arXiv subjects

Carmelo Rosales-Guzman

Publications and source records attributed to Carmelo Rosales-Guzman.

11 recordsLinked to original sources

arXiv2026

Carrier-Envelope Phase Control of Orbital Angular Momentum in Solid-State High-Harmonic Generation

High-order harmonic generation (HHG) driven by optical vortices is a powerful route to produce structured light in different spectral regions. The nonlinear process transfers orbital angular momentum (OAM) from the driving field to the emitted harmonics according to the scaling law $l_q = q\times l$, a consequence of the rotational invariance and angular momentum conservation. Here, we show that, in the regime of few-cycle pulses, the topological charge (TC) of the harmonic radiation detected within a finite spectral window is no longer fixed by this scaling law alone, but is governed by the interplay between broken crystal inversion symmetry and carrier-envelope phase (CEP)-sensitive sub-cycle electron dynamics. By driving HHG in a ZnO crystal with few-cycle ($\approx 1.5$ cycles) vortex beams centered at 3.2~$μ$m, we observed that the measured TC becomes strongly CEP-dependent, switching between adjacent integer values, but only when the inversion symmetry is broken and the harmonic emission is CEP-sensitive. The TC switching vanishes when either condition is removed. Numerical analysis reveals that the TC switching originates from a CEP-controlled redistribution of spectral weight among spectrally overlapping harmonic orders, which changes the dominant OAM channel within the detection window. These results identify the CEP as a degree of freedom for tailoring the topological structure of high-harmonic radiation, pointing toward waveform-controlled structured attosecond light sources.

physics.optics↗

arXiv2026

Twisting harmonics: Transfer of orbital angular momentum in solid-state high-harmonic generation

Although solid-state platforms underpin modern electronics, little is known about how intense ultrashort light pulses carrying orbital angular momentum (OAM) interact with solids. This gap persists even though, for more conventional light-matter interactions, the complex underlying electron dynamics can often be confined to a single Brillouin zone and described well within the dipole approximation. Previous studies were restricted to nonlinear, perturbative regimes, largely because the generation of intense ultrashort vortex pulses, particularly in the mid-infrared spectral regime, has remained a long-standing challenge. Consequently, the role of structured light in driving nonlinear, non-perturbative processes in solids, and the associated transfer of angular momentum during these interactions, has not been systematically explored. Here, we investigate solid-state high-harmonic generation (HHG) driven by intense ultrashort structured light using a versatile experimental approach applicable to different materials and geometries. We demonstrate that the OAM of the driving field is coherently transferred to the emitted harmonics. In particular, we show that the OAM is conserved independently of the crystal symmetry, the range of electronic interactions, and the presence of strong spin-orbit coupling. These results establish OAM-resolved HHG as a robust framework for characterizing and controlling angular momentum transfer in solid-state HHG and open new avenues for structured-light-driven quantum technologies and topological materials investigations.

physics.optics↗

arXiv2026

Sculpting ultrafast mid-infrared light for solid-state high harmonic generation

The ability to sculpt light in space, time, and polarization has revolutionized studies of light-matter interaction and enabled breakthroughs in optical communication, imaging, and ultrafast science. Among the many degrees of freedom of light, orbital angular momentum (OAM) further expands these capabilities by unlocking new regimes of control in information encoding, particle trapping and manipulation, and symmetry-driven selection rules. However, exploiting OAM to drive nonlinear, non-perturbative effects in solids remains challenging, especially in the mid-infrared (MIR) spectral regime-a key region for accessing these effects in ambient air, where spatial light modulators do not operate. Here, we circumvent this limitation by generating femtosecond, few-cycle MIR Bessel-Gauss vortex (BGV) and perfect optical vortices (POVs), using a robust, static spatial-shaping strategy. By utilizing these beams to drive nonlinear optical processes such as second-harmonic generation (SHG) and high-harmonic generation (HHG) in various solid-state materials, we show that the resulting harmonic beams faithfully inherit the structural characteristics of the drivers: the constant-intensity ring of the POVs is preserved across harmonic orders, while the BGV harmonic beams retain their intrinsic topological charge-dependent intensity profiles. Furthermore, by verifying the linear OAM up-scaling law, we confirm the conservation of OAM during SHG and HHG in solids. These results establish strong-field HHG in solids as a robust platform for synthesizing ultrafast structured harmonic light with controllable, high-value OAM.

physics.optics↗

arXiv2025

A curvilinear framework for vector light fields

Vector beams are often regarded as non-separable superpositions of spatial and polarization degrees of freedom that satisfy the wave equation. This interpretation ties their polarization structure to their spatial shape. Here, we introduce a generalized method to construct vector beams whose structure is entirely encoded in the polarization degree of freedom. Using conformal maps, we construct orthonormal polarization bases from the geometry of the coordinates and encode them experimentally via phase-only spatial light modulators. We apply our method to four systems, elliptical, parabolic, bipolar, and dipole, that represent algebraic and transcendental families of conformal maps. Stokes polarimetry measurements confirm agreement with theoretical predictions.

physics.optics↗

arXiv2020

Polarisation-insensitive generation of vector modes using a digital micromirror device

