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Baoli Liu

Publications and source records attributed to Baoli Liu.

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Re-evaluation of bottleneck effect via a coupled monolayer WS_2/photonic crystal heterostructure

Exciton-polariton condensates is an important type of Bose-Einstein condensate whose realization requires efficient relaxation of polaritons to the band-energy minima. However, this process is often obstructed by bottleneck effect near the anticrossing region of polariton dispersion. Although the exciton-polariton bottleneck effect has been extensively observed in various polariton system, but there is no a unified views of physical origin. Here, we construct an exciton-trion-photon coupling system in monolayer WS_2/photonic-crystal slab heterostructures. Momentum-resolved photoluminescence reveals the anticrossing polariton dispersions for the exciton resonance with a ~57 meV Rabi splitting and there is no characteristic anticrossing for trion resonance with a ~5 meV splitting at ~12 K. Enhanced polariton emission is observed around the trion-polariton crossing with elevating temperature. We attributes this exotic phenomenon to bottleneck effect and indicating that small Rabi splitting is the unified origin of bottleneck effect in polariton systems.

physics.optics

Visualization of Photonic Band Structures via Far-field Measurements in SiNx Photonic Crystal Slabs

The band structures of the photonic crystal slabs play a significant role in manipulating the flow of light and pre-dicting exotic physics in photonics. In this letter, we show that the key features of photonic band structures can be achieved experimentally by the polarization- and momentum-resolved photoluminescence spectroscopy utilizing the light emission properties of SiNx. The two-dimensional spectra clearly reveal the energy-momentum dispersion of band structures which is in perfect agreement with the simulation results. The isofrequency contours can be measured easily by adding a bandpass filter with a desired photon energy. Furthermore, it is convenient to observe clearly and directly the optical singularity -- the optical bound states in the continuum featured by dark point in three-dimensional photoluminescence spectra. The polarization-resolved isofrequency contours clearly show that this dark point is the center of an azimuthally polarized vortex. Finally, the helical topological edge states can be easily observed in photonic topological insulators with deformed hexagonal lattices. Our work provides a simple and effective approach for exploring topological photonics and other intriguing phenomena hidden in the photonic crystal slabs.

physics.optics

Probing Phase Transition of Band Topology via Radiation Topology

Topological photonics has received extensive attention from researchers because it provides brand new physical principles to manipulate light. Band topology of optical materials is characterized using the Berry phase defined by Bloch states. Until now, the criteria for experimentally probing the topological phase transition of band topology has always been relatively lacking in topological physics. Moreover, radiation topology can be aroused by the far-field polarizations of the radiating Bloch states, which is described by the Stokes phase. Although such two types of topologies are both related to Bloch states on the band structure, it is rather surprising that their development is almost independent. Here, we reveal that the phase transition of band topology can be probed by the radiation topology. We theoretically design and experimentally demonstrate such an intriguing phenomenon by constructing photonic crystals that support optical analogs of quantum spin Hall effects. The results show that the topological charge of the far-field polarization vortex changes from +1 to -2 or from -2 to +1 when the band topology changes from trivial to non-trivial, which provides a new criterion to probe the phase transition of band topology using radiation topology. Our findings not only provide an insightful understanding of band topology and radiation topology, but also can serve as a novel route to manipulate the near and far fields of light.

physics.optics

Polarized exciton emission enhancement of monolayer MoS2 coupled with plasmonic Salisbury-type absorber

The plasmon-mediated manipulation of light-matter interaction in two-dimensional atomically transition-metal dichalcogenides (TMDs) critically depends on the design of plasmonic nanostructures to achieve the maximum optical field in TMDs. Here, a metal-isolator-metal Salisbury-type perfect absorber was fabricated to serve as a generator of the localized surface plasmons. The significant photoluminescence (PL) enhancement up to 60-fold was observed experimentally in the monolayer (ML) MoS2 on the top of this gold plasmonic hybrid nanostructures. Furthermore, the PL linear polarization can approach ~60 % around the peak of exciton emission and is independent on the polarization of the excitation laser. This Salisbury-type plasmon-exciton hybrid system paves a new way to develop optoelectronic devices based on TMDs.

physics.optics

Experimental valley qubit state tomography and coherence induced uncertainty relations in monolayer WSe$_2$

Velleytronics as a new electronic conception is an emerging exciting research field with wide potential applications, which is attracting great research interests for their extraordinary properties. The localized electronic spins by optical generation of valley polarization with spin-like quantum numbers are promising candidates for implementing quantum-information processing in solids. It is expected that a single qubit preparation can be realized optically by using combination of left- and right-circularly polarized lights. Significantly in a series of experiments, this has already been well achieved by linearly polarized laser representing equal weights of left- and right-circular components resulting in formation of a valley exciton as a specific pseudo-spin qubit with equal amplitudes for spin up and spin down. Further researches on the control of valley pseudospin using longitudinal magnetic field and optical Stark effect have been reported. However, a general qubit preparation has not yet been demonstrated. Moreover as a platform for quantum information processing, the precise readout of a qubit state is necessary, for which the state tomography is a standard method in obtaining all information of a qubit state density matrix.

quant-ph

Electron Density Dependence of in-plane Spin Relaxation Anisotropy in GaAs/AlGaAs Two-Dimensional Electron Gas

We investigated the spin dynamics of two-dimensional electrons in (001) GaAs/AlGaAs heterostructure using the time resolved Kerr rotation technique under a transverse magnetic field. The in-plane spin lifetime is found to be anisotropic below 150k due to the interference of Rashba and Dresselhaus spin-orbit coupling and D'yakonov-Perel' spin relaxation. The ratio of in-plane spin lifetimes is measured directly as a function of temperature and pump power, showing that the electron density in 2DEG channel strongly affects the Rashba spin-orbit coupling.

cond-mat.mes-hall

Experimental Observation of the Inverse Spin Hall Effect at Room Temperature

We observe the inverse spin Hall effect in a two-dimensional electron gas confined in AlGaAs/InGaAs quantum wells. Specifically, we find that an inhomogeneous spin density induced by the optical injection gives rise an electric current transverse to both the spin polarization and its gradient. The spin Hall conductivity can be inferred from such a measurement through the Einstein relation and the Onsager relation, and is found to have the order of magnitude of $0.5(e^{2}/h)$. The observation is made at the room temperature and in samples with macroscopic sizes, suggesting that the inverse spin Hall effect is a robust macroscopic transport phenomenon.

cond-mat.mes-hall