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C. Ritter

Publications and source records attributed to C. Ritter.

At least 55 records · Page 3Linked to original sources
arXiv2017

Evolution of spin correlations in SrDy2O4 in an applied magnetic field

The development of short- and long-range magnetic order induced in a frustrated zig-zag ladder compound SrDy2O4 by an applied field is studied using neutron diffraction techniques. In zero field, SrDy2O4 lacks long-range magnetic order down to temperatures as low as 60 mK, and the observed powder neutron diffraction (PND) patterns are dominated by very broad diffuse scattering peaks. Single crystal neutron diffraction reveals that the zero-field magnetic structure consists of a collection of antiferromagnetic chains running along the c axis and that there is very little correlation between the chains in the ab plane. In an applied magnetic field, the broad diffuse scattering features in PND are gradually replaced by much sharper peaks, however, the pattern remains rather complex, reflecting the highly anisotropic nature of SrDy2O4. Single crystal neutron diffraction shows that a moderate field applied along the b axis induces an up-up-down magnetic order associated with a 1/3-magnetisation plateau, in which magnetic correlation length in the ab plane is significantly increased, but it nevertheless remains finite. The resolution limited k = 0 peaks associated with a ferromagnetic arrangement appear in powder and single crystal neutron diffraction patterns in fields of 2.5 T and above.

cond-mat.str-el↗
arXiv2016

Experimental Evidences for Static Charge Density Waves in Iron Oxy-pnictides

In this Letter we report high-resolution synchrotron X-ray powder diffraction and transmission electron microscope analysis of Mn-substituted LaFeAsO samples, demonstrating that a static incommensurate modulated structure develops across the low-temperature orthorhombic phase, whose modulation wave-vector depends on the Mn content. The incommensurate structural distortion is likely originating from a charge-density-wave instability, a periodic modulation of the density of conduction electrons associated with a modulation of the atomic positions. Our results add a new component in the physics of Fe-based superconductors, indicating that the density wave ordering is charge-driven.

cond-mat.supr-con↗
arXiv2016

Direct determination of the spin structure of Nd$_2$Ir$_2$O$_7$ by means of neutron diffraction

We report on the spin structure of the pyrochlore iridate Nd$_2$Ir$_2$O$_7$ that could be directly determined by means of powder neutron diffraction. Our magnetic structure refinement unravels a so-called all-in/all-out magnetic structure that appears in both, the Nd and the Ir sublattice. The ordered magnetic moments at 1.8 K amount to 0.34(1) $μ_\mathrm{B}$/Ir$^{4+}$ and 1.27(1) $μ_\mathrm{B}$/Nd$^{3+}$. The Nd$^{3+}$ moment size at 1.8 K is smaller than that expected for the Nd$^{3+}$ ground state doublet. On the other hand, the size of the ordered moments of the Ir$^{4+}$ ions at 1.8 K agrees very well with the value expected for a $J_\mathrm{eff}$ = 1/2 state based on the presence of strong spin-orbit coupling in this system. Finally, our measurements reveal a parallel alignment of the Nd$^{3+}$ moments with the net moment of its six nearest neighboring Ir$^{4+}$ ions.

cond-mat.str-el↗
arXiv2016

Zigzag antiferromagnetic ground state with anisotropic correlation lengths in the quasi-2D honeycomb lattice compound Na2Co2TeO6

