Searcharxiv⌕ Search

arXiv subjects

Binghai Yan

Publications and source records attributed to Binghai Yan.

At least 145 records · Page 8Linked to original sources

Momentum-inversion symmetry breaking on the Fermi surface of magnetic topological insulators

Magnetic topological insulators (MnBi$_2$Te$_4$)(Bi$_2$Te$_3$)$_n$ were anticipated to exhibit magnetic energy gaps while recent spectroscopic studies did not observe them. Thus, magnetism on the surface is under debate. In this work, we propose another symmetry criterion to probe the surface magnetism. Because of both time-reversal symmetry-breaking and inversion symmetry-breaking, we demonstrate that the surface band structure violates momentum-inversion symmetry and leads to a three-fold rather than six-fold rotational symmetry on the Fermi surface if corresponding surface states couple strongly to the surface magnetism. Such a momentum-inversion symmetry violation is significant along the $Γ-K$ direction for surface bands on the (0001) plane.

cond-mat.mtrl-sci↗

Imaging Chern mosaic and Berry-curvature magnetism in magic-angle graphene

Charge carriers in magic angle graphene come in eight flavors described by a combination of their spin, valley, and sublattice polarizations. When the inversion and time reversal symmetries are broken by the substrate or by strong interactions, the degeneracy of the flavors can be lifted and their corresponding bands can be filled sequentially. Due to their non-trivial band topology and Berry curvature, each of the bands is classified by a topological Chern number, leading to the quantum anomalous Hall and Chern insulator states at integer fillings $ν$ of the bands. It has been recently predicted, however, that depending on the local atomic-scale arrangements of the graphene and the encapsulating hBN lattices, rather than being a global topological invariant, the Chern number C may become position dependent, altering transport and magnetic properties of the itinerant electrons. Using a SQUID-on-tip, we directly image the nanoscale Berry-curvature-induced equilibrium orbital magnetism, the polarity of which is governed by the local Chern number, and detect its two constituent components associated with the drift and the self-rotation of the electronic wave packets. At $ν=1$, we observe local zero-field valley-polarized Chern insulators forming a mosaic of microscopic patches of C=-1, 0, or 1, governed by the local sublattice polarization, consistent with predictions. Upon further filling, we find a first-order phase transition due to recondensation of electrons from valley K to K', which leads to irreversible flips of the local Chern number and the magnetization, and to the formation of valley domain walls giving rise to hysteretic global anomalous Hall resistance. The findings shed new light on the structure and dynamics of topological phases and call for exploration of the controllable formation of flavor domain walls and their utilization in twistronic devices.

cond-mat.mes-hall↗

Charge density wave order in kagome metal AV$_3$Sb$_5$ (A= Cs, Rb, K)

We employ polarization-resolved electronic Raman spectroscopy and density functional theory to study the primary and secondary order parameters, as well as their interplay, in the charge density wave (CDW) state of the kagome metal AV3Sb5. Previous x-ray diffraction data at 15K established that the CDW order in CsV3Sb5 comprises of a 2x2x4 structure: one layer of inverse-star-of-David and three consecutive layers of star-of-David pattern. We analyze the lattice distortions based the 2x2x4 structure at 15K, and find that U lattice distortion is the primary order parameter while M and L distortions are secondary order parameters for Vanadium displacements. This conclusion is confirmed by the calculation of bare susceptibility that shows a broad peak at around qz=0.25 along the hexagonal Brillouin zone face central line (U-line). We also identify several phonon modes emerging in the CDW state, which are lattice vibration modes related to V and Sb atoms as well as alkali atoms. The detailed temperature evolution of these modes' frequencies, HWHM, and integrated intensities support a phase diagram with two successive structural phase transitions in CsV3Sb5: the first one with a primary order parameter appearing at TS=94K and the second isostructural one appearing at around 70K.

