arXiv subjects

C. L. Zhang

Publications and source records attributed to C. L. Zhang.

At least 19 recordsLinked to original sources

arXiv2024

Superconductivity Discovered in Niobium Polyhydride at High Pressures

Niobium polyhydride was synthesized at high pressure and high temperature conditions by using diamond anvil cell combined with in situ high pressure laser heating techniques. High pressure electric transport experiments demonstrate that superconducting transition occurs with critical temperature(Tc) 42 K at 187 GPa. The shift of Tc as function of external applied magnetic field is in consistent to the nature of superconductivity while the upper critical field at zero temperature Hc2(0) is estimated to~16.8 Tesla while the GL coherent length ~57 angstrom is estimated. The structure investigation using synchrotron radiation implies that the observed superconductivity may come from Fm-3m phase of NbH3.

cond-mat.supr-con↗

arXiv2024

Superconductivity with Tc 116K discovered in antimony polyhydrides

Superconductivity (SC) was experimentally observed for the first time in antimony polyhydride. The diamond anvil cell combined with laser heating system was used to synthesize the antimony polyhydride sample at high pressure and high temperature conditions. In-situ high pressure transport measurements as function of temperature with applied magnet are performed to study the SC properties. It was found that the antimony polyhydride samples show superconducting transition with critical temperature Tc 116 K at 184 GPa. The investigation of SC at magnetic field revealed that the superconducting coherent length ~40 angstroms based on Ginzburg Landau (GL) equation. Antimony polyhydride superconductor has the second highest Tc in addition to sulfur hydride among the polyhydrides of elements from main group IIIA to VIIA in periodic table.

cond-mat.supr-con↗

arXiv2023

Superconductivity Observed in Tantalum Polyhydride at High Pressure

We report experimental discovery of tantalum polyhydride superconductor. It was synthesized at high pressure and high temperature conditions using diamond anvil cell combined with in-situ high pressure laser heating techniques. The superconductivity was investigated via resistance measurements at pressures. The highest superconducting transition temperature Tc was found to be ~30 K at 197 GPa in the sample that was synthesized at the same pressure with ~2000 K heating. The transitions are shifted to low temperature upon applying magnetic fields that supports the superconductivity nature. The upper critical field at zero temperature μ0Hc2(0) of the superconducting phase is estimated to be ~20 T that corresponds to GL coherent length ~40 angstroms. Our results suggest that the superconductivity may arise from I-43d phase of TaH3. It is, for the first time to our best knowledge, experimental realization of superconducting hydrides for the VB group of transitional metals.

cond-mat.supr-con↗

arXiv2022

Record High Tc Element Superconductivity Achieved In Titanium

It is challenging to search for high Tc superconductivity (SC) in transition metal elements wherein d electrons are usually not favored by conventional BCS theory. Here we report discovery of surprising SC up to 310 GPa with Tc above 20 K in wide pressure range from 108 GPa to 240 GPa in titanium. The maximum Tc^onset above 26 K and zero resistance Tc^zero of 21 K are record high values hitherto achieved among element superconductors. The Hc2(0) is estimated to be about 32 Tesla with coherence length 32 angstrom. The results show strong s-d transfer and d-band dominance, indicating correlation driven contributions to high Tc SC in dense titanium. This finding is in sharp contrast to the theoretical predications based on pristine electron-phonon coupling scenario. The study opens a fresh promising avenue for rational design and discovery of high Tc superconductors among simple materials via pressure tuned unconventional mechanism.

cond-mat.supr-con↗

arXiv2022

Superconductivity above 80 K in polyhydrides of hafnium

Studies on polyhydrides are attracting growing attentions recently due to their potential high temperature superconductivity (SC). We here report the discovery of SC in hafnium polyhydrides at high pressures. The hafnium superhydrides are synthesized at high pressure and high temperature conditions using diamond anvil cell in combination with in-situ high pressure laser heating technique. The SC was investigated by in-situ high pressure resistance measurements in applied magnetic fields. A superconducting transition with onset Tc ~83 K was observed at 243 GPa. The upper critical field Hc2(0) was estimated to be 24 Tesla by GL theory and the consequent superconducting coherent length to be ~37 angstrom. Our results suggest that the superconducting phase is from C2/m-HfH14. This is the first 5d transition metal polyhydride superconductor with Tc above the liquid nitrogen temperature.

