arXiv subjects

Ania C. Bleszynski Jayich

Publications and source records attributed to Ania C. Bleszynski Jayich.

At least 19 recordsLinked to original sources

arXiv2026

Engineering and Probing a One-Dimensional Dipolar Spin Ensemble in Diamond

Dimensionality plays a central role in determining the collective behavior of interacting quantum systems. Engineering strongly interacting ensembles of solid-state spin defects in reduced dimensions remains a significant challenge at the interface between the applied and fundamental sciences. Here, we create and characterize a positionally disordered, quasi-one-dimensional spin chain in diamond, consisting of optically dark substitutional nitrogen defects (P1 centers) and optically addressable probe nitrogen-vacancy (NV) centers. Our approach exploits the preferential incorporation of nitrogen along step bunches formed during chemical vapor deposition to achieve both lateral and vertical confinement. Combining spatially resolved materials characterization with nanoscale quantum sensing, we establish the one-dimensional character of the optically dark, unpolarized P1 spin ensemble. We then use correlation spectroscopy to probe local spin autocorrelations and investigate infinite-temperature dipolar spin transport. Our results establish a materials-based route for engineering low-dimensional quantum spin systems.

quant-ph↗

arXiv2026

Direct Observation of Dipolar-Driven Anisotropic Quantum Projection Noise in a Solid-State Spin Ensemble

The nitrogen-vacancy (NV) center in diamond is a prominent quantum-sensing platform. Combining readout at the quantum projection noise limit with strong dipolar interactions promises substantial gains in sensitivity. However, experimentally accessing this regime has remained a longstanding challenge. In this work, we demonstrate quantum-projection-noise-resolved readout of a strongly-interacting, two-dimensional ensemble of NV centers. Our approach leverages repetitive readout via the NV's intrinsic $^{15}$N nuclear memory at a moderate magnetic field ($\sim 0.3$ T), improving the readout fidelities by nearly an order of magnitude. This enables us to directly resolve the quantum projection noise of a coherent spin state and to watch the ensemble's intrinsic dipolar interactions shear this noise into an anisotropic profile. Our results open the door to direct measurements of spin squeezing and entanglement-enhanced sensing in the solid state.

quant-ph↗

arXiv2026

Nanoscale magnetometry via collective many-body dynamics in diamond

Many-body dynamics constitutes a promising approach for creating correlations between quantum particles which can be used for applications in sensing and metrology. However, utilizing this potential for substantial gains in practical settings is a challenging task with only a very few applications realized to date. Here, we demonstrate an approach to nanoscale magnetic sensing enabled by strongly interacting electronic spins in a room temperature solid. By coherently controlling collective many-body dynamics of a dipolar ensemble of $\sim 10^4$ nitrogen-vacancy (NV) centres in diamond with pulsed magnetic field gradients, we demonstrate practical metrological gain up to $7.9(2)\,\mathrm{dB}$ for magnetic signal detection and $8.8(3)\,\mathrm{dB}$ for magnetic noise sensing, fully accounting for experimental overheads. Finally, we combine these methods to demonstrate a momentum-space-resolved sensing modality that enables detection of spatially correlated magnetic noise at continuously tunable length scales down to 50 nanometers. These observations open the door toward practical applications of interaction-enhanced quantum sensors for nanoscale biological imaging and material characterization.

