arXiv subjects

Changzhi Gu

Publications and source records attributed to Changzhi Gu.

14 recordsLinked to original sources

arXiv2026

Re-evaluation of bottleneck effect via a coupled monolayer WS_2/photonic crystal heterostructure

Exciton-polariton condensates is an important type of Bose-Einstein condensate whose realization requires efficient relaxation of polaritons to the band-energy minima. However, this process is often obstructed by bottleneck effect near the anticrossing region of polariton dispersion. Although the exciton-polariton bottleneck effect has been extensively observed in various polariton system, but there is no a unified views of physical origin. Here, we construct an exciton-trion-photon coupling system in monolayer WS_2/photonic-crystal slab heterostructures. Momentum-resolved photoluminescence reveals the anticrossing polariton dispersions for the exciton resonance with a ~57 meV Rabi splitting and there is no characteristic anticrossing for trion resonance with a ~5 meV splitting at ~12 K. Enhanced polariton emission is observed around the trion-polariton crossing with elevating temperature. We attributes this exotic phenomenon to bottleneck effect and indicating that small Rabi splitting is the unified origin of bottleneck effect in polariton systems.

physics.optics↗

arXiv2023

Giant photon-drag-induced ultrafast photocurrent in diamond for nonlinear photonics

Diamond is emerging as an attractive third-generation wide-bandgap semiconductor for future on-chip nonlinear photonics and quantum optics due to its unique thermal, optical, and mechanical properties. However, the light-driven current under below-bandgap excitation from the second-order nonlinear optical effect in diamond is still challenging. Herein, a giant second-order nonlinear photocurrent is observed in the chemical vapor deposition (CVD) diamond by utilizing terahertz (THz) emission spectroscopy. This ultrafast photocurrent originates from the photon drag effect (PDE), during which the momentum transfer from the incident photons to the charge carriers at the rich grain boundaries of the CVD diamond after the exclusive subgap π-π* transition upon femtosecond laser excitation. Especially, the interplay between circular and linear PDE to the THz generation has been clarified and distinguished under elliptically polarized light excitation. Furthermore, the picosecond ultrafast dynamics of these charge carriers are also verified by the infrared spectroscopy. Owing to the giant photon-drag-induced ultrafast photocurrent, the CVD diamond presents the highest THz emission efficiency compared with the reported carbon allotropes, which expands the new functionality of diamond nonlinear photonics into on-chip THz devices.

physics.optics↗

arXiv2023

Visualization of Photonic Band Structures via Far-field Measurements in SiNx Photonic Crystal Slabs

The band structures of the photonic crystal slabs play a significant role in manipulating the flow of light and pre-dicting exotic physics in photonics. In this letter, we show that the key features of photonic band structures can be achieved experimentally by the polarization- and momentum-resolved photoluminescence spectroscopy utilizing the light emission properties of SiNx. The two-dimensional spectra clearly reveal the energy-momentum dispersion of band structures which is in perfect agreement with the simulation results. The isofrequency contours can be measured easily by adding a bandpass filter with a desired photon energy. Furthermore, it is convenient to observe clearly and directly the optical singularity -- the optical bound states in the continuum featured by dark point in three-dimensional photoluminescence spectra. The polarization-resolved isofrequency contours clearly show that this dark point is the center of an azimuthally polarized vortex. Finally, the helical topological edge states can be easily observed in photonic topological insulators with deformed hexagonal lattices. Our work provides a simple and effective approach for exploring topological photonics and other intriguing phenomena hidden in the photonic crystal slabs.

physics.optics↗

arXiv2022

Probing Phase Transition of Band Topology via Radiation Topology

Topological photonics has received extensive attention from researchers because it provides brand new physical principles to manipulate light. Band topology of optical materials is characterized using the Berry phase defined by Bloch states. Until now, the criteria for experimentally probing the topological phase transition of band topology has always been relatively lacking in topological physics. Moreover, radiation topology can be aroused by the far-field polarizations of the radiating Bloch states, which is described by the Stokes phase. Although such two types of topologies are both related to Bloch states on the band structure, it is rather surprising that their development is almost independent. Here, we reveal that the phase transition of band topology can be probed by the radiation topology. We theoretically design and experimentally demonstrate such an intriguing phenomenon by constructing photonic crystals that support optical analogs of quantum spin Hall effects. The results show that the topological charge of the far-field polarization vortex changes from +1 to -2 or from -2 to +1 when the band topology changes from trivial to non-trivial, which provides a new criterion to probe the phase transition of band topology using radiation topology. Our findings not only provide an insightful understanding of band topology and radiation topology, but also can serve as a novel route to manipulate the near and far fields of light.

