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Arun Bansil

Publications and source records attributed to Arun Bansil.

At least 19 recordsLinked to original sources

Nanoscale imaging of ferromagnetic vortex dynamics with scanning NV magnetometry

The generation and manipulation of spin waves at the nanoscale via magnetic vortices are of considerable importance because of their broad applications across magnonic and quantum technologies. Previously, fixed nitrogen-vacancy (NV) centers in diamond have been used to locally characterize vortex dynamics, and scanning NV magnetometry (SNVM) has been used to image vortices' static stray fields. Here, we demonstrate SNVM imaging of both the static and microwave fields generated by vortices in mesoscopic permalloy structures with $\sim$50 nm spatial resolution, achieving excellent agreement with micromagnetic simulations, while revealing the effects of disorder. We further demonstrate a 40$\times$ microwave field enhancement near a vortex core and image the disorder-dependent, spatially varying, evanescent decay of these microwaves. Our ambient, tabletop technique surpasses diffraction-limited techniques' resolutions by at least 5$\times$, with far greater accessibility and throughput than synchrotron radiation-based techniques, offering new opportunities in the study and development of magnonic devices.

cond-mat.mes-hall

Helical Domain-Wall-Ring Networks Reshape Superconducting Correlations

Extended domain-wall networks that emerge in moir\'e materials provide a distinct platform for quasi-one-dimensional electronic states. However, the interaction-driven orders in confined networks remain largely unexplored. Here, we discuss superconducting (SC) correlations in interacting helical domain-wall-ring networks in the closed topological domains formed within the moir\'e patterns of an underlying twisted bilayer honeycomb lattice. We first analyze the system within the framework of an infinite-size theory and show that inter-ring SC-pair tunneling is renormalization-group relevant and thus enhances SC correlations through inter-ring phase locking. To address finite-size effects resulting from the ring-network geometry, we present a self-consistent variational approach. Our analysis shows that even in the regime where the infinite-size theory predicts strongly coupled pair tunneling, the induced phase-locking scale remains strongly suppressed. In contrast, the SC scaling dimension continues to decrease with stronger inter-ring density-density interaction and a decreasing twist angle, while remaining insensitive to the pair-tunneling strength. This discrepancy demonstrates that ring networks do not simply approach their infinite-size counterparts but can exhibit qualitatively distinct collective behavior. Our study highlights how the interplay of confinement effects and ring-network geometry can reshape SC correlations.

cond-mat.mes-hall

Quantum Geometry Driven Finite-Momentum Exciton Fluctuations in Flat-Band Systems

Quantum geometry is instrumental in stabilizing exotic phenomena in systems ranging from topological insulators to superconductors. In dispersionless flat bands, where the kinetic energy is quenched, the quantum metric emerges as the fundamental driver of macroscopic collective phenomena. Here, we theoretically demonstrate that lattice-geometry-induced flat bands, such as those in kagome and Lieb lattices, provide a fertile platform for realizing a purely quantum-geometry-driven excitonic insulator (EI) phase. By applying an out-of-plane Zeeman field to lift spin degeneracy without spin-orbit coupling, we establish a Ginzburg-Landau framework in which the electron-hole wavefunction-overlap directly maps the flat-band quantum metric onto the macroscopic free energy. This mapping plays a key role in both the EI and the associated superfluid phases, with the coherence length and phase stiffness emerging directly from the quantum metric. Our analysis reveals that under strong interactions, the quantum metric induces a negative effective kinetic coefficient for the amplitude mode. Rather than destabilizing the uniform condensate, this softens the amplitude fluctuations at a finite momentum, giving rise to a finite-momentum superfluid density fluctuation (FMSDF) state. This state is observable as a periodically modulated magnitude of in-plane magnetization fluctuations. Our findings establish a rigorous link between flat-band quantum geometry and dynamic collective excitonic states, with promising pathways for realization in covalent-organic frameworks (COFs).

