arXiv subjects

Arne Laucht

Publications and source records attributed to Arne Laucht.

At least 55 records · Page 3Linked to original sources

arXiv2022

Quantum-Coherent Nanoscience

For the past three decades, nanoscience has widely affected many areas in physics, chemistry, and engineering, and has led to numerous fundamental discoveries as well as applications and products. Concurrently, quantum science and technology has developed into a cross-disciplinary research endeavour connecting these same areas and holds a burgeoning commercial promise. Although quantum physics dictates the behaviour of nanoscale objects, quantum coherence, which is central to quantum information, communication and sensing has not played an explicit role in much of nanoscience. This Review describes fundamental principles and practical applications of quantum coherence in nanoscale systems, a research area we call quantum-coherent nanoscience. We structure this manuscript according to specific degrees of freedom that can be quantum-coherently controlled in a given nanoscale system such as charge, spin, mechanical motion, and photons. We review the current state of the art and focus on outstanding challenges and opportunities unlocked by the merging of nanoscience and coherent quantum operations.

cond-mat.mes-hall↗

arXiv2022

Integrated Room Temperature Single Photon Source for Quantum Key Distribution

High-purity single photon sources (SPS) that can operate at room temperature are highly desirable for a myriad of applications, including quantum photonics and quantum key distribution. In this work, we realise an ultra-bright solid-state SPS based on an atomic defect in hexagonal boron nitride (hBN) integrated with a solid immersion lens (SIL). The SIL increases the source efficiency by a factor of six, and the integrated system is capable of producing over ten million single photons per second at room temperature. Our results are promising for practical applications of SPS in quantum communication protocols.

quant-ph↗

arXiv2022

Precision tomography of a three-qubit donor quantum processor in silicon

Nuclear spins were among the first physical platforms to be considered for quantum information processing, because of their exceptional quantum coherence and atomic-scale footprint. However, their full potential for quantum computing has not yet been realized, due to the lack of methods to link nuclear qubits within a scalable device combined with multi-qubit operations with sufficient fidelity to sustain fault-tolerant quantum computation. Here we demonstrate universal quantum logic operations using a pair of ion-implanted 31P donor nuclei in a silicon nanoelectronic device. A nuclear two-qubit controlled-Z gate is obtained by imparting a geometric phase to a shared electron spin, and used to prepare entangled Bell states with fidelities up to 94.2(2.7)%. The quantum operations are precisely characterised using gate set tomography (GST), yielding one-qubit average gate fidelities up to 99.95(2)%, two-qubit average gate fidelity of 99.37(11)% and two-qubit preparation/measurement fidelities of 98.95(4)%. These three metrics indicate that nuclear spins in silicon are approaching the performance demanded in fault-tolerant quantum processors. We then demonstrate entanglement between the two nuclei and the shared electron by producing a Greenberger-Horne-Zeilinger three-qubit state with 92.5(1.0)% fidelity. Since electron spin qubits in semiconductors can be further coupled to other electrons or physically shuttled across different locations, these results establish a viable route for scalable quantum information processing using donor nuclear and electron spins.

quant-ph↗

arXiv2021

Implementation of the SMART protocol for global qubit control in silicon

Quantum computing based on spins in the solid state allows for densely-packed arrays of quantum bits. While high-fidelity operation of single qubits has been demonstrated with individual control pulses, the operation of large-scale quantum processors requires a shift in paradigm towards global control solutions. Here we report the experimental implementation of a new type of qubit protocol - the SMART (Sinusoidally Modulated, Always Rotating and Tailored) protocol. As with a dressed qubit, we resonantly drive a two-level system with a continuous microwave field, but here we add a tailored modulation to the dressing field to achieve increased robustness to detuning noise and microwave amplitude fluctuations. We implement this new protocol to control a single spin confined in a silicon quantum dot and confirm the optimal modulation conditions predicted from theory. Universal control of a single qubit is demonstrated using modulated Stark shift control via the local gate electrodes. We measure an extended coherence time of $2$ ms and an average Clifford gate fidelity $>99$ $\%$ despite the relatively long qubit gate times ($>15$ $\unicode[serif]{x03BC}$s, $20$ times longer than a conventional square pulse gate), constituting a significant improvement over a conventional spin qubit and a dressed qubit. This work shows that future scalable spin qubit arrays could be operated using global microwave control and local gate addressability, while maintaining robustness to relevant experimental inhomogeneities.

