arXiv subjects

Bao-Sen Shi

Publications and source records attributed to Bao-Sen Shi.

At least 37 records · Page 2Linked to original sources

arXiv2025

Cavity-enhanced symmetric second-harmonic generation

As one of the two types of backward second-harmonic generation (SHG), symmetric SHG exhibits some physical characteristics and application prospects that are distinct from those of forward SHG. It is generally realized through quasi-phase matching, which imposes more stringent requirements on the poling period and thus presents challenges for domain engineering. Although employing larger poling periods can ease fabrication, it inevitably reduces conversion efficiency, a drawback that can be compensated by using a cavity. In this work, we employed a semi-monolithic cavity to enhance the efficiency of 7th-order symmetric SHG, achieving a measured one-sided conversion efficiency of 7.2 %, which corresponds to a theoretical total efficiency of 14.4 %. This represents an improvement of more than three orders of magnitude compared with the single-pass case. In addition, the nonlinear coefficient of the crystal of ${d_{33}} = 4.8$ $\rm pm/V$ was estimated.

physics.optics↗

arXiv2025

Quantum synchronization at the critical point of Floquet driven Rydberg atoms

The criticality enhanced correlations and susceptibility allow weak periodic driving to induce collective synchronization due to critical slowing down, providing a unique platform to study non-equilibrium order emergence. This establishes a powerful paradigm for investigating non-equilibrium order formation, yet the fundamental mechanisms of critical-point synchronization remain poorly understood. Here, we utilize a microwave pulse as a seed to induce quantum synchronization at the critical point of Floquet driven Rydberg atoms. In the experiment, the microwave periodic driving on Rydberg states acts as a seeded temporal order in subspace, which triggers synchronization across the entire ensemble. The behavior of the emergent synchronized oscillation is elaborately linked to alterations in the seed, such as the relative phase shift and the frequency difference, which result in phase-dependent seeding and embryonic synchronization. This result opens up new possibilities for studying and harnessing time-dependent quantum many-body phenomena, offering insight into the behavior of complex many-body systems under seeding.

cond-mat.quant-gas↗

arXiv2025

Fragmented quantum phases in anti-blockade regime of Rydberg atom array

In this Letter, we report a parameter-dependent Hilbert space fragmentation in a one-dimensional Rydberg atom array under anti-blockade conditions. We identify distinct non-equilibrium dynamical phases and show that their quasi-periodic behavior arises from the interplay of multi-path interference and multi-photon cascaded excitations, reflecting fundamental differences in state connectivity and effective dimensionality. By constructing a complete phase diagram, we reveal the transition from thermalization to fragmentation, and further demonstrate a secondary fragmentation process enabled by local constraints. Our results highlight the potential of anti-blockade mechanisms for programmable non-thermal dynamics in many-body systems.

quant-ph↗

arXiv2025

Generation of Near-ideal Indistinguishable Two-Photon State by Incoherent Light

High-quality quantum states lie at the heart of advanced quantum information processing. The degree of photon indistinguishability is critical for applications from photonic quantum computation to precision metrology. The two-photon Hong-Ou-Mandel (HOM) interference effect provides a rigorous quantification method, with its visibility serving as the ultimate benchmark for source quality. Generally, the coherent pumping is widely regarded as indispensable for the preparation of quantum sources. As a result, incoherent light sources have seen limited applications in the current quantum technologies. In this work, we generate an indistinguishable two-photon state by incoherent light generated by frequency doubling of Amplified Spontaneous Emission light. The theoretical analysis indicates that phase randomization of the pumping does not affect the coincidence visibility in two-photon intensity interference. Moreover, temporal incoherence further enhances the symmetry of the generated spectrum in second-harmonic generation. In the experiment, the incoherently pumped photon sources exhibit a heralding efficiency of approximately 60\% and a coincidence-to-accidental ratio exceeding 15000. The observed HOM interference fringes show the visibility of 99.1\% without any spectrum filtering, confirming the near-ideal indistinguishability of the photons. Our study reveals the role of temporal coherence in second-order nonlinear interactions, it provide a potential approach to use an easily accessible incoherent light for engineering high-quality quantum sources.

quant-ph↗

arXiv2025

All-optical convolution utilizing processing in memory based on a cold atomic ensemble

Processing in memory (PIM) has received significant attention due to its high efficiency, low latency, and parallelism. In optical computation, coherent memory is a crucial infrastructure for PIM frameworks. This study presents an all-optical convolution experiment conducted within computational storage based on a cold atomic ensemble. By exploiting the light-atom phase transfer facilitated by the electromagnetically induced transparency, we demonstrated spiral phase contrast processing of photon images in memory, resulting in the edge enhancement of retrieved images recorded using time-correlated photon imaging. In particular, adopting state-of-the-art atomic techniques provides a coherent memory lifetime exceeding 320 us for PIM operations. Our results highlight the significant potential of cold atomic ensembles as computational storage for developing all-optical PIM systems.

