arXiv subjects

Andrey Surzhykov

Publications and source records attributed to Andrey Surzhykov.

At least 19 recordsLinked to original sources

arXiv2026

Spatio-spectral vector light created by optical activity in rubidium vapor

We demonstrate a pump-probe scheme in which an atomic vapor is optically pumped with circularly polarized light and probed with a vector vortex beam. The pump induces a macroscopic magnetization in the medium, which gives rise to frequency-dependent circular dichroism and birefringence. The vortex probe, characterized by spatially varying polarization, maps this optical activity onto the spatial structure of the transmitted light, thereby generating correlations between the frequency, polarization, and spatial degrees of freedom. Measuring the intensity profile in a suitable polarization component then allows us to perform spatially resolved polarization spectroscopy. We demonstrate the translation of frequency shifts into an image rotation, observing on resonance a rotation in the order of 98 mrad per MHz. These findings may find applications in high-precision spectroscopy, magnetometry, and the generation of hybrid entanglement.

physics.atom-ph↗

arXiv2026

Bound-state Compton scattering of linearly polarized photons

We present a theoretical study of Compton scattering of X- and $\gamma$-rays by a $K$-shell electron. Special attention is paid to the double-differential cross section and polarization of the scattered photons for linearly polarized incident photons. To investigate these observables, we employ the scattering matrix (S-matrix) approach based on relativistic Green's functions. The S-matrix results are moreover compared with predictions of the free-electron and impulse approximations, allowing us to assess the role of electron binding effects. Detailed calculations are carried out for hydrogen-like Ne$^{9+}$ and Pb$^{81+}$ targets over a wide range of incident photon energies and scattering angles. The calculations reveal kinematic regimes in which the impulse approximation agrees reasonably well with the S-matrix results. We also explore the polarization of scattered photons for slightly depolarized incident radiation, including the highly sensitive case of scattering at $90^\circ$.

physics.atom-ph↗

arXiv2025

Excited-state magnetic properties of carbon-like $\text{Ca}^{14+}$

We measured the $g$-factor of the excited state $^3\text{P}_1$ in $\text{Ca}^{14+}$ ion to be $g = 1.499032(6)$ with a relative uncertainty of $4\times10^{-6}$. The magnetic field magnitude is derived from the Zeeman splitting of a $\text{Be}^+$ ion, co-trapped in the same linear Paul trap as the highly charged $\text{Ca}^{14+}$ ion. Furthermore, we experimentally determined the second-order Zeeman coefficient $C_2$ of the $^3\text{P}_0$ - $^3\text{P}_1$ clock transition. For the $m_J=0\rightarrow m_{J'}=0$ transition, we obtain $C_2 = 0.39\pm0.04\text{HzmT}^{-2}$, which is to our knowledge the smallest reported for any atomic transition to date. This confirms the predicted low sensitivity of highly charged ions to higher-order Zeeman effects, making them ideal candidates for high-precision optical clocks. Comparison of the experimental results with our state-of-the art electronic structure calculations shows good agreement, and demonstrates the significance of the frequency-dependent Breit contribution, negative energy states and QED effects on magnetic moments.

physics.atom-ph↗

arXiv2025

Resonant photon scattering in the presence of external fields and its applications for the Gamma Factory

This theoretical study explores resonant elastic photon scattering in the presence of external electric and magnetic fields, motivated by potential applications in storage ring experiments, such as the Gamma Factory project at CERN. In this framework, resonant scattering involves head-on collisions of relativistic ion beams and counter-propagating laser photons, leading to a strong enhancement of the external field strength due to the Lorentz transformation between ion rest and laboratory frame. Calculations for He-like Ca ions reveal a notable impact of the external fields on the scattering rate as well as the angular distribution and polarization of emitted photons. This opens interesting avenues for diverse applications for the Gamma Factory project, such as as resonance condition tuning, beam cooling, and polarization control.

physics.acc-ph↗

arXiv2024

Hanle Effect for Lifetime Analysis: Li-like Ions

Accurate lifetime measurements of excited states of highly charged ions (HCIs) are essential for advancing diagnostics in both laboratory and astrophysical plasmas, especially in the X-ray regime. The Hanle effect, which utilizes external magnetic fields to modify photon scattering patterns, provides a powerful technique for these measurements. Previously, this method has been successfully employed for He-like ions. Here, we present a theoretical study of the prospects of the Hanle effect for lifetime determinations of Li-like ions. Our results highlight the potential for plasma diagnostics and X-ray spectral analysis.

