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Anke Lindner

Publications and source records attributed to Anke Lindner.

At least 19 recordsLinked to original sources

Orientation Dynamics of Rigid Fibers in a Microfluidic Burgers-like Vortex

Fiber suspensions are common in biological and environmental flows and are widely used in industrial applications. Fiber transport and orientation dynamics are affected by interactions with the surrounding fluid and strongly depend on the nature of the flow. The complexity of realistic flows, which are often heterogeneous or time-dependent, hinders a full understanding of fiber dynamics. In this study, we combine microfluidic experiments, theory and numerical simulations to investigate the orientation dynamics of rigid neutrally buoyant fibers in a well-controlled model system, a streamwise stationary vortex at moderate Reynolds number. Despite the three-dimensional nature of the flow, the orientation dynamics are remarkably simple: the fiber orientation is accurately described by Jeffery equations coupled with the Burgers-vortex model. We show that fibers undergo uniform precession about the vortex axis driven by fluid vorticity while simultaneously aligning with the latter due to strain in the vortex core. These two motions are decoupled, with the alignment timescale determined by the local strain rate and the fiber aspect ratio. Finite particle size and inertia induce weak deviations from the base flow streamlines while leaving the orientational dynamics largely unaffected. These results establish a simple framework for understanding the behavior of elongated particles in stretched vortex flows, which constitute key building blocks of turbulence

physics.flu-dyn

Swimming-limited aggregation of bacteria in liquid crystals

Aggregation and fragmentation processes are widespread in engineering and the natural world. Here, we investigate a distinct colloidal aggregation mechanism in an active system of motile bacteria in highly anisotropic environments. Specifically, we examine \textit{Escherichia coli} bacteria swimming in one-dimensional confinement within nematic liquid crystals and observe long-lived chains of bacteria swimming along the nematic director. Crucially, we find that longer chains swim faster, in apparent contradiction to fundamental force-balance models that predict the swimming speed to be independent of chain length, as chains should swim at the average speed of their individual components. The seeming discrepancy is resolved by recognizing that chains do not form randomly but self-organize due to the relative velocities between bacteria. To elucidate the physical mechanism behind this active aggregation process, we combine our experimental findings with a minimal model of nearest-neighbour aggregation and agent-based simulations of active particles aggregating in one dimension. Consistent with experimental observations, our agent-based simulations reveal a positive correlation between the length and speed of dynamically self-assembled chains of active particles, with the correlation depending on the variance of the individual speed distribution and diminishing over time. Together, our experiments and theoretical models indicate a distinct regime of swimming-limited aggregation whose evolution is constrained by the intrinsic speed distribution of active agents, providing new insight into bacterial self-organization.

cond-mat.soft

Microfluidic Oscillatory Rheology of Transported Soft Particles

Microfluidic channels have emerged as useful tools to control dynamic forcing on transported microscale objects, as encountered in emulsions, biological flows, and other soft matter systems. Tailored channel designs enable precise interfacial and bulk rheological measurements of complex materials over a wide range of forcing timescales. After a brief overview of recent experiments illustrating these techniques, we discuss perspectives for future research in this direction, including the study of lubrication films in highly confined droplets, the measurement of fast relaxation dynamics of complex interfaces, and the high-throughput rheological characterization of microscopic soft matter systems ranging from single macromolecules to cells.

cond-mat.soft

Reversibility, Chaos, and Attractors in Periodically Sheared Elastic Filaments

The dynamics of filaments in flow are central to understanding a wide range of biological and soft-matter systems, yet their behavior under time-dependent forcing remains poorly understood. Here, we investigate the long-time dynamics of Brownian inextensible elastic filaments subjected to strong uniform oscillatory shear by combining microfluidic experiments on actin filaments with numerical simulations based on a fluctuating Euler-Bernoulli elastica model in a viscous fluid. As the oscillation period increases, irreversibility emerges from the interplay of flow-induced deformations and thermal noise. This leads to a departure from reversible, deterministic rigid-body dynamics: in this regime, the filaments cycle between nearly straight, flow-aligned conformations at full periods and buckled shapes at half periods. Owing to the time-glide symmetry of the system, two such attracting states in fact coexist with a phase shift of half a period. The system spontaneously selects one, but occasionally switches between them as a result of noise, producing intermittent transitions between apparent order and disorder. This system constitutes an experimentally accessible realization of stochastic symmetry breaking, attractor hopping, and intermittency in a minimal nonequilibrium soft-matter system, with novel implications for the design and control of soft matter systems under time-dependent flows.

