arXiv subjects

C. A. Marrache-Kikuchi

Publications and source records attributed to C. A. Marrache-Kikuchi.

At least 19 recordsLinked to original sources

arXiv2026

The CROSS experiment: detector construction, background projection, and sensitivity to $^{100}$Mo $0\nu2β$ decay

The CROSS experiment to search for neutrinoless double-beta ($0\nu2β$) decay in $^{100}$Mo with the help of an array of scintillating cryogenic calorimeters, containing 4.9 kg of $^{100}$Mo, has been ongoing in a low-background setup at the Canfranc underground laboratory (Spain) since mid-November 2025. In this paper, we present the construction of the CROSS detector and the description of Geant4-based Monte Carlo simulations of expected background in the region of interest. The simulations predict the background index in a 100-keV-wide interval centered at the $Q$-value of $^{100}$Mo (3034 keV) on the level of 3.2(5) $\times$ 10$^{-3}$ cnts/keV/kg/yr. Taking into account an 18% deadtime induced by the muon veto cut and a typical 90% duty cycle of the facility, such background level would allow to reach the world-leading sensitivity to $^{100}$Mo $0\nu2β$ decay (lim $T_{1/2} \sim 4 \times 10^{24}$ yr) in 1 year of data taking. Considering conservatively a factor 3 (10) worse background index due to unpredictable radioactive contamination of construction materials and/or detector performance, a 2-yr-long operation of the CROSS array would be still compatible with the best (competitive) sensitivity to $0\nu2β$ decay in $^{100}$Mo.

physics.ins-det↗

arXiv2025

Muon veto system for the CROSS double-beta decay search experiment

In preparation to the CROSS experiment at the Canfranc underground laboratory (Spain) $-$ aiming to search for neutrinoless double-beta ($0νββ$) decay of $^{100}$Mo using low-temperature detectors with heat-scintillation readout $-$ we report on development of a dedicated muon veto system. The need for the muon veto in CROSS is caused by a comparatively high residual cosmic muon flux at the experimental site ($\sim$20 $μ$/m$^2$/h), being a dominant background in the region of interest (ROI) at $\sim$3 MeV. Thus, we installed the muon veto system around the CROSS low-background setup, forming four lateral, one top, and four bottom sectors. In this paper we describe the design, construction and operation of the CROSS muon veto system, as well as its optimization and validation by comparing dedicated Monte Carlo (MC) simulations of muons with low-temperature measurements in the setup. We demonstrate a stable operation of the veto system with the average trigger rates compatible with MC simulations. Also, we investigated two muon trigger logics based on coincidences with either 2 sectors or a single sector of the veto. The MC study shows that, in combination with the multiplicity cut of thermal detectors, these trigger logics allow to reject 99.2\% and 99.7\% of muon-induced events in the ROI, respectively. Despite a comparatively high dead time ($\sim$18\%) introduced by coincidences with any of nine sectors of the veto $-$ the adopted strategy $-$ the muon-induced background in the ROI of the CROSS experiment can be reduced down to $\sim$2 $\times 10^{-3}$ cnts/keV/kg/yr, i.e., an acceptable level compatible with a high-sensitivity $0νββ$ decay search foreseen in CROSS.

physics.ins-det↗

arXiv2025

Cryogenic light detectors with thermal signal amplification for $0νββ$ search experiments

As a step towards the realization of cryogenic-detector experiments to search for neutrinoless double-beta decay (such as CROSS, BINGO, and CUPID), we investigated a batch of 10 Ge light detectors (LDs) assisted by Neganov-Trofimov-Luke (NTL) signal amplification. Each LD was assembled with a large cubic light-emitting crystal (45 mm side) using the recently developed CROSS mechanical structure. The detector array was operated at milli-Kelvin temperatures in a pulse-tube cryostat at the Canfranc underground laboratory in Spain. We achieved good performance with scintillating bolometers from CROSS, made of Li$_{2}$$^{100}$MoO$_4$ crystals and used as reference detectors of the setup, and with all LDs tested (except for a single device that encountered an electronics issue). No leakage current was observed for 8 LDs with an electrode bias up to 100 V. Operating the LDs at an 80 V electrode bias applied in parallel, we obtained a gain of around 9 in the signal-to-noise ratio of these devices, allowing us to achieve a baseline noise RMS of $O$(10 eV). Thanks to the strong current polarization of the temperature sensors, the time response of the devices was reduced to around half a millisecond in rise time. The achieved performance of the LDs was extrapolated via simulations of pile-up rejection capability for several configurations of the CUPID detector structure. Despite the sub-optimal noise conditions of the LDs (particularly at high frequencies), we demonstrated that the NTL technology provides a viable solution for background reduction in CUPID.

