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Artem Ryabov

Publications and source records attributed to Artem Ryabov.

At least 19 recordsLinked to original sources

Hidden periodicities allow the prediction of locked particle motions on quasicrystalline surfaces

Motion of particles across quasicrystalline surfaces exhibits peculiar features due to the presence of long-range order without translational periodicity. Under time-periodic forcing, this motion can become locked in directions thatn deviate strongly from the mean driving direction. We show that for surface potentials with a quasicrystalline pattern of minima generated by a superposition of plane waves, particle trajectories are nonperiodic, yet their mean direction and speed are determined by hidden periodic potentials. The lattice vectors of these underlying potentials define characteristic velocities that dictate both directional and speed locking. The particle motion does not synchronize with the driving, and it is possible for the mean speed to remain nonlocked even in directionally locked states. These findings are demonstrated using a model directly amenable to experimental realization.

cond-mat.stat-mech

Nonequilibrium phase transition in single-file transport at high crowding

Driven particle transport in crowded and confining environments is fundamental to diverse phenomena across physics, chemistry, and biology. A main objective in studying such systems is to identify novel emergent states and phases of collective dynamics. Here, we report on a nonequilibrium phase transition occurring in periodic structures at high particle densities. This transition separates a weak-current phase of thermally activated transport from a high-current phase of solitary wave propagation. It is reflected also in a change of universality classes characterizing correlations of particle current fluctuations. Our findings demonstrate that sudden changes to high current states can occur when increasing particle densities beyond critical values.

cond-mat.stat-mech

Local quantum coherence with intersource interactions at nonzero temperature

Local quantum coherence in a two-level system (TLS) is typically generated via time-dependent driving. However, it can also emerge autonomously from symmetry-breaking interactions between the TLS and its surrounding environment at a low temperature. Although such environments often consist of interacting atoms or spins, the role of interactions within the environment in generating the autonomous local coherence has remained unexplored. Here, we address this gap by analyzing an exactly solvable model, which comprises a target TLS coupled to $N$ interacting source TLSs that represent the environment, with the whole system being in thermal equilibrium. We show that the local coherence not only persists but can be enhanced at finite temperatures of the environment compared to the case of no inter-source interactions. The temperature dependence of the coherence bears signatures of a quantum phase transition, and our analytical results suggest strategies for its optimization. Our findings reveal generic properties of the autonomously generated quantum coherence and point to viable routes for observing the coherence at nonzero temperatures.

quant-ph

Cluster sizes, particle displacements and currents in transport mediated by solitary cluster waves

In overdamped particle motion across periodic landscapes, solitary cluster waves can occur at high particle densities and lead to particle transport even in the absence of thermal noise. Here we show that for driven motion under a constant drag, the sum of all particle displacements per soliton equals one wavelength of the periodic potential. This unit displacement law is used to determine particle currents mediated by the solitons. We furthermore derive properties of clusters involved in the wave propagation as well as relations between cluster sizes and soliton numbers.

cond-mat.stat-mech

Engineering tunable fractional Shapiro steps in colloidal transport

Shapiro steps are quantized plateaus in the velocity-force or velocity-torque curve of a driven system, when its speed remains constant despite an increase in the driving force. For microscopic particles driven across a sinusoidal potential, integer Shapiro steps have been observed. By driving a single colloidal particle across a time-modulated, non-sinusoidal periodic optical landscape, we here demonstrate that fractional Shapiro steps emerge in addition to integer ones. Measuring the particle position via individual particle tracking, we reveal the underlying microscopic mechanisms that produce integer and fractional steps and demonstrate how these steps can be controlled by tuning the shape and driving protocol of the optical potential. The flexibility offered by optical engineering allows us to generate wide ranges of potential shapes and to study, at the single-particle level, synchronization behavior in driven soft condensed matter systems.

cond-mat.soft

Phase locking and fractional Shapiro steps in collective dynamics of microparticles

