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Angelika Knothe

Publications and source records attributed to Angelika Knothe.

33 records · Page 2Linked to original sources

Shell Filling and Trigonal Warping in Graphene Quantum Dots

Transport measurements through a few-electron circular quantum dot in bilayer graphene display bunching of the conductance resonances in groups of four, eight and twelve. This is in accordance with the spin and valley degeneracies in bilayer graphene and an additional threefold 'minivalley degeneracy' caused by trigonal warping. For small electron numbers, implying a small dot size and a small displacement field, a two-dimensional s- and then a p-shell are successively filled with four and eight electrons, respectively. For electron numbers larger than twelve, as the dot size and the displacement field increase, the single-particle ground state evolves into a three-fold degenerate minivalley ground state. A transition between these regimes is observed in our measurements and can be described by band-structure calculations. Measurements in magnetic field confirm Hund's second rule for spin filling of the quantum dot levels, emphasizing the importance of exchange interaction effects.

cond-mat.mes-hall↗

Theory of tunneling spectra for a few-electron bilayer graphene quantum dot

The tuneability and control of quantum nanostructures in two-dimensional materials offer promising perspectives for their use in future electronics. It is hence necessary to analyze quantum transport in such nanostructures. Material properties such as a complex dispersion, topology, and charge carriers with multiple degrees of freedom, are appealing for novel device functionalities but complicate their theoretical description. Here, we study quantum tunnelling transport across a few-electron bilayer graphene quantum dot. We demonstrate how to uniquely identify single- and two-electron dot states' orbital, spin, and valley composition from differential conductance in a finite magnetic field. Furthermore, we show that the transport features manifest splittings in the dot's spin and valley multiplets induced by interactions and magnetic field (the latter splittings being a consequence of bilayer graphene's Berry curvature). Our results elucidate spin- and valley-dependent tunnelling mechanisms and will help to utilize bilayer graphene quantum dots, e.g., as spin and valley qubits.

cond-mat.mes-hall↗

Kondo effect and spin-orbit coupling in graphene quantum dots

The Kondo effect is a cornerstone in the study of strongly correlated fermions. The coherent exchange coupling of conduction electrons to local magnetic moments gives rise to a Kondo cloud that screens the impurity spin. Whereas complete Kondo screening has been explored widely, realizations of the underscreened scenario - where only some of several Kondo channels participate in the screening - remain rare. Here we report the observation of fully screened and underscreened Kondo effects in quantum dots in bilayer graphene. More generally, we introduce a unique platform for studying Kondo physics. In contrast to carbon nanotubes, whose curved surfaces give rise to strong spin-orbit coupling breaking the SU(4) symmetry of the electronic states relevant for the Kondo effect, we study a nominally flat carbon material with small spin-orbit coupling. Moreover, the unusual two-electron triplet ground state in bilayer graphene dots provides a route to exploring the underscreened spin-1 Kondo effect.

cond-mat.mes-hall↗

Tunable valley splitting and bipolar operation in graphene quantum dots

Quantum states in graphene are four-fold degenerate: two fold in spins, and two fold in valleys.Both degrees of freedom can be utilized for qubit preparations. In our bilayer graphene quantumdots, we demonstrate that the valley g-factorgv, defined analogously as the spin g-factorgsforvalley splitting in perpendicular magnetic field, is tunable by over a factor of 4 from 20 to 90. Wefind that largergvresults from larger electronic dot sizes, determined from the charging energy.This control is achieved by adjusting voltages on merely two gates, which also allows for tuning ofthe dot-lead tunnel coupling. On our versatile device, bipolar operation, charging our quantum dotwith charge carriers of the same or the opposite polarity as the leads, can be performed. Dots ofboth polarity are tunable to the first charge carrier by action of the plunger gate, such that thetransition from an electron to a hole dot can be observed. By adding more gates, this system caneasily be extended to host double dots.