cond-mat.mes-hall

Inter-Dirac-Cone Coherence Beyond the Valley Framework

Although interactions are known to generate exotic phases in pseudospin-1/2 flat-band Dirac materials, it remains an open question whether higher-pseudospin Dirac cones continue to govern low-energy interaction-driven orders even without a well-defined valley degree of freedom. Here, we demonstrate a new form of inter-Dirac-cone coherence beyond the valley framework, which is realized through a staggered virtual-loop-current (SVLC) order in a partially filled pseudospin-1 Dirac flat band. Remarkably, the SVLC order continues to be driven by coherence between the pseudospin-1 Dirac cones even after the conventional valley-based description ceases to apply. The virtual loop currents are shown to originate from interaction-driven quantum fluctuations of charge densities and are found to exhibit an alternating circulation between the neighboring triangular plaquettes. The resulting spontaneous time-reversal symmetry breaking induces finite intrinsic anomalous Hall conductivity and orbital magnetization. The SVLC order is shown to be the lowest-energy solution in restricted real-space Hartree-Fock calculations in the weakly interacting regime. Our study establishes inter-Dirac-cone coherence as the organizing principle for interaction-driven orders in higher-pseudospin Dirac systems and identifies these systems as a new platform for driving exotic emergent phases beyond the valley framework.

cond-mat.str-el

Nodal Topological Superconductivity Driven by Crystalline Antiunitary Symmetry in Altermagnets

Topological superconductivity hosts protected quasiparticles and is central to topological quantum computation, yet its realization in intrinsic materials remains challenging and often relies on engineered platforms. Here we uncover a symmetry-constrained mechanism for nodal topological superconductivity in altermagnets. Focusing on fourfold rotational collinear altermagnets, we show that the native crystalline antiunitary symmetry $\mathcal{T}C_{4z}$ generically forbids pure spin-singlet pairing and selects pairing structures that admit Bogoliubov-de Gennes (BdG) Hamiltonians with emergent chiral symmetries. These symmetries further give rise to robust nodal topological phases over broad parameter regimes, including a nodal-point phase hosting Majorana flat bands (MFBs) and two distinct nodal-loop phases with chiral Majorana edge states. Notably, the nodal structure persists even after spontaneous breaking of the antiunitary symmetry, indicating that the topology originates from symmetry-constrained pairing rather than direct symmetry protection. Finally, we propose tunneling signatures that can distinguish these nodal phases and probe symmetry breaking experimentally.

cond-mat.supr-con

Emergent Quantum-Geometric Equivalence of Injection and Shift Currents

Injection and shift currents are generally regarded as distinct nonlinear optical responses with separate microscopic origins. Here, we uncover a general hidden connection between them through interband Berry-curvature and quantum-metric dipoles. In systems with approximately linear electronic dispersion near the Fermi level and at low photon energies, this relation sharpens into an emergent equivalence, with injection and shift currents governed by the same interband quantum-geometric dipole. This regime is naturally realized in Dirac and Weyl semimetals, as well as in strained graphene, where measurements of injection and shift currents probe a unified geometric property of the electronic wavefunctions rather than distinct dynamical processes. Our results establish a new framework for interpreting nonlinear optical experiments and suggest that quantum geometry may provide a broader organizing principle linking seemingly distinct nonlinear optical responses in solids.

cond-mat.mes-hall

Engineering Nonlinear Optical Responses via Inversion Symmetry Breaking in Bilayer Bi2Se3

Paucity of naturally occurring noncentrosymmetric materials is stimulating growing interest in engineered two-dimensional systems for nonlinear optical applications. Here, we show that breaking inversion symmetry in centrosymmetric bilayer Bi$_2$Se$_3$ through twisting, point-defect insertion, or the application of an external electric field unlocks rich nonlinear optical responses. In twisted bilayer Bi$_2$Se$_3$ at the first commensurate angle of 21.78$^\circ$, we find peak shift and injection current conductivities of -14 $ nm.\mu AV^{-2}$ and 104 $\times 10^8$ $nm.A V^{-2}s^{-1}$, respectively, which lie in the visible spectrum and enable efficient THz applications. The external electric field and point-defect insertion both transform the bilayer into C$_ {3v}$ symmetry, with the selenium vacancy (V$_{Se}$) achieving peak shift and injection current conductivities of -190 nm.$\mu AV^{-2}$ and -170 $\times 10^8$ $nm.A V^{-2}s^{-1}$. In all three cases, the peak nonlinear optical responses are found to be comparable to those of benchmark 2D materials such as GeS, and the broadband responses, including helicity-dependent current generation, make these engineered bilayers viable candidates for next-generation 2D photovoltaics.