In recent time there has been an increasing amount of interest in developing novel techniques for the generation of complex vector light beams. Amongst these, digital holography stands out as one of the most flexible and versatile with almost unlimited freedom to generate scalar and vector light beams with arbitrary polarisation distributions and spatial transverse profile. Recently, we put forward a novel method to quantify the non-separability of vector modes in which we reported first measurements of a compact and robust device to generate such vector modes that fully exploits the polarisation-independence of Digital Micromirror Devices (DMDs). In this manuscript we fully characterise this device and provide qualitative and quantitative analysis of the generated modes. First by reconstructing their transverse polarisation distribution, using stokes polarimetry, followed by a measure of their degree of non-separability, determined through the concurrence.

physics.optics↗

arXiv2019

Full characterization of spin-orbit coupled photons via spatial-Stokes measurement

Characterization and analysis of spin-orbit coupled (SOC) states, as a measurement problem, play a vital role in research on the modern optics and photonics based on structured light. Here, we demonstrate determination of photonic SOC states via spatial-Stokes measurement, in which two spatial complex probability amplitudes of spin-dependent spatial modes within SOC states and their relative (intramode) phase can be measured directly. Compared with the standard quantum-state tomography, by avoiding wavefront-flattening operations, the apparatus can completely record photons' realistic SOC structure, leading to a more accurate and precise determination of wavefunction. This simple and general approach for SOC state determination can provide a powerful toolkit for in-situ measuring photonic SOC state, characterizing the quality of SOC light source and associated geometric-phase devices.

physics.optics↗

arXiv2019

Does the structure of light influence the speckle size?

It is well known that when a laser is reflected from a rough surface or transmitted through a diffusive medium, a speckle pattern will be formed at a given observation plane. Speckle is commonly produced by laser beams with a homogeneous intensity, for which, well-known relations have been derived, relating the speckle size to the area of illumination. Here we investigate the speckle generated by higher-order Laguerre-Gaussian (LG) modes, characterized by a non-uniform intensity distribution of concentric rings.We show that the ring-structure of the LG modes does not play any role in the speckle size, which happens to be the same as that obtained for a homogeneous intensity distribution. This allow us to provide with a simple expression that relates the speckle size to the spot size of the LG modes. Our findings will be of great relevance in many speckle-based applications.

physics.optics↗

arXiv2019

In-situ detecting cooperative-target's speed and rotation inertia using structured light

Laser remote sensing represents a powerful tool that enables the accurate measurement of the speed of moving targets. Crucially, most sensing techniques are 2-Dimensional and only enable direct determination of the speed along the line of sight. A disadvantage that is very often overcome using two-dimensional techniques that in many cases are hard to implement and expensive. Here we put forward a novel 3-Dimensional technique that enables the direct and simultaneous measurement of both, the speed and the spin rate of cooperative targets. This technique is based on the use of complex vector light beams, whose polarization and spatial degree of freedom are coupled in a non-separable way. We present experimental evidence of our technique by performing a laboratory proof-of-principle experiment.

physics.optics↗

arXiv2018

Structured light by discrete-phase orbital angular momentum holograms

Structured light has been created by a myriad of near- and far-field techniques and has found both classical and quantum applications. In the case of orbital angular momentum (OAM), continuous spiral phase patterns in dynamic or geometric phase are often employed with the phase patterns existing across the entire transverse plane. Here we exploit the uncertainty relation between OAM and angle to create structured OAM fields using multilevel OAM holograms. We show theoretically and experimentally that only a multilevel angular phase contour in the near-field is needed to create structured OAM light in the far-field, exploiting the reciprocal nature of angular momentum and angle. We use this approach to demonstrate exotic 3D structured light control to show the evolution of the Poynting vector in such fields and to highlight the physics underlying this phenomenon.

physics.optics↗

arXiv2017

Creation and characterization of vector vortex modes for classical and quantum communication

Vector vortex beams are structured states of light that are non-separable in their polarisation and spatial mode, they are eigenmodes of free-space and many fibre systems, and have the capacity to be used as a modal basis for both classical and quantum communication. Here we outline recent progress in our understanding of these modes, from their creation to their characterization and detection. We then use these tools to study the propagation behaviour of such modes in free-space and optical fibre and show that modal cross-talk results in a decay of vector states into separable scalar modes, with a concomitant loss of information. We present a comparison between probabilistic and deterministic detection schemes showing that the former, while ubiquitous, negates the very benefit of increased dimensionality in quantum communication while reducing signal in classical communication links. This work provides a useful introduction to the field as well as presenting new findings and perspectives to advance it further.

physics.optics↗

arXiv2016

Process tomography of quantum channels using classical light

High-dimensional entanglement with spatial modes of light promises increased security and information capacity over quantum channels. Unfortunately, entanglement decays due to perturbations, corrupting quantum links which cannot be repaired without a tomography of the channel. Paradoxically, the channel tomography itself is not possible without a working link. Here we overcome this problem with a robust approach to characterising quantum channels by means of classical light. Using free-space communication in a turbulent atmosphere as an example, we show that the state evolution of classically entangled degrees of freedom is equivalent to that of quantum entangled pho- tons, thus providing new physical insights into the notion of classical entanglement. The analysis of quantum channels by means of classical light in real time unravels stochastic dynamics in terms of pure state trajectories and thus enables precise quantum error-correction in short and long haul optical communication, in both free-space and fibre.

quant-ph↗