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C. Schneider

Publications and source records attributed to C. Schneider.

At least 127 records · Page 7Linked to original sources
arXiv2016

Impact of ex-situ rapid thermal annealing on the magneto-optical properties and the oscillator strength of In(Ga)As quantum dots

We discuss the influence of a rapid thermal annealing step on the magneto-optical emission properties of In(Ga)As/GaAs quantum dots. We map out a strong influence of the growth- and anneling parameters on the quantum excitons' effective Landé g-factors and in particular on their diamagnetic coefficients, which we directly correlate with the modification of the emitters shape and material composition. In addition, we study the excitons' spontaneous emission lifetime as a function of the annealing temperature and the dot height, and observe a strong increase of the emission rate with the quantum dot volume. The corresponding increase in oscillator strenth yields fully consistent results with the analysis of the diamagenic behavior. In particular, we demonstrate that a rapid thermal annealing step of 850$^\circ$ C can be employed to increase the oscillator strength of as-grown InAs/GaAs QDs by more than a factor of $2$.

cond-mat.mes-hall↗
arXiv2016

Dynamics of spatial coherence and momentum distribution of polaritons in a semiconductor microcavity under conditions of Bose-Einstein condensation

The dynamics of spatial coherence and momentum distribution of polaritons in the regime of Bose-Einstein condensation are investigated in a GaAs microcavity with embedded quantum wells under nonresonant excitation with picosecond laser pulses. It is shown that the onset of the condensate first order sparial coherence is accompanied by narrowing of the polariton momentum distribution. At the same time, at sufficiently high excitation densities, there is significant qualitative discrepancy between the dynamic behavior of the width of the polariton momentum distribution determined from direct measurements and that calculated from the coherence spatial distribution. This discrepancy is observed at the fast initial stage of the polariton system kinetics and, apparently, results from the strong spatial nonuniformity of the phase of the condensate wave function, which equilibrates on a much longer time scale.

cond-mat.quant-gas↗
arXiv2016

Monolayer MoSe2: A candidate for room temperature polaritonics

Monolayered MoSe2 is a promising new material to investigate advanced light-matter coupling as it hosts stable and robust excitons with comparably narrow optical resonances. In this work, we investigate the evolution of the lowest lying excitonic transition, the so-called A-valley exciton, with temperature. We find a strong, phonon-induced temperature broadening of the resonance, and more importantly, a reduction of the oscillator strength for increased temperatures. Based on these experimentally extracted, temperature dependent parameters, we apply a coupled oscillator model to elucidate the possibility to observe the strong coupling regime between the A-exciton and a microcavity resonance in three prototypical photonic architectures with varying mode volumes. We find that the formation of exciton-polaritons up to ambient conditions in short, monolithic dielectric and Tamm-based structures seems feasible. In contrast, a temperature-induced transition into the weak coupling regime can be expected for structures with extended effective cavity length. Based on these findings, we calculate and draw the phase diagram of polariton Bosonic condensation in a MoSe2 cavity.

cond-mat.mes-hall↗
arXiv2016

Talbot effect for exciton-polaritons

We demonstrate, experimentally and theoretically, a Talbot effect for hybrid light-matter waves -- exciton-polariton condensate formed in a semiconductor microcavity with embedded quantum wells. The characteristic 'Talbot carpet' is produced by loading the exciton-polariton condensate into a microstructured one dimensional periodic array of mesa traps, which creates an array of sources for coherent polariton flow in the plane of the quantum wells. The spatial distribution of the Talbot fringes outside the mesas mimics the near-field diffraction of a monochromatic wave on a periodic amplitude and phase grating with the grating period comparable to the wavelength. Despite the lossy nature of the polariton system, the Talbot pattern persists for distances exceeding the size of the mesas by an order of magnitude.

cond-mat.quant-gas↗
arXiv2016

Photon echo transients from an inhomogeneous ensemble of semiconductor quantum dots

An ensemble of quantum dot excitons may be used for coherent information manipulation. Due to the ensemble inhomogeneity any optical information retrieval occurs in form of a photon echo. We show that the inhomogeneity can lead to a significant deviation from the conventional echo timing sequence. Variation of the area of the initial rotation pulse, which generates excitons in a dot sub-ensemble only, reveals this complex picture of photon echo formation. We observe a retarded echo for π/2 pulses, while for 3π/2 the echo is advanced in time as evidenced through monitoring the Rabi oscillations in the time-resolved photon echo amplitude from (In,Ga)As/GaAs self-assembled quantum dot structures and confirmed by detailed calculations.