The crystal structure, magnetic ground state, and the temperature dependent microscopic spin-spin correlations of the frustrated honeycomb lattice antiferromagnet Na2Co2TeO6 have been investigated by powder neutron diffraction. A three dimensional (3D) long-range antiferromagnetic ordering has been found below TN ~ 24.8 K. The magnetic ground state, determined to be zigzag antiferromagnet [k = (1/2 0 0)], occurs due to the competing exchange interactions up to third nearest neighbors within the honeycomb lattice. The exceptional existence of a limited magnetic correlation length along the c axis (perpendicular to the honeycomb layers in the ab planes) has been found within the 3D long-range ordered state, even at 1.8 K, well below TN. The observed limited correlation along the c axis is explained by the disorder distribution of the Na ions within the intermediate layers. The reduced ordered moments mCo(1) = 2.77(3) muB/Co2+ and mCo(2) = 2.45(2) muB/Co2+ at 1.8 K reflect the persistence of spin fluctuations in the ordered state. Above TN, the presence of short-range magnetic correlations, manifested by broad diffuse magnetic peaks, has been found. Reverse Monte Carlo analysis of the experimental diffuse magnetic scattering data reveals that the spin correlations are mainly confined within the 2D honeycomb layers (ab plane) with a correlation length of ~ 12 Å at 25 K. The nature of spin arrangements is found to be similar in both the short-range and long-range ordered magnetic states. This implies that the short-range correlation grows with decreasing temperature and leads to the zigzag AFM ordering at T < TN. The present study provides a comprehensive picture of the magnetic correlations over the temperature range above and below TN and their relation to the crystal structure. The role of intermediate soft Na-layers on the magnetic coupling between honeycomb planes is discussed.

cond-mat.str-el↗
arXiv2016

Application of a Theory and Simulation based Convective Boundary Mixing model for AGB Star Evolution and Nucleosynthesis

The $s$-process nucleosynthesis in Asymptotic Giant Branch (AGB) stars depends on the modeling of convective boundaries. We present models and s-process simulations that adopt a treatment of convective boundaries based on the results of hydrodynamic simulations and on the theory of mixing due to gravity waves in the vicinity of convective boundaries. Hydrodynamics simulations suggest the presence of convective boundary mixing (CBM) at the bottom of the thermal pulse-driven convective zone. Similarly, convection-induced mixing processes are proposed for the mixing below the convective envelope during third dredge-up where the 13C pocket for the s process in AGB stars forms. In this work we apply a CBM model motivated by simulations and theory to models with initial mass $M = 2$ and $M = 3M_\odot$, and with initial metal content Z = 0.01 and Z = 0.02. As reported previously, the He-intershell abundance of 12C and 16O are increased by CBM at the bottom of pulse-driven convection zone. This mixing is affecting the $^{22}Ne(α,n)^{25}Mg$ activation and the s-process effciency in the 13C-pocket. In our model CBM at the bottom of the convective envelope during the third dredgeup represents gravity wave mixing. We take further into account that hydrodynamic simulations indicate a declining mixing efficiency already about a pressure scale height from the convective boundaries, compared to mixing-length theory. We obtain the formation of the 13C-pocket with a mass of $\approx 10^{-4}M_\odot$. The final $s$-process abundances are characterized by 0.36 < [s=Fe] < 0.78 and the heavy-to-light s-process ratio is 0.23 < [hs=ls] < 0.45. Finally, we compare our results with stellar observations, pre-solar grain measurements and previous work.

astro-ph.SR↗
arXiv2016

Dimensional Reduction in Quantum Dipolar Antiferromagnets

We report ac susceptibility, specific heat, and neutron scattering measurements on a dipolar-coupled antiferromagnet LiYbF$_4$. For the thermal transition, the order-parameter critical exponent is found to be 0.20(1) and the specific-heat critical exponent -0.25(1). The exponents agree with the 2D XY/h$_4$ universality class despite the lack of apparent two-dimensionality in the structure. The order-parameter exponent for the quantum phase transitions is found to be 0.35(1) corresponding to (2+1)D. These results are in line with those found for LiErF$_4$ which has the same crystal structure, but largely different T$_N$, crystal field environment and hyperfine interactions. Our results therefore experimentally establish that the dimensional reduction is universal to quantum dipolar antiferromagnets on a distorted diamond lattice.

cond-mat.str-el↗
arXiv2016

NuGrid stellar data set I. Stellar yields from H to Bi for stars with metallicities Z = 0.02 and Z = 0.01

