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C. M. O'Shaughnessy

Publications and source records attributed to C. M. O'Shaughnessy.

18 recordsLinked to original sources
arXiv2026

Comparative measurements of DC electrical breakdown distributions in liquid nitrogen, liquid helium, and liquid argon

We present a comparative study of DC electrical breakdown in liquid nitrogen, liquid helium, and liquid argon using a common cryostat, electrode assembly, voltage-ramp protocol, and analysis procedure. This common experimental configuration minimizes systematic differences that often complicate comparisons among cryogenic liquids, including variations in electrode geometry, stressed area, surface finish, and gap spacing. For each liquid, breakdown was characterized as a statistical distribution rather than by a single characteristic voltage, allowing the stochastic nature of the process to be examined. Measurements were performed both near saturated vapor pressure and under modest pressurization to assess the influence of bubble formation and related thermodynamic effects. Liquid argon exhibited a non-stationary "turn-on" behavior, with breakdown voltage increasing over repeated discharges, consistent with evolution of the local impurity environment or electrode surface state. Near saturated vapor pressure, liquid helium showed a bimodal breakdown distribution, with a lower-field component consistent with bubble-mediated processes. Liquid nitrogen exhibited higher breakdown fields than liquid argon and fields comparable to those measured in pressurized liquid helium, within the observed run-to-run variation associated with surface state. Taken together, these results support a comparative framework in which breakdown strength reflects both thermodynamic stability against bubble formation and the transport properties of the dominant negative charge carrier.

physics.chem-ph↗
arXiv2026

Demonstration of 255-kV high-voltage generation with a Cavallo multiplier system

Many cryogenic precision measurements require large electric fields in environments where conventional high-voltage feedthroughs are impractical. To address this, we developed a Cavallo electrostatic multiplier designed for in situ high-voltage generation under such conditions. Here, we report a room-temperature demonstration of this device. Using a mechanically translated transfer electrode and a custom rotary field mill for noncontact voltage measurement, the system reached output voltages up to approximately $255~\mathrm{kV}$ from a $25~\mathrm{kV}$ DC-biased input voltage in approximately $600~\mathrm{Torr}$ of SF$_6$. The charging curves are quantitatively described by a capacitance-based model once realistic electrode misalignment is included. Voltage-hold measurements show picoampere-scale leakage currents on long time scales, whereas operation near the maximum voltage is limited by transient discharge processes associated with electrode surface condition and local field enhancement, rather than by the intrinsic dielectric strength of the gas. These results demonstrate the Cavallo multiplier as a viable low-current, in situ high-voltage source and indicate that electrode surface preparation, alignment tolerances, and insulation performance are the principal requirements for reliable operation in future cryogenic implementations.

physics.ins-det↗
arXiv2025

High voltage and electrode system for a cryogenic experiment to search for the neutron electric dipole moment

The cryogenic approach to the search for the neutron electric dipole moment--performing the experiment in superfluid liquid helium--holds promise for a substantial increase in sensitivity, potentially enabling a sensitivity level of $10^{-28}$ e-cm. A crucial component in realizing such an experiment is the high voltage and electrode system capable of providing an electric field of 75 kV/cm. This, in turn, requires an electric potential of 635 kV to be applied to the high voltage electrode, while simultaneously satisfying other experimental constraints, such as those on heat load and magnetic noise requirements. This paper describes the outcome of a comprehensive development program addressing these challenges. It outlines the system requirements, discusses new insights into relevant physical phenomena, and details selected technical solutions with their corresponding experimental demonstrations and expected performance. The results collectively demonstrate the successful development of the necessary technology for the high-voltage and electrode system for this approach.

physics.ins-det↗
arXiv2024

Measurement of the Free Neutron Lifetime in a Magneto-Gravitational Trap with In Situ Detection

Here we publish three years of data for the UCNtau experiment performed at the Los Alamos Ultra Cold Neutron Facility at the Los Alamos Neutron Science Center. These data are in addition to our previously published data. Our goals in this paper are to better understand and quantify systematic uncertainties and to improve the lifetime statistical precision. We report a measured value for these runs from 2020-2022 for the neutron lifetime of 877.94+/-0.37 s; when all the data from UCNtau are averaged we report an updated value for the lifetime of 877.82+/-0.22 (statistical)+0.20-0.17 (systematic) s. We utilized improved monitor detectors, reduced our correction due to UCN upscattering on ambient gas, and employed four different main UCN detector geometries both to reduce the correction required for rate dependence and explore potential contributions due to phase space evolution.