quant-ph↗

arXiv2026

Imaging flat band electron hydrodynamics in biased bilayer graphene

Hydrodynamic electron transport arises when carrier kinetics are dominated by interelectron collisions rather than the relaxation of momentum out of the electron system. In recent years, signatures of electron hydrodynamics have been reported in graphene devices owing to the low disorder and weak electron-phonon coupling. However, these experiments have been performed in regimes where the carrier mass is light, and the electron-electron collision length--though smaller than corresponding lengths for phonon or impurity scattering--remains large in absolute terms, typically several hundred nanometers. This restricts hydrodynamic transport phenomena to large length scales, limiting miniaturization of devices based on hydrodynamic flow. The advent of dual-gated rhombohedral graphene multilayers introduces a new route toward enhanced hydrodynamic behavior via their large--and tunable--effective mass. Here, we employ a scanning superconducting magnetic sensor to image local current flow in dual-gated bilayer graphene. Exploiting a sample geometry sensitive to both laminar and vortical flow, we identify three distinct transport regimes--ballistic, hydrodynamic, and diffusive--across the full phase space spanned by carrier density and displacement field. The strongest hydrodynamic transport is observed in the flat band regime, where fitting our results to a unified Boltzmann transport model reveals the electron-electron scattering length to be comparable to the Fermi wavelength of ~50 nm. High-current measurements, meanwhile, reveal striking nonlinearities in the flow pattern. Our results pave the way for miniaturized electronic devices based on linear and nonlinear electron hydrodynamics.

cond-mat.mes-hall↗

arXiv2026

Quantum Nanophotonic Interface for Tin-Vacancy Centers in Thin-Film Diamond

The negatively charged tin-vacancy center in diamond (SnV$^-$) is an excellent solid state qubit with optically-addressable transitions and a long electron spin coherence time at elevated ($\sim1.7$ K). However, implementing scalable quantum nodes with high-fidelity optical readout of the electron spin state requires efficient photon emission and collection from the system. In this manuscript, we report a quantum photonic interface for SnV$^-$ centers based on one-dimensional photonic crystal cavities fabricated in diamond thin films. Furthermore, we provide a rigorous description of the spontaneous emission dynamics of our system, taking into account individual contributions from both the C and D transitions of the emitter. This allows for determination of Purcell factors per transition and, by extension, the C/D branching ratio SnV$^{-}$ zero phonon line. We observe quality factors up to $\sim$6000 across this sample, and measure up to a 12-fold lifetime reduction, which translates into a Purcell factor of $F_C=26.2\pm1.5$ for a targeted C transition. By considering the cavity mode polarization alignment with the C and D transition dipole moments, we validate the C/D branching ratio to be $η_{\text{BR}}=0.75\pm0.01$, in line with previous theoretical and experimental findings.

quant-ph↗

arXiv2026

Detecting quantum noise of a solid-state spin ensemble with dispersive measurement

We theoretically explore protocols for measuring the spin polarization of an ensemble of solid-state spins, with precision at or below the standard quantum limit. Such measurements in the solid-state are challenging, as standard approaches based on optical fluorescence are often limited by poor readout fidelity. Indirect microwave resonator-mediated measurements provide an attractive alternative, though a full analysis of relevant sources of measurement noise is lacking. In this work we study dispersive readout of an inhomogeneously broadened spin ensemble via coupling to a driven resonator measured via homodyne detection. We derive generic analytic conditions for when the homodyne measurement can be limited by the fundamental spin-projection noise, as opposed to microwave-drive shot noise or resonator phase noise. By studying fluctuations of the measurement record in detail, we also propose an experimental protocol for directly detecting spin squeezing, i.e. a reduction of the spin ensemble's intrinsic projection noise from entanglement. Our protocol provides a method for benchmarking entangled states for quantum-enhanced metrology.

quant-ph↗

arXiv2025

Creation of Depth-Confined, Shallow Nitrogen-Vacancy Centers in Diamond With Tunable Density

Engineering shallow nitrogen-vacancy (NV) centers in diamond holds the key to unlocking new advances in nanoscale quantum sensing. We find that the creation of near-surface NVs through delta doping during diamond growth allows for tunable control over both NV depth confinement (with a twofold improvement relative to low-energy ion implantation) and NV density, ultimately resulting in highly-sensitive single defects and ensembles with coherence limited by NV-NV interactions. Additionally, we demonstrate the utility of our shallow delta-doped NVs by imaging magnetism in few-layer CrSBr, a two-dimensional magnet. We anticipate that the control afforded by near-surface delta doping will enable new developments in NV quantum sensing from nanoscale NMR to entanglement-enhanced metrology.