cond-mat.mtrl-sci

Breakdown of Topological Inheritance and Twist-Induced Quantum Geometry Reconfiguration in Moir\'e Flat Bands

Since the inception of moir\'e quantum matter, a foundational tenet of the field has been that the quantum geometry of emergent flat bands is faithfully inherited from the low-energy valleys of the constituent monolayers. Here, we demonstrate a breakdown of this longstanding tenet in twisted bilayers of loop-current-ordered kagome lattices (tb-LCK). Using microscopic tight-binding modeling, we reveal a twist-induced reconfiguration of quantum geometry where realistic interlayer hybridization quenches topological inheritance from the monolayer. By tuning the loop-current phase, we identify distinct regimes in which the monolayer Berry curvature is either substantially redistributed or entirely suppressed in the moir\'e flat bands. We further show that this quantum geometric collapse is expected to be readily accessible in vanadium-based kagome metals such as AV$_{\text{3}}$Sb$_{\text{5}}$, and that Floquet engineering via waveguide laser illumination offers a practical route to turn topological inheritance on and off. Our findings uncover a universal mechanism for quantum geometric reconstruction, establishing interlayer coupling strength as an independent parameter for tuning band topology beyond the weakly coupled van der Waals heterostructure paradigm.

cond-mat.mes-hall

Quantum Geometry of Moir\'e Flat Bands Beyond the Valley Paradigm

Flat bands in moir\'e superlattices provide a fertile ground for correlated and topological phases, governed by their quantum geometric properties. While the valley-based paradigm captures key features in select materials, it breaks down in a growing class of systems lacking valley structure, where exotic phenomena such as twist-angle-tunable numbers of flat bands emerge. In this work, we develop and analyze tight-binding models for twisted heterobilayers of bipartite lattices, with a focus on the role of interlayer hybridization in generating flat-band quantum geometry. We demonstrate that sublattice-selective interlayer tunnelings in twisted dice lattice and graphene heterobilayers induce isolated flat bands at zero energy, whose number is tunable by the twist angle. Most importantly, these flat bands exhibit finite Berry curvature and a quantum metric of the Chern-insulator scale, generated through interlayer hybridization. This establishes a mechanism to induce quantum geometry in moir\'e flat bands beyond the valley paradigm. Our results chart a route to flat-band quantum geometry engineering in twisted bilayer bipartite lattices, with potential material realizations in oxide heterostructures, molecular lattices, and synthetic quantum matter.

cond-mat.mes-hall

Extending Topological Bound on Quantum Weight Beyond Symmetry-Protected Topological Phases

The quantum metric encodes the geometric structure of Bloch wave functions and governs a wide range of physical responses. Its Brillouin-zone integral, the quantum weight, appears in the structure factor and provides lower bounds on observables such as the optical gap and dielectric constant. In symmetry-protected topological (SPT) phases, the nontrivial band topology imposes a lower bound on the quantum weight and constraints on the observables. Here, we generalize the topological bound on quantum geometry to encompass systems beyond the SPT phases. We show that topological invariants defined via the projected spectrum lower-bound the quantum weight with a symmetry-breaking correction to the quantum metric. Our proposed bound holds even when the underlying symmetries are broken, and it would be amenable to experimental verification via the optical conductivity sum rule under external fields. We illustrate our theory by adding a nonzero spin-orbit coupling term to a spin Chern insulator model, where we show that our proposed bound applies even though the conventional topological bound does not hold.

cond-mat.mes-hall

Conductivity scaling of the anomalous Hall effect in the altermagnetic semiconductor {\alpha}-MnTe