cond-mat.mes-hall↗
arXiv2015

Multi-Wave Coherent Control of a Solid State Single Emitter

Coherent control of individual two-level systems (TLSs) is at the basis of any implementation of quantum information. An impressive level of control is now achieved using nuclear, vacancies and charge spins. Manipulation of bright exciton transitions in semiconductor quantum dots (QDs) is less advanced, principally due to the sub-nanosecond dephasing. Conversely, owing to their robust coupling to light, one can apply tools of nonlinear spectroscopy to achieve all-optical command. Here, we report on the coherent manipulation of an exciton via multi-wave mixing. Specifically, we employ three resonant pulses driving a single InAs QD. The first two induce a four-wave mixing (FWM) transient, which is projected onto a six-wave mixing (SWM) depending on the delay and area of the third pulse, in agreement with analytical predictions. Such a switch enables to demonstrate the generation of SWM on a single emitter and to engineer the spectro-temporal shape of the coherent response originating from a TLS. These results pave the way toward multi-pulse manipulations of solid state qubits via implementing the NMR-like control schemes in the optical domain.

cond-mat.mes-hall↗
arXiv2015

Exciton-Polariton Trapping and Potential Landscape Engineering

Exciton-polaritons in semiconductor microcavities have advanced to become a model system for studying dynamical Bose-Einstein condensation, macroscopic coherence, many-body effects, nonclassical states of light and matter, and possibly quantum phase transitions in a solid state. Being low mass bosons, these light-matter quasiparticles can condense at comparably high temperatures up to 300K, while preserving fundamental properties such as coherence in space and time domain even when they are out of equilibrium with the environment. Although the presence of an in-plane polariton confinement potential is not strictly necessary in order to observe condensation of polaritons, engineering the polariton confinement is a key to controlling, shaping and directing the flow of polaritons. Prototype polariton-based optoelectronic devices rely on ultrafast photon-like velocities and strong nonlinearities, as well as on tailored confinement. Nanotechnology provides several pathways to achieving such a confinement, and the specific features and advantages of the different techniques are discussed in this paper. As hybrid exciton-photon quasiparticles, polaritons can be trapped via their excitonic as well as their photonic component, which leads to a wide choice of highly complementary techniques. Here we highlight the almost free choice of trapping geometries and depths of confinement that provides a powerful tool for control and manipulation of polariton systems both in semi-classical and quantum domain. Furthermore, the possibility to observe effects of polariton blockade, Mott insulator physics, and population of higher-order bands in sophisticated lattice potentials is discussed. The observation of such effects will signify the opportunity for the realization of novel polaritonic non-classical light sources and quantum simulators.

cond-mat.quant-gas↗
arXiv2015

Collective state transitions of exciton-polaritons loaded into a periodic potential

We study the loading of a nonequilibrium, dissipative system of composite bosons -- exciton polaritons -- into a one dimensional periodic lattice potential. Utilizing momentum resolved photoluminescence spectroscopy, we observe a transition between an incoherent Bose gas and a polariton condensate, which undergoes further transitions between different energy states in the band-gap spectrum of the periodic potential with increasing pumping power. We demonstrate controlled loading into distinct energy bands by modifying the size and shape of the excitation beam. The observed effects are comprehensively described in the framework of a nonequilibrium model of polariton condensation. In particular, we implement a stochastic treatment of quantum and thermal fluctuations in the system and confirm that polariton-phonon scattering is a key energy relaxation mechanism enabling transitions from the highly nonequilibrium polariton condensate in the gap to the ground band condensation for large pump powers.

cond-mat.mes-hall↗
arXiv2015

Calculating Three Loop Ladder and V-Topologies for Massive Operator Matrix Elements by Computer Algebra

