arXiv subjects

Bao-Sen Shi

Publications and source records attributed to Bao-Sen Shi.

At least 55 records · Page 3Linked to original sources

arXiv2024

All-optically tunable enantio-selectivity and chirality transfer

Detecting and controlling the chirality of materials play an essential role in exploring nature, providing new avenues for material creation, discrimination, and manipulation. In such tasks, chiral reagents are essential in defining or enhancing the chiral dichroism response. However, ignoring their influences on the symmetry of the medium hamper the ability to control and induce asymmetric synthesis. Here, we propose a simple but versatile chirality transfer method for synthesizing and manipulating the chirality of medium. The proposed method induces the dispersion of light in a neutral atomic system, allowing to deterministically and tunably control the chirality transfer using a helical field. First, we theoretically analyze the mechanism for this optically induced chirality transfer. Afterwards, we experimentally study the enantio-sensitive feature of the medium exposed to the auxiliary chiral field. This result can be suppressed or enhanced in a deterministic enantio-selection, opening up an efficient way to manipulate asymmetric synthesis.

physics.optics↗

arXiv2024

Ultra-Wide Dual-band Rydberg Atomic Receiver Based on Space Division Multiplexing RF-Chip Modules

Detecting microwave signals over a wide frequency range has numerous advantages as it enables simultaneous transmission of a large amount of information and access to more spectrum resources. This capability is crucial for applications such as microwave communication, remote sensing, and radar. However, conventional microwave receiving systems are limited by amplifiers and band-pass filters that can only operate efficiently in a specific frequency range. Typically, these systems can only process signals within a three-fold frequency range, which limits the data transfer bandwidth of the microwave communication systems. Developing novel atom-integrated microwave sensors, for example, radio frequency (RF)-chip coupled Rydberg atomic receiver, provides opportunities for a large working bandwidth of microwave sensing at the atomic level. Here, an ultra-wide dual-band RF sensing scheme is demonstrated by space-division multiplexing two RF-chip-integrated atomic receiver modules. The system can simultaneously receive dual-band microwave signals that span a frequency range exceeding 6 octaves (300 MHz and 24 GHz). This work paves the way for multi-band microwave reception applications within an ultra-wide range by RF-chip-integrated Rydberg atomic sensor.

physics.atom-ph↗

arXiv2024

Floquet engineering Rydberg sub-THz frequency comb spectroscopy

Engineering a Terahertz (THz) frequency comb spectroscopy at atomic level advances the precisely measurement in spectroscopy and sensing. Current progresses on THz frequency comb rely on difference-frequency generation, optical parametric oscillation, and other methods. Generating a THz frequency comb poses challenges in source stability and achieving a narrow bandwidth, which traditional THz devices are difficult to achieve. Furthermore, accurately measuring the generated THz frequency comb necessitates a high-performance THz detector. Rydberg atoms are well-suited for electric field sensing due to their ultra-wide radio frequency transition energy levels, making them especially sensitive to external electric fields in the DC to THz bandwidth. However, there have been no reports about generating THz frequency comb spectroscopy at the atomic level until now. This work presents a THz frequency comb spectroscopy with Rydberg atoms, in which a Floquet comb-like transition is engineered through a time-periodic drive field. Our approach simplifies the setup required for THz frequency comb spectroscopy while extending the working bandwidth for Rydberg atomic sensors. The THz frequency comb spectroscopy at the atomic level reported in this article shows great potential for various applications in astronomy, remote sensing, spectral detection of biological samples, and other related fields.

physics.atom-ph↗

arXiv2024

Cavity-enhanced Rydberg atom microwave receiver

Developing microwave electric field sensing based on Rydberg atom has received significant attention due to its unique advantages. However, achieving effective coupling between Rydberg atom and the microwave electric field in the sensing process is a challenging problem that greatly impacts the sensitivity. To address this, we propose the use of a microwave resonant cavity to enhance the effective coupling between the Rydberg atoms and the microwave electric field. In our experiment, we use a three-photon excitation scheme to prepare Rydberg atoms, make measurements of electric fields without and with a microwave cavity in which the vapor cell is put inside. Through experimental testing, we achieve an 18 dB enhancement of power sensitivity. The experiment shows an effective enhancement in electric field pulse signal detection. This result provides a promising direction for enhancing the sensitivity of Rydberg atomic electric field sensors and paves the way for their application in precision electric field measurements.