physics.app-ph↗

arXiv2025

High resolution up-conversion imaging in the 10 μm band under incoherent illumination

Long-wavelength infrared band exhibits significant utility in thermal signature acquisition and molecular spectral analysis, among other applications. The up-conversion detection technique enables effective signal transduction into the detection bandwidth of silicon-based photodetectors, thereby facilitating high-sensitivity photonic measurements. We realized high-resolution up-conversion imaging for incoherent thermal targets in the 10 μm spectral regime for the first time. Furthermore, this work presents the first derivation of analytical models characterizing depth of field and astigmatic aberration in up-conversion imaging systems, which show excellent agreement between theoretical and experimental results. The results demonstrate generalisability to various up-conversion imaging systems, thus providing critical insights for the design and optimisation of such systems.

physics.optics↗

arXiv2025

On Chip Quantum States Generation by Incoherent Light

On-chip quantum sources based on nonlinear processes are pivotal components in integrated photonics, driving significant advancements in quantum information technologies over recent decades. Usually, the pump coherence has been considered to be crucial for ensuring the quality of generated states, therefore incoherent light is rarely used in quantum information processing. In this work, we explore and reveal the constructive influence of pumped temporal incoherence on the quantum properties of photon sources. Taking silicon waveguides as nonlinear media, we theoretically show that temporal incoherence of light can improve pumping utilization efficiency, resulting in higher source brightness in a spontaneous four-wave mixing process, and the spectrally uncorrelated nature of incoherent light is transferred to the generated photon source, allowing high-purity state preparation. Experimentally, we obtain a higher photon pair generation rate and the lower heralded second-order autocorrelation with an Amplified Spontaneous Emission source. Additionally, we successfully generate a polarization-entangled state with Bell inequality violation of S = 2.64 and a fidelity of 95.7%. Our study reveals the mechanism behind incoherently pumped quantum states and presents a method for generating photon sources using an easily accessible incoherent light.

quant-ph↗

arXiv2025

An all optical broadband tunable quantum frequency shifter

A frequency shifter of the photon is a key component for frequency-multiplexed high-capacity quantum communications and frequency-encoded quantum computation. Existed methods for shifting the frequency of a photon based on electro-optical, or acousto-optical effect, however, suffer the limited frequency shift up to a few hundreds of GHz, furthermore, high-quality micro-wave electronics are required. The frequency of a photon can also be shifted with the frequency difference equal to the frequency of pump laser by using an all optical-wave-mixing approach, which is usually about tens of THz. So, there is a big frequency shifting gap between these methods. Here, we propose a new scheme of a quantum frequency shifter based on an all-optical wave-mixing process, which can theoretically achieve a frequency shift ranging from GHz to a few THz, therefore bridging the gap. As a principle of poof, by using two pump beams in a three-wave mixing cascading process, a heralded single photon is frequency-shifted more than 400GHz, and the shift can be tuned continuously over broadband by changing the frequency difference between two pump lasers. Besides, high coincidence to accidence ratio between the shifted photons and the heralded photon indicates the preserve of quantum properties. The present quantum frequency shifter is in analog to an electro-optical based shifter, but with much broader tuning ability. Our all-optical quantum frequency shifter will become a fundamental building block for high-speed quantum communication networks and frequency domain photonic quantum computation.

quant-ph↗

arXiv2025

Diatomic and Polyatomic Heteronuclear Ultralong-Range Rydberg Molecules

Ultra-long-range Rydberg molecules (ULRMs) have attracted significant interest due to their unique electronic properties and potential applications in quantum technologies. We theoretically investigate the formation and characteristics of heteronuclear ULRMs, focusing on Rb-Cs systems. We explore the vibrational energy levels of heteronuclear nD ULRMs and compare them with homonuclear counterparts. We also predict the formation of polyatomic heteronuclear ULRMs, discussing how the binding energy and spectral features evolve as the number of ground-state atoms increases. Our theoretical predictions are presented in terms of molecular spectra and provide insight into the formation dynamics of these systems. The study further explores the potential applications of heteronuclear ULRMs in quantum information processing, quantum simulation, and precision measurements, offering new avenues for future research in many-body physics and quantum technologies.