cond-mat.mes-hall↗

arXiv2021

Fast coherent control of an NV- spin ensemble using a KTaO3 dielectric resonator at cryogenic temperatures

Microwave delivery to samples in a cryogenic environment can pose experimental challenges such as restricting optical access, space constraints and heat generation. Moreover, existing solutions that overcome various experimental restrictions do not necessarily provide a large, homogeneous oscillating magnetic field over macroscopic lengthscales, which is required for control of spin ensembles or fast gate operations in scaled-up quantum computing implementations. Here we show fast and coherent control of a negatively charged nitrogen vacancy spin ensemble by taking advantage of the high permittivity of a KTaO3 dielectric resonator at cryogenic temperatures. We achieve Rabi frequencies of up to 48 MHz, with the total field-to-power conversion ratio $C_{\rm P} = $ 9.66 mT/$\sqrt{\rm W}$ ($\approx191$ MHz/$\sqrt{\rm W}$). We use the nitrogen vacancy center spin ensemble to probe the quality factor, the coherent enhancement, and the spatial distribution of the magnetic field inside the diamond sample. The key advantages of the dielectric resonator utilised in this work are: ease of assembly, in-situ tuneability, a high magnetic field conversion efficiency, a low volume footprint, and optical transparency. This makes KTaO3 dielectric resonators a promising platform for the delivery of microwave fields for the control of spins in various materials at cryogenic temperatures.

quant-ph↗

arXiv2021

The SMART protocol -- Pulse engineering of a global field for robust and universal quantum computation

Global control strategies for arrays of qubits are a promising pathway to scalable quantum computing. A continuous-wave global field provides decoupling of the qubits from background noise. However, this approach is limited by variability in the parameters of individual qubits in the array. Here we show that by modulating a global field simultaneously applied to the entire array, we are able to encode qubits that are less sensitive to the statistical scatter in qubit resonance frequency and microwave amplitude fluctuations, which are problems expected in a large scale system. We name this approach the SMART (Sinusoidally Modulated, Always Rotating and Tailored) qubit protocol. We show that there exist optimal modulation conditions for qubits in a global field that robustly provide improved coherence times. We discuss in further detail the example of spins in silicon quantum dots, in which universal one- and two-qubit control is achieved electrically by controlling the spin-orbit coupling of individual qubits and the exchange coupling between spins in neighbouring dots. This work provides a high-fidelity qubit operation scheme in a global field, significantly improving the prospects for scalability of spin-based quantum computer architectures.

quant-ph↗

arXiv2021

A near-ideal degenerate parametric amplifier

Degenerate parametric amplifiers (DPAs) exhibit the unique property of phase-sensitive gain and can be used to noiselessly amplify small signals or squeeze field fluctuations beneath the vacuum level. In the microwave domain, these amplifiers have been utilized to measure qubits in elementary quantum processors, search for dark matter, facilitate high-sensitivity spin resonance spectroscopy and have even been proposed as the building blocks for a measurement based quantum computer. Until now, microwave DPAs have almost exclusively been made from nonlinear Josephson junctions, which exhibit high-order nonlinearities that limit their dynamic range and squeezing potential. In this work we investigate a new microwave DPA that exploits a nonlinearity engineered from kinetic inductance. The device has a simple design and displays a dynamic range that is four orders of magnitude greater than state-of-the-art Josephson DPAs. We measure phase sensitive gains up to 50 dB and demonstrate a near-quantum-limited noise performance. Additionally, we show that the higher-order nonlinearities that limit other microwave DPAs are almost non-existent for this amplifier, which allows us to demonstrate its exceptional squeezing potential by measuring the deamplification of coherent states by as much as 26 dB.

