum impurity coupled to a multichannel bath of Majorana fermions and present the numerically exact solution using Wilson's numerical renormalization group technique. Quantum phase transitions occur as a function of Kondo coupling and locally applied field. At zero field, the impurity moment is partially screened only when it binds an emergent gauge flux, and otherwise becomes free at low temperatures. We show how Majorana degrees of freedom determine the fixed-point properties, make contact with Kondo screening in pseudogap Fermi systems, and discuss effects away from the dilute limit.

cond-mat.str-el↗

arXiv2016

Universality and scaling in a charge two-channel Kondo device

We study a charge two-channel Kondo model, demonstrating that recent experiments [Iftikhar et al, Nature 526, 233 (2015)] realize an essentially perfect quantum simulation -- not just of its universal physics, but also nonuniversal effects away from the scaling limit. Numerical renormalization group (NRG) calculations yield conductance lineshapes encoding RG flow to a critical point involving a free Majorana fermion. By mimicking the experimental protocol, the experimental curve is reproduced quantitatively over 9 orders of magnitude, although we show that far greater bandwidth/temperature separation is required to obtain the universal result. Fermi liquid instabilities are also studied: In particular, our exact analytic results for non-linear conductance provide predictions away from thermal equilibrium, in the regime of existing experiments.

cond-mat.str-el↗

arXiv2016

Signatures of Weyl semimetals in quasiparticle interference

Impurities act as in situ probes of nontrivial electronic structure, causing real-space modulations in the density of states detected by scanning tunneling spectroscopy on the sample surface. We show that distinctive topological features of Weyl semimetals can be revealed in the Fourier transform of this map, interpreted in terms of quasiparticle interference (QPI). We develop an exact Green's function formalism and apply it to generalized models of Weyl semimetals with an explicit surface. The type of perturbation lifting the Dirac node degeneracy to produce the three-dimensional bulk Weyl phase determines the specific QPI signatures appearing on the surface. QPI Fermi arcs may or may not appear, depending on the relative surface orientation and quantum interference effects. Line nodes give rise to tube projections of width controlled by the bias voltage. We consider the effect of crystal warping, distinguishing dispersive arclike features from true Fermi arcs. Finally, we demonstrate that the commonly used joint-density-of-states approach fails qualitatively, and cannot describe QPI extinction.

cond-mat.mes-hall↗

arXiv2015

Screening mechanisms in magnetic nanostructures

A theoretical concept is presented for the screening of several magnetic moments locally exchange coupled to conduction electrons in a metallic nanostructure. We consider a quantum confined multi-impurity Kondo model which exhibits the competition between finite-size effects, RKKY interactions, and Kondo physics. In the limit of weak coupling, Kondo correlations are cut by the finite system size; perturbation theory can then be used to derive the low-energy effective model, which is of generalized central-spin form. The theory successfully predicts the degeneracy, total spin, and spin correlations of the ground state, and allows the number of screening channels to be identified. This is demonstrated for a two-impurity model on a finite one-dimensional ring. Density-matrix renormalization-group calculations confirm the physical picture at weak coupling. The non-trivial crossovers to RKKY and strong-coupling regimes are also studied. The numerical renormalization group, tailored to treat finite systems, is used to examine the crossover to the thermodynamic limit.

cond-mat.mes-hall↗

arXiv2015

Validity of the local self-energy approximation: Application to coupled quantum impurities

We examine the quality of the local self-energy approximation, applied here to models of multiple quantum impurities coupled to an electronic bath. The local self-energy is obtained by solving a single-impurity Anderson model in an effective medium that is determined self-consistently, similar to the dynamical mean-field theory (DMFT) for correlated lattice systems. By comparing to exact results obtained using the numerical renormalization group, we determine situations where "impurity-DMFT" is able to capture the physics of highly inhomogeneous systems, and those cases where it fails. For two magnetic impurities separated in real-space, the onset of the dilute limit is captured, but RKKY-dominated inter-impurity singlet formation cannot be described. For parallel quantum dot devices, impurity-DMFT succeeds in capturing underscreened Kondo physics by self-consistent generation of a critical pseudogapped effective medium. However, the quantum phase transition between high- and low-spin states on tuning interdot coupling cannot be described.