cond-mat.soft

Bacteria collective motion is scale-free

Suspensions of swimming bacteria interact hydrodynamically over long ranges, organizing themselves into collective states that drive large-scale chaotic flows, often referred to as "bacterial turbulence". Despite extensive experimental and theoretical work, it remains unclear whether an intrinsic length scale underlies the observed patterns. To shed light on the mechanism driving active turbulence, we investigate the emergence of large-scale flows in E. coli suspensions confined within cylindrical chambers, systematically varying confinement height over more than two orders of magnitude. We first demonstrate that the critical density for the onset of collective motion scales inversely with this confinement height without saturation, even for the smallest densities observed. Near the onset, both the observed length and time scales increase sharply, with the length scale bounded only by the vertical confinement. Importantly, both scales exhibit clear power-law dependence on the confinement height, demonstrating the absence of an intrinsic length scale in bacterial collective motion. This holds up to scales nearly 10,000 times the size of a single bacterium, as evidenced by transient coherent vortices spanning the full chamber width near the onset. Our experimental results demonstrating that bacterial turbulence is scale-free provide important constraints for theories aiming to capture the dynamics of wet active matter.

cond-mat.soft

Pathways to Elastic Turbulence in Giant Micelles Through Curvature Ratios in Taylor-Couette Flow

In the past fifteen years, flow instabilities reminiscent of the Taylor-like instabilities driven by hoop stresses, have been observed in wormlike micelles based on surfactant molecules. In particular, purely elastic instabilities and turbulence have been shown to develop on top of shear banding, a type of flow specific to the semi-dilute and concentrated regimes. These instabilities have been identified as the origin of the large body of data showing complex spatio-temporal fluctuations, collected in shear-banded systems using multiple experimental techniques. Different categories of banding have been suggested depending on their stability, which involve intrinsic properties of the system and streamline curvature. It has been shown qualitatively that instabilities are promoted by an increase of the surfactant concentration or of the curvature of the flow geometry, while an increase in temperature stabilizes the flow. Here, using benchmark shear banding micellar systems, we quantify, for the first time, the effect of the streamline curvature on these flow instabilities, focusing more specifically on the transition towards purely elastic turbulence. Using various optical visualizations, we identify two transitional pathways to elastic turbulence. We construct a generic state diagram in a parameter space based on the curvature ratio and the Weissenberg number. The nature -- supercritical \textit{vs} subcritical -- of the transition to elastic turbulence is discussed. The stress evolution is in favor of a change of nature from subcritical to supercritical transition as the curvature ratio increases. However we show that finite size effects cannot be neglected and may smooth artificially the stress response. Furthermore, each domain of this diagram is characterized using velocimetry measurements. Finally a scaling for the onset of elastic turbulence is determined.

cond-mat.soft

Strain dependent viscous response describes the mechanics of cohesionless soft granular materials

Granular materials are ubiquitous in nature and are used extensively in daily life and in industry. The modeling of these materials remains challenging; therefore, finding models with acceptable predictive accuracy that at the same time also reflect the complexity of the granular dynamics is a central research theme in the field. Soft particle packings present additional modeling challenges, as it has become clear that soft particles also have particle-level relaxation timescales that affect the packing behavior. We construct a simple one-dimensional, one-timescale model that replicates much of the essence of compressed hydrogel packing mechanics. We verify the model performance against both 3D and 2D packings of hydrogel particles, under both controlled strain and stress deformation conditions. We find that the modification of a Standard Linear Solid model with a strain dependent prefactor for the relaxation captures the time-history and rate dependence, as well as the necessary absence of cohesion effectively. We also indicate some directions of future improvement of the modeling.

