arXiv subjects

Antonio Ambrosio

Publications and source records attributed to Antonio Ambrosio.

24 records · Page 2Linked to original sources

arXiv2017

Guided Modes of Anisotropic van der Waals Materials Investigated by Near-Field Scanning Optical Microscopy

Guided modes in anisotropic two-dimensional van der Waals materials are experimentally investigated and their refractive indices in visible wavelengths are extracted. Our method involves near-field scanning optical microscopy of waveguide (transverse electric) and surface plasmon polariton (transverse magnetic) modes in h-BN/SiO2/Si and Ag/h-BN stacks, respectively. We determine the dispersion of these modes and use this relationship to extract anisotropic refractive indices of h-BN flakes. In the wavelength interval 550-700 nm, the in-plane and out-of-plane refractive indices are in the range 1.98-2.12 and 1.45-2.12, respectively. Our approach of using near-field scanning optical microscopy allows for direct study of interaction between light and two-dimensional van der Waals materials and heterostructures.

physics.optics↗

arXiv2017

Mechanical detection and imaging of hyperbolic phonon polaritons in hexagonal Boron Nitride

Mid-infrared nano-imaging and spectroscopy of two-dimensional (2D) materials have been limited so far to scattering-type Scanning Near-field Optical Microscopy (s-NSOM) experiments where light from the sample is scattered by a metallic-coated Atomic Force Microscope (AFM) tip interacting with the material at the nanoscale. These experiments have recently allowed imaging of plasmon polaritons in graphene as well as hyperbolic phonon polaritons (HP2) in hexagonal Boron Nitride (hBN). Here we show that the high mechanical sensitivity of an AFM cantilever can be exploited for imaging hyperbolic phonon polaritons in hBN. In our imaging process, the lattice vibrations of hBN micrometer-sized flakes are locally enhanced by the launched phonon polaritons. These enhanced vibrations are coupled to the AFM tip in contact to the sample surface and recorded during scanning. Imaging resolution better than λ/20 is showed, comparable to the best resolution in s-NSOM. Importantly, this detection mechanism is free from light background and it is in fact the first photon-less detection of phonon polaritons.

cond-mat.mtrl-sci↗

arXiv2016

Spin-to-orbital angular momentum conversion in dielectric metasurfaces

Spin-to-orbital-angular-momentum conversion has attracted considerable interest as a tool to create exotic light beams, leading to the emergence of novel devices that implement this function. These converters exploit the geometrical phase to create helical beams of handedness determined by the chirality of the incident light. This property is finding important applications in quantum optics thanks to the demonstration of liquid crystal spin-to-orbital angular momentum converters (SOC) known as q-plates. Here we demonstrate high-efficiency SOCs in the visible based on dielectric metasurfaces that generate vortex beams with high and even fractional topological charge and show for the first time the simultaneous generation of collinear helical beams with different and arbitrary orbital angular momentum. We foresee that this versatile method of creating vortex beams, which circumvents the limitations of q-plates, will significant impact microscopy and vector beam shaping.

physics.optics↗

arXiv2016

Dispersion-compensated meta-holograms based on detour phase

Subwavelength structured surfaces, known as metasurfaces, hold promise for future compact and optically thin devices with versatile functionalities. Here, by revisiting the concept of detour phase at the basis of the first computer generated holograms we have designed high-performance transmissive dielectric meta-holograms with new functionalities. In one class of such devices wavelength- independent phase masks have been generated by compensating the inherent dispersion of the detour phase with that of the subwavelength structures. This leads to broadband operation from the visible to the near infrared with efficiency as high as 75% in the 1000 to 1400 nm range. We have also shown that we can fully control the effective focal length of the imaging optical system by incorporating a lens-like function in the meta-hologram. In a second class of devices we have incorporated in the phase map a geometric phase to achieve for the first time chiral imaging: the projection of different images depends on the handedness of the reference beam. The compactness, lightweight and ability to produce images even at large angles of our devices have significant potential for important emerging applications such as wearable optics.

physics.optics↗

arXiv2014

Holographic patterning of graphene-oxide films by light-driven reduction

We report on the patterning and reduction of graphene-oxide films by holographic lithography. Light reduction can be used to engineer low-cost graphene-based devices by performing a local conversion of insulating oxide into the conductive graphene. In this work, computer generated holograms have been exploited to realize complex graphene patterns in a single shot, differently from serial laser writing or mask-based photolithographic processes. The technique has been further improved by achieving speckle noise reduction: submicron and diffraction-limited features have been obtained. In addition we have also demonstrated that the gray-scale lithography capability can be used to obtain different reduction levels in a single exposure.

cond-mat.mtrl-sci↗

arXiv2012

Light-induced spiral mass transport in azo-polymer films under vortex-beam illumination

When an azobenzene-containing polymer film is exposed to a non-uniform illumination, a light-induced mass migration process may be induced, leading to the formation of relief patterns on the polymer free surface. Despite a research effort of many years and several proposed models many aspects of this phenomenon remain not well understood. Here we report the appearance of spiral-shaped relief patterns on the polymer under the illumination of focused Laguerre-Gauss beams, having helical wavefront and an optical vortex at their axis. The induced spiral reliefs are sensitive to the vortex topological charge and to the wavefront handedness. These findings are unexpected, because the "doughnut"-shaped intensity profile of Laguerre- Gauss beams contains no information about the wavefront handedness. We propose a model that explains the main features of this phenomenon from the surface-mediated interference of the longitudinal and the transverse components of the optical field. These results may find applications in optical micro- and nanolithography and optical-field.

physics.optics↗