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Baohua Jia

Publications and source records attributed to Baohua Jia.

32 records · Page 2Linked to original sources

BiOBr 2D materials for integrated nonlinear photonics devices

As a new group of advanced 2D layered materials, bismuth oxyhalides, i.e., BiOX (X = Cl, Br, I), have recently become of great interest. In this work, we characterize the third-order optical nonlinearities of BiOBr, an important member of the BiOX family. The nonlinear absorption and Kerr nonlinearity of BiOBr nanoflakes at both 800 nm and 1550 nm are characterized via the Z-Scan technique. Experimental results show that BiOBr nanoflakes exhibit a large nonlinear absorption coefficient = \b{eta} = 10-7 m/W as well as a large Kerr coefficient n2 = 10-14 m2/W. We also note that the n2 of BiOBr reverses sign from negative to positive as the wavelength is changed from 800 nm to 1550 nm. We further characterize the thickness-dependent nonlinear optical properties of BiOBr nanoflakes, finding that the magnitudes of \b{eta} and n2 increase with decreasing thickness of the BiOBr nanoflakes. Finally, we integrate BiOBr nanoflakes into silicon integrated waveguides and measure their insertion loss, with the extracted waveguide propagation loss showing good agreement with mode simulations based on ellipsometry measurements. These results confirm the strong potential of BiOBr as a promising nonlinear optical material for high-performance hybrid integrated photonic devices.

physics.optics↗

Enhanced four-wave-mixing and 3rd order optical nonlinearity in SiN nanowires integrated with graphene oxide films

Layered 2D graphene oxide (GO) films are integrated with silicon nitride (SiN) waveguides to experimentally demonstrate an enhanced Kerr nonlinearity via four wave mixing (FWM). Owing to the strong light matter interaction between the SiN waveguides and the highly nonlinear GO films, the FWM performance of the hybrid waveguides is significantly improved. SiN waveguides with both uniformly coated and patterned GO films are fabricated based on a transfer free, layer by layer GO coating method together with standard photolithography and lift off processes, yielding precise control of the film thickness, placement and coating length. Detailed FWM measurements are carried out for the fabricated devices with different numbers of GO layers and at different pump powers. By optimizing the trade off between the nonlinearity and loss, we obtain a significant improvement in the FWM conversion efficiency of 7.3 dB for a uniformly coated device with 1 layer of GO and 9.1 dB for a patterned device with 5 layers of GO. We also obtain a significant increase in FWM bandwidth for the patterned devices. A detailed analysis of the influence of pattern length and position on the FWM performance is performed. Based on the FWM measurements, the dependence of GOs third-order nonlinearity on layer number and pump power is also extracted, revealing interesting physical insights about the 2D layered GO films. Finally, we obtain an enhancement in the effective nonlinear parameter of the hybrid waveguides by over a factor of 100. These results verify the enhanced nonlinear optical performance of SiN waveguides achievable by incorporating 2D layered GO films.

physics.optics↗

Large and negative Kerr nonlinearity in PdSe2 dichalcogenide 2D films

We report a large third order nonlinear optical response of palladium diselenide (PdSe2) films, a two dimensional (2D) noble metal dichalcogenide material. Both open aperture (OA) and closed aperture (CA) Z scan measurements are performed with a femtosecond pulsed laser at 800 nm to investigate the nonlinear absorption and nonlinear refraction, respectively. In the OA experiment, we observe optical limiting behaviour originating from large two photo absorption (TPA) in the PdSe2 film of beta = 3.26 x 10-8 m/W. In the CA experiment, we measure a peak-valley response corresponding to a large and negative Kerr nonlinearity of n2 = -1.33 x 10-15 m2/W, two orders of magnitude larger than bulk silicon. We also characterize the variation of n2 as a function of laser intensity, observing that n2 decreases in magnitude with incident laser intensity, becoming saturated at n2 = -9.96 x 10-16 m2/W at high intensities. These results verify the large third order nonlinear optical response of 2D PdSe2 as well as its strong potential for high performance nonlinear photonic devices.