cond-mat.mes-hall↗

Coherent Jetting behind a gate-defined Channel in Bilayer Graphene

Graphene has evolved as a platform for quantum transport that can compete with the best and cleanest semiconductor systems. Recently, many interesting local properties of carrier transport in graphene have been investigated by various scanning probe techniques. Here, we report on the observation of distinct electronic jets emanating from a narrow split-gate defined channel in bilayer graphene. We find that these jets, which are visible via their interference patterns, occur predominantly with an angle of 60° between each other. This observation is related to the specific bandstructure of bilayer graphene, in particular trigonal warping, which leads to a valley-dependent selection of momenta for low-energy conduction channels. This experimental observation of electron jetting has consequences for carrier transport in graphene in general as well as for devices relying on ballistic and valley selective transport.

cond-mat.mes-hall↗

Tunable Valley Splitting due to Topological Orbital Magnetic Moment in Bilayer Graphene Quantum Point Contacts

In multivalley semiconductors, the valley degree of freedom can be potentially used to store, manipulate and read quantum information, but its control remains challenging. The valleys in bilayer graphene can be addressed by a perpendicular magnetic field which couples by the valley g-factor. However, control over the valley g-factor has not been demonstrated yet. We experimentally determine the energy spectrum of a quantum point contact realized by a suitable gate geometry in bilayer graphene. Using finite bias spectroscopy we measure the energy scales arising from the lateral confinement as well as the Zeeman splitting and find a spin g-factor of 2. The valley g-factor can be tuned by a factor of 3 using vertical electric fields, reaching values between 40 and 120. The results are quantitatively explained by a calculation considering topological magnetic moment and its dependence on confinement and the vertical displacement field.

cond-mat.mes-hall↗

Quartet states in two-electron quantum dots in bilayer graphene

Trapping electrons in quantum dots and controlling their collective quantum states is crucial for converting semiconductor structures into bits of quantum information processing. Here, we study single- and two-particle states in quantum dots formed in gapped bilayer graphene (BLG), where the electron's valley states appear in pair with their spin quantum number and we analyse spin- and valley-singlet and triplet states for various BLG and dot parameters, as well as two-particle interaction strength and external magnetic field.

cond-mat.mes-hall↗

Composite super-moiré lattices in double aligned graphene heterostructures

When two-dimensional atomic crystals are brought into close proximity to form a van der Waals heterostructure, neighbouring crystals can start influencing each others electronic properties. Of particular interest is the situation when the periodicity of the two crystals closely match and a moiré pattern forms, which results in specific electron scattering, reconstruction of electronic and excitonic spectra, crystal reconstruction, and many other effects. Thus, formation of moiré patterns is a viable tool of controlling the electronic properties of 2D materials. At the same time, the difference in the interatomic distances for the two crystals combined, determines the range in which the electronic spectrum is reconstructed, and thus is a barrier to the low energy regime. Here we present a way which allows spectrum reconstruction at all energies. By using graphene which is aligned simultaneously to two hexagonal boron nitride layers, one can make electrons scatter in the differential moiré pattern, which can have arbitrarily small wavevector and, thus results in spectrum reconstruction at arbitrarily low energies. We demonstrate that the strength of such a potential relies crucially on the atomic reconstruction of graphene within the differential moiré super-cell. Such structures offer further opportunity in tuning the electronic spectra of two-dimensional materials.

cond-mat.mes-hall↗

Semimetallic features in quantum transport through a gate-defined point contact in bilayer graphene

We demonstrate that, at the onset of conduction, an electrostatically defined quantum wire in bilayer graphene (BLG) with an interlayer asymmetry gap may act as a 1D semimetal, due to the multiple minivalley dispersion of its lowest subband. Formation of a non-monotonic subband coincides with a near-degeneracy between the bottom edges of the lowest two subbands in the wire spectrum, suggesting an $8e^2/h$ step at the conduction threshold, and the semimetallic behaviour of the lowest subband in the wire would be manifest as resonance transmission peaks on an $8e^2/h$ conductance plateau.

cond-mat.mes-hall↗

Influence of minivalleys and Berry curvature on electrostatically induced quantum wires in gapped bilayer graphene