physics.ins-det↗

arXiv2024

Precise $^{113}$Cd $β$ decay spectral shape measurement and interpretation in terms of possible $g_A$ quenching

Highly forbidden $β$ decays provide a sensitive test to nuclear models in a regime in which the decay goes through high spin-multipole states, similar to the neutrinoless double-$β$ decay process. There are only 3 nuclei ($^{50}$V, $^{113}$Cd, $^{115}$In) which undergo a $4^{\rm th}$ forbidden non-unique $β$ decay. In this work, we compare the experimental $^{113}$Cd spectrum to theoretical spectral shapes in the framework of the spectrum-shape method. We measured with high precision, with the lowest energy threshold and the best energy resolution ever, the $β$ spectrum of $^{113}$Cd embedded in a 0.43 kg CdWO$_4$ crystal, operated over 26 days as a bolometer at low temperature in the Canfranc underground laboratory (Spain). We performed a Bayesian fit of the experimental data to three nuclear models (IBFM-2, MQPM and NSM) allowing the reconstruction of the spectral shape as well as the half-life. The fit has two free parameters, one of which is the effective weak axial-vector coupling constant, $g_A^{\text{eff}}$, which resulted in $g_A^{\text{eff}}$ between 1.0 and 1.2, compatible with a possible quenching. Based on the fit, we measured the half-life of the $^{113}$Cd $β$ decay including systematic uncertainties as $7.73^{+0.60}_{-0.57} \times 10^{15}$ yr, in agreement with the previous experiments. These results represent a significant step towards a better understanding of low-energy nuclear processes.

nucl-ex↗

arXiv2024

Development of large-volume $^{130}$TeO$_2$ bolometers for the CROSS $2β$ decay search experiment

We report on the development of thermal detectors based on large-size tellurium dioxide crystals (45x45x45 mm), containing tellurium enriched in $^{130}$Te to about 91%, for the CROSS double-beta decay experiment. A powder used for the crystals growth was additionally purified by the directional solidification method, resulting in the reduction of the concentration of impurities by a factor 10, to a few ppm of the total concentration of residual elements (the main impurity is Fe). The purest part of the ingot (the first ~200 mm, about 80% of the total length of the cylindrical part of the ingot) was determined by scanning segregation profiles of impurities and used for the $^{130}$TeO$_2$ powder production with no evidence of re-contamination. The crystal growth was verified with precursors produced from powder with natural Te isotopic composition, and two small-size (20x20x10 mm) samples were tested at a sea-level laboratory showing high bolometric and spectrometric performance together with acceptable $^{210}$Po content (below 10 mBq/kg). This growth method was then applied for the production of six large cubic $^{130}$TeO$_2$ crystals and 4 of them were taken randomly to be characterized at the Canfranc underground laboratory, in the CROSS-dedicated low-background cryogenic facility. Two $^{130}$TeO$_2$ samples were coated with a thin, $O$(100 nm), metal film in form of Al layer (on 4 sides) or AlPd grid (on a single side) to investigate the possibility to tag surface events by pulse-shape discrimination. Similarly to the small natural precursors, large-volume $^{130}$TeO$_2$ bolometers show high performance and even better internal purity ($^{210}$Po activity $\sim$ 1 mBq/kg, while activities of $^{228}$Th and $^{226}$Ra are below 0.01 mBq/kg), satisfying requirements for the CROSS and, potentially, next-generation experiments.

physics.ins-det↗

arXiv2024

A novel mechanical design of a bolometric array for the CROSS double-beta decay experiment