{\alpha}-MnTe is a prototypical altermagnet exhibiting a strong anomalous Hall effect (AHE), despite having a nearly vanishing magnetization. Lately, sample-to-sample variations of the amplitude of the AHE have raised concerns of a possible defect related origin, especially in thin films. Here, we study the AHE in {\alpha}-MnTe films grown on SrF2 that have the crystal structure and m'm'm magnetic point group symmetry expected for bulk. By studying the scaling of the AHE with conductivity for those films and previously reported measurements in the literature, we find that sample-to-sample variations are well explained by a scaling law consistent with a hopping origin. Importantly, a comparison with other magnetic semiconductors reveals the colossal amplitude of the AHE of {\alpha}-MnTe compared to its measured spontaneous magnetization from magnetometry and polarized neutron reflectivity. Our findings address the important fundamental question of the origin of the AHE of {\alpha}-MnTe and further demonstrate the potential of altermagnets as promising spintronic materials.

cond-mat.str-el

Rotational Phonons Drive Low-Energy Kinks in Cuprate Superconductors

Angle-resolved photoemission spectroscopy (ARPES) reveals ubiquitous quasiparticle ``kinks'' near $\sim$70 meV and $\sim$40 meV across cuprate superconductors, often accompanied by peak--dip--hump (PDH) structures. These features point to strong coupling between electrons and low-energy bosonic excitations, but the microscopic origin has remained elusive due to the limitations of conventional density-functional theory (DFT) and the high cost of beyond-DFT methods. Here, we systematically study the electron--phonon coupling (EPC) in hole-doped infinite-layer CaCuO$_2$ using the Strongly Constrained and Appropriately Normed (SCAN) density functional, explicitly including magnetic effects. We find a substantial EPC strength $\lambda$ of $\sim$0.5 in the magnetic phase, producing kinks and PDH structures in the 40-80~meV window in excellent agreement with experiments. The dominant contribution arises from rotational oxygen phonons, while breathing modes contribute little. Our results establish strong EPC in cuprates, highlight the key role of rotational phonons, and provide a framework for understanding spectral anomalies in cuprates and beyond.

cond-mat.str-el

Investigating the Electronic and Magnetic Properties of Na$_x$Fe$_{1/2}$Mn$_{1/2}$O$_2$ Cathode Materials with X-ray Compton Scattering

We discuss electronic and magnetic properties of Na$_x$Fe$_{1/2}$Mn$_{1/2}$O$_2$, a promising Na-ion battery cathode material. Using x-ray Compton scattering, SQUID magnetometry, and density-functional-theory based modeling, we probe how electrons and spins evolve during sodiation. By comparing Compton profiles of sodiated and desodiated samples, we show that oxygen 2$p$ orbitals drive the redox process, while transition-metal 3$d$ electrons become more delocalized, explaining the metallic phase at $x=2/3$. These profile differences define a quantitative descriptor for the sodiation range associated with improved conductivity. Electron holes on oxygen, reflected in oxygen magnetization, confirm the important role of oxygen in the electrochemical activity of the cathode.

cond-mat.mtrl-sci

Layer-dependent antiferromagnetic Chern and axion insulating states in UOTe

Magnetic topological insulators have received significant interest due to their dissipationless edge states, which promise advances in energy-efficient electronic transport. However, the magnetic topological insulator state has typically been found in ferromagnets (FMs) that suffer from low magnetic ordering temperatures and stray fields. Identifying an antiferromagnetic topological insulator that exhibits the quantum anomalous Hall effect (QAHE) with a relatively high N\'eel temperature has been a longstanding challenge. Here, we focus on the recently discovered van der Waals (vdW) antiferromagnet (AFM) UOTe, which not only features a high N\'eel temperature (\(\sim\)150K) but also exhibits intriguing Kondo interaction and topological characteristics. Our systematic analysis of the layer-dependent topological phases based on \textit{ab} initio computations predicts the two-layer UOTe film to be an ideal 2D AFM Chern insulator in which the Hall conductivity is quantized with a fully compensated spin magnetization. By applying an in-plane strain or electric field, we show how the itinerancy of U-5f electrons can be manipulated to trigger a transition between the nontrivial ($C = 1$) and trivial ($C = 0$) phases. Interestingly, the 3-layer UOTe film is found to have zero charge conductance but it hosts a quantized spin Hall conductivity (SHC) with finite magneto-electric coupling, suggesting the presence of an axion insulator-like state. The unique magnetic structure of UOTe supports a layer-tunable topology in which films with an odd number of layers are axion-like insulators, while films with an even number of layers are Chern insulators, and the bulk material is a Dirac semimetal. Our study offers a new intrinsic AFM materials platform for realizing correlated topological phases for next-generation spintronics applications and fundamental science studies.