We provide a set of stellar evolution and nucleosynthesis calculations that applies established physics assumptions simultaneously to low- and intermediate-mass and massive star models. Our goal is to provide an internally consistent and comprehensive nuclear production and yield data base for applications in areas such as pre-solar grain studies. Our non-rotating models assume convective boundary mixing where it has been adopted before. We include 8 (12) initial masses for $Z = 0.01$ ($0.02$). Models are followed either until the end of the asymptotic giant branch phase or the end of Si burning, complemented by a simple analytic core-collapse supernova models with two options for fallback and shock velocities. The explosions show which pre-supernova yields will most strongly be effected by the explosive nucleosynthesis. We discuss how these two explosion parameters impacts the light elements and the $s$ and $p$ process. For low- and intermediate-mass models our stellar yields from H to Bi include the effect of convective boundary mixing at the He-intershell boundaries and the stellar evolution feedback of the mixing process that produces the $^{13}$C pocket. All post-processing nucleosynthesis calculations use the same nuclear reaction rate network and nuclear physics input. We provide a discussion of the nuclear production across the entire mass range organized by element group. All our stellar nucleosynthesis profile and time evolution output is available electronically, and tools to explore the data on the NuGrid VOspace hosted by the Canadian Astronomical Data Centre are introduced.

astro-ph.SR↗
arXiv2016

Sensitivity study for s process nucleosynthesis in AGB stars

In this paper we present a large-scale sensitivity study of reaction rates in the main component of the $s$ process. The aim of this study is to identify all rates, which have a global effect on the $s$ process abundance distribution and the three most important rates for the production of each isotope. We have performed a sensitivity study on the radiative $^{13}$C-pocket and on the convective thermal pulse, sites of the $s$ process in AGB stars. We identified 22 rates, which have the highest impact on the $s$-process abundances in AGB stars.

astro-ph.SR↗
arXiv2015

Nd2Sn2O7: an all-in-all-out pyrochlore magnet with no divergence-free field and anomalously slow paramagnetic spin dynamics

We report measurements performed on a polycrystalline sample of the pyrochlore compound Nd2Sn2O7. It undergoes a second order magnetic phase transition at Tc ~ 0.91 K to a noncoplanar all-in-all-out magnetic structure of the Nd3+ magnetic moments. The thermal behavior of the low temperature specific heat fingerprints excitations with linear dispersion in a three-dimensional lattice. The temperature independent spin-lattice relaxation rate measured below Tc and the anomalously slow paramagnetic spin dynamics detected up to ~ 30 Tc are suggested to be due to magnetic short-range correlations in unidimensional spin clusters, i.e., spin loops. The observation of a spontaneous field in muon spin relaxation measurements is associated with the absence of a divergence-free field for the ground state of an all-in-all-out pyrochlore magnet as predicted recently.

cond-mat.str-el↗
arXiv2015

Observation of long range magnetic ordering in pyrohafnate Nd2Hf2O7: A neutron diffraction study

We have investigated the physical properties of a pyrochlore hafnate Nd2Hf2O7 using ac magnetic susceptibility χ_ac(T), dc magnetic susceptibility χ(T), isothermal magnetization M(H) and heat capacity C_p(T) measurements, and determined the magnetic ground state by neutron powder diffraction study. An upturn is observed below 6 K in C_p(T)/T, however both C_p(T) and χ(T) do not show any clear anomaly down to 2 K. The χ_ac(T) shows a well pronounced anomaly indicating an antiferromagnetic transition at T_N = 0.55 K. The long range antiferromagnetic ordering is confirmed by neutron diffraction. The refinement of neutron diffraction pattern reveals an all-in/all-out antiferromagnetic structure, where for successive tetrahedra, the four Nd3+ magnetic moments point alternatively all-into or all-out-of the tetrahedron, with an ordering wavevector k = (0, 0, 0) and an ordered state magnetic moment of m = 0.62(1) μ_B/Nd at 0.1 K. The ordered moment is strongly reduced reflecting strong quantum fluctuations in ordered state.

