arXiv subjects

C. H. Lee

Publications and source records attributed to C. H. Lee.

At least 91 records · Page 5Linked to original sources

arXiv2010

Possible hydrogen doping and enhancement of Tc (= 35 K) in a LaFeAsO-based superconductor

We report that the incorporation of hydroxide ions (OH)- significantly enhances the superconducting transition temperature (Tc) in the LnFeAsO-based superconductors (Ln1111: Ln = La, Ce and Pr). For La1111, Tc of the (OH)- incorporated sample synthesized using high-pressure technique becomes 35 K, which is higher by 7 K than the typical optimally-doped La1111 superconductors. Similar enhancement in Tc is also observed for Ce1111 and Pr1111. 1H-NMR measurement have confirmed the existence of hydrogen atoms in the samples. Accompanying the (OH)- incorporation, the lattice parameters are largely contracted, down to the values which have never been attained by any other dopings/substitutions.

cond-mat.supr-con↗

arXiv2008

Effect of Structural Parameters on Superconductivity in Fluorine-Free LnFeAsO1-y (Ln=La,Nd)

The crystal structure of LnFeAsO$_{1-y}$ (Ln = La, Nd) has been studied by the powder neutron diffraction technique. The superconducting phase diagram of NdFeAsO$_{1-y}$ is established as a function of oxygen content which is determined by Rietveld refinement. The small As-Fe bond length suggests that As and Fe atoms are connected covalently. FeAs$_4$-tetrahedrons transform toward a regular shape with increasing oxygen deficiency. Superconducting transition temperatures seem to attain maximum values for regular FeAs$_4$-tetrahedrons.

cond-mat.supr-con↗

arXiv2006

Low-lying optical phonon modes in the filled skutterudite CeRu4Sb12

The phonon dynamics of filled skutterudite CeRu4Sb12 have been studied at room temperature by inelastic neutron scattering. Optical phonons associated with a large vibration of Ce atoms are observed at a relatively low energy of E = 6 meV, and show anticrossing behavior with acoustic phonons. We propose that the origin of the low lattice thermal conductivity in filled skutterudites can be attributed to intensive Umklapp scattering originating from low-lying optical phonons. By an analysis based on a Born-von Karman force model, the longitudinal force constants of the nearest Ce-Sb and Ce-Ru pairs are estimated to be 0.025 mdyn/A, while that of the nearest Ru-Sb pair is estimated to be 1.4 mdyn/A, indicating that the Ce atoms are bound very weakly to the surrounding rigid RuSb6-octahedron cages.

cond-mat.str-el↗

arXiv2004

Charge-Density-Wave Ordering in the Metal-Insulator Transition Compound PrRu4P12

X-ray and electron diffraction measurements on the metal-insulator (M-I) transition compound PrRu$_4$P$_{12}$ have revealed the emergence of a periodic ordering of charge density around the Pr atoms. It is found that the ordering is associated with the onset of a low temperature insulator phase. These conclusions are supported by the facts that the space group of the crystal structure transforms from Im$\bar{3}$ to Pm$\bar{3}$ below the M-I transition temperature and also that the temperature dependence of the superlattice peaks in the insulator phase follows the squared BCS function. The M-I transition could be originated from the perfect nesting of the Fermi surface and/or the instability of the $f$ electrons.

cond-mat.str-el↗

arXiv2003

Single Crystal Growth of Skutterudite CoP3 under High Pressure

A new method to grow single crystals of skutterudite compounds is examined. Using a wedge-type, cubic-anvil, high-pressure apparatus, single crystals of CoP3 were grown from stoichiometric melts under a pressure of 3.5 GPa. Powder x-ray diffraction and electron probe microanalysis measurements indicate that the as-grown boules are a single phase of CoP3. The results suggest that CoP3 is a congruent melting compound under high pressure.

cond-mat.str-el↗

arXiv2003

Evidence for an incommensurate magnetic resonance in La(2-x)Sr(x)CuO(4)

We study the effect of a magnetic field (applied along the c-axis) on the low-energy, incommensurate magnetic fluctuations in superconducting La(1.82)Sr(0.18)CuO(4). The incommensurate peaks at 9 meV, which in zero-field were previously shown to sharpen in q on cooling below T_c [T. E. Mason et al., Phys. Rev. Lett. 77, 1604 (1996)], are found to broaden in q when a field of 10 T is applied. The applied field also causes scattered intensity to shift into the spin gap. We point out that the response at 9 meV, though occurring at incommensurate wave vectors, is comparable to the commensurate magnetic resonance observed at higher energies in other cuprate superconductors.