physics.optics↗

Enhanced nonlinear optical figure-of-merit at 1550nm for silicon nanowires integrated with graphene oxide layered films

Layered 2D GO films are integrated with silicon on insulator (SOI) nanowire waveguides to experimentally demonstrate an enhanced Kerr nonlinearity, observed through selfphase modulation (SPM). The GO films are integrated with SOI nanowires using a large area, transfer free, layer by layer coating method that yields precise control of the film thickness. The film placement and coating length are controlled by opening windows in the silica cladding of the SOI nanowires. Owing to the strong mode overlap between the SOI nanowires and the highly nonlinear GO films, the Kerr nonlinearity of the hybrid waveguides is significantly enhanced. Detailed SPM measurements using picosecond optical pulses show significant spectral broadening enhancement for SOI nanowires coated with 2.2 mm long films of 1 to 3 layers of GO, and 0.4 mm long films with 5 to 20 layers of GO. By fitting the experimental results with theory, the dependence of the n2 for GO on layer number and pulse energy is obtained, showing interesting physical insights and trends of the layered GO films from 2D monolayers to quasi bulk like behavior. Finally, we show that by coating SOI nanowires with GO films the effective nonlinear parameter of SOI nanowires is increased 16 times, with the effective nonlinear figure of merit (FOM) increasing by about 20 times to greater than 5. These results reveal the strong potential of using layered GO films to improve the Kerr nonlinear optical performance of silicon photonic devices.

physics.optics↗

Multidimensional sound propagation in 3D high-order topological sonic insulator

High-order topological insulators (TIs) develop the conventional bulk-boundary correspondence theory and rise the interest in searching innovative topological materials. To realize a high-order TI with a wide passband of 1D and 2D transportation modes, we design non-trivial and trivial 3D sonic crystals whose combination mimics the Su-Schrieffer-Heeger model. The high-order topological boundary states can be found at the interfaces, including 0D corner state, 1D hinge state, and 2D surface state. The fabricated sample with the bent two-dimensional and one-dimensional acoustic channels exhibits the multidimensional sound propagation in space, and also verifies the transition between the complete band gap, hinge states, and surface states within the bulk band gap. Among them, the bandwidth of the single-mode hinge state achieves a large relative bandwidth 9.1%, in which sound transports one-dimensionally without significant leak into the surfaces or the bulk. The high-order topological states in the study pave the way for multidimensional sound manipulation in space.

physics.app-ph↗

Enhanced four-wave-mixing with 2D layered graphene oxide films integrated with CMOS compatible micro-ring resonators

Layered 2D graphene oxide (GO) films are integrated with microring resonators (MRRs) to experimentally demonstrate enhanced nonlinear optics in the form of four wave mixing (FWM). Both uniformly coated and patterned GO films are integrated on CMOS compatible doped silica MRRs using a large area, transfer free, layer by layer GO coating method together with photolithography and lift off processes, yielding precise control of the film thickness, placement, and coating length. The high Kerr nonlinearity and low loss of the GO films combined with the strong light matter interaction within the MRRs results in a significant improvement in the FWM efficiency in the hybrid MRRs. Detailed FWM measurements are performed at different pump powers and resonant wavelengths for the uniformly coated MRRs with 1 to 5 layers of GO as well as the patterned devices with 10 to 50 layers of GO. The experimental results show good agreement with theory, achieving up to 7.6 dB enhancement in the FWM conversion efficiency (CE) for an MRR uniformly coated with 1 layer of GO and 10.3 dB for a patterned device with 50 layers of GO. By fitting the measured CE as a function of pump power for devices with different numbers of GO layers, we also extract the dependence of the third-order nonlinearity on layer number and pump power, revealing interesting physical insights about the evolution of the layered GO films from 2D monolayers to quasi bulk like behavior. These results confirm the high nonlinear optical performance of integrated photonic resonators incorporated with 2D layered GO films.

