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Baoqi Shi

Publications and source records attributed to Baoqi Shi.

At least 19 recordsLinked to original sources

Material-Anisotropy-Driven Topological Optical Lattices on Thin-Film Lithium Niobate

Integrated structured-light sources usually obtain high-dimensional orbital angular momentum (OAM) states by encoding each channel into separate gratings, waveguides or metasurfaces, which ties modal capacity to structural complexity. Here we show that intrinsic material anisotropy can instead act as a built-in angular-momentum coupler. In an X-cut thin-film lithium niobate (TFLN) microring vortex emitter, the in-plane optical axis causes a circulating whispering-gallery mode to sample a periodically varying effective index, producing continuous azimuthal phase modulation. This modulation converts each resonance from a nominal single-charge emitter into a coherent topological sideband lattice with charges l=l_p+2n and Bessel-weighted amplitudes. Broadband measurements resolve a representative principal-charge series from l_p=-13 to +13, while additional devices with 100 and 200 GHz free spectral ranges (FSRs) show scalable resonance addressability. The emitted lattices are reproduced by a forward-calculated Fourier--Bessel model, supported by OAM projection measurements, and exhibit focusing into annular perfect-vortex fields and self-healing after obstruction. Waveguide-induced circular polarization further adds a vectorial spin--orbit channel. These results turn TFLN anisotropy from a material constraint into a compact mechanism for resonance-addressed high-dimensional structured-light generation.

physics.optics

Kramers-Kronig causality in integrated photonics: The spectral tension between ultraviolet transition and mid-infrared absorption

Dispersion engineering via geometric confinement is essential to integrated photonics, enabling phenomena such as soliton microcombs, supercontinua, parametric oscillators, and entangled photons. However, prevailing methodologies rely on semi-empirical Sellmeier models that assume idealized material purity, neglecting the pronounced dispersion shifts induced by residual impurities like hydrogen-related bonds. Here, we demonstrate that these residual bonds fundamentally alter the dispersion landscape spanning from the ultraviolet (UV) to the mid-infrared (MIR) spectra. Specifically, they introduce MIR vibrational absorption while simultaneously modifying UV electronic transition, shifting the bandgap and UV pole. We show that the spectral tension between these UV and MIR modifications dictates the group velocity dispersion from the visible to the near-infrared (NIR) via the Kramers-Kronig causality. We experimentally validate this phenomenon through systematic characterization of broadband loss and dispersion in ultralow-loss silicon nitride photonic integrated circuits. By rigorously incorporating these effects, we bridge the gap between empirical fitting and predictive physical modelling. Our study resolves long-standing discrepancies in dispersion engineering, providing precision control essential for next-generation integrated photonics.

physics.optics

Enhancement of vacuum-ultraviolet dispersive-wave emission using gas-filled tapered hollow-core fibers

The recent breakthroughs in laser-driving 229Th nuclear transition have created an urgent demand for coherent vacuum-ultraviolet (VUV) sources delivering high spectral brightness at the critical 148.38 nm isomer energy. However, generating sufficient photon flux to overcome the low nuclear excitation probability remains a challenge for compact setups. While resonant dispersive wave emission in gas-filled hollow-core fibers offers a promising route, standard capillaries face a fundamental trade-off: maximizing input coupling requires large core diameters, whereas efficient nonlinear VUV conversion demands the high intensities using small cores. Here, we resolve this conflict using a gas-filled tapered capillary fiber. This architecture utilizes a longitudinally decreasing core diameter to combine a large input aperture with adiabatic field concentration, thereby continuously enhancing the nonlinear interaction. Experimentally, we demonstrate a widely tunable source (135-240 nm) that achieves a twofold efficiency enhancement specifically at the 148.38 nm wavelength compared to uniform geometries. By providing a scalable route to high-flux VUV generation, this work establishes a critical tabletop tool for advancing solid-state nuclear clocks and time-resolved spectroscopy.