nucl-ex↗
arXiv2024

An experimental search for an explanation of the difference between beam and bottle neutron lifetime measurements

The past two decades have yielded several new measurements and reanalysis of older measurements of the neutron lifetime. These have led to a 4.4 standard deviation discrepancy between the most precise measurements of the neutron decay rate producing protons in cold neutron beams and the most precise lifetime measured in neutron storage experiments. Here we publish an analysis of the recently published UCN aimed a searching for an explanation of this difference using the model proposed by Koch and Hummel.

nucl-ex↗
arXiv2024

Scintillation characteristics of the EJ-299-02H scintillator

A study of the dead layer thickness and quenching factor of a plastic scintillator for use in ultracold neutron (UCN) experiments is described. Alpha spectroscopy was used to determine the thickness of a thin surface dead layer, and the relative light outputs from the decay of $^{241}$Am and Compton scattering of electrons were used to extract the quenching parameter. With these characteristics of the material known, the light yield of the scintillator can be calculated. The ability to make these scintillators deuterated, accompanied by its relatively thin dead layer, make it ideal for use in UCN experiment, where the light yield of decay electrons and alphas from neutron capture are critical for counting events.

physics.ins-det↗
arXiv2024

YAP:Ce scintillator as an absolute ultracold neutron detector

The upcoming UCNProBe experiment at Los Alamos National Laboratory will measure the $β$-decay rate of free neutrons with different systematic uncertainties than previous beam-based neutron lifetime experiments. We have developed a new $^{10}$B-coated YAP:Ce scintillator whose properties are presented. The advantage of the YAP:Ce scintillator is its high Fermi potential, which reduces the probability for upscattering of ultracold neutrons, and its short decay time, which is important at high counting rates. Birks' coefficient of YAP:Ce was measured to be ($5.56^{+0.05}_{-0.30})\times 10^{-4}$ cm/MeV and light losses due to 120 nm of $^{10}$B-coating to be about 60%. The loss of light from YAP:Ce due to transmission through deuterated polystyrene scintillator was about 50%. The efficiency for counting neutrons that are captured on the $^{10}$B coating is (86.82 $\pm$ 2.61)%. Measurement with ultracold neutrons showed that YAP:Ce crystal counted 8% to 28% more UCNs compared to ZnS screen. This may be due to an uneven coating of $^{10}$B on the rough surface.

physics.ins-det↗
arXiv2023

Fundamental Neutron Physics: a White Paper on Progress and Prospects in the US

Fundamental neutron physics, combining precision measurements and theory, probes particle physics at short range with reach well beyond the highest energies probed by the LHC. Significant US efforts are underway that will probe BSM CP violation with orders of magnitude more sensitivity, provide new data on the Cabibbo anomaly, more precisely measure the neutron lifetime and decay, and explore hadronic parity violation. World-leading results from the US Fundamental Neutron Physics community since the last Long Range Plan, include the world's most precise measurement of the neutron lifetime from UCN$τ$, the final results on the beta-asymmetry from UCNA and new results on hadronic parity violation from the NPDGamma and n-${^3}$He runs at the FNPB (Fundamental Neutron Physics Beamline), precision measurement of the radiative neutron decay mode and n-${}^4$He at NIST. US leadership and discovery potential are ensured by the development of new high-impact experiments including BL3, Nab, LANL nEDM and nEDM@SNS. On the theory side, the last few years have seen results for the neutron EDM from the QCD $θ$ term, a factor of two reduction in the uncertainty for inner radiative corrections in beta-decay which impacts CKM unitarity, and progress on {\it ab initio} calculations of nuclear structure for medium-mass and heavy nuclei which can eventually improve the connection between nuclear and nucleon EDMs. In order to maintain this exciting program and capitalize on past investments while also pursuing new ideas and building US leadership in new areas, the Fundamental Neutron Physics community has identified a number of priorities and opportunities for our sub-field covering the time-frame of the last Long Range Plan (LRP) under development. This white paper elaborates on these priorities.

nucl-ex↗
arXiv2023

Characterization of electroless nickel-phosphorus plating for ultracold-neutron storage