In driven nonlinear systems, phase locking is an intriguing effect leading to robust stationary states that are stable over extended ranges of control parameters. Recent experiments allow for exploring microscopic mechanisms underlying such phenomena in collective dynamics of micro- and nanoparticles. Here we show that phase-locked dynamics of hardcore-interacting microparticles in a densely populated periodic potential under time-periodic driving arises from running solitary cluster waves. We explain how values of phase-locked currents are related to soliton velocities and why collective particle dynamics synchronize with the driving for certain particle diameters only. Our analysis is based on an effective potential for the solitary wave propagation and a unit displacement law, saying that the total average shift of all particle positions per soliton period equals one wavelength of the periodic potential.

cond-mat.stat-mech

Solitary cluster waves in periodic potentials: Formation, propagation, and soliton-mediated particle transport

Transport processes in crowded periodic structures are often mediated by cooperative movements of particles forming clusters. Recent theoretical and experimental studies of driven Brownian motion of hard spheres showed that cluster-mediated transport in one-dimensional periodic potentials can proceed in form of solitary waves. We here give a comprehensive description of these solitons. Fundamental for our analysis is a static presoliton state, which is formed by a periodic arrangement of basic stable clusters. Their size follows from a geometric principle of minimum free space. Adding one particle to the presoliton state gives rise to solitons. We derive the minimal number of particles needed for soliton formation, number of solitons at larger particle numbers, soliton velocities and soliton-mediated particle currents. Incomplete relaxations of the basic clusters are responsible for an effective repulsive soliton-soliton interaction seen in measurements. A dynamical phase transition is predicted to occur in current-density relations at low temperatures. Our results provide a theoretical basis for describing experiments on cluster-mediated particle transport in periodic potentials.

cond-mat.stat-mech

Fast Brownian cluster dynamics

We present an efficient method to perform overdamped Brownian dynamics simulations in external force fields and for particle interactions that include a hardcore part. The method applies to particle motion in one dimension, where it is possible to update particle positions by repositioning particle clusters as a whole. These clusters consist of several particles in contact. They form because particle collisions are treated as completely inelastic rather than elastic ones. Updating of cluster positions in time steps is carried out by cluster fragmentation and merging procedures. The presented method is particularly powerful at high collision rates in densely crowded systems, where collective movements of particle assemblies is governing the dynamics. As an application, we simulate the single-file diffusion of sticky hard spheres in a periodic potential.

cond-mat.stat-mech

Nanoswimmers in a ratchet potential: Effects of a transverse rocking force

We study the dynamics of a chemical nanoswimmer in a ratchet potential, which is periodically rocked in the transverse direction. As a result of the mechanochemical coupling, the self-propulsion velocity becomes force-dependent and particle trajectories are rectified in the direction of the ratchet modulation. The magnitude and direction of the nanoswimmer mean velocity depend upon both the rocking amplitude and the frequency. Remarkably, for frequencies larger than the inverse correlation time of the rotational diffusion, the velocity exhibits oscillatory behaviour as a function of the amplitude and the frequency with multiple reversals of the sign. These findings suggest that mechanochemical coupling can be utilized for controlling the motion of chemically active particles at the nanoscale.

cond-mat.stat-mech

Mechanochemical Active Ratchet

Self-propelled nanoparticles moving through liquids offer the possibility of creating advanced applications where such nanoswimmers can operate as artificial molecular-sized motors. Achieving control over the motion of nanoswimmers is a crucial aspect for their reliable functioning. While the directionality of micron-sized swimmers can be controlled with great precision, steering nano-sized active particles poses a real challenge. One of the reasons is the existence of large fluctuations of active velocity at the nanoscale. Here, we describe a mechanism that, in the presence of a ratchet potential, transforms these fluctuations into a net current of active nanoparticles. We demonstrate the effect using a generic model of self-propulsion powered by chemical reactions. The net motion along the easy direction of the ratchet potential arises from the coupling of chemical and mechanical processes and is triggered by a constant, transverse to the ratchet, force. The current magnitude sensitively depends on the amplitude and the periodicity of the ratchet potential and the strength of the transverse force. Our results highlight the importance of thermodynamically consistent modeling of chemical reactions in active matter at the nanoscale and suggest new ways of controlling dynamics in such systems.

