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Benjamin Sacépé

Publications and source records attributed to Benjamin Sacépé.

At least 19 recordsLinked to original sources

Quantum critical collapse of a pinned vortex glass in high-field superconducting resonators

The interplay between disorder and vortex--vortex interactions in strongly disordered superconductors in a magnetic field can stabilize a vortex-glass state, characterized by strong pinning and the absence of positional order. Yet its role in the destruction of superconductivity at the field-driven superconductor--insulator transition has remained unresolved. Here we use plasmonic microwave spectroscopy of superconducting resonators patterned from amorphous indium oxide thin films to directly track the superfluid density up to the critical field $B_c$. We find an unexpected resilience of the superfluid density, which decreases only logarithmically over nearly three orders of magnitude in field, in stark contrast to the rapid power-law suppression expected for vortex lattices. We attribute this anomalously slow decay to a collective vortex-pinning mechanism counterintuitively enhanced by vortex--vortex interactions. The superfluid density then vanishes linearly at $B_c$, where independent magnetoresistance measurements identify a continuous quantum critical point, unlike the abrupt transition observed at zero field. We further uncover an exceptionally large nonlinear electromagnetic response of the vortex glass, manifested as a pronounced positive-Kerr effect with potential for quantum sensing. These results show how disorder controls the critical magnetic field and identify the vortex glass as the key intermediate state governing the magnetic-field-induced superconductor--insulator transition.

cond-mat.supr-con↗

Universal bound on microwave dissipation in superconducting circuits

Improving the coherence of superconducting qubits is essential for advancing quantum technologies. While superconductors are theoretically perfect conductors, they consistently exhibit residual energy dissipation when driven by microwave currents, limiting coherence times. Here, we report an empirical scaling relation between microwave dissipation and the superfluid density, a bulk property of superconductors related to charge carrier density and disorder. Our analysis spans a wide range of superconducting materials and device geometries, from highly disordered amorphous films to ultra-clean systems with record-high quality factors, including resonators, 3D cavities, and transmon qubits. This scaling reveals an intrinsic bulk dissipation channel, independent of surface dielectric losses, which we attribute to nonequilibrium quasiparticles trapped within disorder-induced spatial variations of the superconducting gap, with a density set by a universal material parameter. Our findings identify an empirical coherence limit associated with intrinsic material properties and provide a data-driven basis for materials selection in future superconducting quantum circuits.

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Chiral-helical junctions in screened graphene

Reproducibility and quantization in quantum spin Hall platforms is a persisting challenge, limiting their use in hybrid realizations of topological superconductivity. We report robust and reproducible quantized transport in a graphene quantum Hall topological insulator, stabilized at low magnetic fields by screening long-range Coulomb interactions with a metallic Bi$_2$Se$_3$ back gate. Beyond quantized resistance plateaus, we demonstrate mode-resolved control via gate-defined chiral-helical junctions that selectively transmit or backscatter a single helical channel, a capability inaccessible in time-reversal symmetric quantum spin Hall systems. Targeted experiments and simulations identify contact-induced doping, effectively creating unintended chiral-helical interfaces, as a generic mechanism for quantization breakdown, which is mitigated by large area contacts that enhance edge-channel equilibration. Our findings establish metal screened graphene as a gate-tunable, interaction-driven helical system with quantized transport, spatially separable helical channels, and compatibility with superconducting proximity for topological devices.

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Evidence for correlated electron pairs and triplets in quantum Hall interferometers