cond-mat.str-el↗

arXiv2015

Kondo effect in three-dimensional Dirac and Weyl systems

Magnetic impurities in three-dimensional Dirac and Weyl systems are shown to exhibit a fascinatingly diverse range of Kondo physics, with distinctive experimental spectroscopic signatures. When the Fermi level is precisely at the Dirac point, Dirac semimetals are in fact unlikely candidates for a Kondo effect due to the pseudogapped density of states. However, the influence of a nearby quantum critical point leads to the unconventional evolution of Kondo physics for even tiny deviations in the chemical potential. Separating the degenerate Dirac nodes produces a Weyl phase: time-reversal symmetry-breaking precludes Kondo due to an effective impurity magnetic field, but different Kondo variants are accessible in time-reversal invariant Weyl systems.

cond-mat.str-el↗

arXiv2015

Quasiparticle interference from magnetic impurities

Fourier transform scanning tunneling spectroscopy (FT-STS) measures the scattering of conduction electrons from impurities and defects, giving information about the electronic structure of both the host material and adsorbed impurities. We interpret such FT-STS measurements in terms of the quasiparticle interference (QPI), investigating the QPI due to magnetic impurities adsorbed on a range of representative non-magnetic host surfaces, and contrasting with the case of a simple scalar impurity or point defect. We demonstrate how the electronic correlations present for magnetic impurities markedly affect the QPI, showing e.g. a large intensity enhancement due to the Kondo effect, and universality at low temperatures/scanning-energies. The commonly-used joint density of states (JDOS) interpretation of FT-STS measurements is also considered, and shown to be insuffcient in many cases, including that of magnetic impurities.

cond-mat.str-el↗

arXiv2015

Multiple magnetic impurities on surfaces: Scattering and quasiparticle interference

We study systems of multiple interacting quantum impurities deposited on a metallic surface in a 3D host. For the real-space two-impurity problem, using numerical renormalization group calculations, a rich range of behavior is shown to arise due to the interplay between Kondo physics and effective RKKY interactions - provided the impurity separation is small. Such calculations allow identification of the minimum impurity separation required for a description in terms of independent impurities, and thereby the onset of the 'dilute impurity limit' in many-impurity systems. A 'dilute cluster' limit is also identified in systems with higher impurity density, where inter-impurity interactions are only important within independent clusters. We calculate the quasiparticle interference (QPI) due to two and many impurities, and explore the consequences of the independent impurity/cluster paradigms. Our results provide a framework to investigate the effects of disorder due to interacting impurities at experimentally relevant surface coverages.

cond-mat.str-el↗

arXiv2014

Local moment formation and Kondo screening in impurity trimers

We study theoretically a triangular cluster of three magnetic impurities, hybridizing locally with conduction electrons of a metallic host. Such a cluster is the simplest to exhibit frustration - an important generic feature of many complex molecular systems in which different interactions compete. Here, low-energy doublet states of the trimer are favored by effective exchange interactions produced by strong electronic repulsion in localized impurity orbitals. Parity symmetry protects a level-crossing of such states on tuning microscopic parameters, while an avoided crossing arises in the general distorted case. On coupling to a metallic host, the behavior is shown to be immensely rich, since collective quantum many-body effects now also compete. In particular, impurity degrees of freedom are totally screened at low temperatures in a Kondo-screened Fermi liquid phase, while degenerate ground states persist in a local moment phase. Local frustration drives the quantum phase transition between the two, which may be first order or of Kosterlitz-Thouless type, depending on symmetries. Unusual mechanisms for local moment formation and Kondo screening are found, due to the orbital structure of the impurity trimer. Our results are of relevance for triple quantum dot devices. The problem is studied by a combination of analytical arguments and the numerical renormalization group.

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