physics.optics↗

Inverse design of higher-order photonic topological insulators

Topological photonics revolutionizes some of the traditional approaches to light propagation and manipulation, and it provides unprecedented means for developing novel photonic devices. Recently discovered higher-order topological phases go beyond the conventional bulk-edge correspondence for photonic crystals and introduce novel opportunities for topological protection. Here, we introduce an intelligent numerical approach for inverse design of higher-order photonic topological insulators with great flexibility for controlling both topological edge and topological corner states. In particular, we consider the second-order photonic topological insulator and design several structures supporting both edge and corner states at different frequencies. By carefully programming these structures, we suggest a novel approach for topological routing of the edge and corner states by changing the operational frequency. Our finding paves the way to integrated topological photonic devices with novel functionalities.

physics.app-ph↗

High third-order Kerr optical nonlinearity in BiOBr 2D films measured by the Z-scan method

We investigate the nonlinear optical properties of BiOBr nanoflakes, a novel two-dimensional (2D) layered material from the Bismuth oxyhalide family. We measure the nonlinear absorption and Kerr nonlinearity of BiOBr nanoflakes at both 800 nm and 1550 nm via the Z scan technique. We observe a large nonlinear absorption coefficient beta = 10^-7 m/W as well as a large Kerr coefficient n2 = 10^-14 m^2/W. We also observe strong dispersion in n2, with it reversing sign from negative to positive as the wavelength varies from 800 nm to 1550 nm. In addition, we characterize the thickness-dependence of the nonlinear optical properties of BiOBr nanoflakes, observing that both the magnitudes of beta and n2 increase for very thin flakes. Finally, we integrate BiOBr nanoflakes onto silicon integrated waveguides and characterize the linear optical properties of the resulting hybrid integrated devices, with the measurements agreeing with calculated parameters using independent ellipsometry measurements. These results verify the strong potential of BiOBr as an advanced nonlinear optical material for high-performance hybrid integrated photonic devices.

physics.optics↗

Far-field three-dimensional deep-subwavelength focal spot with azimuthal polarization

This work focuses on the generation of far-field super-resolved pure-azimuthal focal field based on the fast Fourier transform. A self-designed differential filter is first pioneered to robustly reconfigure a doughnut-shaped azimuthal focal field into a bright one with a sub-wavelength lateral scale (0.392λ), which offers a 27.3% reduction ratio relative to that of tightly focused azimuthal polarization modulated by a spiral phase plate. By further uniting the versatile differential filter with spatially shifted beam approach, in addition to allowing for an extremely sharper focal spot, whose size is in turn reduced to 0.228λ and 0.286λ in the transverse as well as axial directions, the parasitic sidelobes are also lowered to an inessential level (< 20%), thereby enabling an excellent three-dimensional deep-subwavelength focal field (λ3/128). The relevant phase profiles are further exhibited to unravel the annihilation of field singularity and locally linear (i.e. azimuthal) polarization. Our scheme opens a promising route toward efficiently steer and tailor the redistribution of the focal field.

physics.optics↗

Integrated polarizers based on graphene oxide in waveguides and ring resonators

Integrated waveguide polarizers and polarization-selective micro-ring resonators (MRRs) incorporated with graphene oxide (GO) films are experimentally demonstrated. CMOS-compatible doped silica waveguides and MRRs with both uniformly coated and patterned GO films are fabricated based on a large-area, transfer-free, layer-by-layer GO coating method that yields precise control of the film thickness. Photolithography and lift-off processes are used to achieve photolithographic patterning of GO films with precise control of the placement and coating length. Detailed measurements are performed to characterize the performance of the devices versus GO film thickness and coating length as a function of polarization, wavelength and power. A high polarization dependent loss of ~53.8 dB is achieved for the waveguide coated with 2-mm-long patterned GO films. It is found that intrinsic film material loss anisotropy dominates the performance for less than 20 layers whereas polarization dependent mode overlap dominates for thicker layers. For the MRRs, the GO coating length is reduced to 50 microns, yielding a ~ 8.3-dB polarization extinction ratio between TE and TM resonances. These results offer interesting physical insights and trends of the layered GO films and demonstrate the effectiveness of introducing GO films into photonic integrated devices to realize high-performance polarization selective components.