cond-mat.mtrl-sci

Anomalous Nodal Gap in a Doped Spin-1/2 Antiferromagnetic Mott Insulator

Many emergent phenomena appear in doped Mott insulators near the insulator-to-metal transition. In high-temperature cuprate superconductors, superconductivity arises when antiferromagnetic (AFM) order is gradually suppressed by carrier doping, and a $\textit{d}$-wave superconducting gap forms when an enigmatic nodal gap evolves into a point node. Here, we examine electron-doped Sr$_{2}$IrO$_{4}$, the 5$\textit{d}$-electron counterpart of cuprates, using angle-resolved photoemission spectroscopy. At low doping levels, we observe the formation of electronic states near the Fermi level, accompanied by a gap at the AFM zone boundary, mimicking the AFM gap in electron-doped cuprates. With increasing doping, a distinct gap emerges along the (0,0)-($\pi$,$\pi$) nodal direction, paralleling that observed in hole-doped cuprates. This anomalous nodal gap persists after the collapse of the AFM gap and gradually decreases with further doping. It eventually vanishes into a point node of the reported $\textit{d}$-wave gap. These observations replicate the characteristic features in both electron- and hole-doped cuprates, indicating a unified route toward nodal metallicity in doped spin-1/2 AFM Mott insulators.

cond-mat.supr-con

Green's Function Methods for Computing Supercurrents in Josephson Junctions

Interest in Josephson junctions (JJs) has increased rapidly in recent years not only because of their use in qubits and other quantum devices but also due to the unique physics supported by the JJs. The advent of various novel quantum materials for both the barrier region and the superconducting leads has led to the possibility of adding new functionalities to the JJs. Thus, there is a growing need for accurate modeling of the JJs and related systems to enable their predictive control and atomistic level understanding. This review presents an in-depth discussion of a Green's function-based formalism for computing supercurrents in JJs. The formulation is tailored for large-scale atomistic simulations and encompasses both dc and ac supercurrents. We hope that this review will provide a timely and comprehensive reference for researchers as well as beginning practitioners interested in Green's-function-based methods to model supercurrents in JJs.

cond-mat.supr-con

Giant Shift Current in Electrically-Tunable Superlattice Bilayer Graphene

Recent introduction of superlattice potentials has opened new avenues for engineering tunable electronic band structures featuring topologically nontrivial moir\'{e}-like bands. Here we consider optoelectronic properties of Bernal-stacked graphene subjected to a superlattice potential either electrostatically or through lattice twisting to show that it exhibits a giant shift current response that is orders of magnitude larger than existing predictions in twisted mulitlayer systems. Effects of gate voltage and the strength and phase of the superlattice potential on the shift current are delineated systematically across various topological regimes. Our study gives insight into the nature of nonlinear responses of materials and how these responses could be optimized by tuning the superlattice potential.

cond-mat.mes-hall

Physics-Guided Dual Implicit Neural Representations for Source Separation

Significant challenges exist in efficient data analysis of most advanced experimental and observational techniques because the collected signals often include unwanted contributions--such as background and signal distortions--that can obscure the physically relevant information of interest. To address this, we have developed a self-supervised machine-learning approach for source separation using a dual implicit neural representation framework that jointly trains two neural networks: one for approximating distortions of the physical signal of interest and the other for learning the effective background contribution. Our method learns directly from the raw data by minimizing a reconstruction-based loss function without requiring labeled data or pre-defined dictionaries. We demonstrate the effectiveness of our framework by considering a challenging case study involving large-scale simulated as well as experimental momentum-energy-dependent inelastic neutron scattering data in a four-dimensional parameter space, characterized by heterogeneous background contributions and unknown distortions to the target signal. The method is found to successfully separate physically meaningful signals from a complex or structured background even when the signal characteristics vary across all four dimensions of the parameter space. An analytical approach that informs the choice of the regularization parameter is presented. Our method offers a versatile framework for addressing source separation problems across diverse domains, ranging from superimposed signals in astronomical measurements to structural features in biomedical image reconstructions.

cs.CV