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Baigeng Wang

Publications and source records attributed to Baigeng Wang.

At least 55 records · Page 3Linked to original sources

D-wave superconductivity induced by proximity to the non-uniform chiral spin liquid on a square lattice

We use the tensor network algorithm to show evidences of a non-uniform chiral spin-liquid (CSL) ground state in a frustrated spin-1/2 model on a square lattice, in the regime of moat-like band structure of the lattice, i.e., a band with infinitely degenerate energy minima attained along a closed contour in the Brillouin zone. The analytical description of the state is given by the effective field theory of a topological square-lattice fermionic Chern insulator coupled to the Chern-Simons gauge field. The observed non-uniform CSL has a substantial effect on a nearby free-fermion environment. We show that, in the presence of arbitrarily small spin exchange interaction, the CSL can endow a gauge-field-modulated effective interaction between the environmental fermions. The induced effective interaction can be attractive within a significant parameter region, leading to an instability towards d-wave superconductivity in the fermionic bath.

cond-mat.str-el↗

Emergence of excitonic superfluid at topological-insulator surfaces

Excitons are spin integer particles that are predicted to condense into a coherent quantum state at sufficiently low temperature, and exciton condensates can be realized at much higher temperature than condensates of atoms because of strong Coulomb binding and small mass. Signatures of exciton condensation have been reported in double quantum wells1-4, microcavities5, graphene6, and transition metal dichalcogenides7. Nonetheless, transport of exciton condensates is not yet understood and it is unclear whether an exciton condensate is a superfluid8,9 or an insulating electronic crystal10,11. Topological insulators (TIs) with massless particles and unique spin textures12 have been theoretically predicted13 as a promising platform for achieving exciton condensation. Here we report experimental evidence of excitonic superfluid phase on the surface of three-dimensional (3D) TIs. We unambiguously confirmed that electrons and holes are paired into charge neutral bound states by the electric field independent photocurrent distributions. And we observed a millimetre-long transport distance of these excitons up to 40 K, which strongly suggests dissipationless propagation. The robust macroscopic quantum states achieved with simple device architecture and broadband photoexcitation at relatively high temperature are expected to find novel applications in quantum computations and spintronics.

cond-mat.mes-hall↗

Oscillating planar Hall response from the surface electrons in bulk crystal Sn doped Bi1.1Sb0.9Te2S

We report the low-temperature magneto-transport in the bulk-insulating single crystal of topological insulator Sn doped Bi1.1Sb0.9Te2S. The Shubnikov-de Haas oscillations appear with their reciprocal frequency proportional to cos/theta , demonstrating the dominant transport of topological surface states. While the magnetic field is rotating in the sample surface, the planar Hall effect arises with sizeable oscillations following a relation of cos/theta sin/theta . Its amplitude reaches the maximum at the lowest temperature and drops to nearly zero at the temperature higher than 100 K. All these evidences consolidate such planar Hall oscillations as a new golden criterion on the topological surface transport.

cond-mat.mes-hall↗

Antiferromagnetic magnons from fractionalized excitations

We develop an approach to describe antiferromagnetic magnons on a bipartite lattice supporting the Néel state using fractionalized degrees of freedom typically inherent to quantum spin liquids. In particular we consider a long-range magnetically ordered state of interacting two-dimensional quantum spin$-1/2$ models using the Chern-Simons (CS) fermion representation of interacting spins. The interaction leads to Cooper instability and pairing of CS fermions, and to CS superconductivity which spontaneously violates the continuous $\mathrm{U}(1)$ symmetry generating a linearly-dispersing gapless Nambu-Goldstone mode due to phase fluctuations. We evaluate this mode and show that it is in high-precision agreement with magnons of the corresponding Néel antiferromagnet irrespective to the lattice symmetry. Using the fermion formulation of a system with competing interactions, we show that the frustration gives raise to nontrivial long-range four, six, and higher-leg interaction vertices mediated by the CS gauge field, which are responsible for restoring of the continuous symmetry at sufficiently strong frustration. We identify these new interaction vertices and discuss their implications to unconventional phase transitions. We also apply the proposed theory to a model of anyons that can be tuned continuously from fermions to bosons.

cond-mat.str-el↗

Topological Phase Transition-Induced Tri-Axial Vector Magnetoresistance in (Bi1-xInx)2Se3 Nanodevices

