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C. Ciuti

Publications and source records attributed to C. Ciuti.

At least 19 recordsLinked to original sources

Nonlinear Terahertz Electroluminescence from Dirac Landau Polaritons

We report Dirac Landau polaritons observed by terahertz (THz) magnetoreflectivity spectroscopy, demonstrating strong coupling between cyclotron transitions of two-dimensional (2D) Dirac fermions in HgTe quantum wells and optical cavity modes. Under pulsed electrical injection we observe efficient nonlinear electroluminescence, with a strongly out-of-equilibrium polariton distribution dominated by emission from the upper polariton branches. Model analysis of the bias-dependent emission intensity and spectral narrowing indicates a polariton occupancy per mode approaching unity, with a possible contribution from stimulated polariton emission in the spectral region of the upper anticrossing. These results open prospects toward Dirac Landau polariton condensates and low-threshold, tunable THz polariton lasers based on cyclotron emission.

cond-mat.mes-hall

Dissipative phase transition with driving-controlled spatial dimension and diffusive boundary conditions

We investigate theoretically and experimentally a first-order dissipative phase transition, with diffusive boundary conditions and the ability to tune the spatial dimension of the system. The considered physical system is a planar semiconductor microcavity in the strong light-matter coupling regime, where polariton excitations are injected by a quasi-resonant optical driving field. The spatial dimension of the system from 1D to 2D is tuned by designing the intensity profile of the driving field. We investigate the emergence of criticality by increasing the spatial size of the driven region. The system is nonlinear due to polariton-polariton interactions and the boundary conditions are diffusive because the polaritons can freely diffuse out of the driven region. We show that no phase transition occurs using a 1D driving geometry, while for a 2D geometry we do observe both in theory and experiments the emergence of a first-order phase transition.

cond-mat.other

Tailored subcycle nonlinearities of ultrastrong light-matter coupling

We explore the nonlinear response of tailor-cut light-matter hybrid states in a novel regime, where both the Rabi frequency induced by a coherent driving field and the vacuum Rabi frequency set by a cavity field are comparable to the carrier frequency of light. In this previously unexplored strong-field limit of ultrastrong coupling, subcycle pump-probe and multi-wave mixing nonlinearities between different polariton states violate the normal-mode approximation while ultrastrong coupling remains intact, as confirmed by our mean-field model. We expect such custom-cut nonlinearities of hybridized elementary excitations to facilitate non-classical light sources, quantum phase transitions, or cavity chemistry with virtual photons.

quant-ph

Nonlinear Polariton Fluids in a Flatband Reveal Discrete Gap Solitons

Phase frustration in periodic lattices is responsible for the formation of dispersionless flat bands. The absence of any kinetic energy scale makes flat band physics critically sensitive to perturbations and interactions. We report here on the experimental investigation of the nonlinear dynamics of cavity polaritons in the gapped flat band of a one-dimensional Lieb lattice. We observe the formation of gap solitons with quantized size and very abrupt edges, signature of the frozen propagation of switching fronts. This type of gap solitons belongs to the class of truncated Bloch waves, and had only been observed in closed systems up to now. Here the driven-dissipative character of the system gives rise to a complex multistability of the nonlinear domains generated in the flat band. These results open up interesting perspective regarding more complex 2D lattices and the generation of correlated photon phases.

cond-mat.mes-hall

Critical behavior of dissipative two-dimensional spin lattices

We explore critical properties of two-dimensional lattices of spins interacting via an anisotropic Heisenberg Hamiltonian and subject to incoherent spin flips. We determine the steady-state solution of the master equation for the density matrix via the corner-space renormalization method. We investigate the finite-size scaling and critical exponent of the magnetic linear susceptibility associated to a dissipative ferromagnetic transition. We show that the Von Neumann entropy increases across the critical point, revealing a strongly mixed character of the ferromagnetic phase. Entanglement is witnessed by the quantum Fisher information which exhibits a critical behavior at the transition point, showing that quantum correlations play a crucial role in the transition even though the system is in a mixed state.

quant-ph

Superradiant phase transition in the ultrastrong coupling regime of the two-photon Dicke model

The controllability of current quantum technologies allows to implement spin-boson models where two-photon couplings are the dominating terms of light-matter interaction. In this case, when the coupling strength becomes comparable with the characteristic frequencies, a spectral collapse can take place, i.e. the discrete system spectrum can collapse into a continuous band. Here, we analyze the thermodynamic limit of the two-photon Dicke model, which describes the interaction of an ensemble of qubits with a single bosonic mode. We find that there exists a parameter regime where two-photon interactions induce a superradiant phase transition, before the spectral collapse occurs. Furthermore, we extend the mean-field analysis by considering second-order quantum fluctuations terms, in order to analyze the low-energy spectrum and compare the critical behavior with the one-photon case.