Pairing of electrons is ubiquitous in electronic systems featuring attractive inter-electron interactions, as exemplified in superconductors. Counter-intuitively, it can also be mediated in certain circumstances by the repulsive Coulomb interaction alone. Quantum Hall (QH) Fabry-Pérot interferometers (FPIs) tailored in two-dimensional electron gas under a perpendicular magnetic field has been argued to exhibit such unusual electron pairing seemingly without attractive interaction. Here, we show evidence in graphene QH FPIs revealing not only a similar electron pairing at bulk filling factor nu=2 but also an unforeseen emergence of electron tripling characterized by a fractional Aharonov-Bohm flux period h/3e (h is the Planck constant and e the electron charge) at nu=3. Leveraging a novel plunger-gate spectroscopy, we demonstrate that electron pairing (tripling) involves correlated charge transport on two (three) entangled QH edge channels. This spectroscopy indicates a quantum interference flux-periodicity determined by the sum of the phases acquired by the distinct QH edge channels having slightly different interfering areas. While recent theory invokes the dynamical exchange of neutral magnetoplasmons -- dubbed neutralons -- as mediator for electron pairing, our discovery of three entangled QH edge channels with apparent electron tripling defies understanding and introduces a new three-body problem for interacting fermions.

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First-order quantum breakdown of superconductivity in amorphous superconductors

Continuous quantum phase transitions are widely assumed and frequently observed in various systems of quantum particles or spins. Their characteristic trait involves scaling laws governing a second-order, gradual suppression of the order parameter as the quantum critical point is approached. The localization of Cooper pairs in disordered superconductors and the resulting breakdown of superconductivity have long stood as a prototypical example. Here, we show a departure from this paradigm, showcasing that amorphous superconducting films of indium oxide undergo a distinctive, discontinuous first-order quantum phase transition tuned by disorder. Through systematic measurements of the plasmon spectrum in superconducting microwave resonators, we provide evidence for a marked jump of both the zero-temperature superfluid stiffness and the transition temperature at the critical disorder. This discontinuous transition sheds light on the previously overlooked role of repulsive interactions between Cooper pairs and the subsequent competition between superconductivity and insulating Cooper-pair glass. Furthermore, our investigation shows that the critical temperature of the films no longer relates to the pairing amplitude but aligns with the superfluid stiffness, consistent with the pseudogap regime of preformed Cooper pairs. Our findings raise fundamental new questions into the role of disorder in quantum phase transitions and carry implications for superinductances in quantum circuits.

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Near-power-law temperature dependence of the superfluid stiffness in strongly disordered superconductors

In BCS superconductors, the superfluid stiffness is virtually constant at low temperature and only slightly affected by the exponentially low density of thermal quasiparticles. Here, we present an experimental and theoretical study on the temperature dependence of superfluid stiffness $Θ\left(T\right)$ in a strongly disordered pseudo-gaped superconductor, amorphous $\text{InO}_{x}$, which exhibits non-BCS behavior. Experimentally, we report an unusual power-law suppression of the superfluid stiffness $δΘ\left(T\right)\propto T^{b}$ at $T\ll T_{c}$, with $b\sim1.6$, which we measured via the frequency shift of microwave resonators. Theoretically, by combining analytical and numerical methods to a model of a disordered superconductor with pseudogap and spatial inhomogeneities of the superconducting order parameter, we found a qualitatively similar low-temperature power-law behavior with exponent $b\sim1.6-3$ being disorder-dependent. This power-law suppression of the superfluid density occurs mainly due to the broad distribution of the superconducting order parameter that is known to exist in such superconductors [arXiv:1012.3630], even moderately far from the superconductor-insulator transition. The presence of the power-law dependence $δΘ\left(T\right)\propto T^{b}$ at low $T\ll T_{c}$ demonstrates the existence of low-energy collective excitations; in turn, it implies the presence of a new channel of dissipation in inhomogeneous superconductors caused by sub-gap excitations that are not quasiparticles. Our findings have implications for the use of strongly disordered superconductors as superinductance in quantum circuits.