cond-mat.supr-con↗

arXiv2022

Superconductivity above 200 K Observed in Superhydrides of Calcium

Searching for superconductivity with Tc near room temperature is of great interest both for fundamental science & many potential applications. Here we report the experimental discovery of superconductivity with maximum critical temperature (Tc) above 210 K in calcium superhydrides, the new alkali earth hydrides experimentally showing superconductivity above 200 K in addition to sulfur hydride & rare-earth hydride system. The materials are synthesized at the synergetic conditions of 160~190 GPa and ~2000 K using diamond anvil cell combined with in-situ laser heating technique. The superconductivity was studied through in-situ high pressure electric conductance measurements in an applied magnetic field for the sample quenched from high temperature while maintained at high pressures. The upper critical field Hc(0) was estimated to be ~268 T while the GL coherent length is ~11 angstrom. The in-situ synchrotron X-ray diffraction measurements suggest that the synthesized calcium hydrides are primarily composed of CaH6 while there may also exist other calcium hydrides with different hydrogen contents.

cond-mat.supr-con↗

arXiv2022

Superconductivity in Zirconium Polyhydrides with Tc above 70 K

We report the experimental discovery of superconductivity with critical temperature Tc above 70 K in zirconium polyhydrides, the record high so far for 3d transition metal hydrides. The superconducting zirconium polyhydrides are synthesized at the extreme conditions above 200 GPa & 2000 K by using diamond anvil cell combined with in-situ laser heating. Superconductivity was observed in the samples maintained at the same pressure upon quenched from heating.

cond-mat.supr-con↗

arXiv2020

Orbital selectivity of layer resolved tunneling on iron superconductor Ba0.6K0.4Fe2As2

We use scanning tunneling microscopy/spectroscopy (STM/S) to elucidate the Cooper pairing of the iron pnictide superconductor Ba0.6K0.4Fe2As2. By a cold-cleaving technique, we obtain atomically resolved termination surfaces with different layer identities. Remarkably, we observe that the low-energy tunneling spectrum related to superconductivity has an unprecedented dependence on the layer-identity. By cross-referencing with the angle-revolved photoemission results and the tunneling data of LiFeAs, we find that tunneling on each termination surface probes superconductivity through selecting distinct Fe-3d orbitals. These findings imply the real-space orbital features of the Cooper pairing in the iron pnictide superconductors, and propose a new and general concept that, for complex multi-orbital material, tunneling on different terminating layers can feature orbital selectivity.

cond-mat.supr-con↗

arXiv2019

Insight-HXMT observation on 4U~1608--52: evolving spectral properties of a bright type-I X-ray burst

The evidences for the influence of thermonuclear (type-I) X-ray bursts upon the surrounding environments in neutron star low-mass X-ray binaries (LMXB) were detected previously via spectral and timing analyses. Benefitting from a broad energy coverage of Insight-HXMT, we analyze one photospheric radius expansion (PRE) burst, and find an emission excess at soft X-rays. Our spectral analysis shows that, such an excess is not likely relevant to the disk reflection induced by the burst emission and can be attributed to an enhanced pre-burst/persistent emission. We find that the burst and enhanced persistent emissions sum up to exceed Eddington luminosity by $\sim$ 40 percentages. We speculate that the enhanced emission is from a region beyond the PRE radius, or through the Comptonization of the corona.

astro-ph.HE↗

arXiv2019

Insight-HXMT observations of 4U~1636-536: Corona cooling revealed with single short type-I X-ray burst

Corona cooling was detected previously from stacking a series of short type-I bursts occurred during the low/had state of atoll outburst. Type-I bursts are hence regarded as sharp probe to our better understanding on the basic property of the corona. The launch of the first Chinese X-ray satellite Insight-HXMT has large detection area at hard X-rays which provide almost unique chance to move further in this research field. We report the first detection of the corona cooling by Insight-HXMT from single short type-I burst showing up during {\bf flare} of 4U 1636-536. This type-I X-ray burst has a duration of $\sim$13 seconds and hard X-ray shortage is detected with significance 6.2~$σ$ in 40-70 keV. A cross-correlation analysis between the lightcurves of soft and hard X-ray band, shows that the corona shortage lag the burst emission by 1.6 $\pm$1.2~s. These results are consistent with those derived previously from stacking a large amount of bursts detected by RXTE/PCA within a series of {\bf flares} of 4U 1636-536. Moreover, the broad bandwidth of Insight-HXMT allows as well for the first time to infer the burst influence upon the continuum spectrum via performing the spectral fitting of the burst, which ends up with the finding that hard X-ray shortage appears at around 40 keV in the continuum spectrum. These results suggest that the evolution of the corona along with the outburst{\bf /flare} of NS XRB may be traced via looking into a series of embedded type-I bursts by using Insight-HXMT.