Three loop ladder and $V$-topology diagrams contributing to the massive operator matrix element $A_{Qg}$ are calculated. The corresponding objects can all be expressed in terms of nested sums and recurrences depending on the Mellin variable $N$ and the dimensional parameter $\varepsilon$. Given these representations, the desired Laurent series expansions in $\varepsilon$ can be obtained with the help of our computer algebra toolbox. Here we rely on generalized hypergeometric functions and Mellin-Barnes representations, on difference ring algorithms for symbolic summation, on an optimized version of the multivariate Almkvist-Zeilberger algorithm for symbolic integration, and on new methods to calculate Laurent series solutions of coupled systems of differential equations. The solutions can be computed for general coefficient matrices directly for any basis also performing the expansion in the dimensional parameter in case it is expressible in terms of indefinite nested product-sum expressions. This structural result is based on new results of our difference ring theory. In the cases discussed we deal with iterative sum- and integral-solutions over general alphabets. The final results are expressed in terms of special sums, forming quasi-shuffle algebras, such as nested harmonic sums, generalized harmonic sums, and nested binomially weighted (cyclotomic) sums. Analytic continuations to complex values of $N$ are possible through the recursion relations obeyed by these quantities and their analytic asymptotic expansions. The latter lead to a host of new constants beyond the multiple zeta values, the infinite generalized harmonic and cyclotomic sums in the case of $V$-topologies.

hep-ph↗
arXiv2015

Controlling circular polarization of light emitted by quantum dots using chiral photonic crystal slab

We study the polarization properties of light emitted by quantum dots that are embedded in chiral photonic crystal structures made of achiral planar GaAs waveguides. A modification of the electromagnetic mode structure due to the chiral grating fabricated by partial etching of the wave\-guide layer has been shown to result in a high circular polarization degree $ρ_c$ of the quantum dot emission in the absence of external magnetic field. The physical nature of the phenomenon can be understood in terms of the reciprocity principle taking into account the structural symmetry. At the resonance wavelength, the magnitude of $|ρ_c|$ is predicted to exceed 98%. The experimentally achieved value of $|ρ_c|=81$% is smaller, which is due to the contribution of unpolarized light scattered by grating defects, thus breaking its periodicity. The achieved polarization degree estimated removing the unpolarized nonresonant background from the emission spectra can be estimated to be as high as 96%, close to the theoretical prediction.

physics.optics↗
arXiv2015

The O(α_s^3) Heavy Flavor Contributions to the Charged Current Structure Function xF_3(x,Q^2) at Large Momentum Transfer

We calculate the massive Wilson coefficients for the heavy flavor contributions to the non-singlet charged current deep-inelastic scattering structure function $xF_3^{W^+}(x,Q^2)+xF_3^{W^-}(x,Q^2)$ in the asymptotic region $Q^2 \gg m^2$ to 3-loop order in Quantum Chromodynamics (QCD) at general values of the Mellin variable $N$ and the momentum fraction $x$. Besides the heavy quark pair production also the single heavy flavor excitation $s \rightarrow c$ contributes. Numerical results are presented for the charm quark contributions and consequences on the Gross-Llewellyn Smith sum rule are discussed.

hep-ph↗
arXiv2015

Broadband indistinguishability from bright parametric downconversion in a semiconductor waveguide

Parametric downconversion (PDC) in semiconductor Bragg-reflection waveguides (BRW) is routinely exploited for photon-pair generation in the telecommunication range. Contrary to many conventional PDC sources, BRWs offer possibilities to create spectrally broadband but nevertheless indistinguishable photon pairs in orthogonal polarizations that simultaneously incorporate high frequency entanglement. We explore the characteristics of co-propagating twin beams created in a type-II ridge BRW. Our PDC source is bright and efficient, which serves as a benchmark of its performance and justifies its exploitation for further use in quantum photonics. We then examine the coalescence of the twin beams and investigate the effect of their inevitable multi-photon contributions on the observed photon bunching. Our results show that BRWs have a great potential for producing broadband indistinguishable photon pairs as well as multi-photon states.

quant-ph↗
arXiv2015

Modally Resolved Fabry-Perot Experiment with Semiconductor Waveguides

Based on the interaction between different spatial modes, semiconductor Bragg-reflection waveguides provide a highly functional platform for non-linear optics. Therefore, the control and engineering of the properties of each spatial mode is essential. Despite the multimodeness of our waveguide, the well-established Fabry-Perot technique for recording fringes in the optical transmission spectrum can successfully be employed for a detailed linear optical characterization when combined with Fourier analysis. A prerequisite for the modal sensitivity is a finely resolved transmission spectrum that is recorded over a broad frequency band. Our results highlight how the features of different spatial modes, such as their loss characteristics and dispersion properties, can be separated from each other allowing their comparison. The mode-resolved measurements are important for optimizing the performance of such multimode waveguides by tailoring the properties of their spatial modes.