cond-mat.supr-con↗

arXiv2003

Spin Pseudo Gap in La2-xSrxCuO4 Studied by Neutron Scattering

Spin excitations of La2-xSrxCuO have been studied using inelastic neutron scattering techniques in the energy range of 2 meV =< w =< 12 meV and the temperature range of 8 K =< T =< 150 K. We observed a signature of a spin pseudo gap in the excitation spectrum above Tc for the slightly overdoped sample with x = 0.18. On heating, the spin pseudo gap gradually collapses between T = 80 K and 150 K. For the x = 0.15 and 0.20, although the visibility of gap-like structure at T ~ Tc is lower compared to the x = 0.18 sample, the broad bump of kai"(w) appears at w ~ 5 meV,close to the spin-gap energy at base temperature, suggests the existence of the spin pseudo gap in the normal state.

cond-mat.supr-con↗

arXiv2001

Optical Cooper Pair Breaking Spectroscopy of Cuprate Superconductors

The photon energy dependence of optical Cooper pair breaking rate (CPBR) is studied for compressibly strained La1.85Sr0.15CuO4 (LSCO) films and YBa2Cu2.92Zn0.08O7-delta (YBCZO) thin films, and compared to that in YBa2Cu3O7-delta (YBCO). Unlike in the case of YBCO, the CPBR for LSCO does not show obvious photon energy dependence. In YBCZO the CPBR shows strong photon energy dependence similar to YBCO, but with a red shift in the peak position. Analysis of these results strongly favours a physical picture based on electronic phase separation in high Tc superconductivity.

cond-mat.supr-con↗

arXiv2001

Sharp resonant multiplet in femto-second optical pair-breaking spectroscopy of YBa2Cu3O7-delta

Femto-second optical pair breaking spectroscopy is performed on optimally doped YBa2Cu3O7-delta near 1.5eV. Dramatic photon energy dependence with a sharp triplet fine structure is seen for the first time. The peak separations are attributable to the reported phonon and magnetic excitations in the system. The power dependence is non-linear with differing exponents for the three contributions. These results imply the presence of insulating antiferromagnetic domains in the superconducting state of YBCO over sub-picosecond time scale, and thereby favor an electronic phase separation picture.

cond-mat.supr-con↗

arXiv2000

Structural Phase Transition Accompanied by Metal - Insulator Transition in PrRu4P12

A structural phase transition has been found using electron diffraction technique in PrRu4P12 accompanied by a metal - insulator (M - I) transition (TMI = 60K). Weak superlattice spots appeared at (H, K, L) (H + K + L = 2n + 1; n is an integer) position at a temperature of T = 12 K and 40 K. Above T = 70 K, the spots completely vanished. The space group of the low temperature phase is probably Pm3. This is the first observation of a symmetry other than Im3 in skutterudite compounds.

cond-mat.str-el↗

arXiv2000

XANES study of rare-earth valency in LRu4P12 (L = Ce and Pr)

Valency of Ce and Pr in LRu4P12 (L = Ce and Pr) was studied by L2,3-edge x-ray absorption near-edge structure (XANES) spectroscopy. The Ce-L3 XANES spectrum suggests that Ce is mainly trivalent, but the 4f state strongly hybridizes with ligand orbitals. The band gap of CeRu4P12 seems to be formed by strong hybridization of 4f electrons. Pr-L2 XANES spectra indicate that Pr exists in trivalent state over a wide range in temperature, 20 < T < 300 K. We find that the metal-insulator (MI) transition at TMI = 60 K in PrRu4P12 does not originate from Pr valence fluctuation.

cond-mat.str-el↗

arXiv1999

Apertureless Near-Field Second Harmonic Microscopy with Bare Tapered Optical Fiber Tips

We present a near-field optical technique for second harmonic imaging using bare tapered optical fiber tip illuminated with femtosecond laser pulses. Enhancement of electric field at the tip of the fiber results in enhanced second harmonic generation (SHG) from the sample region near the tip. This SH emission is collected by the same tapered fiber. Spatial distribution of SHG from thin ferroelectric Pb(Zr_xTi_1-x)O_3 films and model metal-ferroelectric devices has been studied. Spatial resolution on the order of 80 nm has been achieved. This is the first time diffraction limit is surpassed in SH microscopic measurements. Electric field induced changes in SHG from individual grains and/or domains of ferroelectric thin films have been observed.

