arXiv subjects

B. A. Piot

Publications and source records attributed to B. A. Piot.

At least 19 recordsLinked to original sources

arXiv2026

Magnetic-field-induced magnon portfolio in a van der Waals magnet

Magnonic excitations are investigated in chromium oxychloride (CrOCl), a van der Waal (vdW) antiferromagnet prone to a multitude of magnetic phase transitions, with absorption experiments in a broad continuous energy range. At low magnetic fields, the magnon spectra show a strong bi-axial anisotropy and inform on the relative weights of the effective exchange coupling and the system anisotropies. As the magnetic field increases, magnons characteristic of a canted phase are first observed, with peculiarities attributed to in-plane anisotropies and magnon-magnon coupling. Subsequently, a hysteretic magnon spectrum appears as the system transitions to a ferrimagnetic state, with two new magnon branches partly coexisting with the lower energy canted phase branch, indicating the formation of spatially separated magnetic phases. Further changes in the magnon spectrum in higher magnetic fields accompany transitions to the different canted magnetic phases previously reported. Our experiments show that competing exchange interactions and ground states broaden the options to generate different kinds of magnonic excitations in the same vdW material upon the variation of external parameters.

cond-mat.mtrl-sci↗

arXiv2026

Dynamics of surface electrons in a topological insulator: cyclotron resonance at room temperature

The ability to manipulate the surface states of topological insulators using electric or magnetic fields under ambient conditions is a key step toward their integration into future electronic and optoelectronic devices. Here, we demonstrate - using cyclotron resonance measurements on a tin-doped BiSbTe$_2$S topological insulator - that moderate magnetic fields can quantize massless surface electrons into Landau levels even at room temperature. This finding suggests that surface-state electrons can behave as long-lived quasiparticles at unexpectedly high temperatures.

cond-mat.mes-hall↗

arXiv2025

Spontaneous Breaking of the SU(3) Flavor Symmetry in a Quantum Hall Valley Nematic

Two-dimensional quantum materials can host original electronic phases that arise from the interplay of electronic correlations, symmetry and topology. In particular, the spontaneous breaking of internal symmetry that acts simultaneously on the pseudospin and the spatial degree of freedom realizes a nematic ordering. We report evidence of a quantum Hall valley nematic phase with an underlying SU(3) order parameter space obtained by a spontaneous polarization between the threefold degenerate valley pseudospins in Pb1-xSnxSe quantum wells. In the presence of a Zeeman field, we demonstrate a further control of the nematic ordering with an explicit symmetry breaking. Evidence of both spontaneous and explicit SU(3) symmetry breaking, reminiscent of the quark flavor paradigm, is of fundamental interest to shape the many body physics in a SU(3) system.

cond-mat.mes-hall↗

arXiv2025

Magnetic phases and zone-folded phonons in a frustrated van der Waals magnet

2D magnetic materials have attracted extensive research interest due to their potential application in nanospintronics, optospintronics, and in magnonics. Ferromagnetic as well as antiferromagnetic layered materials have been demonstrated and successfully inserted into van der Waals heterostructures. However, the effects of magnetic frustration in van der Waals materials and the possibilities offered by spin configurations characterized by nonlinear spin arrangements have not been fully considered yet. Herein, we establish the magnetic phase diagram of bulk CrOCl, a frustrated van der Waals magnet, using magnetization and magneto-optical spectroscopy techniques. In particular, we use the magnetic superstructures relative to the crystallographic unit cell and the associated rich zone-folded phonon series to describe the magnetic field induced phases. Theoretical calculations taking into account the competing nearest neighbors magnetic exchange interactions provide a unique insight into the lattice vibrations of this class of magnetic system. This study expands the scope of 2D magnetic materials and provides a methodology to characterize frustrated van der Waals magnets.

cond-mat.mes-hall↗

arXiv2024

Electronic band structure of Sb2Te3

Here we report on Landau level spectroscopy of an epitaxially grown thin film of the topological insulator Sb2Te3, complemented by ellipsometry and magneto-transport measurements. The observed response suggests that Sb2Te3 is a direct-gap semiconductor with the fundamental band gap located at the Γpoint, or along the trigonal axis, and its width reaches Eg = 190 meV at low temperatures. Our data also indicate the presence of other low-energy extrema with a higher multiplicity in both the conduction and valence bands. The conclusions based on our experimental data are confronted with and to a great extent corroborated by the electronic band structure calculated using the GW method.

cond-mat.mtrl-sci↗

arXiv2023

Magneto-optical sensing of the pressure driven magnetic ground states in bulk CrSBr

