arXiv subjects
Publications and source records attributed to C. Petrovic.
We report on a positive colossal magnetoresistance (MR) induced by metallization of FeSb$_{2}$, a nearly magnetic or "Kondo" semiconductor with 3d ions. We discuss contribution of orbital MR and quantum interference to enhanced magnetic field response of electrical resistivity.
Temperature dependence of the London penetration depth $λ$ measured in single crystals of CeCoIn$_5$ is interpreted as caused by a strong pair-breaking scattering that makes the superconductivity in this compound gapless. For a gapless d-wave superconductor, we derive $λ=λ_0/\sqrt{1-(T/T_c)^2}$ caused by combined effect of magnetic and non-magnetic scattering in excellent agreement with the data in the full temperature range and with the gapless s-wave case of Abrikosov and Gor'kov. We also obtain the slope of the upper critical field at $T_c$ that compares well with the measured slope.
Specific heat, magnetic susceptibility and electrical transport measurements were performed at ambient pressure on high-quality single crystal specimens of CeRhIn5 down to ultra-low temperatures. We report signatures of an anomaly observed in all measured quantities consistent with a bulk phase transition to a superconducting state at T_c=110 mK. Occurring far below the onset of antiferromagnetism at T_N=3.8 K, this transition appears to involve a significant portion of the available low-temperature density of electronic states, exhibiting an entropy change in line with that found in other members of the 115 family of superconductors tuned away from quantum criticality.
Neutron scattering is used to probe antiferromagnetic spin fluctuations in the d-wave heavy fermion superconductor CeCoIn$_{5}$ (T$_{c}$=2.3 K). Superconductivity develops from a state with slow ($\hbarΓ$=0.3 $\pm$ 0.15 meV) commensurate (${\bf{Q_0}}$=(1/2,1/2,1/2)) antiferromagnetic spin fluctuations and nearly isotropic spin correlations. The characteristic wavevector in CeCoIn$_{5}$ is the same as CeIn$_{3}$ but differs from the incommensurate wavevector measured in antiferromagnetically ordered CeRhIn$_{5}$. A sharp spin resonance ($\hbarΓ<0.07$ meV) at $\hbar ω$ = 0.60 $\pm$ 0.03 meV develops in the superconducting state removing spectral weight from low-energy transfers. The presence of a resonance peak is indicative of strong coupling between f-electron magnetism and superconductivity and consistent with a d-wave gap order parameter satisfying $Δ({\bf q+Q_0})=-Δ({\bf q})$.
The thermal Hall conductivity $κ_{xy}$ and Hall conductivity $σ_{xy}$ in CeCoIn$_5$ are used to determine the Lorenz number ${\cal L}_H$ at low temperature $T$. This enables the separation of the observed thermal conductivity into its electronic and non-electronic parts. We uncover evidence for a charge-neutral, field-dependent thermal conductivity, which we identify with spin excitations. At low $T$, these excitations dominate the scattering of charge carriers. We show that suppression of the spin excitations in high fields leads to a steep enhancement of the electron mean-free-path, which leads to an interesting scaling relation between the magnetoresistance, thermal conductivity and $σ_{xy}$.
The heavy-electron superconductor CeCoIn$_5$ exhibits a puzzling precursor state above its superconducting critical temperature at $T_c$ = 2.3 K. The thermopower and Nernst signal are anomalous. Below 15 K, the entropy current of the electrons undergoes a steep decrease reaching $\sim$0 at $T_c$. Concurrently, the off-diagonal thermoelectric current $α_{xy}$ is enhanced. The delicate sensitivity of the zero-entropy state to field implies phase coherence over large distances. The prominent anomalies in the thermoelectric current contrast with the relatively weak effects in the resistivity and magnetization.
The spin-lattice relaxation time, $T_{1}$, of conduction electrons is measured as a function of temperature and magnetic field in MgB$_2$. The method is based on the detection of the $z$ component of the conduction electron magnetization under electron spin resonance conditions with amplitude modulated microwave excitation. Measurement of $T_{1}$ below $T_c$ at 0.32 T allows to disentangle contributions from the two Fermi surfaces of MgB$_{2}$ as this field restores normal state on the Fermi surface part with $π$ symmetry only.
In CeCoIn$_5$, the thermal conductivity $κ_{xx}$ and Hall conductivity $κ_{xy}$ below $T_c$ display large anomalies below $T_c$. The strong suppression of the anomalies in weak fields implies the existence of long-lived quasiparticles. We also discuss briefly the Wiedemann-Franz ratio and the existence of a strongly field-dependent spin-fluctuation heat current.
The thermal conductivity $κ$ of the heavy-fermion superconductor CeIrIn$_5$ was measured as a function of temperature down to $T_c$/8, for current directions perpendicular ($J \parallel a$) and parallel ($J \parallel c$) to the tetragonal c axis. For $J \parallel a$, a sizable residual linear term $κ_0 / T$ is observed, as previously, which confirms the presence of line nodes in the superconducting gap. For $J \parallel c$, on the other hand, $κ/ T \to 0$ as $T \to 0$. The resulting precipitous decline in the anisotropy ratio $κ_c / κ_a$ at low temperature rules out a gap structure with line nodes running along the c-axis, such as the d-wave state favoured for CeCoIn$_5$, and instead points to a hybrid gap of $E_g$ symmetry. It therefore appears that two distinct superconducting states are realized in the Ce$M$In$_5$ family.
