arXiv subjects

B. Canals

Publications and source records attributed to B. Canals.

At least 37 records · Page 2Linked to original sources

arXiv2014

Chiral nature of magnetic monopoles in artificial spin ice

Micromagnetic properties of monopoles in artificial kagome spin ice systems are investigated using numerical simulations. We show that micromagnetics brings additional complexity into the physics of these monopoles that is, by essence, absent in spin models: besides a fractionalized classical magnetic charge, monopoles in the artificial kagome ice are chiral at remanence. Our simulations predict that the chirality of these monopoles can be controlled without altering their charge state. This chirality breaks the vertex symmetry and triggers a directional motion of the monopole under an applied magnetic field. Our results also show that the choice of the geometrical features of the lattice can be used to turn on and off this chirality, thus allowing the investigation of chiral and achiral monopoles.

cond-mat.mes-hall↗

arXiv2013

Magnetic properties of a family of quinternary oxalates

We report on the magnetic properties of four isomorphous compounds of a family of quinternary oxalates down to 60 mK. In all these materials, the magnetic FeII ions with a strong magneto-crystalline anisotropy form a distorted kagome lattice, topologically equivalent to a perfect kagome one if nearest-neighbor interactions only are considered. All the compounds order at low temperature in an antiferromagnetic arrangement with magnetic moments at 120°. A remarkable magnetic behavior emerges below the Néel temperature in three compounds (with inter-kagome-layer Zr, Sn, Fe but not with Al): the spin anisotropy combined with a low exchange path network connectivity lead to domain walls intersecting the kagome planes through strings of free spins. These produce an unfamiliar slow spin dynamics in the ordered phase observed by AC susceptibility, evolving from exchange-released spin-flips towards a cooperative behavior on decreasing the temperature.

cond-mat.str-el↗

arXiv2013

Inhomogeneous magnetism in the doped kagome lattice of LaCuO2.66

The hole-doped kagome lattice of Cu2+ ions in LaCuO2.66 was investigated by nuclear quadrupole resonance (NQR), electron spin resonance (ESR), electrical resistivity, bulk magnetization and specific heat measurements. For temperatures above ~180 K, the spin and charge properties show an activated behavior suggestive of a narrow-gap semiconductor. At lower temperatures, the results indicate an insulating ground state which may or may not be charge ordered. While the frustrated spins in remaining patches of the original kagome lattice might not be directly detected here, the observation of coexisting non-magnetic sites, free spins and frozen moments reveals an intrinsically inhomogeneous magnetism. Numerical simulations of a 1/3-diluted kagome lattice rationalize this magnetic state in terms of a heterogeneous distribution of cluster sizes and morphologies near the site-percolation threshold.

cond-mat.str-el↗

arXiv2012

Heterogeneous freezing in a geometrically frustrated spin model without disorder: spontaneous generation of two time-scales

By considering the constrained motion of classical spins in a geometrically frustrated magnet, we find a dynamical freezing temperature below which the system gets trapped in metastable states with a "frozen" moment and dynamical heterogeneities. The residual collective degrees of freedom are strongly correlated, and by spontaneously forming aggregates, they are unable to reorganize the system. The phase space is then fragmented in a macroscopic number of disconnected sectors (broken ergodicity), resulting in self-induced disorder and "thermodynamic" anomalies, measured by the loss of a finite configurational entropy. We discuss these results in the view of experimental results on the kagome compounds, SrCr(9p)Ga(12-9p)O19, (H30)Fe3(SO4)2(OH)6, Cu3V2O7(OH)2.2H2O and Cu3BaV2O8(OH)2.

cond-mat.str-el↗

arXiv2012

Domain Wall Spin Dynamics in Kagome Antiferromagnets

We report magnetization and neutron scattering measurements down to 60 mK on a new family of Fe based kagome antiferromagnets, in which a strong local spin anisotropy combined with a low exchange path network connectivity lead to domain walls intersecting the kagome planes through strings of free spins. These produce unfamiliar slow spin dynamics in the ordered phase, evolving from exchange-released spin-flips towards a cooperative behavior on decreasing the temperature, probably due to the onset of long-range dipolar interaction. A domain structure of independent magnetic grains is obtained that could be generic to other frustrated magnets.

cond-mat.str-el↗

arXiv2011

Graphene in periodically alternating magnetic field: unusual quantization of the anomalous Hall effect

We study the energy spectrum and electronic properties of graphene in a periodic magnetic field of zero average with a symmetry of triangular lattice. The periodic field leads to formation of a set of minibands separated by gaps, which can be manipulated by external field. The Berry phase, related to the motion of electrons in $k$ space, and the corresponding Chern numbers characterizing topology of the energy bands are calculated analytically and numerically. In this connection, we discuss the anomalous Hall effect in the insulating state, when the Fermi level is located in the minigap. The results of calculations show that in the model of gapless Dirac spectrum of graphene the anomalous Hall effect can be treated as a sum of fractional quantum numbers, related to the nonequivalent Dirac points.