We report the study of a tri-axial vector magnetoresistance (MR) in nonmagnetic (Bi1-xInx)2Se3 nanodevices at the composition of x = 0.08. We show a dumbbell-shaped in-plane negative MR up to room temperature as well as a large out-of-plane positive MR. MR at three directions is about in a -3%: -1%: 225% ratio at 2 K. Through both the thickness and composition-dependent magnetotransport measurements, we show that the in-plane negative MR is due to the topological phase transition enhanced intersurface coupling near the topological critical point. Our devices suggest the great potential for room-temperature spintronic applications, for example, vector magnetic sensors.

physics.app-ph↗

Robust memristors based on layered two-dimensional materials

Van der Waals heterostructure based on layered two-dimensional (2D) materials offers unprecedented opportunities to create materials with atomic precision by design. By combining superior properties of each component, such heterostructure also provides possible solutions to address various challenges of the electronic devices, especially those with vertical multilayered structures. Here, we report the realization of robust memristors for the first time based on van der Waals heterostructure of fully layered 2D materials (graphene/MoS2-xOx/graphene) and demonstrate a good thermal stability lacking in traditional memristors. Such devices have shown excellent switching performance with endurance up to 107 and a record-high operating temperature up to 340oC. By combining in situ high-resolution TEM and STEM studies, we have shown that the MoS2-xOx switching layer, together with the graphene electrodes and their atomically sharp interfaces, are responsible for the observed thermal stability at elevated temperatures. A well-defined conduction channel and a switching mechanism based on the migration of oxygen ions were also revealed. In addition, the fully layered 2D materials offer a good mechanical flexibility for flexible electronic applications, manifested by our experimental demonstration of a good endurance against over 1000 bending cycles. Our results showcase a general and encouraging pathway toward engineering desired device properties by using 2D van der Waals heterostructures.

cond-mat.mtrl-sci↗

Diagnosing the magnetic field-tuned symmetry nature of the topological electrons by conductance fluctuations in bulk-insulating BiSbTeSe2 devices

We extract the quantum conductance fluctuations and study its magnetic field dependence in the gate-dependent transport of the topological electrons in bulk-insulating BiSbTeSe2 devices. While increasing the magnetic field from 0 to 12 Tesla, the fluctuation magnitudes are found reduced by a ratio of sqrt(2) and form a quantized step. The step is observed both in n-type and p-type transport. It is also confirmed in the nonlocal measurements. This essentially demonstrates the breaking of the time reversal symmetry of the three-dimensional Z2 topological insulators.

cond-mat.mes-hall↗

Approaching the Type-II Dirac Point and Concomitant Superconductivity in Pt-doping Stabilized Metastable 1T-phase IrTe2

Topological semimetal is a topic of general interest in material science. Recently, a new kind of topological semimetal called type-II Dirac semimetal with tilted Dirac cones is discovered in PtSe2 family. However, the further investigation is hindered due to the huge energy difference from Dirac points to Fermi level and the irrelevant conducting pockets at Fermi surface. Here we characterize the optimized type-II Dirac dispersions in a metastable 1T phase of IrTe2. Our strategy of Pt doping protects the metastable 1T phase in low temperature and tunes the Fermi level to the Dirac point. As demonstrated by angle-resolved photoemission spectra and first principle calculations, the Fermi surface of Ir1-xPtxTe2 is formed by only a single band with type-II Dirac cone which is tilted strongly along kz momentum direction. Interesting superconductivity is observed in samples for Dirac point close to Fermi level and even survives when Fermi level aligns with the Dirac point as finite density of states created by the tilted cone dispersion. This advantage offers opportunities for possible topological superconductivity and versatile Majorana devices in type-II Dirac semimetals.

cond-mat.mtrl-sci↗

Gated Tuned Superconductivity and Phonon Softening in Mono- and Bilayer MoS$_2$

Superconductors at the atomic two-dimensional (2D) limit are the focus of an enduring fascination in the condensed matter community. This is because, with reduced dimensions, the effects of disorders, fluctuations, and correlations in superconductors become particularly prominent at the atomic 2D limit; thus such superconductors provide opportunities to tackle tough theoretical and experimental challenges. Here, based on the observation of ultrathin 2D superconductivity in mono- and bilayer molybdenum disulfide (MoS$_2$) with electric-double-layer (EDL) gating, we found that the critical sheet carrier density required to achieve superconductivity in a monolayer MoS$_2$ flake can be as low as 0.55*10$^{14}$cm$^{-2}$, which is much lower than those values in the bilayer and thicker cases in previous report and also our own observations. Further comparison of the phonon dispersion obtained by ab initio calculations indicated that the phonon softening of the acoustic modes around the M point plays a key role in the gate-induced superconductivity within the Bardeen-Cooper Schrieffer (BCS) theory framework. This result might help enrich the understanding of 2D superconductivity with EDL gating.

