SearcharxivSearch

arXiv subjects

Arabella Quane

Publications and source records attributed to Arabella Quane.

3 recordsLinked to original sources

Inductance Meets Memory in the Quantum Magnet Mn3Si2Te6

Orbital degrees of freedom offer a largely untapped route to emergent dynamical phenomena in correlated quantum materials. However, it remains unclear whether collective orbital states can intrinsically generate both reactive and memory functionalities in a bulk system. Here we show that in the ferrimagnet Mn3Si2Te6, nonequilibrium reconfiguration of chiral orbital currents produces both emergent inductance and nonvolatile memristance as intrinsic properties of a single crystal. At low frequency and under a magnetic field along the c axis, coherent orbital-current domains generate robust clockwise inductive I-V loops. At higher frequency and low field, current-driven first-order reconfiguration leads to incomplete reversal and metastable trapping, producing an intrinsic electromotive force and a finite remanent voltage at zero current. These results establish orbital currents as a class of quantum state variables that encode both reactive and memory functionalities, opening routes toward intrinsically reconfigurable and energy-efficient electronic systems.

cond-mat.str-el

Hidden Density-Wave Instability in the Trimer Ruthenate Ba$_4$Ru$_3$O$_{10}$

We report a hidden density-wave instability in the trimer-based ruthenate Ba4Ru3O10, previously regarded as a pure antiferromagnet with a phase transition at TA=100 K. This transition is manifested in lattice parameters, transport, thermodynamics, and magnetic susceptibility, yet remains remarkably insensitive to magnetic fields up to at least 14 T, indicating an electronically driven reconstruction. At much lower temperatures T*= 20 K, charge transport becomes strongly nonlinear, exhibiting distinct depinning thresholds, negative differential resistance, pronounced current- and frequency-dependence, and slow collective dynamics in the Hertz range. While each feature is characteristic of density-wave transport, their simultaneous occurrence in an antiferromagnetic oxide is unprecedented. All nonlinear signatures vanish upon only 3% Ir substitution, which preserves the crystal structure and insulating state, ruling out Joule heating or extrinsic artifacts. The wide separation between the electronic reconstruction at TA and the emergence of nonlinear dynamics at T* identifies Ba4Ru3O10 as a rare correlated system hosting a strongly pinned collective electronic state intertwined with antiferromagnetism.

cond-mat.str-el

Field-Tailoring Quantum Materials via Magneto-Synthesis: Metastable Metallic and Magnetically Suppressed Phases in a Trimer Iridate

We demonstrate that applying modest magnetic fields during high-temperature crystal growth can profoundly alter the structure and ground state of a spin-orbit-coupled, antiferromagnetic trimer lattice. Using BaIrO3 as a model system, whose ground state is intricately dictated by the trimer lattice, we show that magneto-synthesis, a field-assisted synthesis approach, stabilizes a structurally compressed, metastable metallic and magnetically suppressed phases inaccessible via conventional methods. These effects include a 0.85% reduction in unit cell, 4-order-of-magnitude decrease in resistivity, a 10-fold enhancement of the Sommerfeld coefficient, and the collapse of long-range magnetic order -- all intrinsic and bulk in origin. First-principles calculations confirm that the field-stabilized structure lies substantially above the ground state in energy, highlighting its metastable character. These large, coherent and correlated changes across multiple bulk properties, unlike those caused by dilute impurities, defects or off-stoichiometry, point to an intrinsic field-induced mechanism. The findings establish magneto-synthesis as a powerful new pathway for accessing non-equilibrium quantum phases in strongly correlated materials.

cond-mat.str-el