cond-mat.mtrl-sci↗

arXiv2011

Artificial Kagome Arrays of Nanomagnets: A Frozen Dipolar Spin Ice

Magnetic frustration effects in artificial kagome arrays of nanomagnets are investigated using x-ray photoemission electron microscopy and Monte Carlo simulations. Spin configurations of demagnetized networks reveal unambiguous signatures of long range, dipolar interaction between the nanomagnets. As soon as the system enters the spin ice manifold, the kagome dipolar spin ice model captures the observed physics, while the short range kagome spin ice model fails.

cond-mat.mes-hall↗

arXiv2009

Voltage induced control and magnetoresistance of noncollinear frustrated magnets

Noncollinear frustrated magnets are proposed as a new class of spintronic materials with high magnetoresistance which can be controlled with relatively small applied voltages. It is demonstrated that their magnetic configuration strongly depends on position of the Fermi energy and applied voltage. The voltage induced control of noncollinear frustrated materials (VCFM) can be seen as a way to intrinsic control of colossal magnetoresistance (CMR) and is the bulk material counterpart of spin transfer torque concept used to control giant magnetoresistance in layered spin-valve structures.

cond-mat.mtrl-sci↗

arXiv2008

Propagation and Ghosts in the Classical Kagome Antiferromagnet

We investigate the classical spin dynamics of the kagome antiferromagnet by combining Monte Carlo and spin dynamics simulations. We show that this model has two distinct low temperature dynamical regimes, both sustaining propagative modes. The expected gauge invariance type of the low energy low temperature out of plane excitations is also evidenced in the non linear regime. A detailed analysis of the excitations allows to identify ghosts in the dynamical structure factor, i.e propagating excitations with a strongly reduced spectral weight. We argue that these dynamical extinction rules are of geometrical origin.

cond-mat.str-el↗

arXiv2006

Subtle competition between ferromagnetic and antiferromagnetic order in a Mn(II) - free radical ferrimagnetic chain

The macroscopic magnetic characterization of the Mn(II) - nitronyl nitroxide free radical chain (Mn(hfac)2(R)-3MLNN) evidenced its transition from a 1-dimensional behavior of ferrimagnetic chains to a 3-dimensional ferromagnetic long range order below 3 K. Neutron diffraction experiments, performed on a single crystal around the transition temperature, led to a different conclusion : the magnetic Bragg reflections detected below 3 K correspond to a canted antiferromagnet where the magnetic moments are mainly oriented along the chain axis. Surprisingly in the context of other compounds in this family of magnets, the interchain coupling is antiferromagnetic. This state is shown to be very fragile since a ferromagnetic interchain arrangement is recovered in a weak magnetic field. This peculiar behavior might be explained by the competition between dipolar interaction, shown to be responsible for the antiferromagnetic long range order below 3 K, and exchange interaction, the balance between these interactions being driven by the strong intrachain spin correlations. More generally, this study underlines the need, in this kind of molecular compounds, to go beyond macroscopic magnetization measurements.

cond-mat.mtrl-sci↗

arXiv2006

Magnetic Frustration on a Kagomé Lattice in R$\_{3}$Ga$\_{5}$SiO$\_{14}$ Langasites with R = Nd, Pr

In the R$\_{3}$Ga$\_{5}$SiO$\_{14}$ compounds, the network R of rare earth cations form well separated planes of corner sharing triangles topologically equivalent to a kagomé lattice. Powder samples and single crystals with R = Nd and Pr were prepared and magnetostatic measurements were performed under magnetic field up to 10 T in the temperature range from 1.6 K to 400 K. Analysis of the magnetic susceptibility at the high temperatures where only the quadrupolar term of the crystal electric field prevails, suggests that the Nd and Pr magnetic moments can be modeled as coplanar elliptic rotators perpendicular to the three fold axis of the crystal structure that interact antiferromagnetically. Nonetheless, a disordered phase that can be ascribed to geometric frustration persists down to the lowest temperature which is about 25 times smaller than the energy scale for the exchange interactions.

cond-mat.str-el↗

arXiv2006

Magnetic ordering in Gd2Sn2O7: the archetypal Heisenberg pyrochlore antiferromagnet