physics.atom-ph↗

arXiv2024

Non-Hermitian unidirectional routing of photonic qubits

Efficient and tunable qubit unidirectional routers and spin-wave diodes play an important role in both classical and quantum information processing domains. Here, we reveal that multi-level neutral cold atoms can mediate both dissipative and coherent couplings. Interestingly, we investigate and practically implement this paradigm in experiments, successfully synthesizing a system with dual functionality as both a photonic qubit unidirectional router and a spin-wave diode. By manipulating the helicity of the field, we can effectively balance the coherence coupling and dissipative channel, thereby ensuring the unidirectional transfer of photonic qubits. The qubit fidelity exceeds 97.49%, and the isolation ratio achieves $16.8\pm0.11$ dB while the insertion loss is lower than 0.36 dB. Furthermore, we show that the spin-wave diode can effectively achieve unidirectional information transfer by appropriately setting the coherent coupling parameters. Our work not only provides new ideas for the design of extensive components in quantum networks, but also opens up new possibilities for non-Hermitian quantum physics, complex quantum networks, and unidirectional quantum information transfer.

quant-ph↗

arXiv2024

Effective multiband synthetic four-wave mixing by cascading quadratic processes

Four wave mixing (FWM) is an important way to generate supercontinuum and frequency combs in the mid-infrared band. Here, we obtain simultaneous synthetic FWM in the visible and mid-infrared bands by cascading quadratic nonlinear processes in a periodically poled lithium niobate crystal (PPLN), which has a 110dB(at 3000nm) higher conversion efficiency than the FWM directly generated by third-order susceptibilities in bulk PPLN crystals. A general model of this process is developed that is in full agreement with the experimental verifications. The frequency difference between the new frequency components can be freely tuned by changing the frequency difference of the dual pump lasers. Furthermore, by increasing the conversion bandwidth and efficiency of the cascaded processes, it is feasible to generate frequency combs in three bands the visible, near-infrared and mid-infrared bands simultaneously through high-order cascaded processes. This work opens up a new avenue toward free-tuning multiband frequency comb generation with multi-octaves frequency spanning, which will have significant applications in fields such as mid-infrared gas sensing, lidar and precision spectroscopy.

physics.optics↗

arXiv2024

Narrowband telecom band polarization-entangled photon source by superposed monolithic cavities

A high-quality narrowband polarization-entangled source in the telecom band is preferred to avoid frequency dispersion for long-distance transmission in optical fibers and to efficiently couple with telecom band quantum memories. Here, we report narrowband, telecom-band, polarization-entangled photon pair generation based on the superposition of single-longitudinal-mode photon pairs from two monolithic nonlinear crystal cavities in a passively stable interferometer based on beam displacers. The photon pairs generated from the cavities exhibit a high coincidence to accidental coincidence ratio of 20000 and a bandwidth below 500 MHz. Two-photon polarization interference, Bell-inequality, and quantum state tomography are performed to indicate the high quality of the entangled source. The current configuration demonstrates greater stability than traditional free space cavity-enhanced polarization-entangled state generation, which is promising for quantum communication applications.

quant-ph↗

arXiv2024

Polarization entanglement by two simultaneous backward phase-matching processes in a single crystal

Entanglement enables many promising applications in quantum technology. Devising new generation methods and harnessing entanglement are prerequisites for practical applications. Here we realize a distinct polarization-entangled source by simultaneously achieving type-0 and type-I backward quasi-phase matching (BQPM) through spontaneous parametric down-conversion in a single bulk crystal, which is different from all previous entangled-source configurations. Pumping the crystal with a single polarized beam generates a non-maximally polarization-entangled state, which can be further projected to a maximal Bell state with a pair of Brewster windows. Hong-Ou-Mandel interference experiments are done on polarization-degenerate photon pairs for both type-0 and type-I BQPM processes for the first time. The emitted photons in both processes have a bandwidth as narrow as 15.7 GHz. The high quality of this source is characterized by various methods. The rather simple configuration, narrow bandwidth, and high entanglement quality make the source very promising for many quantum information tasks.

quant-ph↗

arXiv2024

Bifurcation of time crystals in driven and dissipative Rydberg atomic gas

A time crystal is an exotic phase of matter where time-translational symmetry is broken; this phase differs from the spatial symmetry breaking induced in crystals in space. Lots of experiments report the transition from a thermal equilibrium phase to time crystal phase. However, there is no experimental method to probe the bifurcation effect of distinct time crystals in quantum many-body systems. Here, in a driven and dissipative many-body Rydberg atom system, we observe multiple continuous dissipative time crystals and emergence of more complex temporal symmetries beyond the single time crystal phase. Bifurcation of time crystals in strongly interacting Rydberg atoms is observed; the process manifests as a transition from a time crystal state of long temporal order to one of short temporal order, or vice versa. By manipulating the driving field parameters, we observe the time crystal's bistability and a hysteresis loop. These investigations indicate new possibilities for control and manipulation of the temporal symmetries of non-equilibrium systems.