The CROSS experiment will search for neutrinoless double-beta decay using a specific mechanical structure to hold thermal detectors. The design of the structure was tuned to minimize the background contribution, keeping an optimal detector performance. A single module of the structure holds two scintillating bolometers (with a crystal size of 45x45x45 mm and a Ge slab facing the crystal's upper side) in the Cu frame, allowing for a modular construction of a large-scale array. Two designs are released: the initial $Thick$ version contains around 15% of Cu over the crystal mass (lithium molybdate, LMO), while this ratio is reduced to ~6% in a finer ($Slim$) design. Both designs were tested extensively at aboveground (IJCLab, France) and underground (LSC, Spain) laboratories. In particular, at LSC we used a pulse-tube-based CROSS facility to operate a 6-crystal array of LMOs enriched/depleted in $^{100}$Mo. The tested LMOs show high spectrometric performance in both designs; notably, the measured energy resolution is 5--7 keV FWHM at 2615 keV $γ$s, nearby the Q-value of $^{100}$Mo (3034 keV). Due to the absence of a reflective cavity around LMOs, a low scintillation signal is detected by Ge bolometers: ~0.3 keV (150 photons) for 1-MeV $γ$($β$) LMO-event. Despite that, an acceptable separation between $α$ and $γ$($β$) events is achieved with most devices. The highest efficiency is reached with light detectors in the $Thick$ design thanks to a lower baseline noise width (0.05--0.09 keV RMS) when compared to that obtained in the $Slim$ version (0.10--0.35 keV RMS). Given the pivotal role of bolometric photodetectors for particle identification and random coincidences rejection, we will use the structure here described with upgraded light detectors, featuring thermal signal amplification via the Neganov-Trofimov-Luke effect, as also demonstrated in the present work.

physics.ins-det↗

arXiv2024

BINGO innovative assembly for background reduction in bolometric $0νββ$ experiments

BINGO is a project aiming to set the grounds for large-scale bolometric neutrinoless double-beta-decay experiments capable of investigating the effective Majorana neutrino mass at a few meV level. It focuses on developing innovative technologies (a detector assembly, cryogenic photodetectors and active veto) to achieve a very low background index, of the order of $10^{-5}$ counts/(keV kg yr) in the region of interest. The BINGO demonstrator, called MINI-BINGO, is designed to investigate the promising double-beta-decay isotopes $^{100}$Mo and $^{130}$Te and it will be composed of Li$_2$MoO$_4$ and TeO$_2$ crystals coupled to bolometric light detectors and surrounded by a Bi$_4$Ge$_3$O$_{12}$-based veto. This will allow us to reject a significant background in bolometers caused by surface contamination from $α$-active radionuclides by means of light yield selection and to mitigate other sources of background, such as surface contamination from $β$-active radionuclides, external $γ$ radioactivity, and pile-up due to random coincidence of background events. This paper describes an R\&D program towards the BINGO goals, particularly focusing on the development of an innovative assembly designed to reduce the passive materials within the line of sight of the detectors, which is expected to be a dominant source of background in next-generation bolometric experiments. We present the performance of two prototype modules -- housing four cubic (4.5-cm side) Li$_2$MoO$_4$ crystals in total -- operated in the Canfranc underground laboratory in Spain within a facility developed for the CROSS double-beta-decay experiment.

physics.ins-det↗

arXiv2023

Test of $^{116}$CdWO$_4$ and Li$_2$MoO$_4$ scintillating bolometers in the CROSS underground facility with upgraded detector suspension