Electroless nickel plating is an established industrial process that provides a robust and relatively low-cost coating suitable for transporting and storing ultracold neutrons (UCN). Using roughness measurements and UCN-storage experiments we characterized UCN guides made from polished aluminum or stainless-steel tubes plated by several vendors. All electroless nickel platings were similarly suited for UCN storage with an average loss probability per wall bounce of $2.8\cdot10^{-4}$ to $4.1\cdot10^{-4}$ for energies between 90 neV and 190 neV, or a ratio of imaginary to real Fermi potential $η$ of $1.7\cdot10^{-4}$ to $3.3\cdot10^{-4}$. Measurements at different elevations indicate that the energy dependence of UCN losses is well described by the imaginary Fermi potential. Some special considerations are required to avoid an increase in surface roughness during the plating process and hence a reduction in UCN transmission. Increased roughness had only a minor impact on storage properties. Based on these findings we chose a vendor to plate the UCN-production vessel that will contain the superfluid-helium converter for the new TRIUMF UltraCold Advanced Neutron (TUCAN) source, achieving acceptable UCN-storage properties with ${η=3.5(5)\cdot10^{-4}}$.

nucl-ex↗
arXiv2023

Characterization of the new Ultracold Neutron beamline at the LANL UCN facility

The neutron electric dipole moment (nEDM) experiment that is currently being developed at Los Alamos National Laboratory (LANL) will use ultracold neutrons (UCN) and Ramsey's method of separated oscillatory fields to search for a nEDM. In this paper, we present measurements of UCN storage and UCN transport performed during the commissioning of a new beamline at the LANL UCN source and demonstrate a sufficient number of stored polarized UCN to achieve a statistical uncertainty of $δd_n = 2\times 10^{-27}$~$e\cdot\text{cm}$ in 5 calendar years of running. We also present an analytical model describing data that provides a simple parameterization of the input UCN energy spectrum on the new beamline.

physics.ins-det↗
arXiv2020

Effect of an electric field on liquid helium scintillation produced by fast electrons

The dependence on applied electric field ($0 - 40$ kV/cm) of the scintillation light produced by fast electrons and $α$ particles stopped in liquid helium in the temperature range of 0.44 K to 3.12 K is reported. For both types of particles, the reduction in the intensity of the scintillation signal due to the applied field exhibits an apparent temperature dependence. Using an approximate solution of the Debye-Smoluchowski equation, we show that the apparent temperature dependence for electrons can be explained by the time required for geminate pairs to recombine relative to the detector signal integration time. This finding indicates that the spatial distribution of secondary electrons with respect to their geminate partners possesses a heavy, non-Gaussian tail at larger separations, and has a dependence on the energy of the primary ionization electron. We discuss the potential application of this result to pulse shape analysis for particle detection and discrimination.

physics.ins-det↗
arXiv2019

A New Cryogenic Apparatus to Search for the Neutron Electric Dipole Moment

A cryogenic apparatus is described that enables a new experiment, nEDM@SNS, with a major improvement in sensitivity compared to the existing limit in the search for a neutron Electric Dipole Moment (EDM). It uses superfluid $^4$He to produce a high density of Ultra-Cold Neutrons (UCN) which are contained in a suitably coated pair of measurement cells. The experiment, to be operated at the Spallation Neutron Source at Oak Ridge National Laboratory, uses polarized $^3$He from an Atomic Beam Source injected into the superfluid $^4$He and transported to the measurement cells as a co-magnetometer. The superfluid $^4$He is also used as an insulating medium allowing significantly higher electric fields, compared to previous experiments, to be maintained across the measurement cells. These features provide an ultimate statistical uncertainty for the EDM of $2-3\times 10^{-28}$ e-cm, with anticipated systematic uncertainties below this level.