cond-mat.quant-gas↗

arXiv2024

Quantum entanglement enabled ellipsometer for phase retardance measurement

An ellipsometer is a vital precision tool used for measuring optical parameters with wide applications in many fields, including accurate measurements in film thickness, optical constants, structural profiles, etc. However, the precise measurement of photosensitive materials meets huge obstacles because of the excessive input photons, therefore the requirement of enhancing detection accuracy under low incident light intensity is an essential topic in the precision measurement. In this work, by combining a polarization-entangled photon source with a classical transmission-type ellipsometer, the quantum ellipsometer with the PSA (Polarizer-Sample-Analyzer) and the Senarmount method is constructed firstly to measure the phase retardation of the birefringent materials. The experimental results show that the accuracy can reach to nanometer scale at extremely low input intensity, and the stability are within 1% for all specimens tested with a compensator involved. Our work paves the way for precision measurement at low incident light intensity, with potential applications in measuring photosensitive materials, active-biological samples and other remote monitoring scenarios.

quant-ph↗

arXiv2024

Microwave control of collective quantum jump statistics of a dissipative Rydberg gas

Quantum many-body systems near phase transitions respond collectively to externally applied perturbations. We explore this phenomenon in a laser-driven dissipative Rydberg gas that is tuned to a bistable regime. Here two metastable phases coexist, which feature a low and high density of Rydberg atoms, respectively. The ensuing collective dynamics, which we monitor in situ, is characterized by stochastic collective jumps between these two macroscopically distinct many-body phases. We show that the statistics of these jumps can be controlled using a dual-tone microwave field. In particular, we find that the distribution of jump times develops peaks corresponding to subharmonics of the relative microwave detuning. Our study demonstrates the control of collective statistical properties of dissipative quantum many-body systems without the necessity of fine-tuning or of ultra cold temperatures. Such robust phenomena may find technological applications in quantum sensing and metrology.

quant-ph↗

arXiv2023

Single-shot, full characterization of the spatial wavefunction of light fields via Stokes tomography

Since the diffraction behavior of a light field is fully determined by its spatial wavefunction, i.e., its spatial complex amplitude (SCA), full characterization of spatial wavefunction, plays a vital role in modern optics from both the fundamental and applied aspects. In this work, we present a novel complex-amplitude profiler based on spatial Stokes tomography with the capability to fully determine the SCA of a light field in a single shot with high precision and resolution. The SCA slice observed at any propagation plane provides complete information about the light field, thus allowing us to further retrieve the complete beam structure in 3 dimensions space, as well as the exact modal constitution in terms of spatial degrees of freedom. The principle demonstrated here provides an important advancement for the full characterization of light beams with a broad spectrum of potential applications in various areas of optics, especially for the growing field of structured light.

physics.optics↗

arXiv2023

Optical Memory for Arbitrary Perfect Poincaré States in an Atomic Ensemble

Inherent spin angular momentum (SAM) and orbital angular momentum (OAM) which manifest as polarization and spatial degrees of freedom (DOF) of photons, hold a promise of large capability for applications in classical and quantum information processing. To enable these photonic spin and orbital dynamic properties strongly coupled with each other, Poincaré states have been proposed and offer advantages in data multiplexing, information encryption, precision metrology, and quantum memory. However, since the transverse size of Laguerre Gaussian beams strongly depends on their topological charge numbers $\left| l \right|$, it is difficult to store asymmetric Poincaré states due to the significantly different light-matter interaction for distinct spatial modes. Here, we experimentally realize the storage of perfect Poincaré states with arbitrary OAM quanta using the perfect optical vortex, in which 121 arbitrarily-selected perfect Poincaré states have been stored with high fidelity. The reported work has great prospects in optical communication and quantum networks for dramatically increased encoding flexibility of information.