cond-mat.str-el↗

Twisted photovoltaics at terahertz frequencies from momentum shift current

The bulk photovoltaic effect (BPVE) converts light into a coherent dc current at zero bias, through what is commonly known as the shift current. This current has previously been attributed to the displacement of the electronic wave function center in real space, when the sample is excited by light. We reveal that materials like twisted bilayer graphene (TBG) with a flatband dispersion are uniquely suited to maximize the BPVE because they lead to an enhanced shift in the momentum space, unlike any previously known shift current mechanism. We identify properties of quantum geometry, which go beyond the quantum geometric tensor, and are unrelated to Berry charges, as the physical origin of the large BPVE we observe in TBG. Our calculations show that TBG with a band gap of several meV exhibits a giant BPVE in a range of 0.2-1 THz, which represents the strongest BPVE reported so far at this frequency in a two-dimensional material and partially persists even a room temperature. Our paper provides a design principle for shift current generation, which applies to a broad range of twisted heterostructures with the potential to overcome the so-called "terahertz gap" in THz sensing.

cond-mat.mes-hall↗

Non-reciprocal charge transport in an intrinsic magnetic topological insulator MnBi2Te4

Symmetries, quantum geometries and electronic correlations are among the most important ingredients of condensed matters, and lead to nontrivial phenomena in experiments, for example, non-reciprocal charge transport. Here we report the non-reciprocal charge transport in the intrinsic magnetic topological insulator MnBi2Te4. The current direction relevant resistance is observed at chiral edges, which is magnetically switchable, edge position sensitive and septuple layer number controllable. Applying gate voltage can effectively tune the non-reciprocal resistance. The observation and manipulation of non-reciprocal charge transport indicate the fundamental role of chirality in charge transport of MnBi2Te4, and pave ways to develop van der Waals spintronic devices by chirality engineering.

cond-mat.mes-hall↗

Observation of anomalous amplitude modes in the kagome metal CsV$_3$Sb$_5$

The charge-density wave (CDW) phase is often accompanied by the condensation of a soft acoustic phonon mode, giving rise to lattice distortion and charge density modulation. This picture was challenged for the recently discovered kagome metal CsV$_3$Sb$_5$, based on the evidence of absence of soft phonons. Here we report the observation of Raman-active CDW amplitude modes in this material, which are collective excitations typically thought to emerge out of frozen soft phonons. The amplitude modes strongly hybridize with other superlattice modes, imparting them with clear temperature-dependent frequency shift and broadening, rarely seen in other known CDW materials. Both the mode mixing and the large amplitude mode frequencies suggest that the CDW exhibits the character of strong electron-phonon coupling, a regime in which acoustic phonon softening can cease to exist. The observation of amplitude modes in the absence of soft phonons highlights the unconventional nature of the CDW in CsV$_3$Sb$_5$.

cond-mat.mtrl-sci↗

Exchange-biased topological transverse thermoelectric effects in a Kagome ferrimagnet

Kagome metal TbMn6Sn6 was recently discovered to be a ferrimagnetic topological Dirac material by scanning tunneling microscopy/spectroscopy measurements. Here, we report the observation of large anomalous Nernst effect and anomalous thermal Hall effect in this compound. The anomalous transverse transport is consistent with the Berry curvature contribution from the massive Dirac gaps in the 3D momentum space as demonstrated by our first-principles calculations. Furthermore, the transverse thermoelectric transport exhibits asymmetry with respect to the applied magnetic field, i.e., an exchange-bias behavior. Together, these features place TbMn6Sn6 as a promising system for the outstanding thermoelectric performance based on anomalous Nernst effect.