cond-mat.stat-mech

Single-file transport of binary hard-sphere mixtures through periodic potentials

Single-file transport occurs in various scientific fields, including diffusion through nanopores, nanofluidic devices, and cellular processes. We here investigate the impact of polydispersity on particle currents for single-file Brownian motion of hard spheres, when they are driven through periodic potentials by a constant drag force. Through theoretical analysis and extensive Brownian dynamics simulations, we unveil the behavior of particle currents for random binary mixtures. The particle currents show a recurring pattern in dependence of the hard-sphere diameters and mixing ratio. We explain this recurrent behavior by showing that a basic unit cell exists in the space of the two hard-sphere diameters. Once the behavior of an observable inside the unit cell is determined, it can be inferred for any diameter. The overall variation of particle currents with the mixing ratio and hard-sphere diameters is reflected by their variation in the limit where the system is fully covered by hard spheres. In this limit, the currents can be predicted analytically. Our analysis explains the occurrence of pronounced maxima and minima of the currents by changes of an effective potential barrier for the center-of-mass motion.

cond-mat.stat-mech

Scaling laws for single-file diffusion of adhesive particles

Single-file diffusion refers to the Brownian motion in narrow channels where particles cannot pass each other. In such processes, the diffusion of a tagged particle is typically normal at short times and becomes subdiffusive at long times. For hard-sphere interparticle interaction, the time-dependent mean squared displacement of a tracer is well understood. Here we develop a scaling theory for adhesive particles. It provides a full description of the time-dependent diffusive behavior with a scaling function that depends on an effective strength of adhesive interaction. Particle clustering induced by the adhesive interaction slows down the diffusion at short times, while it enhances subdiffusion at long times. The enhancement effect can be quantified in measurements irrespective of how tagged particles are injected into the system. Combined effects of pore structure and particle adhesiveness should speed up translocation of molecules through narrow pores.

cond-mat.stat-mech

Hydrodynamic interactions hinder transport of flow-driven colloidal particles

The flow-driven transport of interacting micron-sized particles occurs in many soft matter systems spanning from the translocation of proteins to moving emulsions in microfluidic devices. Here we combine experiments and theory to investigate the collective transport properties of colloidal particles along a rotating ring of optical traps. In the co-rotating reference frame, the particles are driven by a vortex flow of the surrounding fluid. When increasing the depth of the optical potential, we observe a jamming behavior that manifests itself in a strong reduction of the current with increasing particle density. We show that this jamming is caused by hydrodynamic interactions that enhance the energetic barriers between the optical traps. This leads to a transition from an over- to an under-critical tilting of the potential in the corotating frame. Based on analytical considerations, the enhancement effect is estimated to increase with increasing particle size or decreasing radius of the ring of traps. Measurements for different ring radii and Stokesian dynamics simulations for corresponding particle sizes confirm this. The enhancement of potential barriers in the flow-driven system is contrasted to the reduction of barriers in a force-driven one. This diverse behavior demonstrates that hydrodynamic interactions can have a very different impact on the collective dynamics of many-body systems. Applications to soft matter and biological systems require careful consideration of the driving mechanism and of the role of hydrodynamic interactions.

cond-mat.soft

Collective excitations in jammed states: ultrafast defect propagation and finite-size scaling