In preparation to the CROSS $2β$ decay experiment, we installed a new detector suspension with magnetic dumping inside a pulse-tube cryostat of a dedicated low-background facility at the LSC (Spain). The suspension was tested with two scintillating bolometers based on large-volume 116CdWO4 (CWO-enr) and Li2MoO4 (LMO) crystals. The former, a reference device, was used for testing new noise conditions and for comparing bolometric performance of an advanced Li2MoO4 crystal developed in the framework of the CLYMENE project, in view of next-generation double-beta decay experiments like CUPID. We cooled down detectors to 15 mK and achieved high performance for all tested devices. In particular both CWO-enr and LMO bolometers demonstrated the energy resolution of 6 keV FWHM for the 2.6 MeV gamma quanta, among the best for thermal detectors based on such compounds. The baseline noise resolution (FWHM) of the CWO-enr detector was improved by 2 keV, compared to the best previous measurement of this detector in the CROSS facility, while the noise of the Ge-based optical bolometer was improved by a factor 2, to 100 eV FWHM. Despite of the evident progress in the improving of noise conditions of the set-up, we see high-frequency harmonics of a pulse-tube induced noise, suggesting a noise pick-up by cabling. Another Ge light detector was assisted with the signal amplification exploiting the Neganov-Trofimov-Luke effect, which allowed to reach 20 eV FWHM noise resolution by applying 60 V electrode bias. Highly-efficient particle identification was achieved with both detectors, despite a low scintillation efficiency of the LMO material. The radiopurity level of the LMO crystal is rather high; only traces of 210Po and 226Ra were detected (0.1 mBq/kg each), while the 228Th activity is expected to be at least an order of magnitude lower, as well as a 40K activity is found to be < 6 mBq/kg.

physics.ins-det↗

arXiv2023

Li$_2$$^{100\textrm{depl}}$MoO$_4$ Scintillating Bolometers for Rare-Event Search Experiments

We report on the development of scintillating bolometers based on lithium molybdate crystals containing molybdenum depleted in the double-$β$ active isotope $^{100}$Mo (Li$_2$$^{100\textrm{depl}}$MoO$_4$). We used two Li$_2$$^{100\textrm{depl}}$MoO$_4$ cubic samples, 45 mm side and 0.28 kg each, produced following purification and crystallization protocols developed for double-$β$ search experiments with $^{100}$Mo-enriched Li$_2$MoO$_4$ crystals. Bolometric Ge detectors were utilized to register scintillation photons emitted by the Li$_2$$^{100\textrm{depl}}$MoO$_4$ crystal scintillators. The measurements were performed in the CROSS cryogenic set-up at the Canfranc underground laboratory (Spain). We observed that the Li$_2$$^{100\textrm{depl}}$MoO$_4$ scintillating bolometers are characterized by excellent spectrometric performance ($\sim$3--6 keV FWHM at 0.24--2.6 MeV $γ$'s), moderate scintillation signal ($\sim$0.3--0.6 keV/MeV depending on light collection conditions) and high radiopurity ($^{228}$Th and $^{226}$Ra activities are below a few $μ$Bq/kg), comparable to the best reported results of low-temperature detectors based on Li$_2$MoO$_4$ with natural or $^{100}$Mo-enriched molybdenum content. Prospects of Li$_2$$^{100\textrm{depl}}$MoO$_4$ bolometers for use in rare-event search experiments are briefly discussed.

physics.ins-det↗

arXiv2023

Enhanced light signal for the suppression of pile-up events in Mo-based bolometers for the $0νββ$ decay search

Random coincidences of events could be one of the main sources of background in the search for neutrino-less double-beta decay of $^{100}$Mo with macro-bolometers, due to their modest time resolution. Scintillating bolometers as those based on Li$_2$MoO$_4$ crystals and employed in the CROSS and CUPID experiments can eventually exploit the coincident fast signal detected in a light detector to reduce this background. However, the scintillation provides a modest signal-to-noise ratio, making difficult a pile-up pulse-shape recognition and rejection at timescales shorter than a few ms. Neganov-Trofimov-Luke assisted light detectors (NTL-LDs) offer the possibility to effectively increase the signal-to-noise ratio, preserving a fast time-response, and enhance the capability of pile-up rejection via pulse shape analysis. In this article we present: a) an experimental work performed with a Li$_2$MoO$_4$ scintillating bolometer, studied in the framework of the CROSS experiment, and utilizing a NTL-LD; b) a simulation method to reproduce, synthetically, randomly coincident two-neutrino double-beta decay events; c) a new analysis method based on a pulse-shape discrimination algorithm capable of providing high pile-up rejection efficiencies. We finally show how the NTL-LDs offer a balanced solution between performance and complexity to reach background index $\sim$$10^{-4}$ counts/keV/kg/year with 280~g Li$_2$MoO$_4$ ($^{100}$Mo enriched) bolometers at 3034 keV, the Q-value of the double-beta decay, and target the goal of a next generation experiment like CUPID.