cond-mat.mtrl-sci↗

Direct observation of vortices in an electron fluid

Vortices are the hallmarks of hydrodynamic flow. Recent studies indicate that strongly-interacting electrons in ultrapure conductors can display signatures of hydrodynamic behavior including negative nonlocal resistance, Poiseuille flow in narrow channels, and a violation of the Wiedemann-Franz law. Here we provide the first visualization of whirlpools in an electron fluid. By utilizing a nanoscale scanning superconducting quantum interference device on a tip (SQUID-on-tip) we image the current distribution in a circular chamber connected through a small aperture to an adjacent narrow current carrying strip in high-purity type-II Weyl semimetal WTe2. In this geometry, the Gurzhi momentum diffusion length and the size of the aperture determine the vortex stability phase diagram. We find that the vortices are present only for small apertures, whereas the flow is laminar (non-vortical) for larger apertures, consistent with the theoretical analysis of the hydrodynamic regime and in contrast to the expectations of ballistic transport in WTe2 at low temperatures. Moreover, near the vortical-to-laminar transition, we observe a single vortex in the chamber splitting into two vortices, a behavior that can occur only in the hydrodynamic regime and cannot be sustained by ballistic transport. These findings suggest a novel mechanism of hydrodynamic flow: instead of the commonly considered electron-electron scattering at the bulk, which becomes extremely weak at low temperatures, the spatial diffusion of charge carriers' momenta is enabled by small-angle scattering at the planar surfaces of thin pure crystals. This surface-induced para-hydrodynamics opens new avenues for exploring and utilizing electron fluidics in high-mobility electron systems.

cond-mat.mes-hall↗

Facet dependent surface energy gap on magnetic topological insulators

Magnetic topological insulators (MnBi$_2$Te$_4$)(Bi$_2$Te$_3$)$_n$ ($n=0,1,2,3$) are promising to realize exotic topological states such as the quantum anomalous Hall effect (QAHE) and axion insulator (AI), where the Bi$_2$Te$_3$ layer introduces versatility to engineer electronic and magnetic properties. However, whether surface states on the Bi$_2$Te$_3$ terminated facet are gapless or gapped is debated, and its consequences in thin-film properties are rarely discussed. In this work, we find that the Bi$_2$Te$_3$ terminated facets are gapless for $n \ge 1$ compounds by calculations. Despite that the surface Bi$_2$Te$_3$ (one layer or more) and underlying MnBi$_2$Te$_4$ layers hybridize and give rise to a gap, such a hybridization gap overlaps with bulk valence bands, leading to a gapless surface after all. Such a metallic surface poses a fundamental challenge to realize QAHE or AI, which requires an insulating gap in thin films with at least one Bi$_2$Te$_3$ surface. In theory, the insulating phase can still be realized in a film if both surfaces are MnBi$_2$Te$_4$ layers. Otherwise, it requires that the film thickness is less than 10$\sim$20 nm to push down bulk valence bands via the size effect. Our work paves the way to understand surface states and design bulk-insulating quantum devices in magnetic topological materials.

cond-mat.mtrl-sci↗

Truly local topological dynamics of driven defects in Chern insulator

Robust zero modes supported by defects is one of the key features of topological matter. Its presence renders a system topologically inhomegeneuous, thus having no well-defined global topological invariant. The quantities labeling different areas of the sample according to their topological state were dubbed local topological markers. Here we study their dynamics and the possibility to control their distribution over the sample. We suggest a new perspective on the evolution of local markers. It gives a clear physical description of the markers evolution in terms of response functions and the ease of measurement. Furthermore, new markers' equations of motion are truly local, being ensured that the current of the marker exists and obeys the lattice continuity equation. The formalism presented does not rely on the single-particle quantities therefore might be extended to interacting systems.

cond-mat.stat-mech↗

Visualization of Topological Boundary Modes Manifesting Topological Nodal-Point Superconductivity

The extension of the topological classification of band insulators to topological semimetals gave way to the topology classes of Dirac, Weyl, and nodal line semimetals with their unique Fermi arc and drum head boundary modes. Similarly, there are several suggestions to employ the classification of topological superconductors for topological nodal superconductors with Majorana boundary modes. Here, we show that the surface 1H termination of the transition metal dichalcogenide compound 4Hb-TaS$_2$, in which 1T-TaS$_2$ and 1H-TaS$_2$ layers are interleaved, has the phenomenology of a topological nodal point superconductor. We find in scanning tunneling spectroscopy a residual density of states within the superconducting gap. An exponentially decaying bound mode is imaged within the superconducting gap along the boundaries of the exposed 1H layer characteristic of a gapless Majorana edge mode. The anisotropic nature of the localization length of the edge mode aims towards topological nodal superconductivity. A zero-bias conductance peak is further imaged within fairly isotropic vortex cores. All our observations are accommodated by a theoretical model of a two-dimensional nodal Weyl-like superconducting state, which ensues from inter-orbital Cooper pairing. The observation of an intrinsic topological nodal superconductivity in a layered material will pave the way for further studies of Majorana edge modes and its applications in quantum information processing.