quant-ph↗

arXiv2024

A Rb-Cs dual-species magneto-optical trap

We describe a three-dimensional (3D) magneto-optical trap (MOT) capable of simultaneously capturing 85Rb and 133Cs atoms. Unlike conventional setups, our system utilizes two separate laser systems that are combined before entering the vacuum chamber, enabling the simultaneous trapping of two different atomic species. Additionally, in our 3D MOT configuration, two (of three) pairs of laser beams are not orthogonal to the chamber surfaces but are aligned at a 45° angle. With a total trapping laser power of 8 mW and repump laser power of 4 mW for Rb atoms, and a total trapping laser power of 7.5 mW and repump laser power of 1.5 mW for Cs atoms, we achieve optical depths (OD) of 3.71 for Rb and 3.45 for Cs, demonstrating efficient trapping for both species. Our 3D MOT setup allows full horizontal optical access to the trapped atomic ensembles without spatial interference from the trapping or repump laser beams. Moreover, the red detuning for trapping both atomic species is smaller than in traditional configurations. This system offers a versatile platform for exploring complex phenomena in ultracold atom physics, such as Rydberg molecule formation and interspecies interactions.

physics.atom-ph↗

arXiv2024

Folded multistability and hidden critical point in microwave-driven Rydberg atoms

The interactions between Rydberg atoms and microwave fields provide a valuable framework for studying the complex dynamics out of equilibrium, exotic phases, and critical phenomena in many-body physics. This unique interplay allows us to explore various regimes of nonlinearity and phase transitions. Here, we observe a phase transition from the state in the regime of bistability to that in multistability in strongly interacting Rydberg atoms by varying the microwave field intensity, accompanying with the breaking of Z3-symmetry. During the phase transition, the system experiences a hidden critical point, in which the multistable states are difficult to be identified. Through changing the initial state of system, we can identify a hidden multistable state and reveal a hidden trajectory of phase transition, allowing us to track to a hidden critical point. In addition, we observe multiple phase transitions in spectra, suggesting higher-order symmetry breaking. The reported results shed light on manipulating multistability in dissipative Rydberg atoms systems and hold promise in the applications of non-equilibrium many-body physics.

cond-mat.quant-gas↗

arXiv2024

Higher-order and fractional discrete time crystals in Floquet-driven Rydberg atoms

Higher-order and fractional discrete time crystals (DTCs) are exotic phases of matter where the discrete time translation symmetry is broken into higher-order and non-integer category. Generation of these unique DTCs has been widely studied theoretically in different systems. However, no current experimental methods can probe these higher-order and fractional DTCs in any quantum many-body systems. We demonstrate an experimental approach to observe higher-order and fractional DTCs in Floquet-driven Rydberg atomic gases. We have discovered multiple $n$-DTCs with integer values of $n$ = 2, 3, and 4, and others ranging up to 14, along with fractional $n$-DTCs with $n$ values beyond the integers. The system response can transition between adjacent integer DTCs, during which the fractional DTCs are investigated. Study of higher-order and fractional DTCs expands fundamental knowledge of non-equilibrium dynamics and is promising for discovery of more complex temporal symmetries beyond the single discrete time translation symmetry.

cond-mat.quant-gas↗

arXiv2024

Observation of Higgs and Goldstone modes in U(1) symmetry-broken Rydberg atomic systems

Higgs and Goldstone modes manifest as fluctuations in the order parameter of system, offering insights into its phase transitions and symmetry properties. Exploring the dynamics of these collective excitations in a Rydberg atoms system advances various branches of condensed matter, particle physics, and cosmology. Here, we report an experimental signature of Higgs and Goldstone modes in a U(1) symmetry-broken Rydberg atomic gases. By constructing two probe fields to excite atoms, we observe the distinct phase and amplitude fluctuations of Rydberg atoms collective excitations under the particle-hole symmetry. Due to the van der Waals interactions between the Rydberg atoms, we detect a symmetric variance spectrum divided by the divergent regime and phase boundary, capturing the full dynamics of the additional Higgs and Goldstone modes. Studying the Higgs and Goldstone modes in Rydberg atoms allows us to explore fundamental aspects of quantum phase transitions and symmetry breaking phenomena, while leveraging the unique properties of these highly interacting systems to uncover new physics and potential applications in quantum simulation.

