arXiv subjects

C. U. Jung

Publications and source records attributed to C. U. Jung.

At least 37 records · Page 2Linked to original sources

arXiv2001

A Magnetization and Microwave Study of Superconducting MgB2

We report magnetic field dependent magnetization and microwave impedance measurements on a MgB2 superconductor prepared by high pressure synthesis. We find that the upper critical field is linearly dependent on temperature near Tc and the dc irreversibility field exponent is ~1.4. The microwave data display an excess surface resistance below Tc which is neither observed in low Tc nor in high temperature superconductors (HTSC). The real part of the complex conductivity, sigma1, shows a huge maximum below Tc and the imaginary part, sigma2, is linear for temperatures less than 20 K, which can not be simply accounted for by the weak coupling BCS model with an s-wave superconducting order parameter. We speculate that this may be due to the two gaps reported by other studies. Unlike measurements on the high temperature superconducting cuprates, we find no evidence of weak-links in the superconducting state. By inverting the magnetic field dependent impedance data, we find a vortex depinning frequency that decreases with increasing magnetic field and evidence for an anisotropic upper critical magnetic field.

cond-mat.supr-con↗

arXiv2001

X-ray Photoemission Study of the Infinite-Layer Cuprate Superconductor Sr0.9La0.1CuO2

The electron-doped infinite-layer superconductor Sr0.9La0.1CuO2 is studied with x-ray photoemission spectroscopy (XPS). A nonaqueous chemical etchant is shown to effectively remove contaminants and to yield surfaces from which signals intrinsic to the superconductor dominate. These data are compared to measurements from hole-doped La1.85Sr0.15CuO4, from undoped La2CuO4, and from electron-doped Nd1.85Ce0.15CuO4-d. The Cu 2p core level is consistent with a lower value of the O 2p to Cu 3d charge transfer energy D than in hole-doped cuprates. A clear Fermi edge is observed in the valence band region.

cond-mat.supr-con↗

arXiv2001

Synthesis and pinning properties of the infinite-layer superconductor Sr0.9La0.1CuO

We report the high-pressure synthesis of the electron-doped infinite-layer superconductor Sr0.9La0.1CuO2 and its superconducting properties. A Rietveld analysis of X-ray powder diffraction data showed that, within the resolution of the measurement, the sample had purely an infinite-layer structure without any discernible impurities. The superconducting volume fraction and the transition width were greatly improved compared to those in previous reports. The irreversibility field line and the intragranular critical current density were much higher than those of La1.85Sr0.15CuO4 and Nd1.85Ce0.15CuO4. The stronger pinning behaviors are consistent with the strong interlayer coupling due to the short distance between CuO2 planes.

cond-mat.supr-con↗

arXiv2001

Substitution for Cu in the electron-doped infinite-layer superconductor Sr0.9La0.1CuO2, Ni reduces Tc much faster than Zn

We report on the effect of substitution for Cu on Tc of electron-doped infinite-layer superconductors Sr0.9La0.1Cu1-xRxO2, R = Zn and Ni. We found that Tc was nearly constant until x = 0.03 for R = Zn, while superconductivity was nearly suppressed for x = 0.02 with dTc/dx = 20 K/% for R = Ni. This behavior is very similar to that of conventional superconductors. These findings are discussed in terms of the superconducting gap symmetry in the cuprate superconductors including another electron-doped superconductor, (Nd,Ce)2CuO4-y.

cond-mat.supr-con↗

arXiv2001

Superconducting properties of well-shaped MgB2 single crystal

We report measurements of the transport and the magnetic properties of high-quality, sub-millimeter-sized MgB2 single crystals with clear hexagonal-plate shapes. The low-field magnetization and the magnetic hysteresis curves show the vortex pinning of these crystals to be very weak. The Debye temperature of $Θ_{D}\sim 1100$ K, obtained from the zero-field resistance curve, suggests that the normal-state transport properties are dominated by electron-phonon interactions. The resistivity ratio between 40 K and 300 K was about 5, and the upper critical field anisotropy ratio was 3 $\pm$ 0.2 at temperatures around 32 K.

cond-mat.supr-con↗

arXiv2001

Three-Dimensional Superconductivity in the Infinite-Layer Compound Sr_{0.9}La_{0.1}CuO_2 in Entire Region below $T_c$

The infinite-layer compound ACuO$_{2}$ (A $=$ alkaline-earth ions) is regarded as the most suitable material for exploring the fundamental nature of the CuO$_2$ plane because it does not contain a charge-reservoir block, such as a rock-salt or a fluorite like block. We report that superconductivity in the infinite-layer compound Sr$_{0.9}$La$_{0.1}$CuO$_2$ is of a three-dimensional nature, in contrast to the quasi two-dimensional superconducting behavior of all other cuprates. The key observation is that the $c$-axis coherence length is longer than the $c$-axis lattice constant even at zero temperature. This means that the superconducting order parameter of one CuO$_{2}$ plane overlaps with those of neighboring CuO$_{2}$ planes all the temperatures below the $T_c$. Among all cuprates, only the infinite-layer superconductor shows such a feature.

