SearcharxivSearch

arXiv subjects

Anindya Das

Publications and source records attributed to Anindya Das.

At least 19 recordsLinked to original sources

Van Hove singularity-driven giant Nernst signal in twisted double bilayer graphene

Twisted graphene layers host van Hove singularities (vHSs), peaks in the electronic density of states, thought to drive exotic phases in moir\'e materials, but their effect on thermal transport has remained unclear. Here we show that vHSs in twisted double bilayer graphene (tDBLG) generate an unusually large Nernst signal-the transverse voltage produced by a longitudinal temperature gradient in a magnetic field. The pronounced Nernst peaks at the vHSs of the conduction and valence bands of tDBLG are tunable by an electric field with a maximum value of $\sim 40$ $\mu V K^{-1} T^{-1}$ at $\sim 1$ $K$, which is comparable to the best-known Nernst materials. Our theoretical calculations show that the large enhancement of the Nernst signal arises from the Lifshitz transitions around the vHSs. These findings establish the Nernst effect as a sensitive probe of Fermi-surface topology in moir\'e materials, and identify a universal thermoelectric signature of van Hove singularities.

cond-mat.mes-hall

Quantum oscillation spectroscopy of Fermi-surface topologies in tetralayer graphene

Quantum oscillations offer a direct probe of Fermi-surface topology and electronic degeneracy, yet disentangling both simultaneously across the Lifshitz transitions of multiband systems has remained an open experimental challenge. Here, we use Shubnikov-de Haas spectroscopy on a high-mobility, dual-gated Bernal-stacked tetralayer graphene (B-4LG) device to quantitatively reconstruct the complete sequence of six distinct Fermi-surface topologies-gully, annular, singly connected, and multiband pockets. The extracted oscillation frequencies determine the extremal momentum-space areas and their spin, valley, and gully-resolved degeneracies, in quantitative agreement with our tight-binding calculations. We further show that a perpendicular magnetic-field, combined with displacement-field lifts the valley degeneracy through an orbital-Zeeman coupling, producing a single-particle valley splitting of several $meV$, far larger than in bilayer or trilayer graphene. Our work demonstrates a framework for tracking Fermi-surface topologies and their flavor degeneracies in multiband quantum materials.

cond-mat.mes-hall

Quantized heat flow in moir\'e chern bands of bilayer graphene

When electrons are subjected simultaneously to a magnetic field and a periodic potential, they form the fractal Hofstadter spectrum, whose topological gaps host quantum Hall and Chern insulating states with distinct Chern numbers. While electrical transport has established the topology of these states, whether their heat transport is likewise universal has remained unexplored. Here, we measure the thermal conductance of quantum Hall, Chern insulator, and interaction-driven symmetry-broken Chern insulator states in a bilayer graphene-hexagonal boron nitride moir\'e superlattice with a moir\`e wavelength of $\sim$14 nm using Johnson-noise thermometry. We find that the thermal conductance ($G_Q$) is quantized in units of the thermal conductance quantum ($G_Q = t\kappa_0T$) and is determined solely by the Chern number ($t$), independent of the microscopic origin of the topological state. By directly revealing universal topological heat transport in Hofstadter bands, our work establishes thermal conductance as a stringent probe of moir\'e topological matter and provides a route to investigating more exotic phases, including fractional Chern insulators.

cond-mat.mes-hall

Moire-Engineered Excitonic Landscape and Phonon-Mediated Recombination in Twisted WSe2 Bilayers

We report light emission from the moire superlattice of a twisted bilayer of tungsten diselenide (WSe2/WSe2) encapsulated in insulating hexagonal boron nitride (hBN). The low-temperature photoluminescence (PL) spectroscopy reveals signatures of moire-potential induced strong interlayer excitonic emission and phonon-assisted recombination, while the twisting significantly suppresses the emission from localized defect-bound excitons. The moire potential redistributes carriers into indirect valleys, thereby enhancing recombination efficiency and stabilizing the interlayer excitons. Our findings establish that precise control of twist angle and dielectric environment provides a new route for engineering excitonic systems for exploring exciton-phonon interactions and associated quantum phenomena in transition metal dichalcogenides.