cond-mat.mtrl-sci↗

arXiv1999

Structural instability associated with the tilting of CuO6 octahedra in La2-xSrxCuO4

Comprehensive inelastic neutron-scattering measurements were performed to study the soft optical phonons in La2-xSrxCuO4 at x=0.10, 0.12 and 0.18. We found at x=0.18 that the softening of Z-point phonon, suggesting incipient structural transition from the low-temperature orthorhombic (LTO) to low-temperature tetragonal (LTT) phase, breaks at Tc, which is consistent with the previous report by Lee et al. for the optimally doped x=0.15 sample. As for x=0.10 and 0.12, on the other hand, the softening continues even below Tc. It is thus clarified that the breaking of soft phonon is characteristic of La2-xSrxCuO4 in the optimally and overdoped regions. In the course of studying the soft phonons, we discovered that a central peak remains above the LTO to high-temperature tetragonal (HTT) phase transition at Ts1 and splits into incommensurate components along the (1 1 0)HTT direction at higher temperatures. This is a common feature for both x=0.12 and 0.18 and their temperature dependences of the splitting 2d can be scaled by using a renormalized temperature T/Ts1. In the high temperature limit, d saturates around d ~ 0.12 r.l.u., which value is close to the splitting of incommensurate magnetic signals. This implies that the incipient lattice modulation starts appearing at very high temperature. Details of this modulation and its relations with other properties are, however, not yet clarified.

cond-mat.supr-con↗

arXiv1998

Correspondence between classical dynamics and energy level spacing distribution in the transition billiard systems

The Robnik billiard is investigated in detail both classically and quantally in the transition range from integrable to almost chaotic system. We find out that a remarkable correspondence between characteristic features of classical dynamics, especially topological structure of integrable regions in the Poincaré surface of section, and the statistics of energy level spacings appears with a system parameter $λ$ being varied. It is shown that the variance of the level spacing distribution changes its behavior at every particular values of $λ$ in such a way that classical dynamics changes its topological structure in the Poincaré surface of section, while the skewness and the excess of the level spacings seem to be closely relevant to the interface structure between integrable region and chaotic sea rather than inner structure of intergrable regoin.

chao-dyn↗

arXiv1998

Transitions to quantum chaos in a generic one-parameter family of billiards

Generic one-parameter billiards are studied both classically and quantally. The classical dynamics for the billiards makes a transition from regular to fully chaotic motion through intermediary soft chaotic system. The energy spectra of the billiards are computed using finite element method which has not been applied to the euclidean billiard. True generic quantum chaotic transitional behavior and its sensitive dependence on classical dynamics are uncovered for the first time. That is, this sensitive dependence of quantum spectral measures on classical dynamics is a genuine manifestation of quantum chaos.

chao-dyn↗

arXiv1997

Propagator for an Aharonov-Bohm-Coulomb system

The propagator of three-dimensional Aharonov-Bohm-Coulomb system is calculated by following the Duru-Kleinert method. It is shown that the system is reduced to two independent two dimensional Aharonov-Bohm plus harmonic oscillator systems through dimensional extension and Kustaanheimo-Stiefel transformation. The energy spectrum is deduced.

quant-ph↗

arXiv1997

Heisenberg-picture approach to the evolution of the scalar fields in an expanding universe

We present the Heisenberg-picture approach to the quantum evolution of the scalar fields in an expanding FRW universe which incorporates relatively simply the initial quantum conditions such as the vacuum state, the thermal equilibrium state, and the coherent state. We calculate the Wightman function, two-point function, and correlation function of a massive scalar field. We find the quantum evolution of fluctuations of a self-interacting field perturbatively and discuss the renormalization of field equations.

gr-qc↗

arXiv1996

Test of dilute gas approximation in quantum mechanical model

The validity of dilute gas approximation is explored by making use of the large-sized instanton in quantum mechanical model. It is shown that the Euclidean probability amplitude derived through a dilute gas approximation not only cannot explain the result of the linear combination of atomic orbitals approximation, but also does not exhibit a proper limiting case when the size of instanton is very large.

hep-th↗