In crowded systems, particle currents can be mediated by propagating collective excitations which are generated as rare events, are localized and have a finite lifetime. The theoretical description of such excitations is hampered by the problem of identifying complex many-particle transition states, calculation of their free energies, and the evaluation of propagation mechanisms and velocities. Here we show that these problems can be tackled for a highly jammed system of hard spheres in a periodic potential. We derive generation rates of collective excitations, their anomalously high velocities, explain the occurrence of an apparent jamming transition and its strong dependence on the system size. The particle currents follow a scaling behavior, where for small systems the current is proportional to the generation rate and for large systems given by the geometric mean of the generation rate and velocity. Our theoretical approach is widely applicable to dense nonequilibrium systems in confined geometries. It provides new perspectives for studying dynamics of collective excitations in experiments.

cond-mat.stat-mech

Brownian dynamics simulations of hard rods in external fields and with contact interactions

We propose a simulation method for Brownian dynamics of hard rods in one dimension for arbitrary continuous external force fields. It is an event-driven procedure based on the fragmentation and mergers of clusters formed by particles in contact. It allows one to treat particle interactions in addition to the hard-sphere exclusion as long as the corresponding interaction forces are continuous functions of the particle coordinates. We furthermore develop a treatment of sticky hard spheres as described by Baxter's contact interaction potential.

cond-mat.stat-mech

Enhanced diffusivity in microscopically reversible active matter

Physics of self-propelled objects at the nanoscale is a rapidly developing research field where recent experiments focused on motion of individual catalytic enzymes. Contrary to the experimental advancements, theoretical understanding of possible self-propulsion mechanisms at these scales is limited. A particularly puzzling question concerns origins of reportedly high diffusivities of the individual enzymes. Here we start with the fundamental principle of microscopic reversibility (MR) of chemical reactions powering the self-propulsion and demonstrate that MR can lead to increase of the particle mobility and of short- and long-time diffusion coefficients as compared to dynamics where MR is neglected. Moreover, the diffusion coefficients can be enhanced by a constant external force. We propose a way to use these effects in experimental investigations of active propulsion mechanisms at the nanoscale. Our results can shed new light on interpretation of the measured diffusivities and help to test and to evaluate relevance of MR for the active motion of individual nanoswimmers.

cond-mat.soft

Diffusion coefficient and power spectrum of active particles with a microscopically reversible mechanism of self-propelling

Catalytically active macromolecules are envisioned as key building blocks in development of artificial nanomotors. However, theory and experiments report conflicting findings regarding their dynamics. The lack of consensus is mostly caused by a limited understanding of specifics of self-propulsion mechanisms at the nanoscale. Here, we study a generic model of a self-propelled nanoparticle that does not rely on a particular mechanism. Instead, its main assumption is the fundamental symmetry of microscopic dynamics of chemical reactions: the principle of microscopic reversibility. Significant consequences of this assumption arise if we subject the particle to an action of an external time-periodic force. The particle diffusion coefficient is then enhanced compared to the unbiased dynamics. The enhancement can be controlled by the force amplitude and frequency. We also derive the power spectrum of particle trajectories. Among new effects stemming from the microscopic reversibility are the enhancement of the spectrum at all frequencies and sigmoid-shaped transitions and a peak at characteristic frequencies of rotational diffusion and external forcing. The microscopic reversibility is a generic property of a broad class of chemical reactions, therefore we expect that the presented results will motivate new experimental studies aimed at testing of our predictions. This could provide new insights into dynamics of catalytic macromolecules.

cond-mat.stat-mech

Solitons in overdamped Brownian dynamics

Solitons are commonly known as waves that propagate without dispersion. Here we show that they can occur for driven overdamped Brownian dynamics of hard spheres in periodic potentials at high densities. The solitons manifest themselves as periodic sequences of different assemblies of particles moving in the limit of zero noise, where transport of single particles is not possible. They give rise to particle currents at even low temperature that appear in band-like structures around certain hard-sphere diameters. At high temperatures, the band-like structures are washed out by the noise, but the particle transport is still dominated by the solitons. All these predicted features should occur in a broad class of periodic systems and are amenable to experimental tests.

cond-mat.stat-mech