quant-ph

Probing a dissipative phase transition via dynamical optical hysteresis

We experimentally explore the dynamic optical hysteresis of a semiconductor microcavity as a function of the sweep time. The hysteresis area exhibits a double power law decay due to the shot noise of the driving laser, which triggers switching between metastable states. Upon increasing the average photon number and approaching the thermodynamic limit, the double power law evolves into a single power law. This algebraic behavior characterizes a dissipative phase transition. Our findings are in good agreement with theoretical predictions, and the present experimental approach is promising for the exploration of critical phenomena in photonic lattices.

physics.optics

Output squeezed radiation from dispersive ultrastrong light-matter coupling

We investigate the output generation of squeezed radiation of a cavity photon mode coupled to another off-resonant bosonic excitation. By modulating in time their linear interaction, we predict high degree of output squeezing when the dispersive ultrastrong coupling regime is achieved, i.e., when the interaction rate becomes comparable to the frequency of the lowest energy mode. Our work paves the way to squeezed light generation in frequency domains where the ultrastrong coupling is obtained, e.g., solid-state resonators in the GHz, THz and mid-IR spectral range.

quant-ph

Exact results for Schrödinger cats in driven-dissipative systems and their feedback control

In quantum optics, photonic Schrödinger cats are superpositions of two coherent states with opposite phases and with a significant number of photons. Recently, these states have been observed in the transient dynamics of driven-dissipative resonators subject to engineered two-photon processes. Here we present an exact analytical solution of the steady-state density matrix for this class of systems, including one-photon losses, which are considered detrimental for the achievement of cat states. We demonstrate that the unique steady state is a statistical mixture of two cat-like states with opposite parity, in spite of significant one-photon losses. The transient dynamics to the steady state depends dramatically on the initial state and can pass through a metastable regime lasting orders of magnitudes longer than the photon lifetime. By considering individual quantum trajectories in photon-counting configuration, we find that the system intermittently jumps between two cats. Finally, we propose and study a feedback protocol based on this behaviour to generate a pure cat-like steady state.

quant-ph

Probing photon correlations in the dark sites of geometrically frustrated cavity lattices

We theoretically explore the driven-dissipative physics of geometrically frustrated lattices of cavity resonators with relatively weak nonlinearities, i.e. a photon-photon interaction smaller than the loss rate. In such systems, photon modes with zero probability at 'dark' sites are present at the single-particle level due to interference effects. In particular, we study the behavior of a cell with three coupled resonators as well as extended Lieb lattices in 1D and 2D. By considering a partial pumping scheme, with the driving field not applied to the dark sites, we predict that even in presence of relatively weak photon-photon interactions the nominally dark sites achieve a finite photonic population with strong correlations. We show that this is a consequence of biphoton and multiphoton states that in the absence of frustration would not be visible in the observables.

quant-ph

Trion-polaritons : How strong coupling to a cavity changes the orbital and spin properties of trions

The elementary optical excitations of a two-dimensional electron system strongly coupled to a microcavity are trion-polaritons. Using a variational approach, we demonstrate that the competition between Coulomb interaction and light-matter coupling plays a crucial role in determining the lowest-energy orbital and spin properties of trion-polaritons. When the light-matter interaction exceeds the bare trion binding, singlet and triplet trion states are mixed due to a cavity-mediated spin-orbit effect, which in turn results in a strong increase of the outer electron Bohr radius. In this strong cavity coupling regime, the trion-polariton consists of an exciton-polariton surrounded by a weakly bound electron and is reminiscent of a coherent Rydberg excitation.

cond-mat.mes-hall

Power-laws in the dynamic hysteresis of quantum nonlinear photonic resonators

We explore theoretically the physics of dynamic hysteresis for driven-dissipative nonlinear photonic resonators. In the regime where the semiclassical mean-field theory predicts bistability, the exact steady-state density matrix is known to be unique, being a statistical mixture of two states: in particular, no static hysteresis cycle of the excited population occurs as a function of the driving intensity. Here, we predict that in the quantum regime a dynamic hysteresis with a rich phenomenology does appear when sweeping the driving amplitude in a finite time. The hysteresis area as a function of the sweep time reveals a double power-law decay, with a behavior qualitatively different from the mean-field predictions. The dynamic hysteresis power-law in the slow sweep limit defines a characteristic time, which depends dramatically on the size of the nonlinearity and on the frequency detuning between the driving and the resonator. In the strong nonlinearity regime, the characteristic time oscillates as a function of the intrinsic system parameters due to multiphotonic resonances. We show that the dynamic hysteresis for the considered class of driven-dissipative systems is due to a non-adiabatic response region with connections to the Kibble-Zurek mechanism for quenched phase transitions. We also consider the case of two coupled driven-dissipative nonlinear resonators, showing that dynamic hysteresis and power-law behavior occur also in presence of correlations between resonators. Our theoretical predictions can be explored in a broad variety of physical systems, e.g., circuit QED superconducting resonators and semiconductor optical microcavities.