cond-mat.soft

Transport of spherical microparticles in a 3D vortex flow

Particles are common in biological and environmental flows and are widely used in industrial and pharmaceutical applications. Their motion and flow dynamics are strongly affected by interactions with the surrounding flow structure. While particle-flow interactions have been extensively studied in low Reynolds number (Re) flows as well as in fully developed turbulence, the transport mechanisms of these particles in intermediate flow regimes remain less explored. Here, we investigate the response of neutrally buoyant spherical particles to a single vortex flow field. Using a microfluidic cross-slot geometry, we generate a well-characterized, stationary, three-dimensional streamwise vortex at moderate $\text{Re}$ ($\sim 50$). Our experimental results, supported by numerical simulations, show that with increasing particle diameter, they are progressively excluded from the vortex core. Initially, small particles follow a Burgers vortex-like self-similar motion, but for larger particle diameters, deviations from this trend emerge due to fluid inertia and finite-size effects. These findings enhance our understanding of particle dynamics in vortical flows and have implications for microfluidic applications involving particle sorting and separation.

physics.flu-dyn

Active bacterial baths in droplets

Suspensions of self-propelled objects represent a novel paradigm in colloidal science. In such active baths traditional concepts, such as Brownian motion, fluctuation-dissipation relations, and work extraction from heat reservoirs, must be extended beyond the conventional framework of thermal baths. Unlike thermal baths, which are characterized by a single parameter, the temperature, the fundamental descriptors of an active bath remain elusive, especially in confined environments. In this study, buoyant, passive tracers are employed as generalized probes to investigate an active bath comprising motile bacteria confined within a droplet. We demonstrate that momentum transfer from the bath to the tracer can be effectively described as colored noise, characterized by temporal memory and an enhanced effective diffusivity significantly larger compared to thermal Brownian motion values. Using a stochastic analytical framework, we extract the temporal memory and diffusivity parameters that define such an active bath. Notably, the diffusivity scales linearly with bacterial concentration, modulated by a factor representing the role of confinement, expressed as the ratio of the confining radius to the probe radius. This finding, while still awaiting a complete theoretical explanation, offers new insights into the transport properties of confined active baths and paves the way for a deeper understanding of active emulsions driven by confined active matter.

cond-mat.soft

Hopper flows of dense suspensions: a 2D microfluidic model system

Flows of particles through bottlenecks are ubiquitous in nature and industry, involving both dry granular materials and suspensions. However, practical limitations of conventional experimental setups hinder the full understanding of these flows in confined geometries. Here, we present a microfluidic setup to investigate experimentally the flow of dense suspensions in a two-dimensional hopper channel. Particles with controlled properties are in-situ fabricated with a photolithographic projection method and compacted at the channel constriction using a Quake valve. The setup is characterized by examining the flow of a dense suspension of hard, monodisperse disks through constrictions of varying widths. We demonstrate that the microfluidic hopper discharges particles at constant rate, resulting from the channel resistance being dominated by the presence of densely packed particles within the tapered section of the hopper. Under imposed flow rate the discharge remains independent of particle and orifice sizes, whereas it exhibits a Beverloo-like scaling under pressure-imposed conditions. Additionally, we show that the statistics of clog formation in our microfluidic hopper follow the same stochastic laws as reported in other systems. Finally, we show how the versatility of our microfluidic model system can be used to investigate the outflow and clogging of suspensions of more complex particles.

cond-mat.soft

The 2024 Motile Active Matter Roadmap

Activity and autonomous motion are fundamental aspects of many living and engineering systems. Here, the scale of biological agents covers a wide range, from nanomotors, cytoskeleton, and cells, to insects, fish, birds, and people. Inspired by biological active systems, various types of autonomous synthetic nano- and micromachines have been designed, which provide the basis for multifunctional, highly responsive, intelligent active materials. A major challenge for understanding and designing active matter is their inherent non-equilibrium nature due to persistent energy consumption, which invalidates equilibrium concepts such as free energy, detailed balance, and time-reversal symmetry. Furthermore, interactions in ensembles of active agents are often non-additive and non-reciprocal. An important aspect of biological agents is their ability to sense the environment, process this information, and adjust their motion accordingly. It is an important goal for the engineering of micro-robotic systems to achieve similar functionality. With many fundamental properties of motile active matter now reasonably well understood and under control, the ground is prepared for the study of physical aspects and mechanisms of motion in complex environments, of the behavior of systems with new physical features like chirality, of the development of novel micromachines and microbots, of the emergent collective behavior and swarming of intelligent self-propelled particles, and of particular features of microbial systems. The vast complexity of phenomena and mechanisms involved in the self-organization and dynamics of motile active matter poses major challenges, which can only be addressed by a truly interdisciplinary effort involving scientists from biology, chemistry, ecology, engineering, mathematics, and physics.