physics.optics

Metrology-grade mid-infrared spectroscopy for multi-dimensional perception

The mid-infrared spectral window is essential for molecular fingerprinting and atmospheric sensing, yet unlocking its full potential is currently constrained by a fundamental instrumental trade-off: existing systems cannot simultaneously deliver broad bandwidth, high photon flux, and metrological frequency fidelity. Here, we resolve this bottleneck by demonstrating a metrology-grade spectroscopic system based on difference frequency generation, driven by widely tunable, near-infrared diode lasers traceable to atomic standards. Our system achieves continuous tunability across the 3-3.7 $μ$m atmospheric window and delivers output power exceeding 45 mW with an absolute frequency accuracy of 7.2 MHz. We harness this convergence to overcome a critical barrier in integrated photonics, unambiguously identifying and eliminating hydrogen-induced absorption in silicon nitride microresonators to achieve an 88-fold reduction in optical loss. We further reveal multi-phonon absorption in the silica cladding as the fundamental limit to mid-infrared integrated photonics. Finally, we demonstrate the system's versatility through scattering-resilient LiDAR capable of penetrating optically dense fog, and dual-modality sensing that simultaneously retrieves target distance and chemical composition. By unifying the rigor of frequency metrology with the versatility of broadband sensing, this architecture establishes a new paradigm for multi-dimensional perception in complex environments.

physics.optics

A scalable near-visible integrated photon-pair source for satellite quantum science

Quantum state distribution over vast distances is essential for global-scale quantum networks and fundamental test of quantum physics at space scale. While satellite platforms have demonstrated thousand-kilometer entanglement distribution, quantum key distribution and quantum teleportation with ground, future constellations and deep-space missions demand photon sources that are robust, compact, and power-efficient. Integrated photonics offers a scalable solution, yet a critical spectral gap persists. Although telecom-band integrated photon-pair sources are well established, near-visible photons offer distinct advantages for satellite-to-ground links by mitigating diffraction loss and maximizing the collection efficiency of optical telescopes. Scalable integrated sources in this regime have remained elusive due to the fundamental challenge of achieving anomalous dispersion in materials transparent at visible wavelengths. Here we bridge this gap by demonstrating an integrated near-visible photon-pair source based on a wide-bandgap, ultralow-loss, silicon nitride (Si$_3$N$_4$) microresonator. By engineering the dispersion of higher-order waveguide modes, we overcome the intrinsic normal dispersion limit to achieve efficient phase matching. The device exhibits a spectral brightness of 4.87$\times$10$^7$ pairs/s/mW$^2$/GHz and a narrow photon linewidth of 357 MHz. We report high-purity heralded single-photon generation with a heralding rate up to 2.3 MHz and a second-order correlation function as low as 0.0041. Furthermore, we observe energy-time entanglement with 98.4% interference visibility, violating the CHSH limit even at flux exceeding 40.6 million pairs/s. Combined with the proven radiation hardness of Si$_3$N$_4$, this source constitutes a flight-ready hardware foundation for daylight quantum communications and protocols requiring on-orbit multiphoton interference.

quant-ph

Light coupling to photonic integrated circuits using optimized lensed fibers

Efficient and reliable light coupling between optical fibers and photonic integrated circuits has arguably been the most essential issue in integrated photonics for optical interconnects, nonlinear signal conversion, neuromorphic computing, and quantum information processing. A commonly used approach is to use inverse tapers interfacing with lensed fibers, particularly for waveguides of relatively low refractive index, such as silicon nitride (Si3N4), silicon oxynitride, and lithium niobate. This approach simultaneously enables broad operation bandwidth, high coupling efficiency, and simplified fabrication. Although diverse taper designs have been invented and characterized to date, lensed fibers play equally important roles here, yet their optimization has long been underexplored. Here, we fill this gap and introduce a comprehensive co-optimization strategy that synergistically refines the geometries of the taper and the lensed fiber. By incorporating the genuine lensed fiber's shape into the simulation, we accurately capture its non-Gaussian emission profile, thereby nullifying the widely accepted approximation based on a paraxial Gaussian mode. We further characterize many lensed fibers and Si3N4 tapers of varying shapes using different fabrication processes. Our experimental and simulation results show remarkable agreement, both achieving maximum coupling efficiencies exceeding 80% per facet. Finally, we summarize the optimal choices of lensed fibers and Si3N4 tapers that can be directly deployed in modern CMOS foundries for scalable manufacturing of Si3N4 photonic integrated circuits. Our study not only contributes to light-coupling solutions but is also critical for photonic packaging and optoelectronic assemblies that are currently revolutionizing data centers and AI.