physics.atom-ph↗

arXiv2024

Quadratic Zeeman and Electric Quadrupole Shifts in Highly Charged Ions

Recent advances in high-precision spectroscopy of highly charged ions necessitate an understanding of energy shifts of ionic levels caused by external electric and magnetic fields. Beyond the well-known Stark and linear Zeeman shifts, trapped ions may also exhibit quadratic Zeeman and electric quadrupole shifts. In this contribution, we present a systematic approach for the theoretical analysis of these shifts for arbitrary many-electron ions. Based on the derived expressions and making use of the multiconfigurational Dirac-Fock approach, we performed calculations of quadratic Zeeman shift coefficients and quadrupole moments for various ionic states in Ca$^{14+}$, Ni$^{12+}$ and Xe$^{q+}$ ions. These ions attract particular interest for ongoing and future experiments in optical clocks and tests of fundamental physics.

physics.atom-ph↗

arXiv2024

Hanle effect for lifetime determinations in the soft X-ray regime

By exciting a series of $1\mathrm{s}^{2}\, ^{1}\mathrm{S}_{0} \to 1\mathrm{s}n\mathrm{p}\, ^{1}\mathrm{P}_{1}$ transitions in helium-like nitrogen ions with linearly polarized monochromatic soft X-rays at the Elettra facility, we found a change in the angular distribution of the fluorescence sensitive to the principal quantum number $n$. In particular it is observed that the ratio of emission in directions parallel and perpendicular to the polarization of incident radiation increases with higher $n$. We find this $n$-dependence to be a manifestation of the Hanle effect, which served as a practical tool for lifetime determinations of optical transitions since its discovery in 1924. In contrast to traditional Hanle effect experiments, in which one varies the magnetic field and considers a particular excited state, we demonstrate a 'soft X-ray Hanle effect' which arises in a static magnetic field but for a series of excited states. By comparing experimental data with theoretical predictions, we were able to determine lifetimes ranging from hundreds of femtoseconds to tens of picoseconds of the $1\mathrm{s}n\mathrm{p}\, ^{1}\mathrm{P}_{1}$ levels, which find excellent agreement with atomic-structure calculations. We argue that dedicated soft X-ray measurements could yield lifetime data that is beyond current experimental reach and cannot yet be predicted with sufficient accuracy.

physics.atom-ph↗

arXiv2024

Interaction of vector light beams with atoms exposed to a time-dependent magnetic field

During recent years interest has been rising for applications of vector light beams towards magnetic field sensing. In particular, a series of experiments were performed to extract information about properties of static magnetic fields from absorption profiles of light passing through an atomic gas target. In the present work, we propose an extension to this method for oscillating magnetic fields. To investigate this scenario, we carried out theoretical analysis based on the time-dependent density matrix theory. We found that absorption profiles, even when averaged over typical observation times, are indeed sensitive to both strength and frequency of the time-dependent field, thus opening the prospect for a powerful diagnostic technique. To illustrate this sensitivity, we performed detailed calculations for the $5s \;\, {}^2S_{1/2}$ ($F=1$) $-$ $5p \;\, {}^2 P_{3/2}$ ($F=0$) transition in rubidium atoms, subject to a superposition of an oscillating (test) and a static (reference) magnetic field.

physics.atom-ph↗

arXiv2024

Coulomb excitation of hydrogen atoms by vortex ion beams

Coulomb excitation of hydrogen atoms by vortex protons is theoretically investigated within the framework of the non--relativistic first--Born approximation and the density matrix approach. Special attention is paid to the magnetic sublevel population of excited atoms and, consequently, to the angular distribution of the fluorescence radiation. We argue that both these properties are sensitive to the projection of the orbital angular momentum (OAM), carried by the projectile ions. In order to illustrate the OAM--effect, detailed calculations have been performed for the $1s \to 2p$ excitation and the subsequent $2p \to 1s$ radiative decay of a hydrogen target, interacting with incident Laguerre--Gaussian vortex protons. The calculation results suggest that Coulomb excitation can be employed for the diagnostics of vortex ion beam at accelerator and storage ring facilities.

physics.atom-ph↗

arXiv2023

Calculation of isotope shifts and King plot nonlinearities in Ca$^+$

Many-body perturbation theory is implemented in order to calculate the isotope shifts of $4s$, $4p_{1/2}$, $4p_{3/2}$, $3d_{3/2}$, and $3d_{5/2}$ energy levels of Ca$^+$, for even isotopes $A=$40, 42, 44, 46, 48. The results are presented for mass shift and field shift, as well as for higher-order field shifts, quadratic mass shift, nuclear polarization correction, and the cross term between field and mass shifts. Additionally, we examine King-plot nonlinearities introduced by the higher-order isotope-shift corrections to the combinations of $3d_{3/2}\rightarrow 4s$, $3d_{5/2}\rightarrow 4s$, and $4p_{1/2}\rightarrow 4s$ transitions. For these transitions, second-order mass shift and nuclear polarization correction are identified as the dominant sources of King plot nonlinearity.