cond-mat.supr-con↗

Tracing out the Berry curvature dipole and multipoles in second harmonic Hall responses of time-reversal symmetric insulators

Various nonlinear characteristics of solid states, such as the circular photogalvanic effect of time-reversal symmetric insulators, the quantized photogalvanic effect of Weyl semimetals, and the nonlinear Hall effect of time-reversal symmetric metals, have been associated with the Berry curvature dipole (BCD). Here, we explore the question of whether the Berry curvature dipole and multipoles of time-reversal symmetric insulators can be traced in the nonlinear optical responses. We performed real-time time-dependent density functional theory calculations and examined the second harmonic generation susceptibility tensors. The two-band term of the susceptibility tensor is sharply proportional to the interband BCD, dominating over the Hall response once the cancellation effect of the multiple reflection symmetries is lifted. We suggest that the nonlinear Hall component of the second-harmonic spectra of insulators can also be utilized as an effective tool to extract the band structure geometry through Berry curvature dipole and possibly multipoles.

cond-mat.mes-hall↗

Mixed axial-gravitational anomaly from emergent curved spacetime in nonlinear charge transport

In 3+1 dimensional spacetime, two vector gauge anomalies are known: The chiral anomaly and the mixed axial-gravitational anomaly. While the former is well documented and tied to the presence of a magnetic field, the latter instead requires a nonzero spacetime curvature, which has made it rather difficult to study. In this work, we show that a quantum anomaly arises in the second-order electrical response for zero magnetic field, which creates a dc-current that can be either longitudinal or transverse to electric field. Consequently, the continuity equation for the chiral current is not conserved at order $τ^{-1}$, where $τ$ is the quasiparticle relaxation time. We can identify the anomaly as a mixed axial-gravitational one, and predict a material in which the anomaly-induced current can be isolated in a purely electrical measurement. Our findings indicate that charge transport generically derives from quasiparticle motion in an emergent curved spacetime, with potentially far-reaching consequences for all types of response functions.

cond-mat.mes-hall↗

Higher-order, quantum magnetic inductions in chiral topological materials

The classic magnetic induction effect is usually considered in electric circuits or conductor coils. In this work, we propose quantum induction effects induced by the Berry curvature in homogenous solids. Two different types of quantum inductions are identified in the higher order of a magnetic field. They are closely related to the magnetic-field-induced anomalous velocity proportional to the Berry curvature so that both quantum inductions become significantly enhanced near Weyl points. Further, we propose an ac-magnetic-field measurement to detect quantum induction effects and distinguish them from classical induction.

cond-mat.mtrl-sci↗

Roton pair density wave and unconventional strong-coupling superconductivity in a topological kagome metal

The transition-metal kagome lattice materials host frustrated, correlated, and topological quantum states of matter. Recently, a new family of vanadium-based kagome metals AV3Sb5 (A=K, Rb, and Cs) with topological band structures has been discovered. These layered compounds are nonmagnetic and undergo charge density wave transitions before developing superconductivity at low temperatures. Here we report the observation of unconventional superconductivity and pair density wave (PDW) in CsV3Sb5 using scanning tunneling microscope/spectroscopy (STM/STS) and Josephson STS. We find that CsV3Sb5 exhibits a V-shaped pairing gap Δ~0.5 meV and is a strong-coupling superconductor (2Δ/kBTc~5) that coexists with 4a0 unidirectional and 2a0X2a0 charge order. Remarkably, we discover a 3Q PDW accompanied by bidirectional 4a0/3 spatial modulations of the superconducting gap, coherence peak and gap-depth in the tunneling conductance. We term this novel quantum state a roton-PDW associated with an underlying vortex-antivortex lattice that can account for the observed conductance modulations. Probing the electronic states in the vortex halo in an applied magnetic field, in strong-field that suppresses superconductivity, and in zero-field above Tc reveals that the PDW is a primary state responsible for an emergent pseudogap and intertwined electronic order. Our findings show striking analogies and distinctions to the phenomenology of high-Tc cuprate superconductors, and provide groundwork for understanding the microscopic origin of correlated electronic states and superconductivity in vanadium-based kagome metals.