physics.optics↗

arXiv2021

Polarized exciton emission enhancement of monolayer MoS2 coupled with plasmonic Salisbury-type absorber

The plasmon-mediated manipulation of light-matter interaction in two-dimensional atomically transition-metal dichalcogenides (TMDs) critically depends on the design of plasmonic nanostructures to achieve the maximum optical field in TMDs. Here, a metal-isolator-metal Salisbury-type perfect absorber was fabricated to serve as a generator of the localized surface plasmons. The significant photoluminescence (PL) enhancement up to 60-fold was observed experimentally in the monolayer (ML) MoS2 on the top of this gold plasmonic hybrid nanostructures. Furthermore, the PL linear polarization can approach ~60 % around the peak of exciton emission and is independent on the polarization of the excitation laser. This Salisbury-type plasmon-exciton hybrid system paves a new way to develop optoelectronic devices based on TMDs.

physics.optics↗

arXiv2020

Diabolical Points in Coupled Active Cavities with Quantum Emitters

In single microdisks, embedded active emitters intrinsically affect the cavity mode of microdisks, which results in a trivial symmetric backscattering and a low controllability. Here we propose a macroscopical control of the backscattering direction by optimizing the cavity size. The signature of positive and negative backscattering directions in each single microdisk is confirmed with two strongly coupled microdisks. Furthermore, the diabolical points are achieved at the resonance of two microdisks, which agrees well with the theoretical calculations considering backscattering directions. The diabolical points in active optical structures pave a way to implement quantum information processing with geometric phase in quantum photonic networks.

physics.optics↗

arXiv2019

Enhanced Strong Interaction between Nanocavities and p-shell Excitons Beyond the Dipole Approximation

Large coupling strengths in exciton-photon interactions are important for quantum photonic network, while strong cavity-quantum-dot interactions have been focused on s-shell excitons with small coupling strengths. Here we demonstrate strong interactions between cavities and p-shell excitons with a great enhancement by the \textit{in situ} wave-function control. The p-shell excitons are demonstrated with much larger wave-function extents and nonlocal interactions beyond the dipole approximation. Then the interaction is tuned from the nonlocal to local regime by the wave-function shrinking, during which the enhancement is obtained. A large coupling strength of $210\ μ\mathrm{eV}$ has been achieved, indicating the great potential of p-shell excitons for coherent information exchange. Furthermore, we propose a distributed delay model to quantitatively explain the coupling strength variation, revealing the intertwining of excitons and photons beyond the dipole approximation.

physics.optics↗

arXiv2018

Ultrahigh Magnetic Fields Produced by Shearing Carbon Nanotubes

In laboratories, ultrahigh magnetic fields are usually produced with very large currents through superconducting, resistive or hybrid magnets, which require extreme conditions, such as low temperature, huge cooling water or tens of megawatts of power. In this work we report that when single walled carbon nanotubes (SWNTs) are cut, there are magnetic moments at the shearing end of SWNTs. The average magnetic moment is found to be 41.5+-9.8uB per carbon atom in the end states with a width of 1 nm at temperature of 300.0K, suggesting ultrahigh magnetic fields can be produced. The dangling sigma and pi bonds of the carbon atoms at the shearing ends play important roles for this unexpectedly high magnetic moments because the oxidation temperature of cut SWNTs is found to be as low as 312 in dry air. Producing ultrahigh magnetic field with SWNTs has the advantage of working at higher working temperature and with low energy consumption, suggesting great potentials of applications.

cond-mat.mtrl-sci↗

arXiv2018

Two-Photon Rabi Splitting in a Coupled System of a Nanocavity and Exciton Complexes

Two-photon Rabi splitting in a cavity-dot system provides a basis for multi-qubit coherent control in quantum photonic network. Here we report on two-photon Rabi splitting in a strongly coupled cavity-dot system. The quantum dot was grown intentionally large in size for large oscillation strength and small biexciton binding energy. Both exciton and biexciton transitions couple to a high quality factor photonic crystal cavity with large coupling strengths over 130 $μ$eV. Furthermore, the small binding energy enables the cavity to simultaneously couple with two exciton states. Thereby two-photon Rabi splitting between biexciton and cavity is achieved, which can be well reproduced by theoretical calculations with quantum master equations.