physics.atom-ph↗

arXiv2023

Excitation of forbidden electronic transitions in atoms by Hermite-Gaussian modes

Photoexcitation of trapped ions by Hermite-Gaussian (HG) modes from guided beam structures is proposed and investigated theoretically. In particular, simple analytical expressions for the Rabi frequencies of induced atomic transitions are derived that depend both on the parameters of HG beams and on the geometry of an experiment. By using these general expressions, we investigate the $^{2}S_{1/2} \to \; ^{2}F_{7/2}$ electric octupole (E3) transition in an Yb$^{+}$ ion, localized in the low--intensity center of the HG$_{10}$ and HG$_{01}$ beams. We show how the corresponding Rabi frequency can be enhanced by properly choosing the polarization of incident light and the orientation of an external magnetic field, which defines the quantization axis of a target ion. The calculations, performed for experimentally feasible beam parameters, indicate that the achieved Rabi frequencies can be comparable or even higher than those observed for the conventional Laguerre-Gaussian (LG) modes. Since HG-like modes can be relatively straightforwardly generated with high purity and stability from integrated photonics, our results suggest that they may form a novel tool for investigating highly-forbidden atomic transitions.

physics.atom-ph↗

arXiv2023

Using gravitational light deflection in optical cavities for laser frequency stabilization

We theoretically investigate the propagation of light in the presence of a homogeneous gravitational field. To model this, we derive the solutions of the wave equation in Rindler spacetime, which account for gravitational redshift and light deflection. The developed theoretical framework is used to explore the propagation of plane light waves in a horizontal Fabry-Perot cavity. We pay particular attention to the cavity output power. It is shown that this power depends not only on the input frequency, but also on the vertical position of a detector. We state that the height-dependent detector signal arising from the cavity internal light deflection effect (CILD-effect) also opens a new alternative way to frequency stabilization in Earth-based laser experiments and to study gravitational light deflection at laboratory scales.

gr-qc↗

arXiv2022

Excitation and probing of low-energy nuclear states at high-energy storage rings

$^{229}$Th with a low-lying nuclear isomeric state is an essential candidate for a nuclear clock as well as many other applications. Laser excitation of the isomeric state has been a long-standing goal. With relativistic $^{229}$Th ions in storage rings, high-power lasers with wavelengths in the visible range or longer can be used to achieve high excitation rates of $^{229}$Th isomers. This can be realized through direct resonant excitation, or excitation via an intermediate nuclear or electronic state, facilitated by the tunability of both the laser-beam and ion-bunch parameters. Unique opportunities are offered by highly charged $^{229}$Th ions due to the nuclear-state mixing. The significantly reduced isomeric-state lifetime corresponds to a much higher excitation rate for direct resonant excitation. Importantly, we propose electric dipole transitions changing both the electronic and nuclear states that are opened by the nuclear hyperfine mixing. We suggest using them for efficient isomer excitation in Li-like $^{229}$Th ions, via stimulated Raman adiabatic passage or single-laser excitation. We also propose schemes for probing the isomers, utilizing nuclear radiative decay or laser spectroscopy on electronic transitions, through which the isomeric-state energy can be determined with an orders-of-magnitude higher precision than the current value. The schemes proposed here for $^{229}$Th could also be adapted to low-energy nuclear states in other nuclei, such as $^{229}$Pa.

nucl-ex↗

arXiv2022

An Optical Atomic Clock Based on a Highly Charged Ion

Optical atomic clocks are the most accurate measurement devices ever constructed and have found many applications in fundamental science and technology. The use of highly charged ions (HCI) as a new class of references for highest accuracy clocks and precision tests of fundamental physics has long been motivated by their extreme atomic properties and reduced sensitivity to perturbations from external electric and magnetic fields compared to singly charged ions or neutral atoms. Here we present the first realisation of this new class of clocks, based on an optical magnetic-dipole transition in Ar$^{13+}$. Its comprehensively evaluated systematic frequency uncertainty of $2.2\times10^{-17}$ is comparable to that of many optical clocks in operation. From clock comparisons we improve by eight and nine orders of magnitude upon the uncertainties for the absolute transition frequency and isotope shift ($^{40}$Ar vs. $^{36}$Ar), respectively. These measurements allow us to probe the largely unexplored quantum electrodynamic nuclear recoil, presented as part of improved calculations of the isotope shift which reduce the uncertainty of previous theory by a factor of three. This work establishes forbidden optical transitions in HCI as references for cutting-edge optical clocks and future high-sensitivity searches for physics beyond the standard model.