astro-ph.HE↗

arXiv2019

Timing analysis of 2S 1417-624 observed with NICER and Insight-HXMT

We present a study of timing properties of the accreting pulsar 2S 1417-624 observed during its 2018 outburst, based on Swift/BAT, Fermi/GBM, Insight-HXMT and NICER observations. We report a dramatic change of the pulse profiles with luminosity. The morphology of the profile in the range 0.2-10.0keV switches from double to triple peaks at $\sim2.5$ $\rm \times 10^{37}{\it D}_{10}^2\ erg\ s^{-1}$ and from triple to quadruple peaks at $\sim7$ $\rm \times 10^{37}{\it D}_{10}^2\ erg\ s^{-1}$. The profile at high energies (25-100keV) shows significant evolutions as well. We explain this phenomenon according to existing theoretical models. We argue that the first change is related to the transition from the sub to the super-critical accretion regime, while the second to the transition of the accretion disc from the gas-dominated to the radiation pressure-dominated state. Considering the spin-up as well due to the accretion torque, this interpretation allows to estimate the magnetic field self-consistently at $\sim7\times 10^{12}$G.

astro-ph.HE↗

arXiv2019

Hot disk of the Swift J0243.6+6124 revealed by Insight-HXMT

We report on analysis of observations of the bright transient X-ray pulsar \src obtained during its 2017-2018 giant outburst with Insight-HXMT, \emph{NuSTAR}, and \textit{Swift} observatories. We focus on the discovery of a sharp state transition of the timing and spectral properties of the source at super-Eddington accretion rates, which we associate with the transition of the accretion disk to a radiation pressure dominated (RPD) state, the first ever directly observed for magnetized neutron star. This transition occurs at slightly higher luminosity compared to already reported transition of the source from sub- to super-critical accretion regime associate with onset of an accretion column. We argue that this scenario can only be realized for comparatively weakly magnetized neutron star, not dissimilar to other ultra-luminous X-ray pulsars (ULPs), which accrete at similar rates. Further evidence for this conclusion is provided by the non-detection of the transition to the propeller state in quiescence which strongly implies compact magnetosphere and thus rules out magnetar-like fields.

astro-ph.HE↗

arXiv2019

In-orbit demonstration of X-ray pulsar navigation with the Insight-HXMT satellite

In this work, we report the in-orbit demonstration of X-ray pulsar navigation with Insight-Hard X-ray Modulation Telescope (Insight-HXMT), which was launched on Jun. 15th, 2017. The new pulsar navigation method 'Significance Enhancement of Pulse-profile with Orbit-dynamics' (SEPO) is adopted to determine the orbit with observations of only one pulsar. In this test, the Crab pulsar is chosen and observed by Insight-HXMT from Aug. 31th to Sept. 5th in 2017. Using the 5-day-long observation data, the orbit of Insight-HXMT is determined successfully with the three telescopes onboard - High Energy X-ray Telescope (HE), Medium Energy X-ray Telescope (ME) and Low Energy X-ray Telescope (LE) - respectively. Combining all the data, the position and velocity of the Insight-HXMT are pinpointed to within 10 km (3 sigma) and 10 m/s (3 sigma), respectively.

astro-ph.IM↗

arXiv2018

Insight-HXMT observations of the New Black Hole Candidate MAXI J1535-571: timing analysis

We present the X-ray timing results of the new black hole candidate (BHC) MAXI J1535-571 during its 2017 outburst from Hard X-ray Modulation Telescope (\emph{Insight}-HXMT) observations taken from 2017 September 6 to 23. Following the definitions given by \citet{Belloni2010}, we find that the source exhibits state transitions from Low/Hard state (LHS) to Hard Intermediate state (HIMS) and eventually to Soft Intermediate state (SIMS). Quasi-periodic oscillations (QPOs) are found in the intermediate states, which suggest different types of QPOs. With the large effective area of \emph{Insight}-HXMT at high energies, we are able to present the energy dependence of the QPO amplitude and centroid frequency up to 100 keV which is rarely explored by previous satellites. We also find that the phase lag at the type-C QPOs centroid frequency is negative (soft lags) and strongly correlated with the centroid frequency. By assuming a geometrical origin of type-C QPOs, the source is consistent with being a high inclination system.