quant-ph↗

arXiv2021

Quantum Computation Protocol for Dressed Spins in a Global Field

Spin qubits are contenders for scalable quantum computation because of their long coherence times demonstrated in a variety of materials, but individual control by frequency-selective addressing using pulsed spin resonance creates severe technical challenges for scaling up to many qubits. This individual resonance control strategy requires each spin to have a distinguishable frequency, imposing a maximum number of spins that can be individually driven before qubit crosstalk becomes unavoidable. Here we describe a complete strategy for controlling a large array of spins in quantum dots dressed by an on-resonance global field, namely a field that is constantly driving the spin qubits, to dynamically decouple from the effects of background magnetic field fluctuations. This approach -- previously implemented for the control of single electron spins bound to electrons in impurities -- is here harmonized with all other operations necessary for universal quantum computing with spins in quantum dots. We define the logical states as the dressed qubit states and discuss initialization and readout utilizing Pauli spin blockade, as well as single- and two-qubit control in the new basis. Finally, we critically analyze the limitations imposed by qubit variability and potential strategies to improve performance.

quant-ph↗

arXiv2021

Materials for Silicon Quantum Dots and their Impact on Electron Spin Qubits

Quantum computers have the potential to efficiently solve problems in logistics, drug and material design, finance, and cybersecurity. However, millions of qubits will be necessary for correcting inevitable errors in quantum operations. In this scenario, electron spins in gate-defined silicon quantum dots are strong contenders for encoding qubits, leveraging the microelectronics industry know-how for fabricating densely populated chips with nanoscale electrodes. The sophisticated material combinations used in commercially manufactured transistors, however, will have a very different impact on the fragile qubits. We review here some key properties of the materials that have a direct impact on qubit performance and variability.

cond-mat.mes-hall↗

arXiv2021

A high-sensitivity charge sensor for silicon qubits above one kelvin

Recent studies of silicon spin qubits at temperatures above 1 K are encouraging demonstrations that the cooling requirements for solid-state quantum computing can be considerably relaxed. However, qubit readout mechanisms that rely on charge sensing with a single-island single-electron transistor (SISET) quickly lose sensitivity due to thermal broadening of the electron distribution in the reservoirs. Here we exploit the tunneling between two quantised states in a double-island SET (DISET) to demonstrate a charge sensor with an improvement in signal-to-noise by an order of magnitude compared to a standard SISET, and a single-shot charge readout fidelity above 99 % up to 8 K at a bandwidth > 100 kHz. These improvements are consistent with our theoretical modelling of the temperature-dependent current transport for both types of SETs. With minor additional hardware overheads, these sensors can be integrated into existing qubit architectures for high fidelity charge readout at few-kelvin temperatures.

cond-mat.mes-hall↗

arXiv2021

Pauli Blockade in Silicon Quantum Dots with Spin-Orbit Control

Quantum computation relies on accurate measurements of qubits not only for reading the output of the calculation, but also to perform error correction. Most proposed scalable silicon architectures utilize Pauli blockade of triplet states for spin-to-charge conversion. In recent experiments, there have been instances when instead of conventional triplet blockade readout, Pauli blockade is sustained only between parallel spin configurations, with $|T_0\rangle$ relaxing quickly to the singlet state and leaving $|T_+\rangle$ and $|T_-\rangle$ states blockaded -- which we call \textit{parity readout}. Both types of blockade can be used for readout in quantum computing, but it is crucial to maximize the fidelity and understand in which regime the system operates. We devise and perform an experiment in which the crossover between parity and singlet-triplet readout can be identified by investigating the underlying physics of the $|T_0\rangle$ relaxation rate. This rate is tunable over four orders of magnitude by controlling the Zeeman energy difference between the dots induced by spin-orbit coupling, which in turn depends on the direction of the applied magnetic field. We suggest a theoretical model incorporating charge noise and relaxation effects that explains quantitatively our results. Investigating the model both analytically and numerically, we identify strategies to obtain on-demand either singlet-triplet or parity readout consistently across large arrays of dots. We also discuss how parity readout can be used to perform full two-qubit state tomography and its impact on quantum error detection schemes in large-scale silicon quantum computers.