physics.optics

Hybrid-integrated dark-pulse microcombs towards visible light spectrum

Leveraging hybrid integration, we demonstrate dark-pulse formation at 780-nm wavelength band in integrated Si$_3$N$_4$ microresonators driven by high-power AlGaAs-based chip-scale lasers. The device outputs coherent frequency combs with electronically detectable repetition rates down to 20 GHz, paving a route to efficient and compact atom-chip interfaces for spectroscopy, metrology and sensing.

physics.optics

A high-resolution microresonator-frequency-comb spectrometer

Spectral analysis is one of the most powerful technologies for studying and understanding matter. As the devices for spectral analysis, spectrometers are widely used in material detection, isotope analysis, trace gas detection, and the study of atomic and molecular hyperfine structures. While high resolution, wide bandwidth and fast speed are essential factors, they are always trade-offs for conventional spectrometers. Here, we present a soliton-microcomb-based spectrometer that overcomes these challenges by integrating dissipative Kerr solitons (DKSs) with double-sideband modulation and parallelized detection. Leveraging a high-quality silicon nitride microresonator, we generate a broadband, fully stabilized soliton microcomb and employ radio-frequency-modulated double sidebands to scan the optical spectrum with the resolution constrained only by the comb-line linewidth. By projecting the comb lines onto a two-dimensional charge-coupled device (CCD) via a virtually imaged phased array (VIPA)-grating system, we enable parallel processing of all spectral components, circumventing sequential scanning delays. The resulting spectrometer achieves 200-kHz resolution across a 4-THz bandwidth with minutes-level processing time while maintaining robustness against environmental fluctuations. Being promising for miniaturization, this work bridges the gap between laboratory-grade performance and field-deployable practicality, unlocking new possibilities for spectroscopy in astronomy, metrology, and integrated photonics.

physics.optics

Space compatibility of emerging, wide-bandgap, ultralow-loss integrated photonics

Integrated photonics has revolutionized optical communication, sensing, and computation, offering miniaturized and lightweight solutions for spacecraft with limited size and payload. Novel chip-scale instruments based on ultralow-loss integrated photonic platforms, including lasers, frequency combs and atomic traps, have been developed for space applications. Therefore, quantifying the space compatibility of ultralow-loss photonic integrated circuits (PICs), particularly their radiation resistance, is critical. This study experimentally evaluates the radiation resistance of ultralow-loss Si$_3$N$_4$, 4H-SiC, and LiNbO$_3$ PICs under intense $γ$-ray and high-energy proton irradiation. Results show that proton irradiation with $1.1 \times 10^{10}$ $\mathrm{p/cm^2}$ total flux does not significantly increase optical loss or alter the refractive index of these PICs, while $γ$-ray irradiation with 1.2 Mrad accumulated dose only marginally increases their optical loss. These findings provide preliminary evidence of the excellent space compatibility of ultralow-loss Si$_3$N$_4$, 4H-SiC, and LiNbO$_3$ PICs, highlighting their potential for compact and lightweight space systems.