physics.ins-det↗

arXiv2021

Phonon-mediated crystal detectors with metallic film coating capable of rejecting $α$ and $β$ events induced by surface radioactivity

Phonon-mediated particle detectors based on single crystals and operated at millikelvin temperatures are used in rare-event experiments for neutrino physics and dark-matter searches. In general, these devices are not sensitive to the particle impact point, especially if the detection is mediated by thermal phonons. In this Letter, we demonstrate that excellent discrimination between interior and surface $β$ and $α$ events can be achieved by coating a crystal face with a thin metallic film, either continuous or in the form of a grid. The coating affects the phonon energy down-conversion cascade that follows the particle interaction, leading to a modified signal shape for close-to-film events. An efficient identification of surface events was demonstrated with detectors based on a rectangular $20 \times 20 \times 10$ mm$^3$ Li$_2$MoO$_4$ crystal coated with a Pd normal-metal film (10~nm thick) and with Al-Pd superconductive bi-layers (100~nm-10~nm thick) on a $20 \times 20$ mm$^2$ face. Discrimination capabilities were tested with $^{238}$U sources emitting both $α$ and $β$ particles. Surface events are identified for energy depositions down to millimeter-scale depths from the coated surface. With this technology, a substantial improvement of the background figure can be achieved in experiments searching for neutrinoless double-beta decay.

physics.ins-det↗

arXiv2020

The CROSS Experiment: Rejecting Surface Events by PSD Induced by Superconducting Films

Neutrinoless double beta ($0νββ$) decay is a hypothetical rare nuclear transition ($T_{1/2}>10^{26}$ y). Its observation would provide an important insight about the nature of neutrinos (Dirac or Majorana particle) demonstrating that the lepton number is not conserved. This decay can be investigated with bolometers embedding the double beta decay isotope ($^{76}$Ge, $^{82}$Se, $^{100}$Mo, $^{116}$Cd, $^{130}$Te...), which perform as low temperature calorimeters (10 mK) detecting particle interactions via a small temperature rise read out by a dedicated thermometer. CROSS (Cryogenic Rare-event Observatory with Surface Sensitivity) aims at the development of bolometric detectors (Li$_{2}$MoO$_{4}$ and TeO$_{2}$) capable of discriminating surface $α$ and $β$ interactions by exploiting superconducting properties of Al film deposited on the crystal surface. We report in this paper the results of tests on prototypes performed at CSNSM (Orsay, France) that showed the capability of a-few-$μ$m-thick superconducting Al film deposited on crystal surface to discriminate surface $α$ from bulk events, thus providing the detector with the required surface sensitivity capability. The CROSS technology would further improve the background suppression and simplify the detector construction with a view to future competitive double beta decay searches.

physics.ins-det↗

arXiv2019

The $0\nu2β$-decay CROSS experiment: preliminary results and prospects

Neutrinoless double-beta decay is a key process in particle physics. Its experimental investigation is the only viable method that can establish the Majorana nature of neutrinos, providing at the same time a sensitive inclusive test of lepton number violation. CROSS (Cryogenic Rare-event Observatory with Surface Sensitivity) aims at developing and testing a new bolometric technology to be applied to future large-scale experiments searching for neutrinoless double-beta decay of the promising nuclei $^{100}$Mo and $^{130}$Te. The limiting factor in large-scale bolometric searches for this rare process is the background induced by surface radioactive contamination, as shown by the results of the CUORE experiment. The basic concept of CROSS consists of rejecting this challenging background component by pulse-shape discrimination, assisted by a proper coating of the faces of the crystal containing the isotope of interest and serving as energy absorber of the bolometric detector. In this paper, we demonstrate that ultra-pure superconductive Al films deposited on the crystal surfaces act successfully as pulse-shape modifiers, both with fast and slow phonon sensors. Rejection factors higher than 99.9% of $α$ surface radioactivity have been demonstrated in a series of prototypes based on crystals of Li$_2$MoO$_4$ and TeO$_2$. We have also shown that point-like energy depositions can be identified up to a distance of $\sim 1$ mm from the coated surface. The present program envisions an intermediate experiment to be installed underground in the Canfranc laboratory (Spain) in a CROSS-dedicated facility. This experiment, comprising $\sim 3\times 10^{25}$ nuclei of $^{100}$Mo, will be a general test of the CROSS technology as well as a worldwide competitive search for neutrinoless double-beta decay, with sensitivity to the effective Majorana mass down to 70 meV in the most favorable conditions.