physics.optics↗

Graphene oxide for enhanced nonlinear optics in low and high index contrast waveguides and nanowires

We demonstrate enhanced four-wave mixing (FWM) in doped silica waveguides integrated with graphene oxide (GO) layers. Owing to strong mode overlap between the integrated waveguides and GO films that have a high Kerr nonlinearity and low loss, the FWM efficiency of the hybrid integrated waveguides is significantly improved. We perform FWM measurements for different pump powers, wavelength detuning, GO coating lengths, and number of GO layers. Our experimental results show good agreement with theory, achieving up to ~9.5-dB enhancement in the FWM conversion efficiency for a 1.5-cm-long waveguide integrated with 2 layers of GO. We show theoretically that for different waveguide geometries an enhancement in FWM efficiency of ~ 20 dB can be obtained in the doped silica waveguides, and more than 30 dB in silicon nanowires and slot waveguides. This demonstrates the effectiveness of introducing GO films into integrated photonic devices in order to enhance the performance of nonlinear optical processes.

physics.optics↗

Diodelike asymmetric transmission in hybrid plasmonic waveguides via breaking polarization symmetry

The ability to control the asymmetric propagation of light in nanophotonic waveguides is of fundamental importance for optical communications and on-chip signal processing. However, in most studies so far, the design of such structures has been based on asymmetric mode conversion where multi-mode waveguides are involved. Here we propose a hybrid plasmonic structure that performs optical diode behavior via breaking polarization symmetry in single mode waveguides. The exploited physical mechanism is based on the combination of polarization rotation and polarization selection. The whole device is ultra-compact with a footprint of 2.95*14.18 μm2, whose dimension is much smaller than the device previously proposed for the similar function. The extinction ratio is greater than 11.8 dB for both forward and backward propagation at λ = 1550 nm (19.43 dB for forward propagation and 11.8 dB for the backward one). The operation bandwidth of the device is as great as 70 nm (form 1510 to 1580 nm) for extinction > 10 dB. These results may find important applications in the integrated devices where polarization handling or unidirectional propagation is required.

physics.optics↗

Optical gears in a nanophotonic directional coupler

Gears are rotating machines, meshing with each other by teeth to transmit torque. Interestingly, the rotating directions of two meshing gears are opposite, clockwise and counterclockwise. Although this opposite handedness motion has been widely investigated in machinery science, the analogue behavior of photons remains undiscovered. Here, we present a simple nanophotonic directional coupler structure which can generate two meshing gears of angular momentum (AM) of light, optical gears. Due to the abrupt phase shift effect and birefringence effect, the AM states of photons vary with the propagation distance in two adjacent waveguides of the coupler. Thus, by the choice of coupling length, it is able to obtain two light beams with opposite handedness of AM, confirming the appearance of optical gears. The full control in the handedness of output beams is achieved via tuning the relative phase between two orthogonal modes at the input ports. Optical gears thus offer the possibility of exploring light-matter interactions in nanoscale, opening up new avenues in fields of integrated quantum computing and nanoscale bio-sensing of chiral molecules.

physics.optics↗

High Performance Atomically Thin Flat Lenses

We experimentally demonstrate ultrathin flat lenses with a thickness of 7 Å, which corresponds to the fundamental physical limit of the thickness of the material, is fabricated in a large area, monolayer, CVD-prepared tungsten chalcogenides single crystals using the low-cost flexible laser writing method. The lenses apply the ultra-high refractive index to introduce abrupt amplitude modulation of the incident light to achieve three-dimensional (3D) focusing diffraction-limited resolution (0.5λ) and a focusing efficiency as high as 31%. An analytical physical model based diffraction theory is derived to simulate the focusing process, which shows excellent agreement with the experimental results.

physics.optics↗