arXiv subjects

C. Sow

Publications and source records attributed to C. Sow.

5 recordsLinked to original sources

arXiv2021

Orbital dichotomy of Fermi liquid properties in Sr$_2$RuO$_4$ revealed by Raman spectroscopy

We report a polarization-resolved Raman spectroscopy study of the orbital dependence of the quasiparticles properties in the prototypical multi-band Fermi liquid Sr\textsubscript{2}RuO\textsubscript{4}. We show that the quasiparticle scattering rate displays $\omega^{2}$ dependence as expected for a Fermi liquid. Besides, we observe a clear polarization-dependence in the energy and temperature dependence of the quasiparticle scattering rate and mass, with the $d_{xz/yz}$ orbital derived quasiparticles showing significantly more robust Fermi liquid properties than the $d_{xy}$ orbital derived ones. The observed orbital dichotomy of the quasiparticles is consistent with the picture of Sr\textsubscript{2}RuO\textsubscript{4} as a Hund's metal. Our study establishes Raman scattering as a powerful probe of Fermi liquid properties in correlated metals.

cond-mat.str-el↗

arXiv2020

Observation of Pines' Demon in Sr$_2$RuO$_4$

The characteristic excitation of a metal is its plasmon, which is a quantized collective oscillation of its electron density. In 1956, David Pines predicted that a distinct type of plasmon, dubbed a "demon," could exist in three-dimensional metals containing more than one species of charge carrier. Consisting of out-of-phase movement of electrons in different bands, demons are acoustic, electrically neutral, and do not couple to light, so have never been detected in an equilibrium, three-dimensional metal. Nevertheless, demons are believed to be critical for diverse phenomena including phase transitions in mixed-valence semimetals, optical properties of metal nanoparticles, "soundarons" in Weyl semimetals, and high temperature superconductivity in, for example, metal hydrides. Here, we present evidence for a demon in Sr$_2$RuO$_4$ from momentum-resolved electron energy-loss spectroscopy (M-EELS). Formed of electrons in the $\beta$ and $\gamma$ bands, the demon is gapless with a room temperature velocity $v=1.065 \pm 0.12 \times 10^5$ m/s and critical momentum $q_c=0.08$ reciprocal lattice units. Its spectral weight violates low-energy partial sum rules, affirming its neutral character. Our study confirms a 66-year old prediction and suggests that demons may be a pervasive feature of multiband metals.

cond-mat.str-el↗

arXiv2019

Anomalous anisotropic behaviour of spin-triplet proximity effect in Au/SrRuO$_3$/Sr$_2$RuO$_4$ junctions

Spin-polarized supercurrents can be generated with magnetic inhomogeneity at a ferromagnet/spin-singlet-superconductor interface. In such systems, complex magnetic inhomogeneity makes it difficult to functionalise the spin-polarized supercurrents. However, spin-polarized supercurrents in ferromagnet/spin-triplet-superconductor junctions can be controlled by angle between magnetization and spin of Copper pairs ($d$-vector), that can effectively be utilized in developing of a field of research known as superconducting spintronics. Recently, we found induction of spin-triplet correlation into a ferromagnet SrRuO$_3$ epitaxially deposited on a spin-triplet superconductor Sr$_2$RuO$_4$, without any electronic spin-flip scattering. Here, we present systematic magnetic field dependence of the proximity effect in Au/SrRuO$_3$/ Sr$_2$RuO$_4$ junctions. It is found that induced triplet correlations exhibit strong anisotropic field response. Such behaviour attributes to the rotation of the $d$-vector of Sr$_2$RuO$_4$. This anisotropic behaviour is in contrast with the vortex dynamic. Our results will stimulate study of interaction between ferromagnetism and unconventional superconductivity.

cond-mat.supr-con↗

arXiv2018

Abnormal $phase$ flip in coherent phonon oscillations of Ca$_2$RuO$_4$

We employ an optical pump-probe technique to study coherent phonon oscillations in Ca$_2$RuO$_4$. We find that oscillation-amplitude of an $A_g$ symmetric phonon mode is strongly suppressed at 260 K, a putative transition point of orbital ordering. The oscillation also shows a gradual but huge change in its $phase$, such that the oscillation even flips over with a 180$^{\circ}$ change across the temperature. Density functional theory calculations indicate that the $A_g$ phonon has an eigenmode of octahedral distortion with conventional tilting along the $a$-axis and antipolar distortion of apical oxygen. Careful inspection of the lattice captures an unusually large antipolar distortion in low-temperature structures, which may play a crucial role for the phase transition at 260 K.

cond-mat.str-el↗

arXiv2018

Strong spin-phonon coupling unveiled by coherent phonon oscillations in Ca2RuO4

We utilize near-infrared femtosecond pulses to investigate coherent phonon oscillations of Ca2RuO4. The coherent Ag phonon mode of the lowest frequency changes abruptly not only its amplitude but also the oscillation-phase as the spin order develops. In addition, the phonon mode shows a redshift entering the magnetically ordered state, which indicates a spin-phonon coupling in the system. Density functional theory calculations reveal that the Ag oscillations result in octahedral tilting distortions, which are exactly in sync with the lattice deformation driven by the magnetic ordering. We suggest that the structural distortions by the spin-phonon coupling can induce the unusual oscillation-phase shift between impulsive and displacive type oscillations.

cond-mat.str-el↗