cond-mat.soft

Color-switching hydrogels as integrated microfluidic pressure sensors

Precisely measuring pressure in microfluidic flows is essential for flow control, fluid characterization, and monitoring, but faces specific challenges such as \RE{achieving} sufficient resolution, non-invasiveness, or ease of use. Here, we demonstrate a fully integrated multiplexed optofluidic pressure sensor, entirely decoupled from the flow path, that enables local pressure measurements along any microfluidic channel without altering its flow geometry. The sensor itself relies on the compression of a soft mechano-actuated hydrogel, changing color in response to a pressure change. The hydrogel is separated from the fluid circulating in the channel by a thin membrane, allowing for the unrestricted use of different types of fluids. Imaging the gel through the transparent PDMS with a color camera provides a direct, easy, and contact-free determination of the fluid pressure at the sensing location for pressures as small as \SI{20}{\milli\bar} with a resolution of around \SI{10}{\milli\bar}. The sensitivity and accessible pressure range can be tuned via the mechanical properties \RE{of the sensing unit}. The photonic gel can also be used to acquire 2D pressure or deformation maps, taking advantage of the fast response time and fine spatial resolution.

physics.flu-dyn

Dynamics of rigid fibers interacting with triangular obstacles in microchannel flows

Fiber suspensions flowing in structured media are encountered in many biological and industrial systems. Interactions between fibers and the transporting flow as well as fiber contact with obstacles can lead to complex dynamics. In this work, we combine microfluidic experiments and numerical simulations to study the interactions of a rigid fiber with an individual equilateral triangular pillar in a microfluidic channel. Four dominant fiber dynamics are identified: transport above or below the obstacle, pole vaulting and trapping, in excellent agreement between experiments and modeling. The dynamics are classified as a function of the length, angle and lateral position of the fibers at the channel entry. We show that the orientation and lateral position close to the obstacle are responsible for the fiber dynamics and we link those to the initial conditions of the fibers at the channel entrance. Direct contact between the fibers and the pillar is required to obtain strong modification of the fiber trajectories, which is associated to irreversible dynamics. Longer fibers are found to be more laterally shifted by the pillar than shorter fibers that rather tend to remain on their initial streamline. Our findings could in the future be used to design and optimize microfluidic sorting devices to sort rigid fibers by length.

physics.flu-dyn

Asymmetric bistability of chiral particle orientation in viscous shear flows

The migration of helical particles in viscous shear flows plays a crucial role in chiral particle sorting. Attaching a non-chiral head to a helical particle leads to a rheotactic torque inducing particle reorientation. This phenomenon is responsible for bacterial rheotaxis observed for flagellated bacteria as Escherichia coli in shear flows. Here we use a high-resolution microprinting technique to fabricate micro-particles with controlled and tunable chiral shape consisting of a spherical head and helical tails of various pitch and handedness. By observing the fully time-resolved dynamics of these micro-particles in microfluidic channel flow, we gain valuable insights into chirality-induced orientation dynamics. Our experimental model system allows us to examine the effects of particle elongation, chirality, and head-heaviness for different flow rates on the orientation dynamics, while minimizing the influence of Brownian noise. Through our model experiments we demonstrate the existence of asymmetric bistability of the particle orientation perpendicular to the flow direction. We quantitatively explain the particle equilibrium orientations as a function of particle properties, initial conditions and flow rates, as well as the time-dependence of the reorientation dynamics through a theoretical model. The model parameters are determined using boundary element simulations and excellent agreement with experiments is obtained without any adjustable parameters. Our findings lead to a better understanding of chiral particle transport, bacterial rheotaxis and might allow the development of targeted delivery applications.