cond-mat.supr-con↗

Electron quantum optics in graphene

In the last decade, graphene has become an exciting platform for electron optical experiments, in many aspects superior to conventional two-dimensional electron gases (2DEGs). A major advantage, besides the ultra-large mobilities, is the fine control over the electrostatics, which gives the possibility of realising gap-less and compact p-n interfaces with high precision. The latter host non-trivial states, \eg, snake states in moderate magnetic fields, and serve as building blocks of complex electron interferometers. Thanks to the Dirac spectrum and its non-trivial Berry phase, the internal (valley and sublattice) degrees of freedom, and the possibility to tailor the band structure using proximity effects, such interferometers open up a completely new playground based on novel device architectures. In this review, we introduce the theoretical background of graphene electron optics, fabrication methods used to realise electron-optical devices, and techniques for corresponding numerical simulations. Based on this, we give a comprehensive review of ballistic transport experiments and simple building blocks of electron optical devices both in single and bilayer graphene, highlighting the novel physics that is brought in compared to conventional 2DEGs. After describing the different magnetic field regimes in graphene p-n junctions and nanostructures, we conclude by discussing the state of the art in graphene-based Mach-Zender and Fabry-Perot interferometers.

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Probing the fractional quantum Hall phases in valley-layer locked bilayer MoS$_{2}$

Semiconducting transition-metal dichalcogenides (TMDs) exhibit high mobility, strong spin-orbit coupling, and large effective masses, which simultaneously leads to a rich wealth of Landau quantizations and inherently strong electronic interactions. However, in spite of their extensively explored Landau levels (LL) structure, probing electron correlations in the fractionally filled LL regime has not been possible due to the difficulty of reaching the quantum limit. Here, we report evidence for fractional quantum Hall (FQH) states at filling fractions 4/5 and 2/5 in the lowest LL of bilayer MoS$_{2}$, manifested in fractionally quantized transverse conductance plateaus accompanied by longitudinal resistance minima. We further show that the observed FQH states sensitively depend on the dielectric and gate screening of the Coulomb interactions. Our findings establish a new FQH experimental platform which are a scarce resource: an intrinsic semiconducting high mobility electron gas, whose electronic interactions in the FQH regime are in principle tunable by Coulomb-screening engineering, and as such, could be the missing link between atomically thin graphene and semiconducting quantum wells.

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Evidence for chiral supercurrent in quantum Hall Josephson junctions

Hybridizing superconductivity with the quantum Hall (QH) effects has major potential for designing novel circuits capable of inducing and manipulating non-Abelian states for topological quantum computation. However, despite recent experimental progress towards this hybridization, concrete evidence for a chiral QH Josephson junction -- the elemental building block for coherent superconducting-QH circuits -- is still lacking. Its expected signature is an unusual chiral supercurrent flowing in QH edge channels, which oscillates with a specific $2ϕ_0$ magnetic flux periodicity ($ϕ_0=h/2e$ is the superconducting flux quantum, $h$ the Planck constant and $e$ the electron charge). Here, we show that ultra-narrow Josephson junctions defined in encapsulated graphene nanoribbons exhibit such a chiral supercurrent, visible up to 8 teslas, and carried by the spin-degenerate edge channel of the QH plateau of resistance $h/2e^2\simeq 12.9$ k$Ω$. We observe reproducible $2ϕ_0$-periodic oscillation of the supercurrent, which emerges at constant filling factor when the area of the loop formed by the QH edge channel is constant, within a magnetic-length correction that we resolve in the data. Furthermore, by varying the junction geometry, we show that reducing the superconductor/normal interface length is pivotal to obtain a measurable supercurrent on QH plateaus, in agreement with theories predicting dephasing along the superconducting interface. Our findings mark a critical milestone along the path to explore correlated and fractional QH-based superconducting devices that should host non-Abelian Majorana and parafermion zero modes.

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Absence of edge reconstruction for quantum Hall edge channels in graphene devices

Electronic edge states in topological insulators have become a major paradigm in physics. The oldest and primary example is that of quantum Hall (QH) edge channels that propagate along the periphery of two-dimensional electron gases (2DEGs) under perpendicular magnetic field. Yet, despite 40 years of intensive studies using a variety of transport and scanning probe techniques, imaging the real-space structure of QH edge channels has proven difficult, mainly due to the buried nature of most 2DEGs in semiconductors. Here, we show that QH edge states in graphene are confined to a few magnetic lengths at the crystal edges by performing scanning tunneling spectroscopy up to the edge of a graphene flake on hexagonal boron nitride. These findings indicate that QH edge states are defined by boundary conditions of vanishing electronic wavefunctions at the crystal edges, resulting in ideal one-dimensional chiral channels, free of electrostatic reconstruction. We further evidence a uniform charge carrier density at the edges, contrasting with conjectures on the existence of non-topological upstream modes. The absence of electrostatic reconstruction of quantum Hall edge states has profound implications for the universality of electron and heat transport experiments in graphene-based systems and other 2D crystalline materials.