quant-ph↗

arXiv2023

Electric field measurement and application based on Rydberg atoms

Microwave sensing has important applications in areas such as data communication and remote sensing, so it has received much attention from international academia, industry, and governments. Atomic wireless sensing uses the strong response of the large electric dipole moment of a Rydberg atom to an external field to achieve precise measurement of a radio frequency (RF) electric field. This has advantages over traditional wireless sensing. The advantage of a Rydberg atom is its ultra-wide energy level transitions, which make it responsive to RF electric fields over a wide bandwidth. Here, we briefly review the progress of electric field measurement based on Rydberg atoms. The main contents include the properties of Rydberg atoms, measurement using Rydberg atoms, and experimental progress in electric field measurement in different bands. We show the different methods for detecting electric fields such as atomic superheterodyne, machine learning, and critically enhanced measurement. The development of Rydberg atomic measurement focuses on the advantages of Rydberg atomic sensing, especially compared with conventional microwave receivers. This is of major significance to developing Rydberg-based measurement in astronomy, remote sensing, and other fields.

physics.atom-ph↗

arXiv2023

Mid-Infrared Upconversion Imaging Under Different Illumination Conditions

Converting the medium infrared field to the visible band is an effective image detection method. We propose a comprehensive theory of image up-conversion under continuous optical pumping, and discuss the relationship between the experimental parameters and imaging field of view, resolution, quantum efficiency, and conversion bandwidth. Theoretical predictions of upconversion imaging results are given based on numerical simulations, which show good agreement with experimental results. In particular, coherent and incoherent light illumination are studied separately and the advantages and disadvantages of their imaging performance are compared and analysed. This work provides a study of the upconversion image detection performance of the system, which is of great value in guiding the design of the detection system and bringing it to practical applications.

physics.optics↗

arXiv2023

Ergodicity breaking from Rydberg clusters in a driven-dissipative many-body system

It is challenging to probe ergodicity breaking trends of a quantum many-body system when dissipation inevitably damages quantum coherence originated from coherent coupling and dispersive two-body interactions. Rydberg atoms provide a test bed to detect emergent exotic many-body phases and non-ergodic dynamics where the strong Rydberg atom interaction competes with and overtakes dissipative effects even at room temperature. Here we report experimental evidence of a transition from ergodic towards ergodic breaking dynamics in driven-dissipative Rydberg atomic gases. The broken ergodicity is featured by the long-time phase oscillation, which is attributed from the formation of Rydberg excitation clusters in limit cycle phases. The broken symmetry in the limit cycle is a direct manifestation of many-body interactions, which is verified by tuning atomic densities in our experiment. The reported result reveals that Rydberg many-body systems are a promising candidate to probe ergodicity breaking dynamics, such as limit cycles, and enable the benchmark of non-equilibrium phase transition.

cond-mat.quant-gas↗

arXiv2023

High-dimensional frequency conversion in hot atomic system

One of the major difficulties in realizing a high-dimensional frequency converter for conventional optical vortex (COV) stems from the difference in ring diameter of COV modes with different topological charge numbers l. Here, we implement a high-dimensional frequency convertor for perfect optical vortex (POV) modes with invariant size through the four-wave mixing (FWM) process by utilizing Bessel-Gaussian beams instead of Laguerre-Gaussian beams. The measured conversion efficiency from 1530 nm to 795 nm is independent of l at least in subspace of {-6,...,6}, and the achieved conversion fidelities for two-dimensional (2D) superposed POV states exceed 97%. We further realize the frequency conversion of 3D, 5D and 7D superposition states with fidelities as high as 96.70%, 89.16% and 88.68%, respectively. The reported scheme is implemented in hot atomic vapor, it's also compatible with the cold atomic system and may find applications in high-capacity and long-distance quantum communication.

physics.optics↗

arXiv2023

Thermal camera based on frequency upconversion and its noise-equivalent temperature difference characterization

We present a scheme for estimating the noise-equivalent temperature difference (NETD) of frequency upconversion detectors (UCDs) that detect mid-infrared (MIR) light. In particular, this letter investigates the frequency upconversion of a periodically polarized crystal based on lithium niobate, where a mid-infrared conversion bandwidth of 220 nm can be achieved in a single poled period by a special design. Experimentally for a temperature target with a central wavelength of 7.89 μm in mid-infrared radiation, we estimated the NETD of the device to be 56 mK. Meanwhile, a direct measurement of the NETD was performed utilizing conventional methods, which resulted in 48 mK. We also compared the NETD of our UCD with commercially available direct mid-infrared detectors. Here, we showed that the limiting factor for further NETD reduction of our device is not primarily from the upconversion process and camera noise, but from the limitations of the heat source performance. Our detectors have good temperature measurement performance and can be used for a variety of applications involving temperature object identification and material structure detection.

physics.optics↗