quant-ph↗

arXiv2025

Dressed-state Hamiltonian engineering in a strongly interacting solid-state spin ensemble

In quantum science applications, ranging from many-body physics to quantum metrology, dipolar interactions in spin ensembles are controlled via Floquet engineering. However, this technique typically reduces the interaction strength between spins, and effectively weakens the coupling to a target sensing field, limiting the metrological sensitivity. In this work, we develop and demonstrate a method for direct tuning of the native interaction in an ensemble of nitrogen-vacancy (NV) centers in diamond. Our approach utilizes dressed-state qubit encoding under a magnetic field perpendicular to the crystal lattice orientation. This method leads to a $3.2\times$ enhancement of the dimensionless coherence parameter $JT_2$ compared to state-of-the-art Floquet engineering, and a $2.6\times$ ($8.3~$dB) enhanced sensitivity in AC magnetometry. Utilizing the extended coherence we experimentally probe spin transport at intermediate to late times. Our results provide a powerful Hamiltonian engineering tool for future studies with NV ensembles and other interacting higher-spin ($S>\frac{1}{2}$) systems.

quant-ph↗

arXiv2025

Collective many-body dynamics in a solid-state quantum sensor controlled through nanoscale magnetic gradients

Coherent collective dynamics of strongly interacting qubits are a central resource in quantum information science, with applications from quantum computing and simulation to metrology. While electronic spins interact strongly via dipolar couplings in dense solid-state ensembles, imperfections and positional disorder pose major obstacles to coherent correlated behavior, limiting their usefulness. Here, we realize collective many-body dynamics by combining time-dependent magnetic field gradients with global coherent control of dense electron spin ensembles in diamond. We control and probe the dynamics of nanometer-scale spin spirals, and, by exploiting Hamiltonian engineering that enhances the microscopic symmetry of the interactions, we observe a disorder-resilient collective spin evolution. Our results establish a pathway to interaction-enhanced quantum metrology and nanoscale imaging of materials and biological systems under ambient conditions.

quant-ph↗

arXiv2025

Patterning programmable spin arrays on DNA origami for quantum technologies

The controlled assembly of solid-state spins with nanoscale spatial precision is an outstanding challenge for quantum technology. Here, we combine DNA-based patterning with nitrogen-vacancy (NV) ensemble quantum sensors in diamond to form and sense programmable 2D arrays of spins. We use DNA origami to control the spacing of chelated Gd$^{3+}$ spins, as verified by the observed linear relationship between proximal NVs' relaxation rate, $1/T_1$, and the engineered number of Gd$^{3+}$ spins per origami unit. We further show that DNA origami provides a robust way of functionalizing the diamond surface with spins as it preserves the charge state and spin coherence of proximal, shallow NV centers. Our work enables the formation and interrogation of ordered, strongly interacting spin networks with applications in quantum sensing and quantum simulation. We quantitatively discuss the prospects of entanglement-enhanced metrology and high-throughput proteomics.

quant-ph↗

arXiv2025

A spin-embedded diamond optomechanical resonator with mechanical quality factor exceeding one million

Diamond optomechanical crystal (OMC) devices with embedded color center spins are promising platforms for a broad range of applications in quantum sensing, networking, and computing applications, offering an interface between a GHz-frequency mechanical mode and both optical photons and coherent spins. A crucial but elusive step towards realizing this platform is to engineer a device with a high-quality factor mechanical mode while preserving the bulk-like coherence of embedded spins. Here we demonstrate sideband-resolved diamond OMCs with mechanical quality factors in excess of $10^6$ at cryogenic temperatures, and find coherence times up to $T_2$ = 270 $μ$s for embedded nitrogen vacancy (NV) centers. Furthermore, we measure these devices across five orders of magnitude in intracavity optical power, demonstrating robust power handling and a high optomechanical cooperativity ($C\gg1$) at cryogenic temperatures that is essential for a broad range of quantum protocols requiring strong, coherent interactions between photons and phonons. These results are enabled by a robust, high-throughput method for forming single-crystal diamond membranes in combination with chemical vapor deposition (CVD) diamond overgrowth with nitrogen $δ$-doping. We discuss the prospects of this platform for hybrid spin-mechanical devices in the quantum regime.