physics.optics

A chip-based optoelectronic-oscillator frequency comb

Microresonator-based Kerr frequency combs ("Kerr microcombs") constitute chip-scale frequency combs of broad spectral bandwidth and repetition rate ranging from gigahertz to terahertz. An appealing application exploiting microcombs' coherence and large repetition rate is microwave and millimeter-wave generation. Latest endeavor applying two-point optical frequency division (OFD) on photonic-chip-based microcombs has created microwaves with exceptionally low phase noise. Nevertheless, microcomb-based OFD still requires extensive active locking, additional lasers, and external RF or microwave sources, as well as sophisticated initiation. Here we demonstrate a simple and entirely passive (no active locking) architecture, which incorporates an optoelectronic oscillator (OEO) and symphonizes a coherent microcomb and a low-noise microwave spontaneously. Our OEO microcomb leverages state-of-the-art integrated chip devices including a high-power DFB laser, a broadband silicon Mach-Zehnder modulator, an ultralow-loss silicon nitride microresonator, and a high-speed photodetector. Each can be manufactured in large volume with low cost and high yield using established CMOS and III-V foundries. Our system synergizes a microcomb of 10.7 GHz repetition rate and an X-band microwave with phase noise of $-$97/$-$126/$-$130 dBc/Hz at 1/10/100 kHz Fourier frequency offset, yet does not demand active locking, additional lasers, and external RF or microwave sources. With potential to be fully integrated, our OEO microcomb can become an invaluable technology and building block for microwave photonics, radio-over-fiber, and optical communication.

physics.optics

Nanometric dual-comb ranging using photon-level microcavity solitons

Absolute distance measurement with low return power, fast measurement speed, high precision, and immunity to intensity fluctuations is highly demanded in nanotechnology. However, achieving all these objectives simultaneously remains a significant challenge for miniaturized systems. Here, we demonstrate dual-comb ranging (DCR) that encompasses all these capabilities by using counter-propagating (CP) solitons generated in an integrated Si$_3$N$_4$ microresonator. We derive equations linking the DCR precision with comb line powers, revealing the advantage of microcomb's large line spacing in precise ranging. Leveraging the advantage, our system reaches 1-nm-precision and measures nm-scale vibration at frequencies up to 0.9 MHz. We also show that precise DCR is possible even in the presence of strong intensity noise and loss, using a mean received photon number as low as 5.5$\times$10$^{-4}$ per pulse. Our work establishes an optimization principle for dual-comb systems and bridges high performance ranging with foundry-manufactured photonic chips.

physics.optics

A microcomb-empowered Fourier domain mode-locked LiDAR

Light detection and ranging (LiDAR) has emerged as an indispensable tool in autonomous technology. Among its various techniques, frequency modulated continuous wave (FMCW) LiDAR stands out due to its capability to operate with ultralow return power, immunity to unwanted light, and simultaneous acquisition of distance and velocity. However, achieving a rapid update rate with sub-micron precision remains a challenge for FMCW LiDARs. Here, we present such a LiDAR with a sub-10 nm precision and a 24.6 kHz update rate by combining a broadband Fourier domain mode-locked (FDML) laser with a silicon nitride soliton microcomb. An ultrahigh frequency chirp rate up to 320 PHz/s is linearized by a 50 GHz microcomb to reach this performance. Our theoretical analysis also contributes to resolving the challenge of FMCW velocity measurements with nonlinear frequency sweeps and enables us to realize velocity measurement with an uncertainty below 0.4 mm/s. Our work shows how nanophotonic microcombs can unlock the potential of ultrafast frequency sweeping lasers for applications including LiDAR, optical coherence tomography and sensing.

physics.optics

An alkali-referenced vector spectrum analyzer for visible-light integrated photonics