cond-mat.mes-hall↗

Possible particle-hole instabilities in interacting type-II Weyl semimetals

Type II Weyl semimetal, a three dimensional gapless topological phase, has drawn enormous interest recently. These topological semimetals enjoy overtilted dispersion and Weyl nodes that separate the particle and hole pocket. Using perturbation renormalization group, we identify possible renormalization of the interaction vertices, which show a tendency toward instability. We further adopt a self-consistent mean-field approach to study possible instability of the type II Weyl semimetals under short-range electron-electron interaction. It is found that the instabilities are much easier to form in type II Weyl semimetals than the type I case. Eight different mean-field orders are identified, among which we further show that the polar charge density wave (CDW) phase exhibits the lowest energy. This CDW order is originated from the nesting of the Fermi surfaces and could be a possible ground state in interacting type II Weyl semimetals.

cond-mat.str-el↗

The study on quantum material WTe2

WTe2 and its sister alloys have attracted tremendous attentions recent years due to the large non-saturating magnetoresistance and topological non-trivial properties. Herein, we briefly review the electrical property studies on this new quantum material.

cond-mat.mtrl-sci↗

Stepwise quantized surface states and delayed Landau level hybridization in Co cluster-decorated BiSbTeSe2 topological insulator devices

In three-dimensional topological insulators (TIs), the nontrivial topology in their electronic bands casts a gapless state on their solid surfaces, using which dissipationless TI edge devices based on the quantum anomalous Hall (QAH) effect and quantum Hall (QH) effect have been demonstrated. Practical TI devices present a pair of parallel-transport topological surface states (TSSs) on their top and bottom surfaces. However, due to the no-go theorem, the two TSSs always appear as a pair and are expected to quantize synchronously. Quantized transport of a separate Dirac channel is still desirable, but has never been observed in graphene even after intense investigation over a period of 13 years, with the potential aim of half-QHE. By depositing Co atomic clusters, we achieved stepwise quantization of the top and bottom surfaces in BiSbTeSe2 (BSTS) TI devices. Renormalization group flow diagrams13, 22 (RGFDs) reveal two sets of converging points (CVPs) in the (Gxy, Gxx) space, where the top surface travels along an anomalous quantization trajectory while the bottom surface retains 1/2 e2/h. This results from delayed Landau-level (LL) hybridization (DLLH) due to coupling between Co clusters and TSS Fermions.

cond-mat.mes-hall↗

Nontrivial Berry phase and type II Dirac transport in layered material PdTe2

Here we report the evidence of the type II Dirac Fermion in the layered crystal PdTe2. The de Haas-van Alphen oscillations find a small Fermi pocket with a cross section of 0.077nm-2 with a nontrivial Berry phase. First-principal calculations reveal that it is originated from the hole pocket of a tilted Dirac cone. Angle Resolved Photoemission Spectroscopy demonstrates a type II Dirac cone featured dispersion. We also suggest PdTe2 is an improved platform to host the topological superconductors.

cond-mat.mes-hall↗

Topological Weyl phase transition in Mo$_x$W$_{1-x}$Te$_2$

Topological phases of matter exhibit phase transitions between distinct topological classes. These phase transitions are exotic in that they do not fall within the traditional Ginzburg-Landau paradigm but are instead associated with changes in bulk topological invariants and associated topological surface states. In the case of a Weyl semimetal this phase transition is particularly unusual because it involves the creation of bulk chiral charges and the nucleation of topological Fermi arcs. Here we image a topological phase transition to a Weyl semimetal in Mo$_x$W$_{1-x}$Te$_2$ with changing composition $x$. Using pump-probe ultrafast angle-resolved photoemission spectroscopy (pump-probe ARPES), we directly observe the nucleation of a topological Fermi arc at $x_c \sim 7\%$, showing the critical point of a topological Weyl phase transition. For Mo dopings $x < x_c$, we observe no Fermi arc, while for $x > x_c$, the Fermi arc gradually extends as the bulk Weyl points separate. Our results demonstrate for the first time the creation of magnetic monopoles in momentum space. Our work opens the way to manipulating chiral charge and topological Fermi arcs in Weyl semimetals for transport experiments and device applications.