Competition between exchange interactions and magnetocrystalline anisotropy may bring new magnetic states that are of great current interest. An applied hydrostatic pressure can further be used to tune their balance. In this work we investigate the magnetization process of a biaxial antiferromagnet in an external magnetic field applied along the easy axis. We find that the single metamagnetic transition of the Ising type observed in this material under ambient pressure transforms under hydrostatic pressure into two transitions, a first-order spin flop transition followed by a second order transition towards a polarized ferromagnetic state near saturation. This reversible tuning into a new magnetic phase is obtained in layered bulk CrSBr at low temperature by varying the interlayer distance using high hydrostatic pressure, which efficiently acts on the interlayer magnetic exchange, and is probed by magneto-optical spectroscopy.

cond-mat.mes-hall↗

arXiv2023

Magnon gap excitations in van der Waals antiferromagnet MnPSe$_3$

Magneto-spectroscopy methods have been employed to study the zero-wavevector magnon excitations in MnPSe$_3$. Experiments carried out as a function of temperature and the applied magnetic field show that two low-energy magnon branches of MnPSe$_3$ in its antiferromagnetic phase are gapped. The observation of two low-energy magnon gaps (at 14 and 0.7 cm$^{-1}$) implies that MnPSe$_3$ is a biaxial antiferromagnet. A relatively strong out-of-plane anisotropy imposes the spin alignment to be in-plane whereas the spin directionality within the plane is governed by a factor of 2.5 $\times$ 10$^{-3}$ weaker in-plane anisotropy.

cond-mat.mtrl-sci↗

arXiv2023

Temperature dependence of the energy band gap in ZrTe$_5$: implications for the topological phase

Using Landau level spectroscopy, we determine the temperature dependence of the energy band gap in zirconium pentatelluride (ZrTe$_5$). We find that the band gap reaches $E_g=(5 \pm 1)$ meV at low temperatures and increases monotonously when the temperature is raised. This implies that ZrTe$_5$ is a weak topological insulator, with non-inverted ordering of electronic bands in the center of the Brillouin zone. Our magneto-transport experiments performed in parallel show that the resistivity anomaly in ZrTe$_5$ is not connected with the temperature dependence of the band gap.

cond-mat.mes-hall↗

arXiv2022

Microscopic parameters of the van der Waals CrSBr antiferromagnet from microwave absorption experiments

Microwave absorption experiments employing a phase-sensitive external resistive detection are performed for a topical van der Waals antiferromagnet CrSBr. The field dependence of two resonance modes is measured in an applied field parallel to the three principal crystallographic directions, revealing anisotropies and magnetic transitions in this material. To account for the observed results, we formulate a microscopic spin model with a bi-axial single-ion anisotropy and inter-plane exchange. Theoretical calculations give an excellent description of full magnon spectra enabling us to precisely determine microscopic interaction parameters for CrSBr.

cond-mat.mes-hall↗

arXiv2022

Lorentz-boost-driven magneto-optics in a Dirac nodal-line semimetal

Optical response of crystalline solids is to a large extent driven by excitations that promote electrons among individual bands. This allows one to apply optical and magneto-optical methods to determine experimentally the energy band gap - a fundamental property crucial to our understanding of any solid - with a great precision. Here we show that such conventional methods, applied with great success to many materials in the past, do not work in topological Dirac semimetals with a dispersive nodal line. There, the optically deduced band gap depends on how the magnetic field is oriented with respect to the crystal axes. Such highly unusual behaviour is explained in terms of band-gap renormalization driven by Lorentz boosts.

cond-mat.mes-hall↗

arXiv2020

Landau level spectroscopy of Bi$_2$Te$_3$

Here we report on Landau level spectroscopy in magnetic fields up to 34 T performed on a thin film of topological insulator Bi$_2$Te$_3$ epitaxially grown on a BaF$_2$ substrate. The observed response is consistent with the picture of a direct-gap semiconductor in which charge carriers closely resemble massive Dirac particles. The fundamental band gap reaches $E_g=(175\pm 5)$~meV at low temperatures and it is not located on the trigonal axis, thus displaying either six or twelvefold valley degeneracy. Notably, our magneto-optical data do not indicate any band inversion. This suggests that the fundamental band gap is relatively distant from the $Γ$ point where profound inversion exists andgives rise to relativistic-like surface states of Bi$_2$Te$_3$.

cond-mat.mes-hall↗

arXiv2020

Magneto-optics of a Weyl semimetal beyond the conical band approximation: the case study of TaP

Landau-level spectroscopy, the optical analysis of electrons in materials subject to a strong magnetic field, is a versatile probe of the electronic band structure and has been successfully used in the identification of novel states of matter such as Dirac electrons, topological materials or Weyl semimetals. The latter arise from a complex interplay between crystal symmetry, spin-orbit interaction and inverse ordering of electronic bands. Here, we report on unusual Landau-level transitions in the monopnictide TaP that decrease in energy with increasing magnetic field. We show that these transitions arise naturally at intermediate energies in time-reversal-invariant Weyl semimetals where the Weyl nodes are formed by a partially gapped nodal-loop in the band structure. We propose a simple theoretical model for electronic bands in these Weyl materials that captures the collected magneto-optical data to great extent.