cond-mat.soft

Pitch Controls the Flexibility of Helical Ribbons

Helical objects are often implemented in electronic or mechanical micro-systems, requiring a precise understanding of their mechanical properties. While helices formed by cylindrical filaments have been intensely investigated, little is known about the role of the cross-section of the filament at the basis of the helical shape. We study experimentally the force-extension response of micro-helices fabricated from ultra-thin PMMA ribbons. Leveraging newly achieved control on the helix geometry, the influence of the helical pitch is quantified and a significant stiffening of the helical ribbons with increasing pitch is highlighted. Two phenomena are identified: a mechanical transition from a regime dominated by twisting of the ribbon at small pitch to a bending-dominated regime at high pitch and a purely geometrical effect, specific to helical ribbons. Excellent agreement is found with a previously established analytical model of inextensible elastic strips.

physics.app-ph

Frustrated run and tumble of swimming E-coli bacteria in nematic liquid crystals

In many situations bacteria move in complex environments, as for example in soils, oceans or the human gut-track microbiome. In these natural environments, carrier fluids such as mucus or reproductive fluids show complex structure associated with non-Newtonian rheology. Many fundamental questions concerning the the ability to navigate in such environments remain unsolved due to the inherent complexity of the natural surroundings. Recently, the interaction of swimming bacteria with nematic liquid crystals has attracted lot of attention. In these structured fluids, the kinetics of bacterial motion is constrained by the orientational molecular order of the liquid crystal (or director field) and novel spatio-temporal patterns arise from this orientational constraint, as well as from the interactions with topological defects. A question unaddressed so far is how bacteria are able to change swimming direction in such an environment. In this work, we study the swimming mechanism of a single bacterium, E. coli, constrained to move along the director field of a lyotropic chromonic liquid crystal (LCLC) that is confined to a planar cell. In such an environment, the spontaneous run and tumble motion of the bacterium gets frustrated: the elasticity of the liquid crystal prevents flagella from unbundling. Interestingly, in order to change direction, bacteria execute a reversal motion along the director field, driven by the relocation of a single flagellum to the other side of the bacterial body, coined as a frustrated tumble. We present a detailed experimental characterization of this phenomenon, exploiting exceptional spatial and temporal resolution of bacteria and flagella dynamics during swimming, obtained using a two color Lagrangian tracking technique. We suggest a possible mechanism behind the frustrated run and tumble motion, accounting for these observations.

cond-mat.soft

Dynamics of flexible filaments in oscillatory shear flows

The fluid-structure interactions between flexible fibers and viscous flows play an essential role in various biological phenomena, medical problems, and industrial processes. Of particular interest is the case of particles freely transported in time-dependent flows. This work elucidates the dynamics and morphologies of actin filaments under oscillatory shear flows by combining microfluidic experiments, numerical simulations, and theoretical modeling. Our work reveals that, in contrast to steady shear flows, in which small orientational fluctuations from a flow-aligned state initiate tumbling and deformations, the periodic flow reversal allows the filament to explore many different configurations at the beginning of each cycle. Investigation of filament motion during half time periods of oscillation highlights the critical role of the initial filament orientation on the emergent dynamics. This strong coupling between orientation and deformation results in new deformation regimes and novel higher-order buckling modes absent in steady shear flows. The primary outcome of our analysis is the possibility of suppression of buckling instabilities for certain combinations of the oscillation frequency and initial filament orientation, even in very strong flows. We explain this unusual behavior through a weakly nonlinear Landau theory of buckling, in which we treat the filaments as inextensible Brownian Euler-Bernoulli rods whose hydrodynamics are described by local slender-body theory.

physics.flu-dyn

Shaping Nanoscale Ribbons into Micro-Helices of Controllable Radius and Pitch

We report fabrication of highly flexible micron-sized helices from nanometer-thick ribbons. Building upon the helical coiling of such ultra-thin ribbons mediated by surface tension, we demonstrate that the enhanced creep properties of highly confined materials can be leveraged to shape helices into the desired geometry with full control of the final shape. The helical radius, total length and pitch angle are all freely and independently tunable within a wide range: radius within $\sim$ 1-100 micrometer, length within $\sim$ 100-3000 micrometer, and pitch angle within $\sim$ 0-70{\deg}. This fabrication method is validated for three different materials: poly(methyl methacrylate), poly(dimethylaminoethyl methacrylate), and transition metal chalcogenide quantum dots, each corresponding to a different solid-phase structure: respectively a polymer glass, a crosslinked hydrogel, and a nanoparticle array. This demonstrates excellent versatility with respect to material selection, enabling further control of the helix mechanical properties.

cond-mat.soft