astro-ph.HE↗

arXiv2017

Nucleon localization and fragment formation in nuclear fission

An electron localization measure was originally introduced to characterize chemical bond structures in molecules. Recently, a nucleon localization based on Hartree-Fock densities has been introduced to investigate $α$-cluster structures in light nuclei. Compared to the local nucleonic densities, the nucleon localization function has been shown to be an excellent indicator of shell effects and cluster correlations. Using the spatial nucleon localization measure, we investigate the emergence of fragments in fissioning heavy nuclei. To illustrate basic concepts of nucleon localization, we employ the self-consistent energy density functional method with a quantified energy density functional optimized for fission studies. We study the particle densities and spatial nucleon localization distributions along the fission pathways of $^{264}$Fm, $^{232}$Th and $^{240}$Pu. We demonstrate that the fission fragments are formed fairly early in the evolution, well before scission. We illustrate the usefulness of the localization measure by showing how the hyperdeformed state of $^{232}$Th can be understood in terms of a quasimolecular state made of $^{132}$Sn and $^{100}$Zr fragments. Compared to nucleonic distributions, the nucleon localization function more effectively quantifies nucleonic clustering: its characteristic oscillating pattern, traced back to shell effects, is a clear fingerprint of cluster/fragment configurations. This is of particular interest for studies of fragment formation and fragment identification in fissioning nuclei.

nucl-th↗

arXiv2016

Role of Arsenic in Iron-based Superconductivity at Atomic Scale

In iron-based superconductors, a unique tri-layer Fe-As (Se, Te, P) plays an essential role in controlling the electronic properties, especially the Cooper pairing interaction. Here we use scanning tunneling microscopy/spectroscopy (STM/S) to investigate the role of arsenic atom in superconducting Ba0.4K0.6Fe2As2 by directly breaking and restoring the Fe-As structure at atomic scale. After the up-As-layer peeled away, the tunneling spectrum of the exposed iron surface reveals a shallow incoherent gap, indicating a severe suppression of superconductivity without arsenic covering. When a pair of arsenic atoms is placed on such iron surface, a localized topographic feature is formed due to Fe-As orbital hybridization, and the superconducting coherent peaks recover locally with the gap magnitude the same as that on the iron-layer fully covered by arsenic. These observations unravel the Fe-As interactions on an atomic scale and imply its essential roles in the iron-based superconductivity.

cond-mat.supr-con↗

arXiv2015

Photoemission study of the electronic structure and charge density waves of Na2Ti2Sb2O

The electronic structure of Na2Ti2Sb2O, a parent compound of the newly discovered titanium-based oxypnictide superconductors, is studied by photon energy and polarization dependent angle-resolved photoemission spectroscopy (ARPES). The obtained band structure and Fermi surface agree well with the band structure calculation of Na2Ti2Sb2O in the non-magnetic state, which indicating that there is no magnetic order in Na2Ti2Sb2O and the electronic correlation is weak. Polarization dependent ARPES results suggest the multi-band and multi-orbital nature of Na2Ti2Sb2O. Photon energy dependent ARPES results suggest that the electronic structure of Na2Ti2Sb2O is rather two-dimensional. Moreover, we find a density wave energy gap forms below the transition temperature and reaches 65 meV at 7 K, indicating that Na2Ti2Sb2O is likely a weakly correlated CDW material in the strong electron-phonon interaction regime.

cond-mat.supr-con↗

arXiv2013

Kerman-Onishi conditions in self-consistent tilted-axis-cranking mean-field calculations

\item[Background] For cranked mean-field calculations with arbitrarily oriented rotational frequency vector $\boldsymbolω$ in the intrinsic frame, one has to employ constraints on average values of the quadrupole-moment tensor, so as to keep the nucleus in the principal-axis reference frame. Kerman and Onishi [Nucl. Phys. A {\bf 361}, 179 (1981)] have shown that the Lagrangian multipliers that correspond to the required constraints are proportional to $\boldsymbolω \times \boldsymbol{J}$, where $\boldsymbol{J}$ is the average angular momentum vector. \item[Purpose] We study the validity and consequences of the Kerman-Onishi conditions in the context of self-consistent tilted-axis-cranking (TAC) mean-field calculations. \item[Methods] We perform a two-dimensional self-consistent calculations (with and without pairing) utilizing the symmetry-unrestricted solver {\sc hfodd}. At each tilting angle, we compare the calculated values of quadrupole-moment-tensor Lagrangian multipliers and $\boldsymbolω \times \boldsymbol{J}$. \item[Results] We show that in self-consistent calculations, the Kerman-Onishi conditions are obeyed with high precision. Small deviations seen in the calculations with pairing can be attributed to the truncation of the quasiparticle spectrum. We also provide results of systematic TAC calculations for triaxial strongly deformed bands in $^{160}$Yb. \item[Conclusions] For non-stationary TAC solutions, Kerman-Onishi conditions link the non-zero values of the angle between rotational-frequency and angular-momentum vectors to the constraints on off-diagonal components of the quadrupole-moment tensor. To stabilize the convergence of self-consistent iterations, such constraints have to be taken into account. Only then one can determine the Routhian surfaces as functions of the tilting angles.

nucl-th↗