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Imaging tunable quantum Hall broken-symmetry orders in graphene

When electrons populate a flat band their kinetic energy becomes negligible, forcing them to organize in exotic many-body states to minimize their Coulomb energy. The zeroth Landau level of graphene under magnetic field is a particularly interesting strongly interacting flat band because inter-electron interactions are predicted to induce a rich variety of broken-symmetry states with distinct topological and lattice-scale orders. Evidence for these stems mostly from indirect transport experiments that suggest that broken-symmetry states are tunable by boosting the Zeeman energy or by dielectric screening of the Coulomb interaction. However, confirming the existence of these ground states requires a direct visualization of their lattice-scale orders. Here, we image three distinct broken-symmetry phases in graphene using scanning tunneling spectroscopy. We explore the phase diagram by tuning the screening of the Coulomb interaction by a low or high dielectric constant environment, and with a magnetic field. In the unscreened case, we unveil a Kekulé bond order, consistent with observations of an insulating state undergoing a magnetic-field driven Kosterlitz-Thouless transition. Under dielectric screening, a sublattice-unpolarized ground state emerges at low magnetic fields, and transits to a charge-density-wave order with partial sublattice polarization at higher magnetic fields. The Kekulé and charge-density-wave orders furthermore coexist with additional, secondary lattice-scale orders that enrich the phase diagram beyond current theory predictions. This screening-induced tunability of broken-symmetry orders may prove valuable to uncover correlated phases of matter in other quantum materials.

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A tunable Fabry-Pérot quantum Hall interferometer in graphene

Electron interferometry with quantum Hall edge channels holds promise for probing and harnessing exotic exchange statistics of non-Abelian anyons. In semiconductor heterostructures, however, quantum Hall interferometry has proven challenging and often obscured by charging effects. Here we show that high-mobility monolayer graphene equipped with a series of gate-tunable quantum point contacts that act as electron beam-splitters provides a model system to perform Fabry-Pérot quantum Hall interferometry. We observe high-visibility Aharonov-Bohm interference free of charging effects and widely tunable through electrostatic gating or magnetic field, in remarkable agreement with theory. A coherence length of $\mathbf{10 \,μm}$ at a temperature of $0.02$ K allows us to further achieve coherently-coupled double Fabry-Pérot interferometry. Our results open a new avenue for quantum Hall interferometry and the exploitation of topological excitations for quantum computation.

cond-mat.mes-hall↗

Quantum breakdown of superconductivity in low-dimensional materials

In order to understand the emergence of superconductivity it is useful to study and identify the various pathways leading to the destruction of superconductivity. One way is to use the increase in Coulomb-repulsion due to the increase in disorder, which overpowers the attractive interaction responsible for Cooper-pair formation. A second pathway, applicable to uniformly disordered materials, is the competition between superconductivity and Anderson localization, which leads to electronic granularity in which phase and amplitude fluctuations of the superconducting order parameter play a role. Finally, a third pathway is an array of superconducting islands coupled by some form of proximity-effect, due to Andreev-reflections, and which leads from a superconducting state to a state with finite resistivity, which appears like a metallic groundstate. This review summarizes recent progress in understanding of these different pathways, including experiments in low dimensional materials and application in superconducting quantum devices.