quant-ph↗

arXiv2020

Roadmap for gallium arsenide spin qubits

Gate-defined quantum dots in gallium arsenide (GaAs) have been used extensively for pioneering spin qubit devices due to the relative simplicity of fabrication and favourable electronic properties such as a single conduction band valley, a small effective mass, and stable dopants. GaAs spin qubits are readily produced in many labs and are currently studied for various applications, including entanglement, quantum non-demolition measurements, automatic tuning, multi-dot arrays, coherent exchange coupling, and teleportation. Even while much attention is shifting to other materials, GaAs devices will likely remain a workhorse for proof-of-concept quantum information processing and solid-state experiments.

cond-mat.mes-hall↗

arXiv2020

Spin thermometry and spin relaxation of optically detected Cr3+ ions in ruby Al2O3

Paramagnetic ions in solid state crystals form the basis for many advanced technologies such as lasers, masers, frequency standards, and quantum-enhanced sensors. One of the most-studied examples is the Cr3+ ion in sapphire (Al2O3), also known as ruby, which has been intensely studied in the 1950s and 1960s. However, despite decades of research on ruby, some of its fundamental optical and spin properties have not yet been characterized at ultra low-temperatures. In this paper, we present optical measurements on a ruby crystal in a dilution refrigerator at ultra-low temperatures down to 20 mK. Analyzing the relative populations of its 4A2 ground state spin levels, we extract a lattice temperature of 143(7) mK under continuous laser excitation. We perform spin lattice relaxation T1 measurements in excellent agreement with the direct, one-phonon model. Furthermore, we perform optically detected magnetic resonance measurements showing magnetically driven transitions between the ground state spin levels for various magnetic fields. Our measurements characterize some of ruby's low temperature spin properties, and lay the foundations for more advanced spin control experiments.

cond-mat.mes-hall↗

arXiv2020

Bell-state tomography in a silicon many-electron artificial molecule

An error-corrected quantum processor will require millions of qubits, accentuating the advantage of nanoscale devices with small footprints, such as silicon quantum dots. However, as for every device with nanoscale dimensions, disorder at the atomic level is detrimental to qubit uniformity. Here we investigate two spin qubits confined in a silicon double-quantum-dot artificial molecule. Each quantum dot has a robust shell structure and, when operated at an occupancy of 5 or 13 electrons, has single spin-$\frac{1}{2}$ valence electron in its $p$- or $d$-orbital, respectively. These higher electron occupancies screen atomic-level disorder. The larger multielectron wavefunctions also enable significant overlap between neighbouring qubit electrons, while making space for an interstitial exchange-gate electrode. We implement a universal gate set using the magnetic field gradient of a micromagnet for electrically-driven single qubit gates, and a gate-voltage-controlled inter-dot barrier to perform two-qubit gates by pulsed exchange coupling. We use this gate set to demonstrate a Bell state preparation between multielectron qubits with fidelity 90.3%, confirmed by two-qubit state tomography using spin parity measurements.