cond-mat.mes-hall

Half-integer thermal conductance in the absence of Majorana mode

Considering a range of candidate quantum phases of matter, half-integer thermal conductance ($κ_{\text{th}}$) is believed to be an unambiguous evidence of non-Abelian states. It has been long known that such half-integer values arise due to the presence of Majorana edge modes, representing a significant step towards topological quantum computing platforms. Here, we challenge this prevailing notion by presenting a comprehensive theoretical and experimental study where half-integer two-terminal thermal conductance plateau is realized employing Abelian phases. Our proposed setup features a confined geometry of bilayer graphene, interfacing distinct particle-like and hole-like integer quantum Hall states. Each segment of the device exhibits full charge and thermal equilibration. Our approach is amenable to generalization to other quantum Hall platforms, and may give rise to other values of fractional (electrical and thermal) quantized transport. Our study demonstrates that the observation of robust non-integer values of thermal conductance can arise as a manifestation of mundane equilibration dynamics as opposed to underlying non-trivial topology.

cond-mat.mes-hall

Anomalies in G and 2D Raman Modes of Twisted Bilayer Graphene Near the Magic Angle

The role of twist angle ($θ_t$) in tailoring the physical properties of heterostructures is emerging as a new paradigm in two-dimensional materials. The influence of flat electronic bands near the magic angle ($\sim$1.1$^{\circ}$) on the phononic properties of twisted bilayer graphene (t-BLG) is not well understood. In this work, we systematically investigate the G and 2D Raman modes of t-BLG samples with twist angles ranging from $\sim$0.3$^{\circ}$ to $\sim$3$^{\circ}$ using micro-Raman spectroscopy. A key finding of our work is the splitting of the G mode near the magic angle due to moiré potential induced phonon hybridization. The linewidth of the low-frequency component of the G mode (G$^-$), as well as the main component of the 2D mode, exhibits enhanced broadening near the magic angle due to increased electron-phonon coupling, driven by the emergence of flat electronic bands. Additionally, temperature-dependent Raman measurements (6-300 K) of magic-angle twisted bilayer graphene sample ($θ_t \sim$ 1$^{\circ}$) reveal an almost tenfold increase in phonon anharmonicity-induced temperature variation in both components of the split G mode, as compared to Bernal-stacked bilayer graphene sample, further emphasizing the role of phonon hybridization in this system. These studies could be important for understanding the thermal properties of the twisted bilayer graphene systems.

cond-mat.mes-hall

Resistance hysteresis in twisted bilayer graphene: Intrinsic versus extrinsic effects

Hysteresis in resistance under magnetic field sweeps is a key signature for identifying magnetism in twisted bilayer graphene and similar systems. However, such sweeps can induce extrinsic thermal effects, complicating interpretations. Distinguishing intrinsic magnetic ordering from extrinsic thermal influences is crucial. In this study, we report hysteresis in the longitudinal resistance ($(R_{xx}$)) of a near magic-angle twisted bilayer graphene (TBG) sample under an in-plane magnetic field ($(B_{||}$)). The hysteresis phase appears at the edge of the superconducting dome, diminishes deep within the superconducting regime, and reemerges near the superconducting critical temperature ($(T \sim T_c$)). The hysteresis magnitude and coercive fields strongly depend on the magnetic field sweep rate ($(dB/dt)$) and exhibit transient relaxation in time-series measurements. Notably, similar hysteresis behavior was observed in the temperature profile of the sample stage, measured using a calibrated temperature sensor under analogous magnetic field cycles, suggesting extrinsic thermal origins rather than intrinsic magnetic ordering. These findings underscore the importance of carefully distinguishing intrinsic and extrinsic effects in resistance hysteresis observed in mesoscopic van der Waals systems.

cond-mat.mes-hall

Thermopower probing emergent local moments in magic-angle twisted bilayer graphene