cond-mat.mes-hall↗

arXiv2019

Two-dimension Dirac fermions system in CdHgTe quantum wells

We report on transport and capacitance spectroscopy study of two kinds of quantum wells, namely Cd$_{0.02}$Hg$_{0.98}$Te and Cd$_{0.06}$Hg$_{0.94}$Te with the thicknesses of 7.4 and 11.5 nm, accordingly. The fraction of Cd was chosen in a way that the both quantum wells are expected to have gapless band structure typical for a Dirac fermions system. We have established that the first quantum well exhibits a massless Dirac fermions system with a quality slightly better then in conventional HgTe quantum wells of critical thickness. Second quantum well exhibits a high-quality two-dimensional topological insulator state with the energy gap of around 10 meV and well-defined edge transport making it as a good candidate for further study and applications of topological insulators.

cond-mat.mes-hall↗

arXiv2018

Landau level spectroscopy of valence bands in HgTe quantum wells: Effects of symmetry lowering

Landau level spectroscopy has been employed to probe the electronic structure of the valence band in a series of p-type HgTe/HgCdTe quantum wells with both normal and inverted ordering of bands. We find that the standard axial-symmetric 4-band Kane model, which is nowadays widely applied in physics of HgTe-based topological materials, does not fully account for the complex magneto-optical response observed in our experiments - notably, for the unexpected avoided crossings of excitations and for the appearance of transitions that are electric-dipole forbidden within this model. Nevertheless, reasonable agreement with experiments is achieved when the standard model is expanded to include effects of bulk and interface inversion asymmetries. These remove the axial symmetry, and among other, profoundly modify the shape of valence bands.

cond-mat.mes-hall↗

arXiv2018

The energy scale of Dirac electrons in Cd3As2

Cadmium arsenide (Cd3As2) has recently became conspicuous in solid-state physics due to several reports proposing that it hosts a pair of symmetry-protected 3D Dirac cones. Despite vast investigations, a solid experimental insight into the band structure of this material is still missing. Here we fill one of the existing gaps in our understanding of Cd3As2, and based on our Landau level spectroscopy study, we provide an estimate for the energy scale of 3D Dirac electrons in this system. We find that the appearance of such charge carriers is limited - contrary to a widespread belief in the solid-state community - to a relatively small energy scale (below 40 meV).

cond-mat.mes-hall↗

arXiv2016

Magneto-optical signature of massless Kane electrons in Cd3As2

We report on optical reflectivity experiments performed on Cd3As2 over a broad range of photon energies and magnetic fields. The observed response clearly indicates the presence of 3D massless charge carriers. The specific cyclotron resonance absorption in the quantum limit implies that we are probing massless Kane electrons rather than symmetry-protected 3D Dirac particles. The latter may appear at a smaller energy scale and are not directly observed in our infrared experiments.

cond-mat.mes-hall↗

arXiv2016

Tuning the valley and chiral quantum state of Dirac electrons in van der Waals heterostructures

Chirality is a fundamental property of electrons with the relativistic spectrum found in graphene and topological insulators. It plays a crucial role in relativistic phenomena, such as Klein tunneling, but it is difficult to visualize directly. Here we report the direct observation and manipulation of chirality and pseudospin polarization in the tunneling of electrons between two almost perfectly aligned graphene crystals. We use a strong in-plane magnetic field as a tool to resolve the contributions of the chiral electronic states that have a phase difference between the two components of their vector wavefunction. Our experiments not only shed light on chirality, but also demonstrate a technique for preparing graphene's Dirac electrons in a particular quantum chiral state in a selected valley.

cond-mat.mes-hall↗

arXiv2016

The hole Fermi surface in Bi$_{2}$Se$_{3}$ probed by quantum oscillations

Transport and torque magnetometry measurements are performed at high magnetic fields and low temperatures in a series of p-type (Ca-doped) Bi$_{2}$Se$_{3}$ crystals. The angular dependence of the Shubnikov-de Haas and de Haas-van Alphen quantum oscillations enables us to determine the Fermi surface of the bulk valence band states as a function of the carrier density. At low density, the angular dependence exhibits a downturn in the oscillations frequency between $0^\circ$ and $90^\circ$, reflecting a bag-shaped hole Fermi surface. The detection of a single frequency for all tilt angles rules out the existence of a Fermi surface with different extremal cross-sections down to $24$~meV. There is therefore no signature of a camel-back in the valence band of our bulk samples, in accordance with the direct band gap predicted by $GW$ calculations.

cond-mat.mes-hall↗