Low-temperature powder neutron diffraction measurements are performed in the ordered magnetic state of the pyrochlore antiferromagnet Gd2Sn2O7. Symmetry analysis of the diffraction data indicates that this compound has the ground state predicted theoretically for a Heisenberg pyrochlore antiferromagnet with dipolar interactions. The difference in magnetic structures of Gd2Sn2O7 and of nominally analogous Gd2Ti2O7 is found to be determined by a specific type of third-neighbor superexchange interaction on the pyrochlore lattice between spins across empty hexagons.

cond-mat.mtrl-sci↗

arXiv2005

Ordering in the pyrochlore antiferromagnet due to Dzyaloshinsky-Moriya interactions

The Heisenberg nearest neighbour antiferromagnet on the pyrochlore (3D) lattice is highly frustrated and does not order at low temperature where spin-spin correlations remain short ranged. Dzyaloshinsky-Moriya interactions (DMI) may be present in pyrochlore compounds as is shown, and the consequences of such interactions on the magnetic properties are investigated through mean field approximation and monte carlo simulations. It is found that DMI (if present) tremendously change the low temperature behaviour of the system. At a temperature of the order of the DMI a phase transition to a long range ordered state takes place. The ordered magnetic structures are explicited for the different possible DMI which are introduced on the basis of symmetry arguments. The relevance of such a scenario for pyrochlore compounds in which an ordered magnetic structure is observed experimentally is dicussed.

cond-mat.str-el↗

arXiv2005

Berry phase of magnons in textured ferromagnets

We study the energy spectrum of magnons in a ferromagnet with topologically nontrivial magnetization profile. In the case of inhomogeneous magnetization corresponding to a metastable state of ferromagnet, the spin-wave equation of motion acquires a gauge potential leading to a Berry phase for the magnons propagating along a closed contour. The effect of magnetic anisotropy is crucial for the Berry phase: we show that the anisotropy suppresses its magnitude, which makes the Berry phase observable in some cases, similar to the Aharonov-Bohm effect for electrons. For example, it can be observed in the interference of spin waves propagating in mesoscopic rings. We discuss the effect of domain walls on the interference in ferromagnetic rings, and propose some experiments with a certain geometry of magnetization. We also show that the nonvanishing average topological field acts on the magnons like a uniform magnetic field on electrons. It leads to the quantization of the magnon spectrum in the topological field.

cond-mat.mtrl-sci↗

arXiv2005

Anomalous Hall effect in a two-dimensional electron gas with spin-orbit interaction

We discuss the mechanism of anomalous Hall effect related to the contribution of electron states below the Fermi surface (induced by the Berry phase in momentum space). Our main calculations are made within a model of two-dimensional electron gas with spin-orbit interaction of the Rashba type, taking into account the scattering from impurities. We demonstrate that such an "intrinsic" mechanism can dominate but there is a competition with the impurity-scattering mechanism, related to the contribution of states in the vicinity of Fermi surface. We also show that the contribution to the Hall conductivity from electron states close to the Fermi surface has the intrinsic properties as well.

cond-mat.mtrl-sci↗

arXiv2003

XY checkerboard antiferromagnet in external field

Ordering by thermal fluctuations is studied for the classical XY antiferromagnet on a checkerboard lattice in zero and finite magnetic fields by means of analytical and Monte Carlo methods. The model exhibits a variety of novel broken symmetries including states with nematic ordering in zero field and with triatic order parameter at high fields.

cond-mat.str-el↗

arXiv2002

Green's function approach to the magnetic properties of the kagome antiferromagnet

The $S=1/2$ Heisenberg antiferromagnet is studied on the kagomé lattice by using a Green's function method based on an appropriate decoupling of the equations of motion. Thermodynamic properties as well as spin-spin correlation functions are obtained and characterize this system as a two-dimensional quantum spin liquid. Spin-spin correlation functions decay exponentially with distance down to low temperature and the calculated missing entropy at T=0 is found to be $0.46\ln{2}$. Within the present scheme, the specific heat exhibits a single peak structure and a $T^2$ dependence at low temperature.

cond-mat.str-el↗

arXiv2002

Symmetry breaking due to Dzyaloshinsky-Moriya interactions in the kagome lattice

Due to the particular geometry of the kagomé lattice, it is shown that antisymmetric Dzyaloshinsky-Moriya interactions are allowed and induce magnetic ordering. The symmetry of the obtained low temperature magnetic phases are studied through mean field approximation and classical Monté Carlo simulations. A phase diagram relating the geometry of the interaction and the ordering temperature has been derived. The order of magnitude of the anisotropies due to Dzyaloshinsky-Moriya interactions are more important than in non-frustrated magnets, which enhances its appearance in real systems. Application to the jarosites compounds is proposed. In particular, the low temperature behaviors of the Fe and Cr-based jarosites are correctly described by this model.

cond-mat.str-el↗