Recent experiments on magic-angle twisted bilayer graphene (MATBLG) have revealed the formation of flatbands, suggesting that correlation effects are likely to dominate in this system. Yet, a global transport measurement showing distinct signatures of strong correlations like local moments arising from the flatbands is missing. Utilizing thermopower as a sensitive global transport probe for measuring entropy, we unveil the presence of emergent local moments through their impact on entropy. Remarkably, in addition to sign changes at the Dirac point ($ν= 0$) and full band filling ($ν= \pm 4$), the thermopower of MATBLG demonstrates additional sign changes at the location, $ν_{cross} \sim \pm 1$, which do not vary with temperature from $5K$ to $\sim 60K$. This is in contrast to sensitive temperature-dependent crossing points seen in our study on twisted bilayer graphene devices with weaker correlations. Further, we have investigated the effect of magnetic field ($B$) on the thermopower, both $B_{\parallel}$ and $B_{\perp}$. Our results show a $30\%$ and $50\%$ reduction, respectively, that is consistent with suppression seen in the layered oxide due to the partial polarization of the spin entropy. The observed robust crossing points, together with suppression in a magnetic field, cannot be explained solely from the contributions of band fermions; instead, our data is consistent with the dominant contribution arising from the entropy of the emergent localized moments of a strongly correlated flatband.

cond-mat.mes-hall

Absence of heat flow in ν = 0 quantum Hall ferromagnet in bilayer graphene

The charge neutrality point of bilayer graphene, denoted as ν = 0 state, manifests competing phases marked by spontaneously broken isospin (spin/valley/layer) symmetries under external magnetic and electric fields. However, due to their electrically insulating nature, identifying these phases through electrical conductance measurements remains challenging. A recent theoretical proposal introduces a novel approach, employing thermal transport measurements to detect these competing phases. Here, we experimentally explore the bulk thermal transport of the ν = 0 state in bilayer graphene to investigate its ground states and collective excitations associated with isospin. While the theory anticipates a finite thermal conductance in the ν = 0 state, our findings unveil an absence of detectable thermal conductance. Through variations in the external electric field and temperature-dependent measurements, our results suggest towards gapped collective excitations at ν = 0 state. Our findings underscore the necessity for further investigations into the nature of ν = 0.

cond-mat.mes-hall

Electric field tunable superconductivity with competing orders in twisted bilayer graphene near magic-angle

Superconductivity (SC) in twisted bilayer graphene (tBLG) has been explored by varying carrier concentrations, twist angles, and screening strength, with the aim of uncovering its origin and possible connections to strong electronic correlations in narrow bands and various resulting broken symmetries. However, the link between the tBLG band structure and the onset of SC and other orders largely remains unclear. In this study, we address this crucial gap by examining in-situ band structure tuning of a near magic-angle ($θ\approx0.95^\circ$) tBLG device with displacement field ($D$) and reveal remarkable competition between SC and other broken symmetries. At zero $D$, the device exhibits superconducting signatures without the resistance peak at half-filling, a characteristic signature with a strong electronic correlation. As $D$ increases, the SC is suppressed, accompanied by the appearance of a resistance peak at half-filling. Hall density measurements reveal that at zero $D$, SC arises around the van Hove singularity (vHs) from an isospin or spin-valley unpolarized band. At higher $D$, the suppression of SC coincides with broken isospin symmetry near half-filling with lifted degeneracy ($g_d \sim 2$). Additionally, as the SC phase becomes weaker with $D$, vHs shifts to higher fillings, highlighting the modification of the underlying band structure with the applied electric field. These findings, with recent theoretical study on SC in tBLG, highlight the competition, rather being connected concomitantly, between SC and other orders promoted by broken symmetries.

cond-mat.mes-hall

Quantized heat flow in graphene quantum Hall phases: Probing the topological order