cond-mat.supr-con↗

arXiv2001

MgB2 superconducting thin films with a transition temperature of 39 Kelvin

We report the growth of high-quality c-axis-oriented epitaxial MgB2 thin films by using a pulsed laser deposition technique. The thin films grown on (1`1 0 2) Al2O3 substrates show a Tc of 39 K. The critical current density in zero field is ~ 6 x 10^6 A/cm2 at 5 K and ~ 3 x 10^5 A/cm^2 at 35 K, suggesting that this compound has great potential for electronic device applications, such as microwave devices and superconducting quantum interference devices. For the films deposited on Al2O3, X-ray diffraction patterns indicate a highly c-axis-oriented crystal structure perpendicular to the substrate surface.

cond-mat.supr-con↗

arXiv2001

Far-infrared transmission studies of c-axis oriented superconducting MgB2 thin film

We reported far-infrared transmission measurements on a c-axis oriented superconducting MgB$_{2}$ thin film in the frequency range of 30 $\sim$ 250 cm$^{-1}$. We found that these measurements were sensitive to values of scattering rate $1/τ$ and superconducting gap $2Δ$. By fitting the experimental transmission spectra at 40 K and below, we obtained $1/τ=$ (700 $\sim$ 1000) cm$^{-1}$ and $2Δ(0)\cong$ 42 cm$^{-1}$. These two quantities suggested that MgB$_{2}$ belong to the dirty limit.

cond-mat.supr-con↗

arXiv2001

Pressure dependent thermoelectric power of MgB$_2$ superconductor

We have measured temperature dependence of thermoelectric power (TEP) on MgB$_2$ superconductor under hydrostatic pressure. The sign and temperature dependence of TEP shows metallic hole carriers are dominant with activation type contribution at higher temperature. TEP increases with pressure while $T_c$ decrease with ratio -0.136 K/kbar. The data are discussed in consideration of carriers from different bands and anisotropy of compressibility.

cond-mat.str-el↗

arXiv2001

X-ray Photoemission Study of MgB2

A c-axis oriented thin film and a high density sintered pellet of MgB2 have been studied by x-ray photoemission spectroscopy, and compared to measurements from MgO and MgF2 single crystals. The as-grown surface has a layer which is Mg-rich and oxidized, which is effectively removed by a nonaqueous etchant. The subsurface region of the pellet is Mg-deficient. This nonideal near-surface region may explain varied scanning tunneling spectroscopy results. The MgB2 core level and Auger signals are similar to measurements from metallic Mg and transition metal diborides, and the measured valence band is consistent with the calculated density of states.

cond-mat.supr-con↗

arXiv2001

Optical phonons of superconducting infinite-layer compounds Sr_{0.9}Ln_{0.1}CuO_2 (Ln = La, Gd, Sm)

We have identifies the otical phonon modes of the superconducting infinite-layer compounds Sr$_{0.9}Ln_{0.1}$CuO$_2$ ($Ln$ = La, Gd, Sm; $T_c$ = 43 K for all) from their infrared reflectivity spectra obtained with a Fourier-transform infrared spectrometer on high-quality high-purity samples synthesized under high pressure. The La- and the Gd-doped compounds exhibited only four (2$A_{\rm 2u}$+2$E_{\rm u}$) out of the five (2$A_{\rm 2u}$+3$E_{\rm u}$) infrared-active phonon modes predicted by a group theoretical analysis whereas the Sm-doped compound exhibited all five modes. We propose the atomic displacement pattern for each phonon mode based on reported lattice dynamics calculations and through comparison with the phonon modes of other single-layer high-$T_{\rm c}$ cuprate superconductors.

cond-mat.supr-con↗

arXiv2001

Prominent bulk pinning effect in the MgB_2 superconductor

We report the magnetic-field dependence of the irreversible magnetization of the recently discovered binary superconductor MgB$_{2}$. For the temperature region of $T< 0.9T_c$, the contribution of the bulk pinning to the magnetization overwhelms that of the surface pinning. This was evident from the fact that the magnetization curves, $M(H)$, were well described by the critical-state model without considering the surface pinning effect. It was also found that the $M(H)$ curves at various temperatures scaled when the field and the magnetization were normalized by the characteristic scaling factors $H^\ast(T)$ and $M^\ast(T)$, respectively. This feature suggests that the pinning mechanism determining the hysteresis in $M(H)$ is unique below $T=T_c$.

cond-mat.supr-con↗

arXiv2001

Temperature- and magnetic-field-dependent resistivity of MgB2 sintered at high temperature and high pressure condition