nucl-ex↗

arXiv2019

Sample-based calibration for cryogenic broadband microwave reflectometry measurements

The characteristic frequencies of a system provide important information on the phenomena that govern its physical properties. In this framework, there has recently been renewed interest in cryogenic microwave characterization for condensed matter systems since it allows to probe energy scales of the order of a few $μ$eV. However, broadband measurements of the absolute value of a sample response in this frequency range are extremely sensitive to its environment and require a careful calibration. In this paper, we present an \textit{in situ} calibration method for cryogenic broadband microwave reflectometry experiments that is both simple to implement and through which the effect of the sample electromagnetic environment can be minimized. The calibration references are here provided by the sample itself, at three reference temperatures where its impedance is assumed or measured, and not by external standards as is usual. We compare the frequency-dependent complex impedance (0.1--2 GHz) of an a-Nb$_{15}$Si$_{85}$ superconducting thin film obtained through this Sample-Based Calibration (SBC) and through an Open-Short-Load Standard Calibration (SC) when working at very low temperature (0.02--4 K) and show that the SBC allows us to obtain the absolute response of the sample. This method brings the calibration planes as close as possible to the sample, so that the environment electrodynamic response does not affect the measurement, provided it is temperature independent. This results in a heightened sensitivity, for a given experimental set--up.

cond-mat.supr-con↗

arXiv2018

Temperature-dependent transport measurements with Arduino

The current performances of single-board microcontrollers render them attractive not only for basic applications but also for more elaborate projects, amongst which physics teaching or research. In this article, we show how temperature-dependent transport measurements can be performed using an Arduino microcontroller, from cryogenic temperatures up to room temperature or above. We focus on two of the main issues for this type of experiments: the determination of the sample temperature and the measurement of its resistance. We also detail two student-led experiments: evidencing the magnetocaloric effect in Gadolinium and measuring the resistive transition of a high critical temperature superconductor.

physics.ed-ph↗

arXiv2014

Destruction of superconductivity in disordered materials : a dimensional crossover

The disorder-induced Superconductor-to-Insulator Transition in amorphous Nb$_{x}$Si$_{1-x}$ two-dimensional thin films is studied for different niobium compositions $x$ through a variation of the sample thickness $d$. We show that the critical thickness $d_c$, separating a superconducting regime from an insulating one, increases strongly with diminishing $x$, thus attaining values of over 100 Å. The corresponding phase diagram in the $(d, x)$ plane is inferred and related to the three-dimensional situation. The two-dimensional Superconductor-to-Insulator Transition well connects with the three-dimensional Superconductor-to-Metal Transition.

cond-mat.supr-con↗

arXiv2013

Effect of annealing on the superconducting properties of a-Nb(x)Si(1-x) thin films

a-Nb(x)Si(1-x) thin films with thicknesses down to 25 Å have been structurally characterized by TEM (Transmission Electron Microscopy) measurements. As-deposited or annealed films are shown to be continuous and homogeneous in composition and thickness, up to an annealing temperature of 500°C. We have carried out low temperature transport measurements on these films close to the superconductor-to-insulator transition (SIT), and shown a qualitative difference between the effect of annealing or composition, and a reduction of the film thickness on the superconducting properties of a-NbSi. These results question the pertinence of the sheet resistance R_square as the relevant parameter to describe the SIT.

cond-mat.supr-con↗

arXiv2011

Tunable Superconducting Properties of a-NbSi Thin Films and Application to Detection in Astrophysics

We report on the superconducting properties of amorphous NbxSi1-x thin films. The normal-state resistance and critical temperatures can be separately adjusted to suit the desired application. Notably, the relatively low electron-phonon coupling of these films makes them good candidates for an "all electron bolometer" for Cosmological Microwave Background radiation detection. Moreover, this device can be made to suit both high and low impedance readouts.

cond-mat.supr-con↗