Topological quantum numbers are often used to characterise the topological order of phase having protected gapless edge modes when the system is kept in a space with the boundary. The famous examples in this category are the quantized electrical Hall conductance and thermal Hall conductance, which encodes the topological order of integer and fractional quantum Hall states. Here, we review the recent thermal transport study of integer and fractional quantum Hall states realized in graphene-based van der Waals heterostructures.

cond-mat.mes-hall

Electric field tunable edge transport in Bernal stacked trilayer graphene

This letter presents a non-local study on the electric field tunable edge transport in an hBN-encapsulated dual-gated Bernal stacked (ABA) trilayer graphene across various displacement fields ($D$) and temperatures ($T$). Our measurements revealed that the non-local resistance ($R_{NL}$) surpassed the expected classical ohmic contribution by a factor of at least two orders of magnitude. Through scaling analysis, we found that the non-local resistance scales linearly with the local resistance ($R_{L}$) only when the $D$ exceeds a critical value of $\sim0.2$ V/nm. Additionally, we observed that the scaling exponent remains constant at unity for temperatures below the bulk-band gap energy threshold ($T<25$ K). Further, the value of $R_{NL}$ decreases in a linear fashion as the channel length ($L$) increases. These experimental findings provide evidence for edge-mediated charge transport in ABA trilayer graphene under the influence of a finite displacement field. Furthermore, our theoretical calculations support these results by demonstrating the emergence of dispersive edge modes within the bulk-band gap energy range when a sufficient displacement field is applied.

cond-mat.mes-hall

Electrical noise spectroscopy of magnons in a quantum Hall ferromagnet

Collective spin-wave excitations-magnons-in a quantum Hall ferromagnet are promising quasi-particles for next-generation spintronics devices, including platforms for information transfer. Detection of these charge-neutral excitations relies on the conversion of magnons into electrical signals in the form of excess electrons and holes, but if these signals are equal the magnon detection remains elusive. In this work, we overcome this shortcoming by measuring the electrical noise generated by magnons. We use the symmetry-broken quantum Hall ferromagnet of the zeroth Landau level in graphene to launch magnons. Absorption of these magnons creates excess noise above the Zeeman energy and remains finite even when the average electrical signal is zero. Moreover, we formulate a theoretical model in which the noise is generated by equilibration (partial or full, depending on the bias voltage) between edge channels and propagating magnons. Our model, which agrees with experimental observations, also allows us to pinpoint the regime of ballistic magnon transport in our device.

cond-mat.mes-hall

Excitonic Metal and Non-Fermi Liquid Behaviour in Twisted Double Bilayer Graphene near Charge Neutrality

Twisted double bilayer graphene is a compensated semi-metal near the charge neutrality point with the presence of small electron and hole pockets in its band structure. We show that strong Coulomb attraction between the electrons and holes can lead to the formation of indirect excitons. Condensation of these excitons at low temperature creates an excitonic metal with charge density wave order for an appropriate range of interaction strength. This has interesting implications for low-temperature transport in the system as a function of carrier density and temperature. The reorganization of the single particle excitations and their density of states in the excitonic metal can lead to peaks in resistivity as a function of carrier density, recently seen in experiments at low temperatures. The fluctuations of the Landau damped order parameter in the quantum critical metal lead to non-Fermi liquid behaviour, which can explain the sublinear $T^{2/3}$ dependence of the resistance near the charge neutrality point.

cond-mat.str-el

Evidence of a compensated semimetal with electronic correlations at the CNP of twisted double bilayer graphene

Recently, magic-angle twisted bilayer graphene (MATBLG) has shown the emergence of various interaction-driven novel quantum phases at the commensurate fillings of the moir'e superlattice, while the charge neutrality point (CNP) remains mostly a vanilla insulator. Here, we show an emerging phase of nearly compensated semimetallicity at the CNP of twisted double bilayer graphene (TDBLG), a close cousin of MATBLG, with signatures of electronic correlation. Using electrical and thermal transport, we find almost two orders of magnitude enhancement of the thermopower in magnetic fields much smaller than the extreme quantum limit, accompanied by a large magnetoresistance($\sim 2500\%$) at CNP. This provides indisputable experimental evidence that TDBLG near CNP is a compensated semimetal. Moreover, at low temperatures, we observe an unusual sublinear temperature dependence of resistance. A recent theory predicts the formation of an excitonic metal near CNP, where small electron and hole pockets coexist. We understand the sublinear temperature dependence in terms of critical fluctuations in this theory.

