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C. H. Lee

Publications and source records attributed to C. H. Lee.

At least 73 records · Page 4Linked to original sources

Universal heat conduction in the iron-arsenide superconductor KFe2As2 : Evidence of a d-wave state

The thermal conductivity of the iron-arsenide superconductor KFe2As2 was measured down to 50 mK for a heat current parallel and perpendicular to the tetragonal c-axis. A residual linear term (RLT) at T=0 is observed for both current directions, confirming the presence of nodes in the superconducting gap. Our value of the RLT in the plane is equal to that reported by Dong et al. [Phys. Rev. Lett. 104, 087005 (2010)] for a sample whose residual resistivity was ten times larger. This independence of the RLT on impurity scattering is the signature of universal heat transport, a property of superconducting states with symmetry-imposed line nodes. This argues against an s-wave state with accidental nodes. It favors instead a d-wave state, an assignment consistent with five additional properties: the magnitude of the critical scattering rate for suppressing Tc to zero; the magnitude of the RLT, and its dependence on current direction and on magnetic field; the temperature dependence of the thermal conductivity.

cond-mat.supr-con↗

Magnetic dispersion and anisotropy in multiferroic BiFeO3

We have determined the full magnetic dispersion relations of multiferroic BiFeO3. In particular, two excitation gaps originating from magnetic anisotropies have been clearly observed. The direct observation of the gaps enables us to accurately determine the Dzyaloshinskii-Moriya (DM) interaction and the single ion anisotropy. The DM interaction supports a strong magneto-electric coupling in this compound.

cond-mat.mtrl-sci↗

Anomalous two peak structure in the Angle-resolved Photoemission Spectra of Ba1-xKxFe2As2

The electronic structure near the Fermi level (EF) of Ba1-xKxFe2As2 (BaK122 ; x = 0.2 - 0.7) is studied using laser ultrahigh-resolution angle-resolved photoemission spectroscopy(ARPES). For the optimally doped case of x = 0.4, we clearly observe two peaks below Tc in the ARPES spectra at a binding energies (BE) of 5 meV and 13meV. The former is assigned to a superconducting (SC) coherence peak since it appears and evolves below the bulk SC transition at Tc (= 36 K), accompanying a gap opening centered at EF. In contrast, the latter peak, which appears below ~ 90 K without any gap formation, is interpreted to be not directly related to a SC coherence peak. This high-BE peak is observed from x = 0.2 to 0.6, reduces in energy with overdoping (x > 0.4) and is absent for x = 0.7. The temperature(T)- and doping-dependent ARPES results suggest that the high-BE peak originates from coupling to a bosonic mode of energy ~ 8 meV.

cond-mat.supr-con↗

Orbital-dependent electron correlation effect on the two- and three-dimensional Fermi surfaces in KFe2As2 revealed by angle-resolved photoemission spectroscopy

We have performed an angle-resolved photoemission study of the hole-overdoped iron pnictide superconductor KFe2As2, which shows a low Tc of ~4 K. Most of the observed Fermi surfaces show nearly two-dimensional shapes, while a band near the Fermi level shows a strong dispersion along the kz direction and forms a small three-dimensional hole pocket centered at the Z point, as predicted by band-structure calculation. However, hole Fermi surfaces of yz and zx orbital character centered at the Γpoint of the two-dimensional Brillouin zone are smaller than those predicted by the calculation while the other hole Fermi surfaces of xy orbital character is much larger. Clover-shaped hole Fermi surfaces around the corner of the 2D BZ are also larger than those predicted by the calculation. These observations are consistent with the de Haas-van Alphen measurement and indicate orbital-dependent electron correlation effects. The effective masses of the energy bands show moderate to strong enhancement, partly due to electron correlation and partly due to energy shifts from the calculated band structure.

cond-mat.str-el↗

Anisotropic Energy Gaps of Iron-based Superconductivity from Intra-band Quasiparticle Interference in LiFeAs

If strong electron-electron interactions between neighboring Fe atoms mediate the Cooper pairing in iron-pnictide superconductors, then specific and distinct anisotropic superconducting energy gaps Δ_i(k) should appear on the different electronic bands i. Here we introduce intra-band Bogoliubov quasiparticle scattering interference (QPI) techniques for determination of Δ_i(k) in such materials, focusing on LiFeAs. We identify the three hole-like bands assigned previously as γ, α_2 and α_1, and we determine the anisotropy, magnitude and relative orientations of their Δ_i(k). These measurements will advance quantitative theoretical analysis of the mechanism of Cooper pairing in iron-based superconductivity.