quant-ph↗
arXiv2015

The 3-Loop Non-Singlet Heavy Flavor Contributions to the Structure Function g_1(x,Q^2) at Large Momentum Transfer

We calculate the massive flavor non-singlet Wilson coefficient for the heavy flavor contributions to the polarized structure function $g_1(x,Q^2)$ in the asymptotic region $Q^2 \gg m^2$ to 3-loop order in Quantum Chromodynamics at general values of the Mellin variable $N$ and the momentum fraction $x$, and derive heavy flavor corrections to the Bjorken sum-rule. Numerical results are presented for the charm quark contribution. Results on the structure function $g_2(x,Q^2)$ in the twist-2 approximation are also given.

hep-ph↗
arXiv2015

Observation of non-Hermitian degeneracies in a chaotic exciton-polariton billiard

Exciton-polaritons are hybrid light-matter quasiparticles formed by strongly interacting photons and excitons (electron-hole pairs) in semiconductor microcavities. They have emerged as a robust solid-state platform for next-generation optoelectronic applications as well as fundamental studies of quantum many-body physics. Importantly, exciton-polaritons are a profoundly open (i.e., non-Hermitian) quantum system: it requires constant pumping of energy and continuously decays releasing coherent radiation. Thus, the exciton-polaritons always exist in a balanced potential landscape of gain and loss. However, the inherent non-Hermitian nature of this potential has so far been largely ignored in exciton-polariton physics. Here we demonstrate that non-Hermiticity dramatically modifies the structure of modes and spectral degeneracies in exciton-polariton systems, and, therefore, will affect their quantum transport, localisation, and dynamical properties. Using a spatially-structured optical pump, we create a chaotic exciton-polariton billiard. Eigenmodes of this billiard exhibit multiple non-Hermitian spectral degeneracies -- exceptional points. These are known to cause remarkable wave phenomena, such as unidirectional transport, anomalous lasing/absorption, and chiral modes. By varying parameters of the billiard, we observe crossing and anti-crossing of energy levels and reveal the nontrivial topological modal structure exclusive to non-Hermitian systems. We also observe the mode switching and topological Berry phase for a parameter loop encircling the exceptional point. Our findings pave the way for studies of non-Hermitian quantum dynamics of exciton-polaritons, which can lead to novel functionalities of polariton-based devices.

cond-mat.quant-gas↗
arXiv2015

Single Semiconductor Quantum Dots in Microcavities: Bright sources of indistinguishable Photons

In this chapter we will discuss the technology and experimental techniques to realize quantum dot (QD) single photon sources combining high outcoupling efficiencies and highest degrees of non-postselected photon indistinguishability. The system, which is based on ultra low density InAs QDs embedded in a quasi planar single sided microcavity with natural photonic traps is an ideal testbed to study quantum light emission from single QDs. We will discuss the influence of the excitation conditions on the purity of the single photon emission, and in particular on the degree of indistinguishability of the emitted photons. While high purity triggered emission of single photons is observed under all tested excitation conditions, single photon interference effects can be almost vanish in experiments relying on non-resonant pumping into the quantum dot wetting layer. In contrast, we can observe nearly perfect indistinguishability of single photons in resonance fluorescence excitation conditions, which underlines the superiority of this excitation scheme to create photon wave packets close to the Fourier limit. As a first step towards the realization of solid state quantum networks based on quantum dot single photon sources we test the overlap of photons emitted from remote QDs yielding non-postselected interference visibilities on the order of ~40% for quasi resonant excitation.

quant-ph↗
arXiv2015

Enhanced single photon emission from positioned InP/GaInP quantum dots coupled to a confined Tamm-plasmon mode

We report on the enhancement of the spontaneous emission in the visible red spectral range from site-controlled InP/GaInP quantum dots by resonant coupling to Tammplasmon modes confined beneath gold disks in a hybrid metal/semiconductor structure. The enhancement of the emission intensity is confirmed by spatially resolved microphotoluminescence area scans and temperature dependent measurements. Single photon emission from our coupled system is verified via second order autocorrelation measurements. We observe bright single quantum dot emission of up to ~173000 detected photons per second at a repetition rate of the excitation source of 82 MHz, and calculate an extraction efficiency of our device as high as 7%.

cond-mat.mes-hall↗