cond-mat.supr-con↗

Spatial symmetry constraint of charge-ordered kagome superconductor CsV$_3$Sb$_5$

Elucidating the symmetry of intertwined orders in exotic superconductors is at the quantum frontier. Recent surface sensitive studies of the topological kagome superconductor CsV$_3$Sb$_5$ discovered a cascade 4a$_0$ superlattice below the charge density wave (CDW) ordering temperature, which can be related to the pair density modulations in the superconducting state. If the 4a$_0$ phase is a bulk and intrinsic property of the kagome lattice, this would form a striking analogy to the stripe order and pair density wave discovered in the cuprate high-temperature superconductors, and the cascade ordering found in twisted bilayer graphene. High-resolution X-ray diffraction has recently been established as an ultra-sensitive probe for bulk translational symmetry-breaking orders, even for short-range orders at the diffusive limit. Here, combining high-resolution X-ray diffraction, scanning tunneling microscopy and scanning transmission electron microscopy, we demonstrate that the 4a$_0$ superstructure emerges uniquely on the surface and hence exclude the 4a$_0$ phase as the origin of any bulk transport or spectroscopic anomaly. Crucially, we show that our detected 2$\times$2$\times$2 CDW order breaks the bulk rotational symmetry to C2, which can be the driver for the bulk nematic orders and nematic surface superlattices including the 4a$_0$ phase. Our high-resolution data impose decisive spatial symmetry constraints on emergent electronic orders in the kagome superconductor CsV$_3$Sb$_5$.

cond-mat.mtrl-sci↗

Geometry of the charge density wave in kagom${é}$ metal AV$_{3}$Sb$_{5}$

Kagom${é}$ lattice is a fertile platform for topological and intertwined electronic excitations. Recently, experimental evidence of an unconventional charge density wave (CDW) is observed in a Z2 kagom${é}$ metal AV$_{3}$Sb$_{5}$ (A= K, Cs, Rb). This observation triggers wide interests on the interplay between frustrated crystal structure and Fermi surface instabilities. Here we analyze the lattice effect and its impact on CDW in AV$_{3}$Sb$_{5}$. Based on published experimental data, we show that the CDW induced structural distortions is consistent with the theoretically predicted inverse star-of-David pattern, which preserves the $D_{6h}$ symmetry in the kagom${é}$ plane but breaks the sixfold rotational symmetry of the crystal due to the phase shift between kagom${é}$ layers. The coupling between the lattice and electronic degrees of freedom yields a weak first order structural transition without continuous change of lattice dynamics. Our result emphasizes the fundamental role of lattice geometry in proper understanding of unconventional electronic orders in AV$_{3}$Sb$_{5}$.

cond-mat.str-el↗

Quasiparticle Interference Studies of Quantum Materials

Exotic electronic states are realized in novel quantum materials. This field is revolutionized by the topological classification of materials. Such compounds necessarily host unique states on their boundaries. Scanning tunneling microscopy studies of these surface states have provided a wealth of spectroscopic characterization, with the successful cooperation of ab initio calculations. The method of quasiparticle interference imaging proves to be particularly useful for probing the dispersion relation of the surface bands. Herein, how a variety of additional fundamental electronic properties can be probed via this method is reviewed. It is demonstrated how quasiparticle interference measurements entail mesoscopic size quantization and the electronic phase coherence in semiconducting nanowires; helical spin protection and energy-momentum fluctuations in a topological insulator; and the structure of the Bloch wave function and the relative insusceptibility of topological electronic states to surface potential in a topological Weyl semimetal.

cond-mat.mes-hall↗