physics.ins-det↗
arXiv2019

The neutron electric dipole moment experiment at the Spallation Neutron Source

Novel experimental techniques are required to make the next big leap in neutron electric dipole moment experimental sensitivity, both in terms of statistics and systematic error control. The nEDM experiment at the Spallation Neutron Source (nEDM@SNS) will implement the scheme of Golub & Lamoreaux [Phys. Rep., 237, 1 (1994)]. The unique properties of combining polarized ultracold neutrons, polarized $^3$He, and superfluid $^4$He will be exploited to provide a sensitivity to $\sim 10^{-28}\,e{\rm \,\cdot\, cm}$. Our cryogenic apparatus will deploy two small ($3\,{\rm L}$) measurement cells with a high density of ultracold neutrons produced and spin analyzed in situ. The electric field strength, precession time, magnetic shielding, and detected UCN number will all be enhanced compared to previous room temperature Ramsey measurements. Our $^3$He co-magnetometer offers unique control of systematic effects, in particular the Bloch-Siegert induced false EDM. Furthermore, there will be two distinct measurement modes: free precession and dressed spin. This will provide an important self-check of our results. Following five years of "critical component demonstration," our collaboration transitioned to a "large scale integration" phase in 2018. An overview of our measurement techniques, experimental design, and brief updates are described in these proceedings.

nucl-ex↗
arXiv2018

Search for the Neutron Decay n$\rightarrow$ X+$γ$ where X is a dark matter particle

In a recent paper submitted to Physical Review Letters, Fornal and Grinstein have suggested that the discrepancy between two different methods of neutron lifetime measurements, the beam and bottle methods can be explained by a previously unobserved dark matter decay mode, n$\rightarrow$ X+$γ$ where X is a dark matter particle. We have performed a search for this decay mode over the allowed range of energies of the monoenergetic gamma ray for X to be a dark matter particle. We exclude the possibility of a sufficiently strong branch to explain the lifetime discrepancy with greater than 4 sigma confidence.

nucl-ex↗
arXiv2015

High-Sensitivity Measurement of 3He-4He Isotopic Ratios for Ultracold Neutron Experiments

Research efforts ranging from studies of solid helium to searches for a neutron electric dipole moment require isotopically purified helium with a ratio of 3He to 4He at levels below that which can be measured using traditional mass spectroscopy techniques. We demonstrate an approach to such a measurement using accelerator mass spectroscopy, reaching the 10e-14 level of sensitivity, several orders of magnitude more sensitive than other techniques. Measurements of 3He/4He in samples relevant to the measurement of the neutron lifetime indicate the need for substantial corrections. We also argue that there is a clear path forward to sensitivity increases of at least another order of magnitude.

physics.ins-det↗
arXiv2015

Stochastic modeling and survival analysis of marginally trapped neutrons for a magnetic trapping neutron lifetime experiment

In a variety of neutron lifetime experiments, in addition to $β-$decay, neutrons can be lost by other mechanisms including wall losses. Failure to account for these other loss mechanisms produces systematic measurement error and associated systematic uncertainties in neutron lifetime measurements. In this work, we develop a physical model for neutron wall losses and construct a competing risks survival analysis model to account for losses due to the joint effect of $β-$decay losses, wall losses of marginally trapped neutrons, and an additional absorption mechanism. We determine the survival probability function associated with the wall loss mechanism by a Monte Carlo method. Based on a fit of the competing risks model to a subset of the NIST experimental data, we determine the mean lifetime of trapped neutrons to be approximately 700 s -- considerably less than the current best estimate of (880.1 $\pm$ 1.1) s promulgated by the Particle Data Group [1]. Currently, experimental studies are underway to determine if this discrepancy can be explained by neutron capture by ${}^3$He impurities in the trapping volume. Analysis of the full NIST data will be presented in a later publication.

nucl-ex↗
arXiv2009

Measuring the Neutron Lifetime Using Magnetically Trapped Neutrons

The neutron beta-decay lifetime plays an important role both in understanding weak interactions within the framework of the Standard Model and in theoretical predictions of the primordial abundance of 4He in Big Bang Nucleosynthesis. In previous work, we successfully demonstrated the trapping of ultracold neutrons (UCN) in a conservative potential magnetic trap. A major upgrade of the apparatus is nearing completion at the National Institute of Standards and Technology Center for Neutron Research (NCNR). In our approach, a beam of 0.89 nm neutrons is incident on a superfluid 4He target within the minimum field region of an Ioffe-type magnetic trap. A fraction of the neutrons is downscattered in the helium to energies <200 neV, and those in the appropriate spin state become trapped. The inverse process is suppressed by the low phonon density of helium at temperatures less than 200 mK, allowing the neutron to travel undisturbed. When the neutron decays the energetic electron ionizes the helium, producing scintillation light that is detected using photomultiplier tubes. Statistical limitations of the previous apparatus will be alleviated by significant increases in field strength and trap volume resulting in twenty times more trapped neutrons.

nucl-ex↗