Integrated photonics has reformed our information society by offering on-chip optical signal synthesis, processing and detection with reduced size, weight and power consumption. As such, it has been successfully established in the near-infrared (NIR) telecommunication bands. With the soaring demand in miniaturized systems for biosensing, quantum information and transportable atomic clocks, extensive endeavors have been stacked on translating integrated photonics into the visible spectrum, i.e. visible-light integrated photonics. Various innovative visible-light integrated devices have been demonstrated, such as lasers, frequency combs, and atom traps, highlighting the capacity and prospect to create chip-based optical atomic clocks that can make timing and frequency metrology ubiquitous. A pillar to the development of visible-light integrated photonics is characterization techniques featuring high frequency resolution and wide spectral coverage, which however remain elusive. Here, we demonstrate a vector spectrum analyzer (VSA) for visible-light integrated photonics, offering spectral bandwidth from 766 to 795 nm and frequency resolution of 415 kHz. The VSA is rooted on a widely chirping, high-power, narrow-linewidth, mode-hop-free laser around 780 nm, which is frequency-doubled from the near-infrared via an efficient, broadband CPLN waveguide. The VSA is further referenced to hyperfine structures of rubidium and potassium atoms, enabling 8.1 MHz frequency accuracy. We apply our VSA to showcase the characterization of loss, dispersion and phase response of passive integrated devices, as well as densely spaced spectra of mode-locked lasers. Combining operation in the NIR and visible spectra, our VSA allows characterization bandwidth exceeding an octave and can be an invaluable diagnostic tool for spectroscopy, nonlinear optical processing, imaging and quantum interfaces to atomic devices.

physics.optics

Ultralow-loss integrated photonics enables bright, narrow-band, photon-pair sources

Photon-pair sources are critical building blocks for photonic quantum systems. Leveraging Kerr nonlinearity and cavity-enhanced spontaneous four-wave mixing, chip-scale photon-pair sources can be created using microresonators built on photonic integrated circuit. For practical applications, a high microresonator quality factor $Q$ is mandatory to magnify photon-pair sources' brightness and reduce their linewidth. The former is proportional to $Q^4$, while the latter is inversely proportional to $Q$. Here, we demonstrate an integrated, microresonator-based, narrow-band photon-pair source. The integrated microresonator, made of silicon nitride and fabricated using a standard CMOS foundry process, features ultralow loss down to $3$ dB/m and intrinsic $Q$ factor exceeding $10^7$. The photon-pair source has brightness of $1.17\times10^9$ Hz/mW$^2$/GHz and linewidth of $25.9$ MHz, both of which are record values for silicon-photonics-based quantum light source. It further enables a heralded single-photon source with heralded second-order correlation $g^{(2)}_\mathrm{h}(0)=0.0037(5)$, as well as a time-bin entanglement source with a raw visibility of $0.973(9)$. Our work evidences the global potential of ultralow-loss integrated photonics to create novel quantum light sources and circuits, catalyzing efficient, compact and robust interfaces to quantum communication and networks.

physics.optics

A chip-integrated comb-based microwave oscillator

Low-noise microwave oscillators are cornerstones for wireless communication, radar and clocks. Optical frequency combs have enabled photonic microwaves with unrivalled noise performance and bandwidth. Emerging interest is to generate microwaves using chip-based frequency combs, namely microcombs. Here, we demonstrate the first, fully integrated, microcomb-based, microwave oscillator chip. The chip, powered by a microelectronic circuit, leverages hybrid integration of a DFB laser, a nonlinear microresonator, and a high-speed photodetector. Each component represents the best of its own class, yet allows large-volume manufacturing with low cost in CMOS foundries. The hybrid chip outputs an ultralow-noise laser of 6.9 Hz linewidth, a microcomb of 10.7 GHz repetition rate, and a 10.7 GHz microwave of 6.3 mHz linewidth -- all three in one entity of 76 mm$^2$ size.The microwave phase noise reaches -75/-105/-130 dBc/Hz at 1/10/100 kHz Fourier offset frequency. Our results can reinvigorate our information society for communication, sensing, timing and precision measurement.