quant-ph↗

arXiv2025

Integrated phononic waveguide on thin-film lithium niobate on diamond

We demonstrate wavelength-scale phononic waveguides formed by transfer-printed thin-film lithium niobate (LN) on bulk diamond (LNOD), a material stack that combines the strong piezoelectricity of LN with the high acoustic velocity and color-center compatibility of diamond. We characterize a delay line based on a 100 micron long phononic waveguide at room and cryogenic temperatures. The total insertion loss through the device at 4 kelvin is -5.8 dB, corresponding to a >50% transducer efficiency, at a frequency of 2.8 gigahertz. Our work represents a step towards phonon-mediated hybrid quantum systems consisting of strain-sensitive color centers in diamond.

cond-mat.mes-hall↗

arXiv2025

Signal amplification in a solid-state quantum sensor via asymmetric time-reversal of many-body dynamics

Electronic spins of nitrogen vacancy (NV) centers in diamond constitute a promising system for micro- and nano-scale magnetic sensing, due to their operation under ambient conditions, ease of placement in close proximity to sensing targets, and biological compatibility. At high densities, the electronic spins interact through dipolar coupling, which typically limits but can also potentially enhance sensing performance. Here we report the experimental demonstration of many-body signal amplification in a solid-state, room temperature quantum sensor. Our approach utilizes time-reversed two-axis-twisting interactions, engineered through dynamical control of the quantization axis and Floquet engineering in a two-dimensional ensemble of NV centers. Strikingly, we observe that the optimal amplification occurs when the backward evolution time equals twice the forward evolution time, in sharp contrast to the conventional Loschmidt echo. These observations can be understood as resulting from an underlying time-reversed mirror symmetry of the microscopic dynamics, providing key insights into signal amplification and opening the door towards entanglement-enhanced practical quantum sensing.

quant-ph↗

arXiv2025

Spin squeezing in an ensemble of nitrogen-vacancy centers in diamond

Spin squeezed states provide a seminal example of how the structure of quantum mechanical correlations can be controlled to produce metrologically useful entanglement. Such squeezed states have been demonstrated in a wide variety of artificial quantum systems ranging from atoms in optical cavities to trapped ion crystals. By contrast, despite their numerous advantages as practical sensors, spin ensembles in solid-state materials have yet to be controlled with sufficient precision to generate targeted entanglement such as spin squeezing. In this work, we present the first experimental demonstration of spin squeezing in a solid-state spin system. Our experiments are performed on a strongly-interacting ensemble of nitrogen-vacancy (NV) color centers in diamond at room temperature, and squeezing (-0.5 $\pm$ 0.1 dB) is generated by the native magnetic dipole-dipole interaction between NVs. In order to generate and detect squeezing in a solid-state spin system, we overcome a number of key challenges of broad experimental and theoretical interest. First, we develop a novel approach, using interaction-enabled noise spectroscopy, to characterize the quantum projection noise in our system without directly resolving the spin probability distribution. Second, noting that the random positioning of spin defects severely limits the generation of spin squeezing, we implement a pair of strategies aimed at isolating the dynamics of a relatively ordered sub-ensemble of NV centers. Our results open the door to entanglement-enhanced metrology using macroscopic ensembles of optically active spins in solids.

quant-ph↗

arXiv2025

Scalable, nanoscale positioning of highly coherent color centers in prefabricated diamond nanostructures