cond-mat.str-el↗
arXiv2015

H ingestion into He-burning convection zones in super-AGB stellar models as a potential site for intermediate neutron-density nucleosynthesis

We investigate the evolution of super-AGB thermal pulse (TP) stars for a range of metallicities (Z) and explore the effect of convective boundary mixing (CBM). With decreasing metallicity and evolution along the TP phase, the He-shell flash and the third dredge-up (TDU) occur closer together in time. After some time (depending upon the CBM parameterisation), efficient TDU begins while the pulse-driven convection zone (PDCZ) is still present, causing a convective exchange of material between the PDCZ and the convective envelope. This results in the ingestion of protons into the convective He-burning pulse. Even small amounts of CBM encourage the interaction of the convection zones leading to transport of protons from the convective envelope into the He layer. H-burning luminosities exceed $10^9$ (in some cases $10^{10}$) $\mathrm{L}_\odot$. We also calculate models of dredge-out in the most massive super-AGB stars and show that the dredge-out phenomenon is another likely site of convective-reactive H-$^{12}$C combustion. We discuss the substantial uncertainties of stellar evolution models under these conditions. Nevertheless, the simulations suggest that in the convective-reactive H-combustion regime of H ingestion the star may encounter conditions for the intermediate neutron capture process (i process). We speculate that some CEMP-s/r stars could originate in i-process conditions in the H-ingestion phases of low-Z SAGB stars. This scenario would however suggest a very low electron-capture supernova rate from super-AGB stars. We also simulate potential outbursts triggered by such H-ingestion events, present their light curves and briefly discuss their transient properties.

astro-ph.SR↗
arXiv2015

The i-process and CEMP-r/s stars

We investigate whether the anomalous elemental abundance patterns in some of the C-enhanced metal-poor-s+r (CEMP-r/s) stars are consistent with predictions of nucleosynthesis yields from the i-process, a neutron-capture regime at neutron densities intermediate between those typical for the slow (s) and rapid (r) processes. Conditions necessary for the i-process are expected to be met at multiple stellar sites, such as the He-core and He-shell flashes in low-metallicity low-mass stars, super-AGB and post-AGB stars, as well as low-metallicity massive stars. We have found that single-exposure one-zone simulations of the i-process reproduce the abundance patterns in some of the CEMP-r/s stars much better than the model that assumes a superposition of yields from s- and r-process sources. Our previous study of nuclear data uncertainties relevant to the i-process revealed that they could have a significant impact on the i-process yields obtained in our idealized one-zone calculations, leading, for example, to ~0.7dex uncertainty in our predicted [Ba/La] ratio. Recent 3D hydrodynamic simulations of convection driven by a He-shell flash in post-AGB Sakurai's object have discovered a new mode of non-radial instabilities: the Global Oscillation of Shell H-ingestion. This has demonstrated that spherically symmetric stellar evolution simulations cannot be used to accurately model physical conditions for the i-process.

astro-ph.SR↗
arXiv2015

Contrasting chemical pressure effect on the moment direction in the Kondo semiconductor CeT$_2$Al$_{10}$ (T = Ru,Os)