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Deficiency of the scaling collapse as an indicator of a superconductor-insulator quantum phase transition

Finite-size scaling analysis is a well-accepted method for identification and characterization of quantum phase transitions (QPTs) in superconducting, magnetic and insulating systems. We formally apply this analysis in the form suitable for QPTs in 2-dimensional superconducting films to magnetic-field driven superconductor-metal transition in 1-dimensional MoGe nanowires. Despite being obviously inapplicable to nanowires, the 2d scaling equation leads to a high-quality scaling collapse of the nanowire resistance in the temperature and resistance ranges comparable or better to what is accepted in the analysis of the films. Our results suggest that the appearance and the quality of the scaling collapse by itself is not a reliable indicator of a QPT. We have also observed a sign-change of the zero-bias anomaly (ZBA) in the non-linear resistance, occurring exactly at the critical field of the accidental QPT. This behavior is often taken as an additional confirmation of the transition. We argue that in nanowires, the non-linearity is caused by electron heating and has no relation to the critical fluctuations. Our observation suggests that similar to the scaling collapse, the sign-change of ZBA can be a misleading indicator of QPT.

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Helical quantum Hall phase in graphene on SrTiO$_3$

The ground state of charge neutral graphene under perpendicular magnetic field was predicted to be a quantum Hall topological insulator with a ferromagnetic order and spin-filtered, helical edge channels. In most experiments, however, an otherwise insulating state is observed and is accounted for by lattice-scale interactions that promote a broken-symmetry state with gapped bulk and edge excitations. We tuned the ground state of the graphene zeroth Landau level to the topological phase via a suitable screening of the Coulomb interaction with a SrTiO$_3$ high-$k$ dielectric substrate. We observed robust helical edge transport emerging at a magnetic field as low as 1 tesla and withstanding temperatures up to 110 kelvins over micron-long distances. This new and versatile graphene platform opens new avenues for spintronics and topological quantum computation.

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Low Magnetic Field Regime of a Gate-Defined Constriction in High-Mobility Graphene

We report on the evolution of the coherent electronic transport through a gate-defined constriction in a high-mobility graphene device from ballistic transport to quantum Hall regime upon increasing the magnetic field. At low field, the conductance exhibits Fabry-Pérot resonances resulting from the npn cavities formed beneath the top-gated regions. Above a critical field $B^*$ corresponding to the cyclotron radius equal to the npn cavity length, Fabry-Pérot resonances vanish and snake trajectories are guided through the constriction with a characteristic set of conductance oscillations. Increasing further the magnetic field allows us to probe the Landau level spectrum in the constriction, with distortions due to the combination of confinement and de-confinement of Landau levels in a saddle potential. These observations are confirmed by numerical calculations.

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Ionic liquid gating of InAs nanowire-based field effect transistors

We report the operation of a field-effect transistor based on a single InAs nanowire gated by an ionic liquid. Liquid gating yields very efficient carrier modulation with a transconductance value thirty time larger than standard back gating with the SiO2 /Si++ substrate. Thanks to this wide modulation we show the controlled evolution from semiconductor to metallic-like behavior in the nanowire. This work provides the first systematic study of ionic-liquid gating in electronic devices based on individual III-V semiconductor nanowires: we argue this architecture opens the way to a wide range of fundamental and applied studies from the phase-transitions to bioelectronics.

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Collective energy gap of preformed Cooper-pairs in disordered superconductors

In most superconductors the transition to the superconducting state is driven by the binding of electrons into Cooper-pairs. The condensation of these pairs into a single, phase coherent, quantum state takes place concomitantly with their formation at the transition temperature, $T_c$. A different scenario occurs in some disordered, amorphous, superconductors: Instead of a pairing-driven transition, incoherent Cooper pairs first pre-form above $T_c$, causing the opening of a pseudogap, and then, at $T_c$, condense into the phase coherent superconducting state. Such a two-step scenario implies the existence of a new energy scale, $Δ_{c}$, driving the collective superconducting transition of the preformed pairs. Here we unveil this energy scale by means of Andreev spectroscopy in superconducting thin films of amorphous indium oxide. We observe two Andreev conductance peaks at $\pm Δ_{c}$ that develop only below $T_c$ and for highly disordered films on the verge of the transition to insulator. Our findings demonstrate that amorphous superconducting films provide prototypical disordered quantum systems to explore the collective superfluid transition of preformed Cooper-pairs pairs.

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