cond-mat.mes-hall

Electrically switchable tunneling across a graphene pn junction: evidence for canted antiferromagnetic phase in $ν=0$ state

The ground state of a graphene sheet at charge neutrality in a perpendicular magnetic field remains enigmatic, with various experiments supporting canted antiferromagnetic, bond ordered, and even charge density wave phases. A promising avenue to elucidating the nature of this state is to sandwich it between regions of different filling factors, and study spin-dependent tunneling across the edge modes at the interfaces. Here we report on tunnel transport through a $ν=0$ region in a graphite-gated, hexagonal boron nitride ($hBN$) encapsulated monolayer graphene device, with the $ν=0$ strip sandwiched by spin-polarized $ν=\pm1$ quantum Hall states. We observe finite tunneling ($t \sim 0.3-0.6$) between the $ν=\pm1$ edges at not too small magnetic fields ($B>3T$) and low tunnel bias voltage ($<30-60μV$), which is surprising because electrons at the edge states nominally have opposite spins. Hartree-Fock calculations elucidate these phenomena as being driven by the formation of a CAF order parameter in the $ν=0$ region at zero bias (for wide enough junctions) leading to non-orthogonal spins at the edges. Remarkably, this tunneling can be controllably switched off by increasing bias; bias voltage leads to a pileup of charge at the junction, leading to a collapse of the CAF order and a suppression of the tunneling.

cond-mat.mes-hall

Determination of topological edge quantum numbers of fractional quantum Hall phases

To determine the topological quantum numbers of fractional quantum Hall (FQH) states hosting counter-propagating (CP) downstream ($N_d$) and upstream ($N_u$) edge modes, it is pivotal to study quantized transport both in the presence and absence of edge mode equilibration. While reaching the non-equilibrated regime is challenging for charge transport, we target here the thermal Hall conductance $G_{Q}$, which is purely governed by edge quantum numbers $N_d$ and $N_u$. Our experimental setup is realized with a hBN encapsulated graphite gated monolayer graphene device. For temperatures up to $35mK$, our measured $G_{Q}$ at $ν= $ 2/3 and 3/5 (with CP modes) match the quantized values of non-equilibrated regime $(N_d + N_u)κ_{0}T$, where $κ_{0}T$ is a quanta of $G_{Q}$. With increasing temperature, $G_{Q}$ decreases and eventually takes the value of equilibrated regime $|N_d - N_u|κ_{0}T$. By contrast, at $ν= $1/3 and 2/5 (without CP modes), $G_Q$ remains robustly quantized at $N_dκ_{0}T$ independent of the temperature. Thus, measuring the quantized values of $G_{Q}$ at two regimes, we determine the edge quantum numbers, which opens a new route for finding the topological order of exotic non-Abelian FQH states.

cond-mat.mes-hall

Effect of boron nitride defects and charge inhomogeneity on 1/f noise in encapsulated graphene

Low frequency 1/f noise is investigated in graphene, encapsulated between hexagonal boron nitride (hBN) substrate in dual gated geometry. The overall noise magnitude is smaller as compared to graphene on Si/SiO2 substrate. The noise amplitude in the hole doped region is independent of carrier density while in the electron doped region, a pronounced peak is observed, at Fermi energy, EF ~ 90 meV. The physical mechanism of the anomalous noise peak in the electron doped region is attributed to the impurity states originating from the Carbon atom replacing the Nitrogen site in hBN crystal. Furthermore, the noise study near Dirac point shows characteristic "M-shape", which is found to be strongly correlated with the charge inhomogeneity region near Dirac point.

cond-mat.mes-hall