The opening of a spin gap in the orthorhombic compounds CeT$_2$Al$_{10}$ (T = Ru and Os) is followed by antiferromagnetic ordering at $T_N$ = 27 K and 28.5 K, respectively, with a small ordered moment (0.29$-$0.34$μ_B$) along the $c-$axis, which is not an easy axis of the crystal field (CEF). In order to investigate how the moment direction and the spin gap energy change with 10\% La doping in Ce$_{1-x}$La$_x$T$_2$Al$_{10}$ (T = Ru and Os) and also to understand the microscopic nature of the magnetic ground state, we here report on magnetic, transport, and thermal properties, neutron diffraction (ND) and inelastic neutron scattering (INS) investigations on these compounds. Our INS study reveals the persistence of spin gaps of 7 meV and 10 meV in the 10\% La-doped T = Ru and Os compounds, respectively. More interestingly our ND study shows a very small ordered moment of 0.18 $μ_B$ along the $b-$axis (moment direction changed compared with the undoped compound), in Ce$_{0.9}$La$_{0.1}$Ru$_2$Al$_{10}$, however a moment of 0.23 $μ_B$ still along the $c-$axis in Ce$_{0.9}$La$_{0.1}$Os$_2$Al$_{10}$. This contrasting behavior can be explained by a different degree of hybridization in CeRu$_2$Al$_{10}$ and CeOs$_2$Al$_{10}$, being stronger in the latter than in the former. Muon spin rotation ($μ$SR) studies on Ce$_{1-x}$La$_x$Ru$_2$Al$_{10}$ ($x$ = 0, 0.3, 0.5 and 0.7), reveal the presence of coherent frequency oscillations indicating a long$-$range magnetically ordered ground state for $x$ = 0 to 0.5, but an almost temperature independent Kubo$-$Toyabe response between 45 mK and 4 K for $x$ = 0.7. We will compare the results of the present investigations with those reported on the electron and hole$-$doping in CeT$_2$Al$_{10}$.

cond-mat.str-el↗
arXiv2014

Magnetic properties of the RbMnPO4 zeolite-ABW type material: a frustrated zigzag spin chain

The crystal structure and magnetic properties of the RbMnPO4 zeolite-ABW type material have been studied by temperature-dependent neutron powder diffraction, low temperature magnetometry and heat capacity measurements. RbMnPO4 represents a rare example of a weak ferromagnetic polar material, containing Mn2+ ions with TN = 4.7 K. The neutron powder diffraction pattern recorded at T = 10 K shows that the compound crystallizes in the chiral and polar monoclinic space group P21 (No. 4) with the unit-cell parameters: a = 8.94635(9) Å, b = 5.43415(5) Å, c = 9.10250(8) Å and beta = 90.4209(6)°. A close inspection of the crystal structure of RbMnPO4 shows that this material presents two different types of zigzag chains running along the b axis. This is a unique feature among the zeolite-ABW type materials exhibiting the P21 symmetry. At low temperature, RbMnPO4 exhibits a canted antiferromagnetic structure characterized by the propagation vector k1 = 0 resulting in the magnetic symmetry P21. The magnetic moments lie mostly along the b axis with the ferromagnetic component being in the ac plane. Due to the geometrical frustration present in this system, an intermediate phase appears within the temperature range 4.7 - 5.1 K characterized by the propagation vector k2 = (kx, 0, kz) with kx/kz = 2. This ratio is reminiscent of the multiferroic phase of the orthorhombic RMnO3 phases (R = rare earth). This suggests that RbMnPO4 could present some multiferroic properties at low temperature. Our density functional calculations confirm the presence of magnetic frustration, which explains this intermediate incommensurate phase. Taking into account the strongest magnetic interactions, we are able to reproduce the magnetic structure observed experimentally at low temperature.

cond-mat.mtrl-sci↗
arXiv2014

Anomalous change of the magnetic moment direction by hole doping in CeRu$_2$Al$_{10}$