We report the temperature- and magnetic-field-dependent resistivity of MgB2 sintered at high temperature and high pressure condition. The superconducting transition width for the resistivity measurement was about 0.4 K, and the low-field magnetization showed a sharp superconducting transition with a transition width of about 1 K. The resistivity in the normal state roughly followed T^2 behavior with smaller residual resistivity ratio (RRR) of 3 over broad temperature region above 100 K rather than reported T^3 behavior with larger RRR value of ~ 20 in the samples made at lower pressures. Also, the resistivity did not change appreciably with the applied magnetic field, which was different from previous report. These differences were discussed with the microscopic and structural change due to the high-pressure sintering.

cond-mat.supr-con↗

arXiv2001

Epitaxial MgB2 superconducting thin films with a transition temperature of 39 Kelvin

We report the growth of high-quality epitaxial MgB2 thin films on (1102) Al2O3 and (001) SrTiO3 substrates by using a pulsed laser deposition technique. The thin films grown on Al2O3 substrates show a Tc of 39 K with a sharp transition width of ~ 0.7 K. The critical current density in zero field is ~ 8 x 10^6 A/cm^2 at 5 K, suggesting that this compound has great potential for industrial applications. Also, Al2O3 is a very promising substrate in terms of superconducting device applications because of its high thermal conductivity and small dielectric constant. For the films deposited on Al2O3, X-ray diffraction patterns indicate a c-axis-oriented crystal structure perpendicular to the substrate surface whereas the films deposited on SrTiO3 show {101} plane as the preferred orientation.

cond-mat.supr-con↗

arXiv2001

Origin of the high DC transport critical current density for the MgB2 superconductor

If the critical current density Jc is very high for a superconductor, then estimating its value from transport measurements is not very easy. In such cases, the value of Jc, called Jcm for magnetic Jc, is usually obtained from the measured magnetic hysteresis loop measurements by using a proper critical state model such as Bean's model (ref. 1). However, for bulk polycrystalline high temperature superconductors, the values of Jcm are much higher than the values, Jct, obtained from the transport measurements. This is due to the fact that the Jct is interrupted by weakly linked grain boundaries. However, for the recently discovered superconductor MgB2 (ref. 2), the grain boundary effect is negligible and these two values seem to coincide. Moreover, Jc increases drastically with decreasing the temperature. Consequently, the critical current densities for bulk wires can be very high, suggesting that numerous applications for the power transport. In this letter, we report the origin of the large current carrying capability of MgB2 based on direct measurements of the current-voltage relation in high magnetic fields. A strong coupling between the grains may be one reason for the absence of the weak link effect. Another reason may be the fact that, instead of a weak pinning mechanism such as thermally activated flux hopping, strong pinning due to a vortex glass phase is found in this material. The vortex phase diagram obtained from transport measurements shows that, in H-T space, a wide region below the Hc2 line is covered by a vortex glass phase.

cond-mat.supr-con↗

arXiv2001

Microstructure of the highly dense MgB2 Superconductor by transmission electron microscope

The microstructure of the MgB2 superconductor sintered at high temperature under a high pressure of about 3 GPa was investigated by using a high-resolution transmission electron microscope (HRTEM). The TEM images did not show any pores in the specimen. All grains were compactly connected, and no discernable empty spaces or impurities at the boundaries existed over the regions investigated. The HRTEM image showed clearly each constituent atom that formed the basal hexagonal plane, without any defect in a single grain. The a-axis lattice parameter, 0.307 nm, from this direct measurement was shorter than the value, 0.314 nm obtained from samples prepared using diffusion techniques. A minor impurity phase, which was most probably MgB4 and did not form interfacial layers was also observed, but was well isolated from the main MgB2 phase. Our results verify that the MgB2 powder was sintered under high temperature and high pressure into its theoretical density without any porosity or grain growth.

cond-mat.supr-con↗

arXiv2001

Effect of sintering temperature under high pressure in the uperconductivity for MgB2

We report the effect of the sintering temperature on the superconductivity of MgB2 pellets prepared under a high pressure of 3 GPa. The superconducting properties of the non-heated MgB2 in this high pressure were poor. However, as the sintering temperature increased, the superconducting properties were vastly enhanced, which was shown by the narrow transition width for the resistivity and the low-field magnetizations. This shows that heat treatment under high pressure is essential to improve superconducting properties. These changes were found to be closely related to changes in the surface morphology observed using scanning electron microscopy.

cond-mat.supr-con↗

arXiv2001

Hole carrier in MgB_{2} characterized by Hall Measurements

The longitudinal resistivity rho_{xx} and Hall coefficient R_H were measured for MgB2 sintered under high pressure. We found that R_H is positive like cuprate high-Tc superconductors, and decreases as the temperature increases for 40 K < T < 300 K. The cotangent of the Hall angle was found to follow a+bT^2 behavior from Tc to 300 K. At T = 100 K, R_H = 4.1 x 10^{-11} m^3/C from which hole carrier density was determined to be 1.5 x 10^{23}/cm^3. This carrier density is 2 - 3 orders of magnitude larger than that of Nb3Sn superconductor and that of optimally doped YBa_2Cu_3O_y.

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