quant-ph

Polariton superfluids reveal quantum hydrodynamic solitons

A quantum fluid passing an obstacle behaves differently from a classical one. When the flow is slow enough, the quantum gas enters a superfluid regime and neither whirlpools nor waves form around the obstacle. For higher flow velocities, it has been predicted that the perturbation induced by the defect gives rise to the turbulent emission of quantised vortices and to the nucleation of solitons. Using an interacting Bose gas of exciton-polaritons in a semiconductor microcavity, we report the transition from superfluidity to the hydrodynamic formation of oblique dark solitons and vortex streets in the wake of a potential barrier. The direct observation of these topological excitations provides key information on the mechanisms of superflow and shows the potential of polariton condensates for quantum turbulence studies.

cond-mat.quant-gas

Corner space renormalization method for driven-dissipative 2D correlated systems

We present a theoretical method to study driven-dissipative correlated systems on lattices with two spatial dimensions (2D). The steady-state density-matrix of the lattice is obtained by solving the master equation in a corner of the Hilbert space. The states spanning the corner space are determined through an iterative procedure, using eigenvectors of the density-matrix of smaller lattice systems, merging in real space two lattices at each iteration and selecting M pairs of states by maximizing their joint probability. Accuracy of the results is then improved by increasing M, the number of states of the corner space, until convergence is reached. We demonstrate the efficiency of such an approach by applying it to the driven-dissipative 2D Bose-Hubbard model, describing, e.g., lattices of coupled cavities with quantum optical nonlinearities.

quant-ph

Comment on "Linear wave dynamics explains observations attributed to dark-solitons in a polariton quantum fluid"

In a recent preprint (arXiv:1401.1128v1) Cilibrizzi and co-workers report experiments and simulations showing the scattering of polaritons against a localised obstacle in a semiconductor microcavity. The authors observe in the linear excitation regime the formation of density and phase patterns reminiscent of those expected in the non-linear regime from the nucleation of dark solitons. Based on this observation, they conclude that previous theoretical and experimental reports on dark solitons in a polariton system should be revised. Here we comment why the results from Cilibrizzi et al. take place in a very different regime than previous investigations on dark soliton nucleation and do not reproduce all the signatures of its rich nonlinear phenomenology. First of all, Cilibrizzi et al. consider a particular type of radial excitation that strongly determines the observed patterns, while in previous reports the excitation has a plane-wave profile. Most importantly, the nonlinear relation between phase jump, soliton width and fluid velocity, and the existence of a critical velocity with the time-dependent formation of vortex-antivortex pairs are absent in the linear regime. In previous reports about dark soliton and half-dark soliton nucleation in a polariton fluid, the distinctive dark soliton physics is supported both by theory (analytical and numerical) and experiments (both continuous wave and pulsed excitation).

physics.optics

Back-action effects in an all-optical model of dynamical Casimir emission

We report a theoretical study of the optical properties of a three-level emitter embedded in an optical cavity including the non-rotating wave terms of the light-matter interaction Hamiltonian. Rabi oscillations induced by a continuous wave drive laser are responsible for a periodic time-modulation of the effective cavity resonance, which results in a significant dynamical Casimir emission. A clear signature of the back-action effect of the dynamical Casimir emission onto the drive laser is visible as a sizable suppression of its absorption.

quant-ph

All-optical control of the quantum flow of a polariton superfluid

While photons in vacuum are massless particles that do not interact with each other, significant photon-photon interactions appear in suitable nonlinear media, leading to novel hydrodynamic behaviors typical of quantum fluids. Here we show the formation of vortex-antivortex pairs in a Bose-Einstein condensate of exciton-polaritons -a coherent gas of strongly dressed photons- flowing at supersonic speed against an artificial potential barrier created and controlled by a light beam in a planar semiconductor microcavity. The observed hydrodynamical phenomenology is in agreement with original theoretical predictions based on the Gross-Pitaevskii equation, recently generalized to the polariton context. However, in contrast to this theoretical work, we show how the initial position and the subsequent trajectory of the vortices crucially depend on the strength and size of the artificial barrier. Additionally, we demonstrate how a suitably tailored optical beam can be used to permanently trap and store the vortices that are hydrodynamically created in the wake of a natural defect. These observations are borne out by time-dependent theoretical simulations.

cond-mat.mes-hall