cond-mat.mtrl-sci↗

Spinon Majorana fermions

A realization of Majorana fermions is proposed in the frustrated magnets via the topological proximity effect. Specifically, we consider a theoretical model, where a topological insulator is coupled to a frustrated magnetic material through the spin exchange interaction. Using the renormalization group-based self-consistent mean-field approach, and calculating the self-energy correction due to the topological insulator, we find that the spin texture and the spin-momentum locking of the Dirac cone will be inherited by the spinons in the nearby frustrated magnets. This leads to a particular topological state of matter that supports the Majorana excitations. Unlike the conventional realization in SC systems, these Majorana fermions are the combination of spinons and anti-spinons, rather than electrons and holes. They can participate in the transport of spinons, leading to nontrivial properties of the spin transport.

cond-mat.str-el↗

Gate-Tunable Negative Longitudinal Magnetoresistance in the Predicted Type-II Weyl Semimetal WTe2

The progress in exploiting new electronic materials and devices has been a major driving force in solid-state physics. As a new state of matter, a Weyl semimetal (WSM), particularly a type-II WSM, hosts Weyl fermions as emergent quasiparticles and may harbor novel electrical transport properties because of the exotic Fermi surface. Nevertheless, such a type-II WSM material has not been experimentally observed in nature. In this work, by performing systematic magneto-transport studies on thin films of a predicted material candidate WTe2, we observe notable angle-sensitive (between the electric and magnetic fields) negative longitudinal magnetoresistance (MR), which can likely be attributed to the chiral anomaly in WSM. This phenomenon also exhibits strong planar orientation dependence with the absence of negative longitudinal MR along the tungsten chains (a axis), which is consistent with the distinctive feature of a type-II WSM. By applying a gate voltage, we demonstrate that the Fermi energy can be tuned through the Weyl points via the electric field effect; this is the first report of controlling the unique transport properties in situ in a WSM system. Our results have important implications for investigating simulated quantum field theory in solid-state systems and may open opportunities for implementing new types of electronic applications, such as field-effect chiral electronic devices.

cond-mat.mes-hall↗

Measuring Chern numbers above the Fermi level in the Type II Weyl semimetal Mo$_x$W$_{1-x}$Te$_2$

It has recently been proposed that electronic band structures in crystals give rise to a previously overlooked type of Weyl fermion, which violates Lorentz invariance and, consequently, is forbidden in particle physics. It was further predicted that Mo$_x$W$_{1-x}$Te$_2$ may realize such a Type II Weyl fermion. One crucial challenge is that the Weyl points in Mo$_x$W$_{1-x}$Te$_2$ are predicted to lie above the Fermi level. Here, by studying a simple model for a Type II Weyl cone, we clarify the importance of accessing the unoccupied band structure to demonstrate that Mo$_x$W$_{1-x}$Te$_2$ is a Weyl semimetal. Then, we use pump-probe angle-resolved photoemission spectroscopy (pump-probe ARPES) to directly observe the unoccupied band structure of Mo$_x$W$_{1-x}$Te$_2$. For the first time, we directly access states $> 0.2$ eV above the Fermi level. By comparing our results with $\textit{ab initio}$ calculations, we conclude that we directly observe the surface state containing the topological Fermi arc. Our work opens the way to studying the unoccupied band structure as well as the time-domain relaxation dynamics of Mo$_x$W$_{1-x}$Te$_2$ and related transition metal dichalcogenides.

cond-mat.mes-hall↗

Evidence of both surface and bulk Dirac bands in ZrSiS and the unconventional magnetoresistance

The unconventional magnetoresistance of ZrSiS single crystals is found unsaturated till the magnetic field of 53 T with the butterfly shaped angular dependence. Intense Shubnikov-de Haas oscillations resolve a bulk Dirac cone with a nontrivial Berry phase, where the Fermi surface area is 1.80*10^-3 Å-2 and reaches the quantum limit before 20 T. Angle resolved photoemission spectroscopy measurement reveals an electronic state with the two-dimensional nature around the X point of Brillouin zone boundary. By integrating the density functional theory calculations, ZrSiS is suggested to be a Dirac material with both surface and bulk Dirac bands.

cond-mat.mtrl-sci↗