cond-mat.supr-con↗

Abrupt change in the energy gap of superconducting Ba1-xKxFe2As2 single crystals with hole doping

We performed a Laser angle-resolved photoemission spectroscopy (ARPES) study on a wide doping range of Ba1-xKxFe2As2 (BaK) and precisely determined the doping evolution of the superconducting (SC) gaps in this compound. The gap size of the outer hole Fermi surface (FS) sheet around the Brillioun zone (BZ) center shows an abrupt drop with overdoping (for x > 0.6) while the inner and middle FS gaps roughly scale with Tc. This is accompanied by the simultaneous disappearance of the electron FS sheet with similar orbital character at the BZ corner. These results browse the different contributions of X2-Y2 and XZ/YZ orbitals to superconductivity in BaK and can be hardly completely reproduced by the available theories on iron-based superconductors.

cond-mat.supr-con↗

Properties of MgB2 Films Grown at Various Temperatures by Hybrid Physical-Chemical Vapour Deposition

A Hybrid Physical-Chemical Vapour Deposition (HPCVD) system consisting of separately controlled Mg-source heater and substrate heater is used to grow MgB2 thin films and thick films at various temperatures. We are able to grow superconducting MgB2 thin films at temperatures as low as 350 C with a Tc0 of 35.5 K. MgB2 films up to 4 um in thickness grown at 550 C have Jc over 10E6 A/cm2 at 5 K and zero applied field. The low deposition temperature of MgB2 films is desirable for all-MgB2 tunnel junctions and MgB2 thick films are important for applications in coated conductors.

cond-mat.supr-con↗

Manifestations of multiple-carrier charge transport in the magnetostructurally ordered phase of undoped BaFe$_2$As$_2$

We investigated the transport properties of BaFe$_2$As$_2$ single crystals before and after annealing with BaAs powder. The annealing remarkably improves transport properties, in particular the magnitude of residual resistivity which decreases by a factor of more than 10. From the resistivity measurement on detwinned crystals we found that the anisotropy of the in-plane resistivity is remarkably diminished after annealing, indicative of dominant contributions to the charge transport from the carriers with isotropic and high mobility below magnetostructural transition temperature $T_{\rm s}$ and the absence of nematic state above $T_{\rm s}$. We found that the Hall resistivity shows strong non-linearity against magnetic field and the magnetoresistance becomes very large at low temperatures. These results give evidence for the manifestation of multiple carriers with distinct characters in the ordered phase below $T_{\rm s}$. By analyzing the magnetic field dependences, we found that at least three carriers equally contribute to the charge transport in the ordered phase, which is in good agreement with the results of recent quantum oscillation measurements.

cond-mat.supr-con↗

Optical to near-infrared transit observations of super-Earth GJ1214b: water-world or mini-Neptune?

GJ1214b is thought to be either a mini-Neptune with a thick, hydrogen-rich atmosphere, or a planet with a composition dominated by water. In the case of a hydrogen-rich atmosphere, molecular absorption and scattering processes may result in detectable radius variations as a function of wavelength. The aim of this paper is to measure these variations. We have obtained observations of the transit of GJ1214b in the r- and I-band with the INT, in the g, r, i and z bands with the 2.2 meter MPI/ESO telescope, in the Ks-band with the NOT, and in the Kc-band with the WHT. By comparing the transit depth between the the different bands, which is a measure for the planet-to-star size ratio, the atmosphere is investigated. We do not detect clearly significant variations in the planet-to-star size ratio as function of wavelength. Although the ratio at the shortest measured wavelength, in g-band, is 2sigma larger than in the other bands. The uncertainties in the Ks and Kc bands are large, due to systematic features in the light curves. The tentative increase in the planet-to-star size ratio at the shortest wavelength could be a sign of an increase in the effective planet-size due to Rayleigh scattering, which would require GJ1214b to have a hydrogen-rich atmosphere. If true, then the atmosphere has to have both clouds, to suppress planet-size variations at red optical wavelengths, as well as a sub-solar metallicity, to suppress strong molecular features in the near- and mid-infrared. However, star spots, which are known to be present on the hoststar's surface, can (partly) cancel out the expected variations in planet-to-star size ratio, due to the lower surface temperature of the spots . A hypothetical spot-fraction of 10% would be able to raise the infrared points sufficiently with respect to the optical measurements to be inconsistent with a water-dominated atmosphere. [abridged]

astro-ph.EP↗

Strong electron-lattice coupling and orbital fluctuations in iron pnictide superconductor Ba(Fe1-xCox)2As2