cond-mat.quant-gas↗

arXiv2024

Early warning signals of the tipping point in strongly interacting Rydberg atoms

The identification of tipping points is essential for prediction of collapses or other sudden changes in complex systems. Applications include studies of ecology, thermodynamics, climatology, and epidemiology. However, detecting early signs of proximity to a tipping is made challenging by complexity and non-linearity. Strongly interacting Rydberg atom gases offer model systems that offer both complexity and non-linearity, including phase transition and critical slowing down. Here, via an external probe we observe prior warning of the proximity of a phase transition of Rydberg thermal gases. This warning signal is manifested as a deviation from linear growth of the variance with increasing probe intensity. We also observed the dynamics of the critical slowing down behavior versus different time scales, and atomic densities, thus providing insights into the study of a Rydberg atom system's critical behavior. Our experiment suggests that the full critical slowing down dynamics of strongly-interacting Rydberg atoms can be probed systematically, thus providing a benchmark with which to identify critical phenomena in quantum many-body systems.

cond-mat.quant-gas↗

arXiv2024

In-Lab High Resolution Mid-infrared Up-conversion Stellar Interferometer Based on Synthetic Long Base-Line

Detecting mid-infrared (MIR) radiation has significant astronomical applications, although limited by unsatisfactory MIR detectors. Here we reported on the realization of a MIR up-conversion interferometer based on synthetic long base-line (SLBL) in the laboratory. The experimental system consisted of an interferometer and subsequent up-conversion detection part of mid-infrared signal, which streamlined the structure and enhanced the reliability of the system. By using a tungsten filament lamp as an imitated star, we not only achieved the single target angle resolution of 1.10 times 10^(-4) rad, but also obtained the field angle resolution of 3.0 times 10^(-4) rad of double star targets. The angular resolution is in inverse proportion to the length of baseline. The maximum length of simulated baseline in the laboratory is about 3cm. In a Keck Interferometer (KI) liked program, the base line can reach up to 85m leading to a corresponding angular resolution of 3.0 times 10^(-9) rad (about 1.8mas). The study will offer potential benefits in extending the usage of mid-infrared light in astronomical exploration.

astro-ph.IM↗

arXiv2024

Quantum key distribution based on mid-infrared and telecom band two-color entanglement source

Due to the high noise caused by solar background radiation, the existing satellite-based free-space quantum key distribution (QKD) experiments are mainly carried out at night, hindering the establishment of a practical all-day real-time global-scale quantum network. Given that the 3-5 μm mid-infrared (MIR) band has extremely low solar background radiation and strong scattering resistance, it is one of the ideal bands for free-space quantum communication. Here, firstly, we report on the preparation of a high-quality MIR (3370 nm) and telecom band (1555 nm) two-color polarization-entangled photon source, then we use this source to realize a principle QKD based on free-space and fiber hybrid channels in a laboratory. The theoretical analysis clearly shows that a long-distance QKD over 500 km of free-space and 96 km of fiber hybrid channels can be reached simultaneously. This work represents a significant step toward developing all-day global-scale quantum communication networks.

quant-ph↗

arXiv2024

Quantum-Enhanced Polarimetric Imaging

Polarimetric imaging, a technique that captures the invisible polarization-related properties of given materials, has broad applications from fundamental physics to advanced fields such as target recognition, stress detection, biomedical diagnosis and remote sensing. The introduction of quantum sources into classical imaging systems has demonstrated distinct advantages, yet few studies have explored their combination with polarimetric imaging. In this study, we present a quantum polarimetric imaging system that integrates polarization-entangled photon pairs into a polarizer-sample-compensator-analyzer (PSRA)-type polarimeter. Our system visualizes the birefringence properties of a periodical-distributed anisotropic material under decreasing illumination levels and diverse disturbing light sources. Compared to the classical system, the quantum approach reveals the superior sensitivity and robustness in low-light conditions, particularly useful in biomedical studies where the low illumination and non-destructive detection are urgently needed. The study also highlights the nonlocality of entangled photons in birefringence measurement, indicating the potential of quantum polarimetric system in the remote sensing domain.

physics.optics↗

arXiv2024

Exceptional point and hysteresis trajectories in cold Rydberg atomic gases

The interplay between strong long-range interactions and the coherent driving contribute to the formation of complex patterns, symmetry, and novel phases of matter in many-body systems. However, long-range interactions may induce an additional dissipation channel, resulting in non-Hermitian many-body dynamics and the emergence of exceptional points in spectrum. Here, we report experimental observation of interaction-induced exceptional points in cold Rydberg atomic gases, revealing the breaking of charge-conjugation parity symmetry. By measuring the transmission spectrum under increasing and decreasing probe intensity, the interaction-induced hysteresis trajectories are observed, which give rise to non-Hermitian dynamics. We record the area enclosed by hysteresis loops and investigate the dynamics of hysteresis loops. The reported exceptional points and hysteresis trajectories in cold Rydberg atomic gases provide valuable insights into the underlying non-Hermitian physics in many-body systems, allowing us to study the interplay between long-range interactions and non-Hermiticity.

cond-mat.quant-gas↗