Nanophotonic devices in color center-containing hosts provide efficient readout, control, and entanglement of the embedded emitters. Yet control over color center formation - in number, position, and coherence - in nanophotonic devices remains a challenge to scalability. Here, we report a controlled creation of highly coherent diamond nitrogen-vacancy (NV) centers with nanoscale three-dimensional localization in prefabricated nanostructures with high yield. Combining nitrogen $δ$-doping during chemical vapor deposition diamond growth and localized electron irradiation, we form shallow NVs registered to the center of diamond nanopillars with wide tunability over NV number. We report positioning precision of ~ 4 nm in depth and 46(1) nm laterally in pillars (102(2) nm in bulk diamond). We reliably form single NV centers with long spin coherence times (average $T_2^{Hahn}$ = 98 $μs$) and 1.8x higher average photoluminescence compared to NV centers randomly positioned in pillars. We achieve a 3x improved yield of NV centers with single electron-spin sensitivity over conventional implantation-based methods. Our high-yield defect creation method will enable scalable production of solid-state defect sensors and processors.

quant-ph↗

arXiv2024

A strongly interacting, two-dimensional, dipolar spin ensemble in (111)-oriented diamond

Systems of spins with strong dipolar interactions and controlled dimensionality enable new explorations in quantum sensing and simulation. In this work, we investigate the creation of strong dipolar interactions in a two-dimensional ensemble of nitrogen-vacancy (NV) centers generated via plasma-enhanced chemical vapor deposition (PECVD) on (111)-oriented diamond substrates. We find that diamond growth on the (111) plane yields high incorporation of spins, both nitrogen and NV centers, where the density of the latter is tunable via the miscut of the diamond substrate. Our process allows us to form dense, preferentially aligned, 2D NV ensembles with volume-normalized AC sensitivity down to $η_{AC}$ = 810 pT um$^{3/2}$ Hz$^{-1/2}$. Furthermore, we show that (111) affords maximally positive dipolar interactions amongst a 2D NV ensemble, which is crucial for leveraging dipolar-driven entanglement schemes and exploring new interacting spin physics.

quant-ph↗

arXiv2024

New opportunities in condensed matter physics for nanoscale quantum sensors

Nitrogen vacancy (NV) centre quantum sensors provide unique opportunities in studying condensed matter systems: they are quantitative, noninvasive, physically robust, offer nanoscale resolution, and may be used across a wide range of temperatures. These properties have been exploited in recent years to obtain nanoscale resolution measurements of static magnetic fields arising from spin order and current flow in condensed matter systems. Compared with other nanoscale magnetic-field sensors, NV centres have the unique advantage that they can probe quantities that go beyond average magnetic fields. Leveraging techniques from magnetic resonance, NV centres can perform high precision noise sensing, and have given access to diverse systems, such as fluctuating electrical currents in simple metals and graphene, as well as magnetic dynamics in yttrium iron garnet. In this review we summarise unique opportunities in condensed matter sensing by focusing on the connections between specific NV measurements and previously established physical characteristics that are more readily understood in the condensed matter community, such as correlation functions and order parameters that are inaccessible by other techniques, and we describe the technical frontier enabled by NV centre sensing.

cond-mat.mes-hall↗

arXiv2024

Role of Oxygen in Laser Induced Contamination at Diamond-Vacuum Interfaces

Many modern-day quantum science experiments rely on high-fidelity measurement of fluorescent signals emitted by the quantum system under study. A pernicious issue encountered when such experiments are conducted near a material interface in vacuum is "laser-induced contamination" (LIC): the gradual accretion of fluorescent contaminants on the surface where a laser is focused. Fluorescence from these contaminants can entirely drown out any signal from e.g. optically-probed color centers in the solid-state. Crucially, while LIC appears often in this context, it has not been systematically studied. In this work, we probe the onset and growth rate of LIC for a diamond nitrogen-vacancy center experiment in vacuum, and we correlate the contamination-induced fluorescence intensities to micron-scale physical build-up of contaminant on the diamond surface. Drawing upon similar phenomena previously studied in the space optics community, we use photo-catalyzed oxidation of contaminants as a mitigation strategy. We vary the residual oxygen pressure over 9 orders of magnitude and find that LIC growth is inhibited at near-atmospheric oxygen partial pressures, but the growth rate at lower oxygen pressure is non-monotonic. Finally, we discuss a model for the observed dependence of LIC growth rate on oxygen content and propose methods to extend in situ mitigation of LIC to a wider range of operating pressures.

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