physics.optics↗

arXiv2017

Transport properties of ultrathin BaFe1.84Co0.16As2 superconducting nanowires

Superconducting nanowire single-photon detectors (SNSPDs) have an absolute advantage over other types of single photon detectors except the low operating temperature. Therefore, many efforts have been devoted to find high-temperature superconducting materials that are suitable for preparing SNSPDs. Copper-based and MgB2 ultra-thin superconducting nanowires have been already reported. However, the transport properties of iron-based ultra-thin superconducting nanowires have not been studied. In this work, a 10 nm thick 200 nm wide 30 μm long high quality superconducting nanowire was fabricated from ultrathin BaFe1.84Co0.16As2 films by a lift-off process. The precursor BaFe1.84Co0.16As2 film with a thickness of 10 nm and root-mean-square roughness of 1 nm was grown on CaF2 substrates by pulsed laser deposition. The nanowire shows a high superconducting critical temperature Tzero c=20 K with a narrow transition width of Delta T=2.5 K and exhibits a high critical current density Jc of 1.8E7 A/cm2 at 10 K. These results of ultrathin BaFe1.84Co0.16As2 nanowire will attract interest in electronic applications, including SNSPDs

cond-mat.supr-con↗

arXiv2015

Tunable mid-infrared coherent perfect absorption in a graphene meta-surface

We exploited graphene nanoribbons based meta-surface to realize coherent perfect absorption (CPA) in the mid-infrared regime. It was shown that quasi-CPA frequencies, at which CPA can be demonstrated with proper phase modulations, exist for the graphene meta-surface with strong resonant behaviors. The CPA can be tuned substantially by merging the geometric design of the meta-surface and the electrical tunability of graphene. Furthermore, we found that the graphene nanoribbon meta-surface based CPA is realizable with experimental graphene data. The findings of CPA with graphene meta-surface can be generalized for potential applications in optical detections and signal processing with two-dimensional optoelectronic materials.

physics.optics↗

arXiv2014

Full control of polarization states and phase distributions of light with dual-metasurfaces

Control of the phase and polarization states of light is an important goal for nearly all optical research. The development of an efficient optical component that allows the simultaneous manipulation of the polarization and phase distribution is needed. Traditional methods require the combination of multiple optical devices, and a single optical device cannot easily realize full control of light. We theoretically predict and experimentally verify that our proposed dual-metasurfaces provide an excellent means to simultaneously manipulate the phase and polarization of transmission light at the nanoscale. By introducing a phase gradient along the interface, we achieved a near-perfect anomalous refraction with controllable polarization in the near-infrared region. On the basis of these properties, we created a dual-metasurface capable of generating radially polarized beam, demonstrating the power of full control of light. This work opens exciting avenues toward improving the degrees of freedom in the manipulation of light, including the propagation direction and distribution of the polarization and phase, and may profoundly affect a wide range of plasmonic applications.

physics.optics↗

arXiv2011

Thickness-Dependent Morphologies of Gold on N-Layer Graphenes

We report that gold thermally deposited onto n-layer graphenes interacts differently with these substrates depending on the number layer, indicating the different surface properties of graphenes. This results in thickness-dependent morphologies of gold on n-layer graphenes, which can be used to identify and distinguish graphenes with high throughput and spatial resolution. This technique may play an important role in checking if n-layer graphenes are mixed with different layer numbers of graphene with a smaller size, which cannot be found by Raman spectra. The possible mechanisms for these observations are discussed.

physics.chem-ph↗

arXiv2008

Critical Fields and Anisotropy of NdO0.82F0.18FeAs Single Crystals

The newly discovered iron-based superconductors have stimulated enormous interests in the field of superconductivity. Since the new superconductor is a layered system, the anisotropy is a parameter with the first priority to know. Meanwhile any relevant message about the critical fields (upper critical field and irreversibility line) are essentially important. By using flux method, we have successfully grown the single crystals NdO0.82F0.18FeAs at ambient pressure. Resistive measurements reveal a surprising discovery that the anisotropy Γ= (mc/mab)^{1/2} is below 5, which is much smaller than the theoretically calculated results. The data measured up to 400 K show a continuing curved feature which prevents a conjectured linear behavior for an unconventional metal. The upper critical fields determined based on the Werthamer-Helfand-Hohenberg formula are H_{c2}^{H||ab}(T=0 K) = 304 T and H_{c2}^{H||c}(T=0 K)=62-70 T, indicating a very encouraging application of the new superconductors.

cond-mat.supr-con↗