This paper has been withdrawn by the author due to some experimental mistakes. In this paper, we reported that C66, C44 and (C11-C12)/2 show remarkable softening toward the structural transition temperature TS. The data reported in this paper were acquired using the ultrasonic frequency lower than 25 MHz. Recently, we performed high-frequency measurements for the same system. We found that the anomaly of C44 and (C11-C12)/2 tend to disappear rapidly with increasing the frequency. On the other hand, C66 anomaly is still there at high frequencies. Therefore, we concluded that the observed anomalies in C44 and (C11-C12)/2 are not true. They would be ascribed to certain influence by the large softening of C66. So, we have checked our data through careful measurements by using ultrasonic frequency higher than 60 MHz, so far. Then, it has been found that C66 shows still nice softening toward TS, but that its temperature dependence is slightly different from the results of this paper. We have accumulated reliable data now. They will be reported in near future.

cond-mat.supr-con↗

Unprecedented anisotropic metallic state in BaFe2As2 revealed by optical spectroscopy

An ordered phase showing remarkable electronic anisotropy in proximity to the superconducting phase is now a hot issue in the field of high-transition-temperature superconductivity. As in the case of copper oxides, superconductivity in iron arsenides competes or coexists with such an ordered phase. Undoped and underdoped iron arsenides have a magnetostructural ordered phase exhibiting stripe-like antiferromagnetic spin order accompanied by an orthorhombic lattice distortion; both the spin order and lattice distortion break the tetragonal symmetry of crystals of these compounds. In this ordered state, anisotropy of in-plane electrical resistivity is anomalous and difficult to attribute simply to the spin order and/or the lattice distortion. Here, we present the anisotropic optical spectra measured on detwinned BaFe2As2 crystals with light polarization parallel to the Fe planes. Pronounced anisotropy is observed in the spectra, persisting up to an unexpectedly high photon energy of about 2 eV. Such anisotropy arises from an anisotropic energy gap opening below and slightly above the onset of the order. Detailed analysis of the optical spectra reveals an unprecedented electronic state in the ordered phase.

cond-mat.str-el↗

Incommensurate spin fluctuations in hole-overdoped superconductor KFe2As2

A neutron scattering study of heavily hole-overdoped superconducting KFe$_2$As$_2$ revealed a well-defined low-energy incommensurate spin fluctuation at [$π(1\pm2δ$),0] with $δ$ = 0.16. The incommensurate structure differs from the previously observed commensurate peaks in electron-doped $A$Fe$_2$As$_2$ ($A$ = Ba, Ca, or Sr) at low energies. The direction of the peak splitting is perpendicular to that observed in Fe(Te,Se) or in Ba(Fe,Co)$_2$As$_2$ at high energies. A band structure calculation suggests interband scattering between bands around the $Γ$ and X points as an origin of this incommensurate peak. The perpendicular direction of the peak splitting can be understood within the framework of multiorbital band structure. The results suggest that spin fluctuation is more robust in hole-doped than in electron-doped samples, which can be responsible for the appearance of superconductivity in the heavily hole-doped samples.

cond-mat.supr-con↗

Quasi-Two-Dimensional Fermi Surfaces and Coherent Interlayer Transport in KFe$_2$As$_2$

We report the results of the angular-dependent magnetoresistance oscillations (AMROs), which can determine the shape of bulk Fermi surfaces in quasi-two-dimensional (Q2D) systems, in a highly hole-doped Fe-based superconductor KFe$_2$As$_2$ with $T_c \approx$ 3.7 K. From the AMROs, we determined the two Q2D FSs with rounded-square cross sections, corresponding to 12% and 17% of the first Brillouin zone. The rounded-squared shape of the FS cross section is also confirmed by the analyses of the interlayer transport under in-plane fields. From the obtained FS shape, we infer the character of the 3d orbitals that contribute to the FSs.