Heat and charge transport were used to probe the magnetic field-tuned quantum critical point in the heavy-fermion metal CeCoIn$_5$. A comparison of electrical and thermal resistivities reveals three characteristic energy scales. A Fermi-liquid regime is observed below $T_{FL}$, with both transport coefficients diverging in parallel and $T_{FL}\to 0$ as $H\to H_c$, the critical field. The characteristic temperature of antiferromagnetic spin fluctuations, $T_{SF}$, is tuned to a minimum but {\it finite} value at $H_c$, which coincides with the end of the $T$-linear regime in the electrical resistivity. A third temperature scale, $T_{QP}$, signals the formation of quasiparticles, as fermions of charge $e$ obeying the Wiedemann-Franz law. Unlike $T_{FL}$, it remains finite at $H_c$, so that the integrity of quasiparticles is preserved, even though the standard signature of Fermi-liquid theory fails.
Using small-angle neutron scattering, we have studied the flux-line lattice (FLL) in superconducting CeCoIn5. The FLL is found to undergo a first-order symmetry and reorientation transition at ~0.55 T at 50 mK. The FLL form factor in this material is found to be independent of the applied magnetic field, in striking contrast to the exponential decrease usually observed in superconductors. This result is consistent with a strongly field-dependent coherence length in CeCoIn5, in agreement with recent theoretical predictions for superclean, high-kappa superconductors.
We present a comprehensive optical study of the narrow gap $FeSb_2$ semiconductor. From the optical reflectivity, measured from the far infrared up to the ultraviolet spectral range, we extract the complete absorption spectrum, represented by the real part $σ_1(ω)$ of the complex optical conductivity. With decreasing temperature below 80 K, we find a progressive depletion of $σ_1(ω)$ below $E_g\sim 280$ cm$^{-1}$, the semiconducting optical gap. The suppressed (Drude) spectral weight within the gap is transferred at energies $ω>E_g$ and also partially piles up over a continuum of excitations extending in the spectral range between zero and $E_g$. Moreover, the interaction of one phonon mode with this continuum leads to an asymmetric phonon shape. Even though several analogies between $FeSb_2$ and $FeSi$ were claimed and a Kondo-insulator scenario was also invoked for both systems, our data on $FeSb_2$ differ in several aspects from those of $FeSi$. The relevance of our findings with respect to the Kondo insulator description will be addressed.
Thermal conductivity and specific heat were measured in the superconducting state of the heavy fermion material Ce_{1-x}La_{x}CoIn_{5}. With increasing impurity concentration x, the suppression of T_{c} is accompanied by the increase in the residual electronic specific heat expected of a d-wave superconductor, but it occurs in parallel with a decrease in residual electronic thermal conductivity. This contrasting behavior reveals the presence of uncondensed electrons coexisting with nodal quasiparticles. An extreme multiband scenario is proposed, with a d-wave superconducting gap on the heavy-electron sheets of the Fermi surface and a negligible gap on the light, three-dimensional pockets.
Heat and charge conduction were measured in the heavy-fermion metal CeRhIn5, an antiferromagnet with T_N=3.8 K. The thermal resistivity is found to be proportional to the magnetic entropy, revealing that spin fluctuations are as effective in scattering electrons as they are in disordering local moments. The electrical resistivity, governed by a q^2 weighting of fluctuations, increases monotonically with temperature. In contrast, the difference between thermal and electrical resistivities, characterized by an omega^2 weighting, peaks sharply at T_N and eventually goes to zero at a temperature T^* ~ 8 K. T^* thus emerges as a measure of the characteristic energy of magnetic fluctuations.
The thermal expansion and heat capacity of FeSb2 at ambient pressure agrees with a picture of a temperature induced spin state transition within the Fe t_{2g} multiplet. However, high pressure powder diffraction data show no sign of a structural phase transition up to 7GPa. A bulk modulus B=84(3)GPa has been extracted and the temperature dependence of the Gruneisen parameter has been determined. We discuss here the relevance of a Kondo insulator description for this material.
Point-contact spectroscopy was performed on single crystals of the heavy-fermion superconductor CeCoIn_5 between 150 mK and 2.5 K. A pulsed measurement technique ensured minimal Joule heating over a wide voltage range. The spectra show Andreev-reflection characteristics with multiple structures which depend on junction impedance. Spectral analysis using the generalized Blonder-Tinkham-Klapwijk formalism for d-wave pairing revealed two coexisting order parameter components, with amplitudes Delta_1 = 0.95 +/- 0.15 meV and Delta_2 = 2.4 +/- 0.3 meV, which evolve differently with temperature. Our observations indicate a highly unconventional pairing mechanism, possibly involving multiple bands.
The resistivity of the heavy-fermion superconductor CeCoIn5 was measured as a function of temperature, down to 25 mK and in magnetic fields of up to 16 T applied perpendicular to the basal plane. With increasing field, we observe a suppression of the non-Fermi liquid behavior, rho ~ T, and the development of a Fermi liquid state, with its characteristic rho = rho_0 + AT^2 dependence. The field dependence of the T^2 coefficient shows critical behavior with an exponent of 1.37. This is evidence for a field-induced quantum critical point (QCP), occuring at a critical field which coincides, within experimental accuracy, with the superconducting critical field H_c2. We discuss the relation of this field-tuned QCP to a change in the magnetic state, seen as a change in magnetoresistance from positive to negative, at a crossover line that has a common border with the superconducting region below ~ 1 K.
The resistivity of CeCoIn_5 was measured down to 20 mK in magnetic fields of up to 16 T. With increasing field, we observe a suppression of the non-Fermi liquid behavior, rho~T, and the development of a Fermi liquid state, with its characteristic rho=rho_0+AT^2 dependence. The field dependence of the T^2 coefficient shows critical behavior with an exponent of ~4/3. This is evidence for a new field-induced quantum critical point, occuring in this case at a critical field which coincides with the superconducting upper critical field H_c2.