We present a detailed investigation of the hole (3\% Re) doping effect on the polycrystalline CeRu$_{2}$Al$_{10}$ sample by magnetization, heat capacity, resistivity, muon spin rotation ($μ$SR), and neutron scattering (both elastic and inelastic) measurements. CeRu$_2$Al$_{10}$ is an exceptional cerium compound with an unusually high Neel temperature of 27 K. Here we study the stability of the unusual magnetic order by means of controlled doping, and we uncover further surprising attributes of this phase transition. The heat capacity, resistivity and $μ$SR measurements reveal an onset of magnetic ordering below 23 K, while a broad peak at 31 K (i.e. above $T_N$), has been observed in the temperature dependent susceptibility, indicating an opening of a spin gap above $T_N$. Our important finding, from the neutron diffraction, is that the compound orders antiferromagnetically with a propagation vector $\bf k$ = (1 0 0) and the ordered state moment is 0.20(1)$μ_B$ along the $b-$axis. This is in sharp contrast to the undoped compound, which shows AFM ordering at 27 K with the ordered moment of 0.39(3)$μ_B$ along the $c-$axis. Similar to CeRu$_2$Al$_{10}$ our inelastic neutron scattering study on the Re doped shows a sharp spin gap-type excitation near 8 meV at 5 K, but with slightly reduced intensity compared to the undoped compound. Further the excitation broadens and shifts to lower energy ($\le$ 4 meV) near 35 K. These results suggest that the low temperature magnetic properties of the hole doped sample is governed by the competition between the anisotropic hybridization effect and crystal field anisotropy as observed in hole-doped CeOs$_2$Al$_{10}$.

cond-mat.str-el↗
arXiv2013

Chemical pressure effects on structural, dielectric and magnetic properties of solid solutions Mn3-xCoxTeO6

The effects of Co2+ doping on the structural, magnetic and dielectric properties of the multiferroic frustrated antiferromagnet Mn3TeO6 have been investigated. Ceramic samples of the solid solution series Mn3-xCoxTeO6 were prepared by a solid-state reaction route. X-ray and neutron powder diffraction and electron microscopy techniques were combined with calorimetric, dielectric and magnetic measurements to investigate the dependence of the crystal structure and physical properties on temperature and composition. It is shown that the compounds with x up to 2.4 all adopt the trigonal corundum-related structure of pure Mn3TeO6 (space group R-3) in the temperature range 5-295 K and that the lattice parameters a and c and the unit-cell volume V decrease linearly with increasing Co2+ concentration. The low- temperature magnetic susceptibility and heat capacity data evidence the antiferromagnetic ordering of all samples. The Neel temperature linearly increases with Co2+ concentration x. Curie-Weiss fits of the high temperature susceptibility indicate that the magnetic frustration decreases with x. The derived magnetic structure of Mn3TeO6 can be described as an incommensurately modulated magnetic spin state with k = [0, 0, kz] and an elliptical spin- spiral order of spins within the chains of MnO6 octahedra. With increasing Co2+ concentration the propagation vector kz changes from 0.453 (x = 0) to 0.516 (x = 2.4). The magnetic anisotropy changes as well, leading to a reorientation of the spiral-basal plane. A possible coexistence of long-range order of electrical dipoles and magnetic moments in Mn3-xCoxTeO6 is discussed.

cond-mat.mtrl-sci↗
arXiv2013

Spin and Dipole Ordering in Ni_2InSbO_6 and Ni_2ScSbO_6 with corundum-related structure

The complex metal oxides Ni2InSbO6 (NISO) and Ni2ScSbO6 (NSSO) have been prepared in form of polycrystalline powders by a solid state reaction route. The crystal structure and magnetic properties of the compounds were investigated using a combination of X-ray and neutron powder diffraction, electron microscopy, calorimetric and magnetic measurements. The compounds adopt a trigonal structure, space group R3, of the corundum related Ni3TeO6 (NTO) type. Only one of the octahedral Ni positions (Ni(2)) of the NTO structure was found to be occupied by In (Sc). NTO has non-centrosymmetric structure and is ferroelectric below 1000 K, dielectric and second harmonic measurements suggest that also NISO and NSSO are correspondingly ferroelectric. Magnetization measurements signified antiferromagnetic ordering below TN=60 K (NSSO) and 76 K (NISO). The magnetic structure is formed by two antiferromagnetically coupled incommensurate helices with the spiral axis along the b-axis and propagation vector k = [0, ky,0] with ky= 0.036(1) (NSSO) and ky= 0.029(1) (NISO). The observed structural and magnetic properties of NISO and NSSO are discussed and compared with those of NTO.

cond-mat.mtrl-sci↗