cond-mat.str-el↗

The pairing state in KFe2As2 studied by measurements of the magnetic vortex lattice

Understanding the mechanism and symmetry of electron pairing in iron-based superconductors represents an important challenge in condensed matter physics [1-3]. The observation of magnetic flux lines - "vortices" - in a superconductor can contribute to this issue, because the spatial variation of magnetic field reflects the pairing. Unlike many other iron pnictides, our KFe2As2 crystals have very weak vortex pinning, allowing small-angle-neutron-scattering (SANS) observations of the intrinsic vortex lattice (VL). We observe nearly isotropic hexagonal packing of vortices, without VL-symmetry transitions up to high fields along the fourfold c-axis of the crystals, indicating rather small anisotropy of the superconducting properties around this axis. This rules out gap nodes parallel to the c-axis, and thus d-wave and also anisotropic s-wave pairing [2, 3]. The strong temperature-dependence of the intensity down to T<<Tc indicates either widely different full gaps on different Fermi surface sheets, or nodal lines perpendicular to the axis.

cond-mat.supr-con↗

Fermi surfaces and quasi-particle band dispersions of the iron pnictides superconductor KFe2As2 observed by angle-resolved photoemission spectroscopy

We have performed an angle-resolved photoemission study of the iron pnictide superconductor KFe2As2 with Tc 4 K. Most of the observed Fermi surfaces show almost two-dimensional shapes, while one of the quasi-particle bands near the Fermi level has a strong dispersion along the kz direction, consistent with the result of a band-structure calculation. However, hole Fermi surfaces αand ζare smaller than those predicted by the calculation while other Fermi surfaces are larger. These observations are consistent with the result of a de Haas-van Alphen study and a theoretical prediction on inter-band scattering, possibly indicating many body effects on the electronic structure.

cond-mat.str-el↗

Evidence for superconducting gap nodes in the zone-centered hole bands of KFe2As2 from magnetic penetration-depth measurements

Among the iron-based pnictide superconductors the material KFe$_2$As$_2$ is unusual in that its Fermi surface does not consist of quasi-nested electron and hole pockets. Here we report measurements of the temperature dependent London penetration depth of very clean crystals of this compound with residual resistivity ratio $>1200$. We show that the superfluid density at low temperatures exhibits a strong linear-in-temperature dependence which implies that there are line nodes in the energy gap on the large zone-centered hole sheets. The results indicate that KFe$_2$As$_2$ is an unconventional superconductor with strong electron correlations.

cond-mat.supr-con↗

Strong carrier-scattering in iron-pnictide superconductors with highest Tc obtained from charge transport experiments

Characteristic normal-state charge transport is found in the oxygen-deficient iron-arsenides LnFeAsO1-y (Ln: La and Nd) with the highest Tc's among known Fe-based superconductors. The effect of "doping" in this system is mainly on the carrier scattering, quite distinct from that in high-Tc cuprates. In the superconducting regime of the La system with maximum Tc = 28 K, the low-temperature resistivity is dominated by a T^2 term. On the other hand, in the Nd system with Tc higher than 40 K, the carriers are subject to stronger scattering showing T-linear resistivity and small magnetoresistance. Such strong scattering appears crucial for high-Tc superconductivity in the iron-based system.

cond-mat.supr-con↗

Evolution of the optical spectrum with doping in iron pnictides Ba(Fe1-xCox)2As2

We investigated the optical spectrum of Ba(Fe1-xCox)2As2 single crystals with various doping levels. It is found that the low-energy optical conductivity spectrum of this system can be decomposed into two components: a sharp Drude term and a broad "incoherent" term. For the compounds showing magnetic order, a gap appears predominantly in the "incoherent" component, while an s-wave like superconducting gap opens in both components for highly doped compounds. The Drude weight steadily increases as doping proceeds, consistent with electron doping in this system. On the other hand, the "incoherent" spectral weight is almost doping independent, but its spectral feature is intimately connected with the magnetism. We demonstrate that the presence of two distinct components in the optical spectrum well explains the doping and temperature dependences of the dc resistivity.

cond-mat.supr-con↗