cond-mat.mes-hall↗

arXiv2020

Coherent control of NV- centers in diamond in a quantum teaching lab

The room temperature compatibility of the negatively-charged nitrogen-vacancy (NV-) in diamond makes it the ideal quantum system for a university teaching lab. Here, we describe a low-cost experimental setup for coherent control experiments on the electronic spin state of the NV- center. We implement spin-relaxation measurements, optically-detected magnetic resonance, Rabi oscillations, and dynamical decoupling sequences on an ensemble of NV- centers. The relatively short times required to perform each of these experiments (<10 minutes) demonstrate the feasibility of the setup in a teaching lab. Learning outcomes include basic understanding of quantum spin systems, magnetic resonance, the rotating frame, Bloch spheres, and pulse sequence development.

physics.ed-ph↗

arXiv2020

Conditional quantum operation of two exchange-coupled single-donor spin qubits in a MOS-compatible silicon device

Silicon nanoelectronic devices can host single-qubit quantum logic operations with fidelity better than 99.9%. For the spins of an electron bound to a single donor atom, introduced in the silicon by ion implantation, the quantum information can be stored for nearly 1 second. However, manufacturing a scalable quantum processor with this method is considered challenging, because of the exponential sensitivity of the exchange interaction that mediates the coupling between the qubits. Here we demonstrate the conditional, coherent control of an electron spin qubit in an exchange-coupled pair of $^{31}$P donors implanted in silicon. The coupling strength, $J = 32.06 \pm 0.06$ MHz, is measured spectroscopically with unprecedented precision. Since the coupling is weaker than the electron-nuclear hyperfine coupling $A \approx 90$ MHz which detunes the two electrons, a native two-qubit Controlled-Rotation gate can be obtained via a simple electron spin resonance pulse. This scheme is insensitive to the precise value of $J$, which makes it suitable for the scale-up of donor-based quantum computers in silicon that exploit the Metal-Oxide-Semiconductor fabrication protocols commonly used in the classical electronics industry.

cond-mat.mes-hall↗

arXiv2020

Single-electron operation of a silicon-CMOS 2x2 quantum dot array with integrated charge sensing

The advanced nanoscale integration available in silicon complementary metal-oxide-semiconductor (CMOS) technology provides a key motivation for its use in spin-based quantum computing applications. Initial demonstrations of quantum dot formation and spin blockade in CMOS foundry-compatible devices are encouraging, but results are yet to match the control of individual electrons demonstrated in university-fabricated multi-gate designs. We show here that the charge state of quantum dots formed in a CMOS nanowire device can be sensed by using floating gates to electrostatically couple it to a remote single electron transistor (SET) formed in an adjacent nanowire. By biasing the nanowire and gates of the remote SET with respect to the nanowire hosting the quantum dots, we controllably form ancillary quantum dots under the floating gates, thus enabling the demonstration of independent control over charge transitions in a quadruple (2x2) quantum dot array. This device overcomes the limitations associated with measurements based on tunnelling transport through the dots and permits the sensing of all charge transitions, down to the last electron in each dot. We use effective mass theory to investigate the necessary optimization of the device parameters in order to achieve the tunnel rates required for spin-based quantum computation.

cond-mat.mes-hall↗

arXiv2020

Exchange coupling in a linear chain of three quantum-dot spin qubits in silicon

Quantum gates between spin qubits can be implemented leveraging the natural Heisenberg exchange interaction between two electrons in contact with each other. This interaction is controllable by electrically tailoring the overlap between electronic wavefunctions in quantum dot systems, as long as they occupy neighbouring dots. An alternative route is the exploration of superexchange - the coupling between remote spins mediated by a third idle electron that bridges the distance between quantum dots. We experimentally demonstrate direct exchange coupling and provide evidence for second neighbour mediated superexchange in a linear array of three single-electron spin qubits in silicon, inferred from the electron spin resonance frequency spectra. We confirm theoretically through atomistic modeling that the device geometry only allows for sizeable direct exchange coupling for neighbouring dots, while next nearest neighbour coupling cannot stem from the vanishingly small tail of the electronic wavefunction of the remote dots, and is only possible if mediated.

quant-ph↗