physics.atom-ph↗

arXiv2022

Parity-violation studies with partially stripped ions

We present a theoretical study of photoexcitation of highly charged ions from their ground states, a process which can be realized at the Gamma Factory at CERN. Special attention is paid to the question of how the excitation rates are affected by the mixing of opposite-parity ionic levels, which is induced both by an external electric field and the weak interaction between electrons and the nucleus. In order to reinvestigate this "Stark-plus-weak-interaction" mixing, well-known in neutral atomic systems, we employ relativistic Dirac theory. Based on the developed approach, detailed calculations are performed for the ${\rm 1s}_{1/2} \to {\rm 2s}_{1/2}$ and ${\rm 1s}^2 \; {\rm 2s}_{1/2} \to {\rm 1s}^2 \; {\rm 3s}_{1/2}$ (M1 + parity-violating-E1) transitions in hydrogen- and lithium-like ions, respectively. In particular, we focus on the difference between the excitation rates obtained for the right- and left-circularly polarized incident light. This difference arises due to the parity violating mixing of ionic levels and is usually characterized in terms of the circular-dichroism parameter. We argue that future measurements of circular dichroism, performed with highly charged ions in the SPS or LHC rings, may provide valuable information on the electron-nucleus weak-interaction coupling.

physics.atom-ph↗

arXiv2021

Radiative recombination of twisted electrons with hydrogen-like heavy ions: Linear polarization of emitted photons

We present a theoretical investigation of the radiative recombination of twisted Bessel electrons with initially hydrogen-like (finally helium-like) heavy ions. In our study, we focus especially on the linear polarization of x-ray photons emitted in the electron capture into the ground $1s^2_{1/2}$ ionic state. Particular emphasis is placed on the question of how this polarization is affected if incident hydrogen-like ions are themselves spin-polarized. To explore such a "polarization transfer" we apply the density matrix theory and derive the Stokes parameters of recombination x-rays for the realistic case of collisions between macroscopic electron and ion beams. Based on the developed general approach two scenarios are discussed that are of interest for the planned experiments at ion storage rings. First, we demonstrate how the use of twisted electrons can empower the known method for the diagnostics of spin-polarized ion beams, based on the rotation of the linear polarization of recombination light. In the second scenario we show how the internal structure of ions beams with inhomogeneous intensity and spin patterns can be probed by the capture of Bessel electrons, carrying different values of angular momentum.

physics.atom-ph↗

arXiv2021

Resonant scattering of plane-wave and twisted photons at the Gamma Factory

We present a theoretical investigation of the resonant elastic scattering of laser photons by ultra-relativistic partially stripped ions, that is the core process of the Gamma Factory project. Special emphasis in our study is placed on the angular distribution and polarization of scattered photons as observed in the collider and ion-rest reference frames. In order to describe these (angular and polarization) properties for arbitrary relativistic many-electron ion, the general approach, based on the application of irreducible polarization tensors, is laid down. By making use of the polarization tensors we explore in detail the scattering of both, conventional plane-wave- and twisted (or vortex) photons. For the former case we show how the propagation directions and polarization states of incident and outgoing photons are related to each other for the $n S_{0} \to n' P_{1} \to n S_{0}$, $n S_{1/2} \to n' P_{1/2} \to n S_{1/2}$ and $n S_{1/2} \to n' P_{3/2} \to n S_{1/2}$ resonant transitions. For the scattering of initially twisted light, that carries non-zero orbital angular momentum, we explore the angular distribution of secondary photons and discuss the conditions under which they are also twisted.

physics.atom-ph↗

arXiv2021

Nonlinearities of King's plot and their dependence on nuclear radii

Investigations of isotope shifts of atomic spectral lines provide insights into nuclear properties. Deviations from the linear dependence of the isotope shifts of two atomic transitions on nuclear parameters, leading to a nonlinearity of the so-called King plot, are actively studied as a possible way of searching for the new physics. In the present work we calculate the King-plot nonlinearities originating from the Standard-Model atomic theory. The calculation is performed both analytically, for a model example applicable for an arbitrary atom, and numerically, for one-electron ions. It is demonstrated that the Standard-Model predictions of the King-plot nonlinearities are hypersensitive to experimental errors of nuclear charge radii. This effect significantly complicates identifications of possible King-plot nonlinearities originating from the new physics.

physics.atom-ph↗