We show that the spectrum of subbands in an electrostatically defined quantum wire in gapped bilayer graphene directly manifests the minivalley structure and reflects Berry curvature via the associated magnetic moment of the states in the low-energy bands of this two-dimensional material. We demonstrate how these appear in degeneracies of the low-energy minibands and their valley splitting, which develops linearly in a weak magnetic field. Consequently, magneto-conductance of a ballistic point contact connecting two non-gapped areas of a bilayer through a gapped (top and bottom gated) barrier would reflect such degeneracies by the heights of the first few conductance steps developing upon the increase of the doping of the BLG conduction channel: $8e^2/h$ steps in a wide channel in BLG with a large gap, $4e^2/h$ steps in narrow channels, all splitting into a staircase of $2e^2/h$ steps upon lifting valley degeneracy by a magnetic field.

cond-mat.mes-hall↗

Topologically non-trivial valley states in bilayer graphene quantum point contacts

We present measurements of quantized conductance in electrostatically induced quantum point contacts in bilayer graphene. The application of a perpendicular magnetic field leads to an intricate pattern of lifted and restored degeneracies with increasing field: at zero magnetic field the degeneracy of quantized one-dimensional subbands is four, because of a twofold spin and a twofold valley degeneracy. By switching on the magnetic field, the valley degeneracy is lifted. Due to the Berry curvature states from different valleys split linearly in magnetic field. In the quantum Hall regime fourfold degenerate conductance plateaus reemerge. During the adiabatic transition to the quantum Hall regime, levels from one valley shift by two in quantum number with respect to the other valley, forming an interweaving pattern that can be reproduced by numerical calculations.

cond-mat.mes-hall↗

Phase diagram of a graphene bilayer in the zero-energy Landau level

Bilayer graphene under a magnetic field has an octet of quasidegenerate levels due to spin, valley, and orbital degeneracies. This zero-energy Landau level is resolved into several incompressible states whose nature is still elusive. We use a Hartree-Fock treatment of a realistic tight-binding four-band model to understand the quantum ferromagnetism phenomena expected for integer fillings of the octet levels. We include the exchange interaction with filled Landau levels below the octet states. This Lamb-shift-like effect contributes to the orbital splitting of the octet. We give phase diagrams as a function of applied bias and magnetic field. Some of our findings are in agreement with experiments. We discuss the possible appearance of phases with orbital coherence.

cond-mat.str-el↗

Edge structure of graphene monolayers in the ν = 0 quantum Hall state

Monolayer graphene at neutrality in the quantum Hall regime has many competing ground states with various types of ordering. The outcome of this competition is modified by the presence of the sample boundaries. In this paper we use a Hartree-Fock treatment of the electronic correlations allowing for space-dependent ordering. The edge influence is modeled by a simple perturbative effective magnetic field in valley space. We find that all phases found in the bulk of the sample, ferromagnetic, canted antiferromagnetic, charge-density wave and Kekul$é$ distortion are smoothly connected to a Kekul$é$-distorted edge. The single-particle excitations are computed taking into account the spatial variation of the order parameters. An eventual metal-insulator transition as a function of the Zeeman energy is not simply related to the type of bulk order.

cond-mat.str-el↗

Frequency correlations in reflection from random media

We present a theoretical study of frequency correlations of light backscattered from a random scattering medium. This statistical quantity provides insight into the dynamics of multiple scattering processes accessible both, in theoretical and experimental investigations. For frequency correlations between field amplitudes, we derive a simple expression in terms of the path length distribution of the underlying backscattering processes. In a second step, we apply this relation to describe frequency correlations between intensities in the regime of weak disorder. Since, with increasing disorder strength, an unexplained breakdown of the angular structure of the frequency correlation function has recently been reported in experimental studies, we explore extensions of our model to the regime of stronger disorder. In particular, we show that closed scattering trajectories tend to suppress the angular dependence of the frequency correlation function.

physics.optics↗

Flux conservation in coherent backscattering and weak localisation of light

The standard theoretical description of coherent backscattering, accord- ing to which maximally crossed diagrams accounting for interference between counter- propagating path amplitudes are added on top of the incoherent background, violates the fundamental condition of flux conservation. In contrast to predictions of previous theories, we show that including maximally crossed diagrams with one additional scat- tering event does not restore flux conservation. Instead, we propose that the latter is recovered when treating the effects of coherent backscattering and weak localisation in a unified framework. On the basis of this framework, we demonstrate explicitly flux conservation in leading order of the weak disorder parameter 1/(kl).

cond-mat.dis-nn↗