physics.optics

Rhythmic soliton interactions for integrated dual-microcomb spectroscopy

Rotation symmetry of microresonators supports the generation of phase-locked counter-propagating (CP) solitons that can potentially miniaturize dual-comb systems. Realization of these dual-comb compatible solitons in photonic integrated circuits remains a challenge. Here, we synthesized such CP solitons in an integrated silicon nitride microresonator and observed forced soliton oscillation due to rhythmic, time-varying soliton interactions. The interactions result in seconds mutual-coherence passively. Temporal motion in the soliton streams is discerned by measuring a quadratic-scaling frequency noise peaks and an inverse quadratic-scaling microcomb sidebands. By generating a CP soliton trimer to have two synchronized solitons in one of the orbiting directions, we resolve the incapability of measuring two unsynchronized CP soliton dimer pulses by optical cross-correlation, and show CP solitons undergo complex motion trajectory. We further prove that precise dual-comb spectroscopy with an acquisition time as short as 0.6 $μ$s is feasible using these solitons, although the temporal motion limits the dynamic range. Besides revealing soliton interactions with different group velocities, our work propels the realization of photonic integrated dual-comb spectrometers with high passive coherence.

physics.optics

A wideband, high-resolution vector spectrum analyzer for integrated photonics

The analysis of optical spectra - emission or absorption -- has been arguably the most powerful approach for discovering and understanding matters. The invention and development of many kinds of spectrometers have equipped us with versatile yet ultra-sensitive diagnostic tools for trace gas detection, isotope analysis, and resolving hyperfine structures of atoms and molecules. With proliferating data and information, urgent and demanding requirements have been placed today on spectrum analysis with ever-increasing spectral bandwidth and frequency resolution. These requirements are especially stringent for broadband laser sources that carry massive information, and for dispersive devices used in information processing systems. In addition, spectrum analyzers are expected to probe the device's phase response where extra information is encoded. Here we demonstrate a novel vector spectrum analyzer (VSA) that is capable of characterizing passive devices and active laser sources in one setup. Such a dual-mode VSA can measure loss, phase response and dispersion properties of passive devices. It also can coherently map a broadband laser spectrum into the RF domain. The VSA features a bandwidth of 55.1 THz (1260 to 1640 nm), frequency resolution of 471 kHz, and dynamic range of 56 dB. Meanwhile, our fiber-based VSA is compact and robust. It requires neither high-speed modulators and photodetectors, nor any active feedback control. Finally, we successfully employ our VSA for applications including characterization of integrated dispersive waveguides, mapping frequency comb spectra, and coherent light detection and ranging (LiDAR). Our VSA presents an innovative approach for device analysis and laser spectroscopy, and can play a critical role in future photonic systems and applications for sensing, communication, imaging, and quantum information processing.

physics.optics

Programmable access to microresonator solitons with modulational sideband heating

Dissipative Kerr solitons formed in high-$Q$ optical microresonators provide a route to miniaturized optical frequency combs that can revolutionize precision measurements, spectroscopy, sensing, and communication. In the last decade, a myriad of integrated material platforms have been extensively studied and developed to create photonic-chip-based soliton combs. However, the photo-thermal effect in integrated optical microresonators has been a major issue preventing simple and reliable soliton generation. Several sophisticated techniques to circumvent the photo-thermal effect have been developed. In addition, instead of the single-soliton state, emerging applications in microwave photonics and frequency metrology prefer multi-soliton states. Here we demonstrate an approach to manage the photo-thermal effect and facilitate soliton generation. The approach is based on a single phase-modulated pump, where the generated blue-detuned sideband synergizes with the carrier and thermally stabilizes the microresonator. We apply this technique and demonstrate deterministic soliton generation of 19.97 GHz repetition rate in an integrated silicon nitride microresonator. Furthermore, we develop a program to automatically address to target $N-$soliton state, in addition to the single-soliton state, with near 100% success rate and as short as 10 s time consumption. Our method is valuable for soliton generation in essentially any platforms even with strong photo-thermal effect, and can promote wider applications of soliton frequency comb systems for microwave photonics, telecommunication and frequency metrology.

physics.optics